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Maria Lugaro

Publications and source records attributed to Maria Lugaro.

At least 37 records · Page 2Linked to original sources

The chemical evolution of the solar neighbourhood for planet-hosting stars

Theoretical physical-chemical models for the formation of planetary systems depend on data quality for the Sun's composition, that of stars in the solar neighbourhood, and of the estimated "pristine" compositions for stellar systems. The effective scatter and the observational uncertainties of elements within a few hundred parsecs from the Sun, even for the most abundant metals like carbon, oxygen and silicon, are still controversial. Here we analyse the stellar production and the chemical evolution of key elements that underpin the formation of rocky (C, O, Mg, Si) and gas/ice giant planets (C, N, O, S). We calculate 198 galactic chemical evolution (GCE) models of the solar neighbourhood to analyse the impact of different sets of stellar yields, of the upper mass limit for massive stars contributing to GCE ($M_{\rm up}$) and of supernovae from massive-star progenitors which do not eject the bulk of the iron-peak elements (faint supernovae). Even considering the GCE variation produced via different sets of stellar yields, the observed dispersion of elements reported for stars in the Milky Way disk is not reproduced. Among others, the observed range of super-solar [Mg/Si] ratios, sub-solar [S/N], and the dispersion of up to 0.5 dex for [S/Si] challenge our models. The impact of varying $M_{\rm up}$ depends on the adopted supernova yields. Thus, observations do not provide a constraint on the M$_{\rm up}$ parametrization. When including the impact of faint supernova models in GCE calculations, elemental ratios vary by up to 0.1-0.2 dex in the Milky Way disk; this modification better reproduces observations.

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Unveiling the chemical fingerprint of phosphorus-rich stars I. In the infrared region of APOGEE-2

The origin of phosphorus, one of the essential elements for life on Earth, is currently unknown. Prevalent models of Galactic chemical evolution (GCE) underestimate the amount of P compared to observations. The recently discovered P-rich ([P/Fe] > 1 dex) and metal-poor giants further challenge current theories on stellar nucleosynthesis. Since the observed stars are low-mass giants, our primary goal is to find clues on their progenitor. By increasing the number of known P-rich stars, we aim to narrow down a reliable chemical abundance pattern and to place robust constraints on the responsible nucleosynthetic mechanism. In the long term, identifying the progenitor of the P-rich stars may contribute to the search for the source of P in our Galaxy. We performed a detailed chemical abundance analysis based on the H-band spectra from APOGEE-2 (DR17). Employing the BACCHUS code, we measured the abundances of 13 elements in the sample, which is mainly composed of a recent collection of Si-enhanced giants. We also analyzed the orbital motions and compared the abundance results to possible nucleosynthetic formation scenarios, and also to detailed GCE models. We enlarged the sample of confirmed P-rich stars from 16 to 78 giants, which represents the largest sample of P-rich stars to date. Significant enhancements in O, Al, Si and Ce, as well as systematic correlations among the elements, unveil the chemical fingerprint of the P-rich stars. The high Mg and C+N found in some of the P-rich stars with respect to P-normal stars is not confirmed over the full sample. Strikingly, the strong over-abundance in the $α$-element Si is accompanied by normal Ca and S abundances. Our analysis of the orbital motion showed that the P-rich stars do not belong to a specific sub-population. In addition, we confirm that the majority of the sample stars are not part of binary systems.

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Representation of s-process abundances for comparison to data from bulk meteorites

Analysis of bulk meteorite compositions has revealed small isotopic variations due to the presence of material (e.g., stardust) that preserved the signature of nuclear reactions occurring in specific stellar sites. The interpretation of such anomalies provides evidence for the environment of the birth of the Sun, its accretion process, the evolution of the solar proto-planetary disk, and the formation of the planets. A crucial element of such interpretation is the comparison of the observed anomalies to predictions from models of stellar nucleosynthesis. To date, however, this comparison has been limited to a handful of model predictions. This is mostly because the calculated stellar abundances need to be transformed into a specific representation, which nuclear astrophysicists and stellar nucleosynthesis researchers are not familiar with. Here, we show in detail that this representation is needed to account for mass fractionation effects in meteorite data that can be generated both in nature and during instrumental analysis. We explain the required internal normalisation to a selected isotopic ratio, describe the motivations behind such representation more widely, and provide the tools to perform the calculations. Then, we present some examples considering two elements produced by the $slow$ neutron-capture ($s$) process: Sr and Mo. We show which specific representations for the Sr isotopic composition calculated by $s$-process models better disentangle the nucleosynthetic signatures from stars of different metallicity. For Mo, the comparison between data and models is improved due to a recent re-analysis of the $^{95}$Mo neutron-capture cross section.

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Inhomogeneous enrichment of radioactive nuclei in the Galaxy: Deposition of live Mn-53, Fe-60, Hf-182, and Pu-244 into deep-sea archives. Surfing the wave?

While modelling the galactic chemical evolution (GCE) of stable elements provides insights to the formation history of the Galaxy and the relative contributions of nucleosynthesis sites, modelling the evolution of short-lived radioisotopes (SLRs) can provide supplementary timing information on recent nucleosynthesis. To study the evolution of SLRs, we need to understand their spatial distribution. Using a 3-dimensional GCE model, we investigated the evolution of four SLRs: Mn-53, Fe-60, Hf-182, and Pu-244 with the aim of explaining detections of recent (within the last $\approx$1-20 Myr) deposition of live Mn-53, Fe-60, and Pu-244 of extrasolar origin into deep-sea reservoirs. We find that core-collapse supernovae (CCSNe) are the dominant propagation mechanism of SLRs in the Galaxy. This results in the simultaneously arrival of these four SLRs on Earth, although they could have been produced in different astrophysical sites, which can explain why live extrasolar Mn-53, Fe-60, and Pu-244 are found within the same, or similar, layers of deep-sea sediments. We predict that Hf-182 should also be found in such sediments at similar depths.

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Origin of Plutonium-244 in the Early Solar System

We investigate the origin in the early Solar System of the short-lived radionuclide 244Pu (with a half life of 80 Myr) produced by the rapid (r) neutron-capture process. We consider two large sets of r-process nucleosynthesis models and analyse if the origin of 244Pu in the ESS is consistent with that of the other r and slow (s) neutron-capture process radioactive nuclei. Uncertainties on the r-process models come from both the nuclear physics input and the astrophysical site. The former strongly affects the ratios of isotopes of close mass (129I/127I, 244Pu/238U, and 247Pu/235U). The 129I/247Cm ratio, instead, which involves isotopes of a very different mass, is much more variable than those listed above and is more affected by the physics of the astrophysical site. We consider possible scenarios for the evolution of the abundances of these radioactive nuclei in the galactic interstellar medium and verify under which scenarios and conditions solutions can be found for the origin of 244Pu that are consistent with the origin of the other isotopes. Solutions are generally found for all the possible different regimes controlled by the interval ($δ$) between additions from the source to the parcel of interstellar medium gas that ended up in the Solar System, relative to decay timescales. If r-process ejecta in interstellar medium are mixed within a relatively small area (leading to a long $δ$), we derive that the last event that explains the 129I and 247Cm abundances in the early Solar System can also account for the abundance of 244Pu. Due to its longer half life, however, 244Pu may have originated from a few events instead of one only. If r-process ejecta in interstellar medium are mixed within a relatively large area (leading to a short $δ$), we derive that the time elapsed from the formation of the molecular cloud to the formation of the Sun was 9-16 Myr.

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Cosmic nucleosynthesis: a multi-messenger challenge

The origins of the elements and isotopes of cosmic material is a critical aspect of understanding the evolution of the universe. Nucleosynthesis typically requires physical conditions of high temperatures and densities. These are found in the Big Bang, in the interiors of stars, and in explosions with their compressional shocks and high neutrino and neutron fluxes. Many different tools are available to disentangle the composition of cosmic matter, in material of extraterrestrial origins such as cosmic rays, meteorites, stardust grains, lunar and terrestrial sediments, and through astronomical observations across the electromagnetic spectrum. Understanding cosmic abundances and their evolution requires combining such measurements with approaches of astrophysical, nuclear theories and laboratory experiments, and exploiting additional cosmic messengers, such as neutrinos and gravitational waves. Recent years have seen significant progress in almost all these fields; they are presented in this review. Models are required to explore nuclear fusion of heavier elements. These have been confirmed by observations of nucleosynthesis products in the ejecta of stars and supernovae, as captured by stardust grains and by characteristic lines in spectra seen from these objects, and also by ejecta material captured by Earth over millions of years in sediments. All these help to piece together how cosmic materials are transported in interstellar space and re-cycled into and between generations of stars. Our description of cosmic compositional evolution needs observational support, as it rests on several assumptions that appear challenged. This overview presents the flow of cosmic matter and the various sites of nucleosynthesis, as understood from combining many techniques and observations, towards the current knowledge of how the universe is enriched with elements.

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Radioactive nuclei in the early Solar System: analysis of the 15 isotopes produced by core-collapse supernovae

Short-lived radioactive isotopes (SLRs) with half-lives between 0.1 to 100 Myr can be used to probe the origin of the Solar System. In this work, we examine the core-collapse supernovae production of the 15 SLRs produced: $^{26}$Al, $^{36}$Cl, $^{41}$Ca, $^{53}$Mn, $^{60}$Fe, $^{92}$Nb, $^{97}$Tc, $^{98}$Tc, $^{107}$Pd, $^{126}$Sn, $^{129}$I, $^{135}$Cs, $^{146}$Sm, $^{182}$Hf, and $^{205}$Pb. We probe the impact of the uncertainties of the core-collapse explosion mechanism by examining a collection of 62 core-collapse models with initial masses of 15, 20, and 25M$_{\odot}$, explosion energies between 3.4$\times$10$^{50}$ and 1.8$\times$10$^{52}$ ergs and compact remnant masses between 1.5M$_{\odot}$and 4.89M$_{\odot}$. We identify the impact of both explosion energy and remnant mass on the final yields of the SLRs. Isotopes produced within the innermost regions of the star, such as $^{92}$Nb and $^{97}$Tc, are the most affected by the remnant mass, $^{92}$Nb varying by five orders of magnitude. Isotopes synthesised primarily in explosive C-burning and explosive He-burning, such as $^{60}$Fe, are most affected by explosion energies. $^{60}$Fe increases by two orders of magnitude from the lowest to the highest explosion energy in the 15M$_{\odot}$model. The final yield of each examined SLR is used to compare to literature models.

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The RADIOSTAR Project

Radioactive nuclei are the key to understanding the circumstances of the birth of our Sun because meteoritic analysis has proven that many of them were present at that time. Their origin, however, has been so far elusive. The ERC-CoG-2016 RADIOSTAR project is dedicated to investigating the production of radioactive nuclei by nuclear reactions inside stars, their evolution in the Milky Way Galaxy, and their presence in molecular clouds. So far, we have discovered that: (i) radioactive nuclei produced by slow ($^{107}$Pd and $^{182}$Hf) and rapid ($^{129}$I and $^{247}$Cm) neutron captures originated from stellar sources - asymptotic giant branch (AGB) stars and compact binary mergers, respectively - within the galactic environment that predated the formation of the molecular cloud where the Sun was born; (ii) the time that elapsed from the birth of the cloud to the birth of the Sun was of the order of 10$^7$ years, and (iii) the abundances of the very short-lived nuclei $^{26}$Al, $^{36}$Cl, and $^{41}$Ca can be explained by massive star winds in single or binary systems, if these winds directly polluted the early Solar System. Our current and future work, as required to finalise the picture of the origin of radioactive nuclei in the Solar System, involves studying the possible origin of radioactive nuclei in the early Solar System from core-collapse supernovae, investigating the production of $^{107}$Pd in massive star winds, modelling the transport and mixing of radioactive nuclei in the galactic and molecular cloud medium, and calculating the galactic chemical evolution of $^{53}$Mn and $^{60}$Fe and of the p-process isotopes $^{92}$Nb and $^{146}$Sm.

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Comparison between core-collapse supernova nucleosynthesis and meteoric stardust grains: investigating magnesium, aluminium, and chromium

Isotope variations of nucleosynthetic origin among Solar System's solid samples are well documented, yet the origin of these variations is still uncertain. The observed variability of \iso{54}Cr among materials formed in different regions of the proto-planetary disk has been attributed to variable amounts of presolar chromium-rich oxide (chromite) grains, which exist within the meteoritic stardust inventory and most likely originated from some type of supernova explosions. To investigate if core-collapse supernovae (CCSNe) could be the site of origin of these grains, we analyse yields of CCSN models of stars with initial mass 15, 20 and 25 M$_{\odot}$, and solar metallicity. We present an extensive abundance data set of the Cr, Mg, and Al isotopes as a function of enclosed mass. We find cases in which the explosive C-ashes produce a composition in good agreement with the observed \iso{54}Cr/\iso{52}Cr and \iso{53}Cr/\iso{52}Cr ratios as well as the \iso{50}Cr/\iso{52}Cr ratios. Taking into account that the signal at atomic mass 50 could also originate from \iso{50}Ti, the ashes of explosive He-burning also match the observed ratios. Addition of material from the He ashes (enriched in Al and Cr relative to Mg to simulate the make-up of chromite grains) to the Solar System composition may reproduce the observed correlation between Mg and Cr anomalies, while material from the C-ashes does not present significant Mg anomalies together with Cr isotopic variations. In all cases, non-radiogenic, stable Mg isotope variations dominate over the variations expected from \iso{26}Al.

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The Radioactive Nuclei $^{\textbf{26}}$Al and $^{\textbf{60}}$Fe in the Cosmos and in the Solar System

The cosmic evolution of the chemical elements from the Big Bang to the present time is driven by nuclear fusion reactions inside stars and stellar explosions. A cycle of matter recurrently re-processes metal-enriched stellar ejecta into the next generation of stars. The study of cosmic nucleosynthesis and of this matter cycle requires the understanding of the physics of nuclear reactions, of the conditions at which the nuclear reactions are activated inside the stars and stellar explosions, of the stellar ejection mechanisms through winds and explosions, and of the transport of the ejecta towards the next cycle, from hot plasma to cold, star-forming gas. Due to the long timescales of stellar evolution, and because of the infrequent occurrence of stellar explosions, observational studies are challenging. Due to their radioactive lifetime of million years, the 26Al and 60Fe isotopes are suitable to characterise simultaneously the processes of nuclear fusion reactions and of interstellar transport. We describe and discuss the nuclear reactions involved in the production and destruction of 26Al and 60Fe, the key characteristics of the stellar sites of their nucleosynthesis and their interstellar journey after ejection from the nucleosynthesis sites. We connect the theoretical astrophysical aspects to the variety of astronomical messengers, from stardust and cosmic-ray composition measurements, through observation of gamma rays produced by radioactivity, to material deposited in deep-sea ocean crusts and to the inferred composition of the first solids that have formed in the Solar System. We show that considering measurements of the isotopic ratio of 26Al to 60Fe eliminate some of the unknowns when interpreting astronomical results, and discuss the lessons learned from these two isotopes on cosmic chemical evolution.

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The stellar beta-decay rate of 134Cs and its impact on the Barium nucleosynthesis in the s process

We have calculated the stellar $β$-decay rate of the important s-process branching point ${}^{134}$Cs based on the state of the art shell model calculations. At typical $s$-process temperatures ($T\sim$ 0.2-0.3 GK), our new rate is one order of magnitude lower than the widely-used rate from Takahashi and Yokoi (hereafter TY87). The impact on the nucleosynthesis in AGB stars is investigated with various masses and metallicities. Our new decay rate leads to an overall decrease in the ${}^{134}$Ba/${}^{136}$Ba ratio, and well explains the measured ratio in meteorities without introducing the $i$ process. We also derive the elapsed time from the last AGB nucleosynthetic event that polluted the early Solar System to be $>$28 Myr based on the ${}^{135}$Cs/${}^{133}$Cs ratio, which is consistent with the elapsed times derived from ${}^{107}$Pd and ${}^{182}$Hf. The $s$-process abundance sum of ${}^{135}$Ba and ${}^{135}$Cs is found to increase, resulting in a smaller $r$-process contribution of ${}^{135}$Ba in the Solar System.

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129I and 247Cm in Meteorites Constrain the Last Astrophysical Source of Solar r-process Elements

The composition of the early Solar System can be inferred from meteorites. Many elements heavier than iron were formed by the rapid neutron-capture process (r process), but the astrophysical sources where this occurred remain poorly understood. We demonstrate that the near-identical half-lives ($\simeq$ 15.6 Myr) of the radioactive r-process nuclei 129I and 247Cm preserve their ratio, irrespective of the time between production and incorporation into the Solar System. We constrain the last r-process source by comparing the measured meteoritic 129I / 247Cm = 438 $\pm$ 184 to nucleosynthesis calculations based on neutron star merger and magneto-rotational supernova simulations. Moderately neutron-rich conditions, often found in merger disk ejecta simulations, are most consistent with the meteoritic value. Uncertain nuclear physics data limit our confidence in this conclusion.

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The Origin of Elements from Carbon to Uranium

To reach a deeper understanding of the origin of elements in the periodic table, we construct Galactic chemical evolution (GCE) models for all stable elements from C (A=12) to U (A=238) from first principles, i.e., using theoretical nucleosynthesis yields and event rates of all chemical enrichment sources. This enables us to predict the origin of elements as a function of time and environment. In the solar neighborhood, we find that stars with initial masses of M>30M_\odot can become failed supernovae if there is a significant contribution from hypernovae (HNe) at M~20-50M_\odot. The contribution to GCE from super asymptotic giant branch (AGB) stars (with M~8-10M_\odot at solar metallicity) is negligible, unless hybrid white dwarfs from low-mass super-AGB stars explode as so-called Type Iax supernovae, or high-mass super-AGB stars explode as electron-capture supernovae (ECSNe). Among neutron-capture elements, the observed abundances of the second (Ba) and third (Pb) peak elements are well reproduced with our updated yields of the slow neutron-capture process (s-process) from AGB stars. The first peak elements, Sr, Y, and Zr, are sufficiently produced by ECSNe together with AGB stars. Neutron star mergers can produce rapid neutron-capture process (r-process) elements up to Th and U, but the timescales are too long to explain observations at low metallicities. The observed evolutionary trends, such as for Eu, can well be explained if ~3% of 25-50 M_\odot hypernovae are magneto-rotational supernovae producing r-process elements. Along with the solar neighborhood, we also predict the evolutionary trends in the halo, bulge, and thick disk for future comparison with galactic archaeology surveys.

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Gas and dust from metal-rich AGB stars

Context: Stars evolving through the asymptotic giant branch (AGB) phase provide significant feedback to their host system, in form of both gas enriched in nuclear-burning products and dust formed in their winds, which they eject into the interstellar medium. Therefore AGB stars are an essential ingredient for the chemical evolution of the Milky Way and other galaxies. Aims: We study AGB models with super-solar metallicity, to complete our large database, so far extending from metal-poor to solar chemical compositions. We provide chemical yields for masses in the range 1-8 Msun and metallicities Z=0.03 and Z=0.04. We also study dust production in this metallicity domain. Methods: We calculated the evolutionary sequences from the pre main sequence through the whole AGB phase. We follow the variation of the surface chemical composition to calculate the chemical yields of the various species and model dust formation in the winds to determine the dust production rate and the total dust mass produced by each star during the AGB phase. Results: The physical and chemical evolution of the star is sensitive to the initial mass: M> 3Msun stars experience hot bottom burning, whereas the surface chemistry of the lower mass counterparts is altered only by third dredge-up. The carbon-star phase is reached by 2.5-3.5Msun stars of metallicity Z=0.03, whereas all the Z=0.04 stars (except the 2.5 Msun) remain O-rich for the whole AGB phase. Most of the dust produced by metal-rich AGBs is in the form of silicates particles. The total mass of dust produced increases with the mass of the star, reaching ~ 0.012 Msun for 8Msun stars.

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Origin of large meteoritic SiC stardust grains in metal-rich AGB stars

Stardust grains that originated in ancient stars and supernovae are recovered from meteorites and carry the detailed composition of their astronomical sites of origin. We present evidence that the majority of large ($μ$m-sized) meteoritic silicon carbide (SiC) grains formed in C-rich asymptotic giant branch (AGB) stars that were more metal-rich than the Sun. In the framework of the slow neutron-captures (the s process) that occurs in AGB stars the lower-than-solar 88Sr/86Sr isotopic ratios measured in the large SiC grains can only be accompanied by Ce/Y elemental ratios that are also lower than solar, and predominately observed in metal-rich barium stars - the binary companions of AGB stars. Such an origin suggests that these large grains represent the material from high-metallicity AGB stars needed to explain the s-process nucleosynthesis variations observed in bulk meteorites (Ek et al. 2020). In the outflows of metal-rich, C-rich AGB stars SiC grains are predicted to be small ($\simeq$ 0.2 $μ$m-sized); large ($\simeq$ $μ$m-sized) SiC grains can grow if the number of dust seeds is two to three orders of magnitude lower than the standard value of $10^{-13}$ times the number of H atoms. We therefore predict that with increasing metallicity the number of dust seeds might decrease, resulting in the production of larger SiC grains.

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The origin of s-process isotope heterogeneity in the solar protoplanetary disk

Rocky asteroids and planets display nucleosynthetic isotope variations that are attributed to the heterogeneous distribution of stardust from different stellar sources in the solar protoplanetary disk. Here we report new high precision palladium isotope data for six iron meteorite groups, which display smaller nucleosynthetic isotope variations than the more refractory neighbouring elements. Based on this observation we present a new model in which thermal destruction of interstellar medium dust results in an enrichment of s-process dominated stardust in regions closer to the Sun. We propose that stardust is depleted in volatile elements due to incomplete condensation of these elements into dust around asymptotic giant branch (AGB) stars. This led to the smaller nucleosynthetic variations for Pd reported here and the lack of such variations for more volatile elements. The smaller magnitude variations measured in heavier refractory elements suggest that material from high-metallicity AGB stars dominated stardust in the Solar System. These stars produce less heavy s-process elements compared to the bulk Solar System composition.

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Stochastic Chemical Evolution of Radioactive Isotopes with a Monte Carlo Approach

Short-lived radionuclides (SLRs) with mean-lives $τ$ of a few to hundreds Myr provide unique opportunities to probe recent nucleosynthesis events in the interstellar medium, and the physical conditions in which the Sun formed. Here we quantify the uncertainty in the predicted evolution of SLRs within a parcel of interstellar gas given the stochastic nature of stellar enrichment events. We assume that an enrichment progenitor is formed at every time interval $γ$. For each progenitor, we randomly sample the delay time between its formation and its enrichment event, based on several delay-time distribution (DTD) functions that cover a wide range of astrophysical sites. For each set of $τ$, $γ$, and DTD function, we follow the abundances of SLRs for 15 Gyr, and repeat this process thousands of times to derive their probability distributions. For $τ/γ\gtrsim2$, the distributions depend on the DTD function and we provide tabulated values and analytical expressions to quantify the spread. The relative abundance uncertainty reaches a maximum of $\sim$ 60% for $τ/γ=1$. For $τ/γ\lesssim1$, we provide the probability for the SLR abundance to carry the signature of only one enrichment event, which is greater than 50% when $τ/γ\lesssim0.3$. For $0.3\lesssimτ/γ\lesssim 2$, a small number of events contributed to the SLR abundance. This case needs to be investigated with a separate statistical method. We find that an isolation time for the birth of the Sun of roughly $9-13$ Myr is consistent with the observed abundances of $^{60}$Fe, $^{107}$Pd, and $^{182}$Hf in the early Solar System, when assuming $τ/γ\sim3$ for these isotopes.

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Learning about the intermediate neutron-capture process from lead abundances

Lead (Pb) is predominantly produced by the slow neutron-capture process (s process) in asymptotic giant branch (AGB) stars. In contrast to significantly enhanced Pb abundances predicted by low-mass, low-metallicity AGB-models, observations of Magellanic post-AGB stars show incompatibly low Pb abundances. Observations of carbon-enhanced metal-poor (CEMP) stars whose s-process enrichments are accompanied by heavy elements traditionally associated with the rapid neutron-capture process (r process) have raised the need for a neutron-capture process operating at neutron densities intermediate to the s and r process: the so-called i process. We study i-process nucleosynthesis with single-zone nuclear-network calculations. Our i-process models can explain the heavy-element abundance patterns measured in Magellanic post-AGB stars including their puzzlingly low Pb abundances. Furthermore, the heavy-element enhancements in the post-AGB and CEMP-i stars, particularly their Pb abundance, allow us to characterise the neutron densities and exposures of the i process that produced the observed abundance patterns. We find that the lower-metallicity CEMP-i stars ($\left[ \mathrm{Fe} / \mathrm{H} \right] \approx -2.5$) have heavy-element abundances best matched by models with higher neutron densities and exposures ($τ> 2.0 \, \mathrm{mbarn}^{-1}$) compared to the higher-metallicity post-AGB stars ($\left[ \mathrm{Fe} / \mathrm{H} \right] \approx -1.3$, $τ< 1.3 \, \mathrm{mbarn}^{-1}$). This offers new constraints and insights regarding the properties of i-process sites and demonstrates that the responsible process operates on time scales of the order of a few years or less.

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