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Maria Schönbächler

Publications and source records attributed to Maria Schönbächler.

At least 19 recordsLinked to original sources

Dust Processing in Protoplanetary Discs From Infall to Dispersal: the Origin of Solar System Isotopic Heterogeneities

The nucleosynthetic heterogeneity between different asteroids and planets is well established. These isotopic variations manifest themselves at the part per millions level or larger, in isotopes that were synthesised in various stellar environments. To escape homogenisation, some of these isotopic signatures must have been preserved in dust, which ended up being heterogeneously distributed in the solar protoplanetary disc. The origin of the nucleosynthetic heterogeneity is still poorly constrained, potentially reflecting inherited isotope variations from the Sun's parental molecular cloud and/or processing and redistribution during the subsequent protoplanetary disc phase with thermal processing and size sorting as major processes. This chapter aims to provide a broad review of the dynamical, collisional, and thermal processes in protoplanetary discs -- from initial infall to gas dispersal -- that may have influenced the distribution and survival of the anomalous carrier phases, which finally accreted into asteroids and planets. While several of these mechanisms have been considered in past studies, they are often examined in isolation, which impedes the assessment of how their effects may be altered or amplified by additional disc processes. Size sorting in particular has received little attention, and here we highlight that this process likely occurred in the disc and can induce nucleosynthetic heterogeneity. By placing previous studies within the context of a comprehensive overview, we aim to clarify the broader physical framework in which anomalous carrier transport occurs and identify previously underexplored mechanisms that may have contributed to the final isotopic structure of the Solar System we see today.

astro-ph.EP↗

Predictions from $s$-process AGB models of the isotopic variations of zirconium and neodymium for comparison to bulk meteorites

Bulk meteoritic data show isotopic variability of $slow$-neutron-capture ($s$-process) origin in a several elements heavier than Fe. One peculiar feature is that the lighter $s$-process elements (e.g., Zr and Mo) present larger anomalies than the heavier $s$-process elements (e.g., Nd and W). To address this observation, we compared Zr and Nd data to model predictions of the s-process abundances at the surface of low-mass asymptotic giant branch (AGB) stars of initial metallicity from solar to twice solar. We found that the relative magnitude of the isotopic variability between these two elements can be matched by models of AGB stars of super-solar metallicity. The match is favoured by stronger convective overshoot, leading to a deeper dredge-up of the H-rich envelope into the He-rich region, and/or a smaller (~ half than standard) mass of the region rich in the $^{13}$C nuclei that produce free neutrons via the $^{13}$C($α$,n)$^{16}$O reaction. We conclude that nucleosynthesis in AGB stars can match the difference in the magnitude of the bulk meteoritic variations in Zr and Nd, provided that super-solar metallicity stars are the original site of these signatures. The AGB stars that produced such variations could have belonged to the current population of old, super-solar metallicity stars seen in the galactic solar neighbourhood.

astro-ph.SR↗

Experimental evidence for granular shear-flow instability in the Epstein regime

Stability analysis of two-fluid protoplanetary disc models has enriched our understanding of how solids can grow into larger bodies called planetesimals. Dust particles entrained in a gas stream modify the flow, creating shear layers prone to instability. In such environments, drag occurs in the free-molecular (Epstein) regime. Recreating these two-phase flows on Earth is difficult due to gravity-driven buoyancy. Here, we use particle image velocimetry to study a low-pressure dust-gas mixture at Knudsen numbers up to 10 in microgravity. We observe a granular shear flow instability, characterized by a periodic velocity field, which can be modeled to first order as a Kelvin-Helmholtz (KH) instability. This behavior resembles a Kelvin-Helmholtz instability and provides a benchmark for two-fluid theories relevant to planet formation.

astro-ph.EP↗

Stellar Interpretation of Meteoritic Data and PLotting for Everyone (SIMPLE): Isotope Mixing Lines for Six Sets of Core-Collapse Supernova Models

Bulk meteorites and their inclusions exhibit, for many chemical elements, isotopic variability produced by nucleosynthetic events in stars and supernovae before the formation of the Sun. While the exact astrophysical origins of these variations are still a matter of debate, their identification provides insights on the environment of the Sun's birth and the formation of the Solar System. Here we present a new Python tool called SIMPLE (Stellar Interpretation of Meteoritic Data and Plotting for Everyone) designed to compare the isotopic composition of the ejecta from core-collapse supernovae (CCSNe) with meteoritic data. In the present version, the SIMPLE toolkit includes a dataset of 18 CCSN models, from 6 different published sets, with initial masses of 15, 20, and 25 M$_{\odot}$ and solar metallicity. SIMPLE is designed to easily extract the isotopic abundances predicted by each CCSN model for any elements and post-process them into the format needed to compare to the meteoritic data, therefore, facilitating their interpretation. As an example of how to use SIMPLE, we analyze the composition of the Ni isotopes in the 18 models and confirm that bulk meteorite Ni anomalies are compatible with material from the innermost Si-rich region of CCSN ejecta. Designed as a collaborative platform, SIMPLE is open-source and welcomes community contributions to enhance its development and dissemination for stellar nucleosynthesis and meteoritic studies. Future enhancements include addition of more model predictions and inclusion of mixing between different layers of supernova ejecta.

astro-ph.SR↗

Interstellar Ices as Carriers of Supernova Material to the Early Solar System

Planetary materials show systematic variations in their nucleosynthetic isotope compositions that resonate with orbital distance. The origin of this pattern remains debated, limiting how these isotopic signatures can be used to trace the precursors of terrestrial planets. Here we test the hypothesis that interstellar ices carried supernova-produced nuclides by searching for a supernova nucleosynthetic fingerprint in aqueous alteration minerals from carbonaceous and non-carbonaceous chondrite meteorites. We focus on zirconium, a refractory element that includes the neutron-rich isotope $^{96}$Zr formed in core-collapse supernovae. Leaching experiments reveal extreme $^{96}$Zr enrichments in alteration minerals, showing that they incorporated supernova material hosted in interstellar ices. We show that the Solar System's zirconium isotope variability reflects mixing between these ices and an ice-free rocky component. Finally, the presence of supernova nuclides in a volatile carrier supports models where the Solar System's nucleosynthetic variability was imparted by thermal processing of material in the protoplanetary disk and during planetary accretion.

astro-ph.EP↗

The Elemental Abundances of Ryugu: Assessment of Chemical Heterogeneities and the Nugget Effect

The Hayabusa 2 spacecraft sampled ~5.4 g of asteroid material from the Cb-type asteroid Ryugu. Initial analysis of the Ryugu materials revealed a mineralogical, chemical, and isotopic kinship to the CI chondrites. In this study, we have summarized the elemental abundances of Ryugu samples published to date, and evaluated their compositional variability associated with the CI chondrite data. The abundances of some elements (e.g., P, Ca, Mn, and rare earth elements) in individual Ryugu particles were found to show large relative dispersions compared to the other elements, presumably due to the nugget effect of aqueously formed minor secondary minerals (e.g., dolomite, apatite, magnetite, and pyrrhotite). Consequently, the mean abundances of Ryugu for these elements, calculated using currently available Ryugu data, are accompanied by a certain degree of uncertainties. We suggest establishing a consortium to determine the representative elemental abundances of Ryugu by measuring aliquots from a large homogenized powder sample that can mitigate the nugget effect. Our statistical calculation shows that at least 750 and 400 mg of homogenized samples from Chambers A and C, respectively, are needed to achieve within +/-5% compositional heterogeneity. The data obtained throughout the consortium activity complement the scientific objectives of the Hayabusa2 mission. Moreover, we anticipate that the obtained Ryugu data, coupled with the elemental abundances of CI chondrites, provide new insights into the chemical composition of the Solar System, which will be used by multidisciplinary communities, including Earth and planetary sciences, astronomy, physics, and chemistry.

astro-ph.EP↗

Presolar Grains As Probes of Supernova Nucleosynthesis

We provide an overview of the isotopic signatures of presolar supernova grains, specifically focusing on 44Ti-containing grains with robustly inferred supernova origins and their implications for nucleosynthesis and mixing mechanisms in supernovae. Recent technique advancements have enabled the differentiation between radiogenic (from 44Ti decay) and nonradiogenic 44Ca excesses in presolar grains, made possible by enhanced spatial resolution of Ca-Ti isotope analyses with the Cameca NanoSIMS (Nano-scale Secondary Ion Mass Spectrometer) instrument. Within the context of presolar supernova grain data, we discuss (i) the production of 44Ti in supernovae and the impact of interstellar medium heterogeneities on the galactic chemical evolution of 44Ca/40Ca, (ii) the nucleosynthesis processes of neutron bursts and explosive H-burning in Type II supernovae, and (iii) challenges in identifying the progenitor supernovae for 54Cr-rich presolar nanospinel grains. Drawing on constraints and insights derived from presolar supernova grain data, we also provide an overview of our current understanding of the roles played by various supernova types - including Type II, Type Ia, and electron capture supernovae - in accounting for the diverse array of nucleosynthetic isotopic variations identified in bulk meteorites and meteoritic components. We briefly overview the potential mechanisms that have been proposed to explain these nucleosynthetic variations by describing the transport and distribution of presolar dust carriers in the protoplanetary disk. We highlight existing controversies in the interpretation of presolar grain data and meteoritic nucleosynthetic isotopic variations, while also outlining potential directions for future research.

astro-ph.SR↗

The Ni isotopic composition of Ryugu reveals a common accretion region for carbonaceous chondrites

The isotopic compositions of samples returned from Cb-type asteroid Ryugu and Ivuna-type (CI) chondrites are distinct from other carbonaceous chondrites, which has led to the suggestion that Ryugu and CI chondrites formed in a different region of the accretion disk, possibly around the orbits of Uranus and Neptune. We show that, like for Fe, Ryugu and CI chondrites also have indistinguishable Ni isotope anomalies, which differ from those of other carbonaceous chondrites. We propose that this unique Fe and Ni isotopic composition reflects different accretion efficiencies of small FeNi metal grains among the carbonaceous chondrite parent bodies. The CI chondrites incorporated these grains more efficiently, possibly because they formed at the end of the disk's lifetime, when planetesimal formation was also triggered by photoevaporation of the disk. Isotopic variations among carbonaceous chondrites may thus reflect fractionation of distinct dust components from a common reservoir, implying CI chondrites and Ryugu may have formed in the same region of the accretion disk as other carbonaceous chondrites.

astro-ph.EP↗

Gas permeability and mechanical properties of dust grain aggregates at hyper- and zero-gravity

Particle-particle and particle-gas processes significantly impact planetary precursors such as dust aggregates and planetesimals. We investigate gas permeability ($κ$) in 12 granular samples, mimicking planetesimal dust regoliths. Using parabolic flights, this study assesses how gravitational compression -- and lack thereof -- influences gas permeation, impacting the equilibrium state of low-gravity objects. Transitioning between micro- and hyper-gravity induces granular sedimentation dynamics, revealing collective dust-grain aerodynamics. Our experiments measure $κ$ across Knudsen number (Kn) ranges, reflecting transitional flow. Using mass and momentum conservation, we derive $κ$ and calculate pressure gradients within the granular matrix. Key findings: 1. As confinement pressure increases with gravitational load and mass flow, $κ$ and average pore space decrease. This implies that a planetesimal's unique dust-compaction history limits sub-surface volatile outflows. 2. The derived pressure gradient enables tensile strength determination for asteroid regolith simulants with cohesion. This offers a unique approach to studying dust-layer properties when suspended in confinement pressures comparable to the equilibrium state on planetesimals surfaces, which will be valuable for modelling their collisional evolution. 3. We observe a dynamical flow symmetry breaking when granular material moves against the pressure gradient. This occurs even at low Reynolds numbers, suggesting that Stokes numbers for drifting dust aggregates near the Stokes-Epstein transition require a drag force modification based on permeability.

astro-ph.IM↗

A community-led calibration of the Zr isotope Reference Materials: NIST candidate RM 8299 and SRM 3169

As the field of Zr stable isotopes is rapidly expanding from the study of mass-independent to that of mass-dependent isotope effects, a variety of Zr standards have appeared in the literature. While several of these standards have been proposed as the ideal isotope reference material (iRM) against which all data should be reported, none of them have been shown to meet the compositional and/or conflict-of-interest-free distribution requirements put forth by the community. To remedy this situation, we report on a community-led effort to develop and calibrate a scale defining iRM for Zr isotopes: NIST RM 8299. Developed in partnership with the National Institute of Standards and Technology (NIST) from the widely used SRM 3169 Zr Standard Solution, the candidate RM 8299 was calibrated through an inter-laboratory study involving three laboratories. Our data show that RM 8299 meets all requirements of an ideal iRM. It is an isotopically homogeneous, high-purity reference material, that is free of isotope anomalies, and whose composition is identical to that of a major geological reservoir (Ocean Island Basalts). Furthermore, RM 8299 will be curated and distributed by NIST, a neutral, conflict-of-interest free organization, and was produced in sufficient quantities to last multiple decades. We recommend that all Zr isotope data to be reported against RM 8299. Our results also show that SRM 3169 lots #130920 and #071226 have identical composition to RM 8299. Therefore, using RM 8299 as the scale defining iRM will enable direct comparison of all future data with the vast majority of the existing literature data, both for mass-independent and mass-dependent isotope effects. To facilitate conversion of d94/90Zr values reported against other Zr standards, we provide high-precision conversion factors to the RM 8299 scale obtained using the double-spike method.

physics.geo-ph↗

Representation of s-process abundances for comparison to data from bulk meteorites

Analysis of bulk meteorite compositions has revealed small isotopic variations due to the presence of material (e.g., stardust) that preserved the signature of nuclear reactions occurring in specific stellar sites. The interpretation of such anomalies provides evidence for the environment of the birth of the Sun, its accretion process, the evolution of the solar proto-planetary disk, and the formation of the planets. A crucial element of such interpretation is the comparison of the observed anomalies to predictions from models of stellar nucleosynthesis. To date, however, this comparison has been limited to a handful of model predictions. This is mostly because the calculated stellar abundances need to be transformed into a specific representation, which nuclear astrophysicists and stellar nucleosynthesis researchers are not familiar with. Here, we show in detail that this representation is needed to account for mass fractionation effects in meteorite data that can be generated both in nature and during instrumental analysis. We explain the required internal normalisation to a selected isotopic ratio, describe the motivations behind such representation more widely, and provide the tools to perform the calculations. Then, we present some examples considering two elements produced by the $slow$ neutron-capture ($s$) process: Sr and Mo. We show which specific representations for the Sr isotopic composition calculated by $s$-process models better disentangle the nucleosynthetic signatures from stars of different metallicity. For Mo, the comparison between data and models is improved due to a recent re-analysis of the $^{95}$Mo neutron-capture cross section.

astro-ph.SR↗

The Dissipation of the Solar Nebula Constrained by Impacts and Core Cooling in Planetesimals

Rapid cooling of planetesimal cores has been inferred for several iron meteorite parent bodies based on metallographic cooling rates, and linked to the loss of their insulating mantles during impacts. However, the timing of these disruptive events is poorly constrained. Here, we used the short-lived 107Pd / 107Ag decay system to date rapid core cooling by determining Pd-Ag ages for iron meteorites. We show closure times for the iron meteorites equate to cooling in the timeframe ~7.8 to 11.7 Myr after CAI, and indicate that an energetic inner Solar System persisted at this time. This likely results from the dissipation of gas in the protoplanetary disk, after which the damping effect of gas drag ceases. An early giant planet instability between 5 and 14 Myr after CAI could have reinforced this effect. This correlates well with the timing of impacts recorded by the Pd Ag system for iron meteorites.

astro-ph.EP↗

TEMPus VoLA: the Timed Epstein Multi-pressure Vessel at Low Accelerations

The field of planetary system formation relies extensively on our understanding of the aerodynamic interaction between gas and dust in protoplanetary disks. Of particular importance are the mechanisms triggering fluid instabilities and clumping of dust particles into aggregates, and their subsequent inclusion into planetesimals. We introduce the Timed Epstein Multi-pressure vessel at Low Accelerations (TEMPusVoLA), which is an experimental apparatus for the study of particle dynamics and rarefied gas under micro-gravity conditions. This facility contains three experiments dedicated to studying aerodynamic processes, i) the development of pressure gradients due to collective particle-gas interaction, ii) the drag coefficients of dust aggregates with variable particle-gas velocity, iii) the effect of dust on the profile of a shear flow and resultant onset of turbulence. The approach is innovative with respect to previous experiments because we access an untouched parameter space in terms of dust particle packing fraction, and Knudsen, Stokes, and Reynolds numbers. The mechanisms investigated are also relevant for our understanding of the emission of dust from active surfaces such as cometary nuclei and new experimental data will help interpreting previous datasets (Rosetta) and prepare future spacecraft observations (Comet Interceptor). We report on the performance of the experiments, which has been tested over the course of multiple flight campaigns. The project is now ready to benefit from additional flight campaigns, to cover a wide parameter space. The outcome will be a comprehensive framework to test models and numerical recipes for studying collective dust particle aerodynamics under space-like conditions.

astro-ph.IM↗

Presolar stardust in asteroid Ryugu

We have conducted a NanoSIMS-based search for presolar material in samples recently returned from C-type asteroid Ryugu as part of JAXA's Hayabusa2 mission. We report the detection of all major presolar grain types with O- and C-anomalous isotopic compositions typically identified in carbonaceous chondrite meteorites: 1 silicate, 1 oxide, 1 O-anomalous supernova grain of ambiguous phase, 38 SiC, and 16 carbonaceous grains. At least two of the carbonaceous grains are presolar graphites, whereas several grains with moderate C isotopic anomalies are probably organics. The presolar silicate was located in a clast with a less altered lithology than the typical extensively aqueously altered Ryugu matrix. The matrix-normalized presolar grain abundances in Ryugu are 4.8$^{+4.7}_{-2.6}$ ppm for O-anomalous grains, 25$^{+6}_{-5}$ ppm for SiC grains and 11$^{+5}_{-3}$ ppm for carbonaceous grains. Ryugu is isotopically and petrologically similar to carbonaceous Ivuna-type (CI) chondrites. To compare the in situ presolar grain abundances of Ryugu with CI chondrites, we also mapped Ivuna and Orgueil samples and found a total of SiC grains and 6 carbonaceous grains. No O-anomalous grains were detected. The matrix-normalized presolar grain abundances in the CI chondrites are similar to those in Ryugu: 23 $^{+7}_{-6}$ ppm SiC and 9.0$^{+5.3}_{-4.6}$ ppm carbonaceous grains. Thus, our results provide further evidence in support of the Ryugu-CI connection. They also reveal intriguing hints of small-scale heterogeneities in the Ryugu samples, such as locally distinct degrees of alteration that allowed the preservation of delicate presolar material.

astro-ph.EP↗

Presolar grain dynamics: creating nucleosynthetic variations through a combination of drag and viscous evolution

Meteoritic studies of solar system objects show evidence of nucleosynthetic heterogeneities that are inherited from small presolar grains (< 10 $μ$m) formed in stellar environments external to our own. The initial distribution and subsequent evolution of these grains are currently unconstrained. Using 3D, gas-dust simulations, we find that isotopic variations on the order of those observed in the solar system can be generated and maintained by drag and viscosity. Small grains are dragged radially outwards without size/density sorting by viscous expansion and backreaction, enriching the outer disc with presolar grains. Meanwhile large aggregates composed primarily of silicates drift radially inwards due to drag, further enriching the relative portion of presolar grains in the outer disc and diluting the inner disc. The late accumulation of enriched aggregates outside Jupiter could explain some of the isotopic variations observed in solar system bodies, such as the enrichment of supernovae derived material in carbonaceous chondrites. We also see evidence for isotopic variations in the inner disc that may hold implications for enstatite and ordinary chondrites that formed closer to the Sun. Initial heterogeneities in the presolar grain distribution that are not continuously reinforced are dispersed by diffusion, radial surface flows, and/or planetary interactions over the entire lifetime of the disc. For younger, more massive discs we expect turbulent diffusion to be even more homogenising, suggesting that dust evolution played a more central role in forming the isotopic anomalies in the solar system than originally thought.

astro-ph.EP↗

Mesosiderite formation on asteroid 4 Vesta by a hit-and-run collision

Collision and disruption processes of proto-planetary bodies in the early solar system are key to understanding the genesis of diverse types of main-belt asteroids. Mesosiderites are stony-iron meteorites that formed by mixing of howardite-eucrite-diogenite-like crust and molten core materials and provide unique insights into the catastrophic break-up of differentiated asteroids. However, the enigmatic formation process and the poorly constrained timing of metal-silicate mixing complicate the assignment to potential parent bodies. Here we report high-precision uranium-lead dating of mesosiderite zircons by isotope dilution thermal ionization mass spectrometry, revealing initial crust formation 4,558.5 +/- 2.1 million years ago and metal-silicate mixing at 4,525.39 +/- 0.85 million years. The two distinct ages coincide with the timing of crust formation and a large-scale reheating event on the eucrite parent body, likely the asteroid Vesta. This chronological coincidence corroborates that Vesta is the parent body of mesosiderite silicates. Mesosiderite formation on Vesta can be explained by a hit-and-run collision 4,525.4 million years ago that caused the thick crust observed by NASA's Dawn mission and explains the missing olivine in mesosiderites, howardite-eucrite-diogenite meteorites, and vestoids.

astro-ph.EP↗

The Sariçiçek howardite fall in Turkey: Source crater of HED meteorites on Vesta and impact risk of Vestoids

The Sariçiçek howardite meteorite shower consisting of 343 documented stones occurred on 2 September 2015 in Turkey and is the first documented howardite fall. Cosmogenic isotopes show that Sariçiçek experienced a complex cosmic ray exposure history, exposed during ~12-14 Ma in a regolith near the surface of a parent asteroid, and that an ca.1 m sized meteoroid was launched by an impact 22 +/- 2 Ma ago to Earth (as did one third of all HED meteorites). SIMS dating of zircon and baddeleyite yielded 4550.4 +/- 2.5 Ma and 4553 +/- 8.8 Ma crystallization ages for the basaltic magma clasts. The apatite U-Pb age of 4525 +/- 17 Ma, K-Ar age of ~3.9 Ga, and the U,Th-He ages of 1.8 +/- 0.7 and 2.6 +/- 0.3 Ga are interpreted to represent thermal metamorphic and impact-related resetting ages, respectively. Petrographic, geochemical and O-, Cr- and Ti- isotopic studies confirm that Sariçiçek belongs to the normal clan of HED meteorites. Petrographic observations and analysis of organic material indicate a small portion of carbonaceous chondrite material in the Sariçiçek regolith and organic contamination of the meteorite after a few days on soil. Video observations of the fall show an atmospheric entry at 17.3 +/- 0.8 kms-1 from NW, fragmentations at 37, 33, 31 and 27 km altitude, and provide a pre-atmospheric orbit that is the first dynamical link between the normal HED meteorite clan and the inner Main Belt. Spectral data indicate the similarity of Sariçiçek with the Vesta asteroid family spectra, a group of asteroids stretching to delivery resonances, which includes (4) Vesta. Dynamical modeling of meteoroid delivery to Earth shows that the disruption of a ca.1 km sized Vesta family asteroid or a ~10 km sized impact crater on Vesta is required to provide sufficient meteoroids <4 m in size to account for the influx of meteorites from this HED clan.

astro-ph.EP↗

Bifurcation of planetary building blocks during Solar System formation

Geochemical and astronomical evidence demonstrate that planet formation occurred in two spatially and temporally separated reservoirs. The origin of this dichotomy is unknown. We use numerical models to investigate how the evolution of the solar protoplanetary disk influenced the timing of protoplanet formation and their internal evolution. Migration of the water snow line can generate two distinct bursts of planetesimal formation that sample different source regions. These reservoirs evolve in divergent geophysical modes and develop distinct volatile contents, consistent with constraints from accretion chronology, thermo-chemistry, and the mass divergence of inner and outer Solar System. Our simulations suggest that the compositional fractionation and isotopic dichotomy of the Solar System was initiated by the interplay between disk dynamics, heterogeneous accretion, and internal evolution of forming protoplanets.

astro-ph.EP↗