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Marcus Doherty

Publications and source records attributed to Marcus Doherty.

6 recordsLinked to original sources

Beyond sensitivity: mechanism-resolved error budgets for designing quantum sensors

Quantum sensors are specified by a headline sensitivity, yet applications also demand accuracy and reliability. The dominant limiter of one metric is often known, but no method resolves how interacting mechanisms combine into a signed, per-mechanism budget for each metric. We introduce a framework that computes a sensor's sensitivity, accuracy, and robustness from one open-system simulation and attributes each to its limiting mechanism. For a nitrogen-vacancy diamond ensemble the attribution inverts across metrics: dephasing limits sensitivity, the thermal ground-state shift limits accuracy, and optical leakage limits robustness. At identical sensitivity the recovered-field bias spans $8$ to $1500$\,nT, so tuning to sensitivity alone can miss the accuracy target by two orders of magnitude. The same modeling transfers to a cesium optically pumped magnetometer recording a human magnetocardiogram. As a digital twin, it predicts the gain from addressing each limiter, so sensors can be designed to the required metrics.

quant-ph

Software for Massively Parallel Quantum Computing

Quantum computing has the potential to offer substantial computational advantages over conventional computing. Recent advances in quantum computing hardware and algorithms have enabled a class of classically parallel quantum workloads, whereby individual quantum circuits can execute independently on many quantum processing units. Here, we present the full-stack software framework developed at Quantum Brilliance to enable multi-modal parallelism for hybrid quantum workloads. Our software provides the capability to distribute quantum workloads across multiple quantum accelerators hosted by nodes of a locally-networked cluster, via the industry-standard MPI (Message Passing Interface) protocol, or to distribute workloads across a large number of cloud-hosted quantum accelerators.

quant-ph

Strain Engineering of Quantum Emitters in Hexagonal Boron Nitride

Quantum emitters in hexagonal boron nitride (hBN) are promising building blocks for the realization of integrated quantum photonic systems. However, their spectral inhomogeneity currently limits their potential applications. Here, we apply tensile strain to quantum emitters embedded in few-layer hBN films and realize both red and blue spectral shifts with tuning magnitudes up to 65 meV, a record for any two-dimensional quantum source. We demonstrate reversible tuning of the emission and related photophysical properties. We also observe rotation of the optical dipole in response to strain, suggesting the presence of a second excited state. We derive a theoretical model to describe strain-based tuning in hBN, and the rotation of the optical dipole. Our work demonstrates the immense potential for strain tuning of quantum emitters in layered materials to enable their employment in scalable quantum photonic networks.

cond-mat.mtrl-sci

Near-deterministic activation of room temperature quantum emitters in hexagonal boron nitride

Applications of quantum science to computing, cryptography and imaging are on their way to becoming key next generation technologies. Owing to the high-speed transmission and exceptional noise properties of photons, quantum photonic architectures are likely to play a central role. A long-standing hurdle, however, has been the realization of robust, device-compatible single photon sources that can be activated and controlled on demand. Here we use strain engineering to create large arrays of quantum emitters in two-dimensional hexagonal boron nitride (hBN). The large energy gap inherent to this Van der Waals material stabilizes the emitters at room temperature within nanoscale regions defined by substrate-induced deformation of the flake. Combining analytical and numerical modeling we show that emitter activation is likely the result of carrier trapping in deformation potential wells localized near the points where the hBN flake reaches the highest curvature. These findings, therefore, hint at novel opportunities for the manipulation of single photon sources through the combined control of strain and external electrostatic potentials under ambient conditions.

cond-mat.mes-hall

Readout and control of a single nuclear spin with a meta-stable electron spin ancilla

Electron and nuclear spins associated with point defects in insulators are promising systems for solid state quantum technology. While the electron spin usually is used for readout and addressing, nuclear spins are exquisite quantum bits and memory systems. With these systems single-shot readout of nearby nuclear spins as well as entanglement aided by the electron spin has been shown. While the electron spin in this example is essential for readout it usually limits nuclear spin coherence. This has set of the quest for defects with spin-free ground states. Here, we isolate a hitherto unidentified defect in diamond and use it at room temperature to demonstrate optical spin polarization and readout with exceptionally high contrast (up to 45%), coherent manipulation of an individual excited triplet state spin, and coherent nuclear spin manipulation using the triplet electron spin as a meta-stable ancilla. By this we demonstrate nuclear magnetic resonance and Rabi oscillations of the uncoupled nuclear spin in the spin-free electronic ground state. Our study demonstrates that nuclei coupled to single metastable electron spins are useful quantum systems with long memory times despite electronic relaxation processes.

quant-ph

Optically induced spin polarisation of the NV- centre in diamond: role of electron-vibration interaction

The novel aspect of the centre (NV-) in diamond is the high degree of spin polarisation achieved through optical illumination. In this paper it is shown that the spin polarisation occurs as a consequence of an electron-vibration interaction combined with spin-orbit interaction, and an electronic model involving these interactions is developed to account for the observed polarisation.

cond-mat.mtrl-sci