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Marie Barthelemy

Publications and source records attributed to Marie Barthelemy.

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Technical design report of a complete and compact broadband high-harmonics femtosecond beamline based on a modular hollow waveguide for photons generation centered on the upper region of the extreme ultraviolet spectral range

We have successfully developed and implemented an entire and compact table-top high-order harmonics generation (HHG) setup from monochromatic and intense femtosecond ($10^{-15}$ s) laser pulses launched in a target composed of a high-purity monoatomic noble gas specie, which can be Argon or Helium, distinctively. Its frequency arrangement is distributed both in the full eXtreme UltraViolet (XUV, $22-124$ eV) spectral region and in the bottom part of the Soft-X Ray range (SXR, $124-132$ eV), at once. Specifically, the core of this coherent secondary light source is based solely on a homemade, modular, affordable, though sturdy, design. We take advantage of this opportunity to present our design guidance of the XUV generation from a hollow capillary waveguide apparatus, and our simple recipe regarding the alignment process of the latter, which is easily carried out thanks to our adjustable design. Then, a comprehensive description of our entire XUV beamline is described, and participate in adding essential contents to the existing literature. Concurrently, we conducted theoretical studies, in order to anticipate or explain our experimental results. Overall, we found very good consistency between the experimental and cost-effective time-consuming numerical results. Finally, our setup provides very good vacuum performance under high gas load pressures, to a few atmospheres. All of these attributes fulfill the requirements regarding ultrafast time-resolved pump-probe configuration in table-top element-sensitive spectroscopy of complex and integrated optoelectronic devices made of magnetic materials.

physics.optics

Robust coherent dynamics of homogeneously limited anisotropic excitons in two-dimensional layered ReS2

The discovery of in-plane anisotropic excitons in two-dimensional layered semiconductors enables state-of-the-art nanophotonic applications. A fundamental yet unknown parameter of these quasiparticles is the coherence time (T_2 ), which governs the quantum dephasing timescale, over which the coherent superposition of excitons can be maintained and manipulated. Here, we report the direct measurement of T_2 within the sub-picosecond range, along with multiple population decay timescales (T_1 ) at resonance for anisotropic excitons in pristine layered rhenium disulfide (ReS2). We observe a notable weak dependence on layer thickness for T_2 , and a quasi-independence for T_1 . The excitonic coherence in few-layer ReS2 exhibits exceptional robustness against optical density and temperature compared to other two-dimensional semiconductors, enabling quantum features even at room temperature. No photon echo fingerprints were observed in pristine ReS2, highlighting the homogeneous character of the anisotropic excitonic transitions and a particularly low level of disorder in exfoliated flakes. Lastly, our results for mono- to bulk-like ReS2 support a direct gap band structure regardless their layer thickness, addressing the ongoing discussion about its nature.

cond-mat.mes-hall