arXiv subjects

Marie Houssin

Publications and source records attributed to Marie Houssin.

17 recordsLinked to original sources

arXiv2020

An analytical approach to symmetry breaking in multipole RF-traps

Radio-frequency linear multipole traps have been shown to be very sensitive to mis-positioning of their electrodes, which results in a symmetry breaking and leads to extra local minima in the trapping potential \cite{pedregosa17} disturbing the operation of the trap. In this work, we analytically describe the RF-potential of a realistic octupole trap by including lower order terms to the well-established equation for a perfectly symmetric octupole trap. We describe the geometry by a combination of identified defects, characterised by simple analytical expressions. A complete equation is proposed for a trap with any electrode deviation relying on a combination of the simple cases where the defects are taken individually. Our approach is validated by comparison between analytical and numerical results for defect sizes up to 4\% of the trap radius. As described in \cite{pedregosa18}, an independent fine-tuning of the amplitude of the RF voltage applied on each electrode can be used to mitigate the geometrical defects of a realistic trap. In a different way than in \cite{pedregosa18}, the knowledge of an analytical equation for the potential allows to design the set of RF-voltages required for this compensation, based on the experimental measurement of the ion position in the trap, without information concerning the exact position of each electrode, and with a small number of iterations. The requirements, performances and limitations of this protocol are discussed via comparison of numerical simulations and analytical results.

quant-ph↗

arXiv2019

Experimental Demonstration of a Terahertz Frequency Reference based on Coherent Population Trapping

A novel protocol of interrogation based on coherent population trapping in an N-level scheme atomic system leads to dark resonances involving three different photons. An ensemble of several hundreds of radiofrequency-trapped ions is probed by three lasers simultaneously locked onto the same optical frequency comb, resulting in high-contrast spectral lines referenced to an atomic transition in the THz domain. We discuss the cause of uncertainties and limitations for this method and show that reaching a sub-kHz resolution is experimentally accessible via this interrogation protocole.

quant-ph↗

arXiv2018

Phase transfer between three visible lasers for coherent population trapping

Stringent conditions on the phase relation of multiple photons are a prerequisite for novel protocols of high-resolution coherent spectroscopy. In a recent experiment we have implemented an interrogation process of a Ca$^+$-ion cloud based on three-photon coherent population trapping, with the potential to serve as a frequency reference in the THz-range. This high-resolution interrogation has been made possible by phase-locking both laser sources for cooling and repumping of the trapped ions to a clock laser at 729~nm by means of an optical frequency comb. The clock laser, a titanium-sapphire laser built in our lab locked onto two high-finesse cavities reaches a linewidth of a few Hertz and a frequency stability below 10$^{-14}$ at one second, performances which can be copied onto the two other sources. In this paper we discuss the performances of the phase-transfer between the three involved lasers via the optical frequency comb.

physics.atom-ph↗

arXiv2017

Symmetry breaking in linear multipole traps

Radiofrequency multipole traps have been used for some decades in cold collision experiments, and are gaining interest for precision spectroscopy due to their low mi-cromotion contribution, and the predicted unusual cold-ion structures. However, the experimental realisation is not yet fully controlled, and open questions in the operation of these devices remain. We present experimental observations of symmetry breaking of the trapping potential in a macroscopic octupole trap with laser-cooled ions. Numerical simulations have been performed in order to explain the appearance of additional local potential minima, and be able to control them in a next step. We characterize these additional potential minima, in particular with respect to their position, their potential depth and their probability of population as a function of the radial and angular displacement of the trapping rods.

physics.atom-ph↗

arXiv2016

Noise characterization of an Optical Frequency Comb using Offline Cross-Correlation

Using an offline cross-correlation technique, we have analyzed the noise behavior of a new type of optical frequency comb (OFC), which is carrier envelope offset (CEO) free by configuration, due to difference frequency generation. In order to evaluate the instrument's ultimate noise floor, the phase and amplitude noise of a stabilized OFC are measured simultaneously using two analog-to-digital converters. Carrier recovery and phase detection are done by post-processing, eliminating the need for external phase-locked loops and complex calibration techniques. In order to adapt the measurement noise floor and the number of averages used in cross correlation, an adaptive frequency resolution for noise measurement is applied. Phase noise results are in excellent agreement with measurements of the fluctuations of the repetition frequency of the OFC obtained from optical signal.

physics.ins-det↗

arXiv2016

Experimental demonstration of an efficient number diagnostic for long 1D ion chains

Very long, one-dimensional (1D) ion chains are the basis for many applications, in particular in quantum information processing and reliable diagnostics are needed to quantify them. To that purpose, we have experimentally validated Dubin's model for very long ion chains [Phys. Rev. Lett. 71, 2753 (1993)]. This diagnostic allows to precisely determine the number of trapped ion with an accuracy of almost 1\% without counting them, by measuring the ion-ion distance of the innermost particles, as well as the trapping potential along the ion chain direction. In our experiment, based on a 155 ion chain, the central 30 ions are measured to be equidistant to better than 2\%, and we can determine the total number of trapped ions with a 4.5\% uncertainty, completely dominated by a conservative estimation of the experimental characterisation of the trap.

quant-ph↗

arXiv2015

Fast and efficient transport of large ion clouds

The manipulation of trapped charged particles by electric fields is an accurate, robust and reliable technique for many applications or experiments in high-precision spectroscopy. The transfer of the ion sample between multiple traps allows the use of a tailored environment in quantum information, cold chemistry, or frequency metrology experiments. In this article, we experimentally study the transport of ion clouds of up to 50 000 ions. The design of the trap makes ions very sensitive to any mismatch between the assumed electric potential and the actual local one. Nevertheless, we show that being fast (100 $\mu$s to transfer over more than 20 mm) increases the transport efficiency to values higher than 90 %, even with a large number of ions. For clouds of less than 2000 ions, a 100 % transfer efficiency is observed.

physics.plasm-ph↗

arXiv2013

Coherent internal state transfer by three-photon STIRAP-like scheme for many-atom samples

A STIRAP-like scheme is proposed to exploit a three-photon resonance taking place in alkaline-earth-metal ions. This scheme is designed for state transfer between the two fine structure components of the metastable D-state which are two excited states that can serve as optical or THz qu-bit. The advantage of a coherent three-photon process compared to two-photon STIRAP lies in the possibility of exact cancellation of the first order Doppler shift which opens the way for an application to a sample composed of many ions. The transfer efficiency and its dependence with experimental parameters are analyzed by numerical simulations. This efficiency is shown to reach a fidelity as high as $(1-8.10^{-5})$ with realistic parameters. The scheme is also extended to the synthesis of a linear combination of three stable or metastable states.

quant-ph↗

arXiv2013

A double ion trap for large Coulomb crystals

While the linear radiofrequency trap finds various applications in high-precision spectroscopy and quantum information, its higher-order cousin, the linear multipole trap, is almost exclusively employed in physical chemistry. Recently, first experiments have shown interesting features by laser-cooling multipole-trapped ion clouds. Multipole traps show a flatter potential in their centre and therefore a modified density distribution compared to quadrupole traps. Micromotion is an important issue and will certainly influence the dynamics of crystallized ion structures. Our experiment tends to investigate possible crystallization processes in the multipole. In a more general way, we are interested in the study of the dynamics and thermodynamics of large ion clouds in traps of different geometry.

physics.atom-ph↗

arXiv2010

An ion ring in a linear multipole trap for optical frequency metrology

A ring crystal of ions trapped in a linear multipole trap is studied as a basis for an optical frequency standard. The equilibrium conditions and cooling possibilities are discussed through an analytical model and molecular dynamics simulations. A configuration which reduces the frequency sensitivity to the fluctuations of the number of trapped ions is proposed. The systematic shifts for the electric quadrupole transition of calcium ions are evaluated for this ring configuration. This study shows that a ring of 10 or 20 ions allows to reach a short term stability better than for a single ion without introducing limiting long term fluctuations.

quant-ph↗

arXiv2010

Anharmonic contributions in real RF linear quadrupole traps

The radiofrequency quadrupole linear ion trap is a widely used device in physics and chemistry. When used for trapping of large ion clouds, the presence of anharmonic terms in the radiofrequency potential limits the total number of stored ions. In this paper, we have studied the anharmonic content of the trapping potential for different implementations of a quadrupole trap, searching for the geometry best suited for the trapping of large ion clouds. This is done by calculating the potential of a real trap using SIMION8.0, followed by a fit, which allows us to obtain the evolution of anharmonic terms for a large part of the inner volume of the trap.

physics.ins-det↗

arXiv2008

Two-step Doppler cooling of a three-level ladder system with an intermediate metastable level

Doppler laser cooling of a three-level ladder system using two near-resonant laser fields is analyzed in the case of the intermediate level being metastable while the upper level is short-lived. Analytical as well as numerical results for e.g. obtainable scattering rates and achievable temperatures are presented. When appropriate, comparisons with two-level single photon Doppler laser cooling is made. These results are relevant to recent experimental Doppler laser cooling investigations addressing intercombination lines in alkali-earth metal atoms and quadrupole transitions in alkali-earth metal ions.

quant-ph↗

arXiv2007

Terahertz frequency standard based on three-photon coherent population trapping

A scheme for a THz frequency standard based on three-photon coherent population trapping in stored ions is proposed. Assuming the propagation directions of the three lasers obey the phase matching condition, we show that stability of few 10$^{-14}$ at one second can be reached with a precision limited by power broadening to $10^{-11}$ in the less favorable case. The referenced THz signal can be propagated over long distances, the useful information being carried by the relative frequency of the three optical photons.

quant-ph↗

arXiv2005

Comment on "Prospect of optical frequency standard based on a 43Ca+ ion"

A recent evaluation of the frequency uncertainty expected for an optical frequency standard based on a single trapped $^{43}$Ca$^+$ ion was published in Phys. Rev. A {\bf 72} (2005) 043404. The paper contains some interesting information like systematic frequency shifts but fails to depict their uncertainty, leading to confuse accuracy and precision. The conclusions about the major contribution to the frequency shift are not consistent with the presented calculations and omit comparisons with data published previously.

physics.atom-ph↗

arXiv2005

Long-term stabilization of the length of an optical reference cavity

To obtain a high degree of long-term length stabilisation of an optical reference cavity, its free-spectral range is locked by means of an accurate and stable frequency synthesizer. The locking scheme is twofold: a laser is locked on the N$^{th}$ mode of a reference Fabry-Perot cavity and part of the laser light is shifted in frequency to be in resonance with the (N+1)$^{th}$ mode of the cavity. This shift is generated by an acousto-optical modulator (AOM) mounted in a double-pass scheme, matching half of the free spectral range of the reference cavity. The resulting absolute stabilization of the length of the cavity reaches the 10$^{-11}$ level per second, limited by the lock transfer properties and the frequency stability of the AOM control synthesizer.

physics.atom-ph↗

arXiv2004

Evaluation of the ultimate performances of a Ca+ single-ion frequency standard

We numerically evaluate the expected performances of an optical frequency standard at 729 nm based on a single calcium ion. The frequency stability is studied through the Allan deviation and its dependence on the excitation method (single Rabi pulse or two Ramsey pulses schemes) and the laser linewidth are discussed. The minimum Allan deviation that can be expected is estimated to $σ_y(τ) \approx 2.5\times 10^{-15}/\sqrtτ$ with $τ$ the integration time. The frequency shifts induced by the environmental conditions are evaluated to minimize the uncertainty of the proposed standard by chosing the most suited environment for the ion. If using the odd isotope $^{43}$Ca$^{+}$ and a vessel cooled to 77 K, the expected relative shift is $-2 \times 10^{-16}$ with an uncertainty of $\pm 4\times10^{-16}$, mainly due to the quadrupole shift induced by the unknown static electric field gradient .

physics.atom-ph↗

arXiv2004

Metastable level lifetimes from electron-shelving measurements with ion clouds and single ions

The lifetime of the 3d^2D_5/2-level in singly-ionized calcium has been measured by the electron-shelving technique on different samples of rf trapped ions. The metastable state has been directly populated by exciting the dipole-forbidden 4S_1/2 - 3D_5/2 transition. In ion clouds, the natural lifetime of this metastable level has been measured to be (1095+-27) ms. For the single-ion case, we determined a lifetime of (1152+-20) ms. The 1sigma-error bars at the 2%-level have different origins for the two kinds of experiments: data fitting methods for lifetime measurements in an ion cloud and control of experimental parameters for a single ion. De-shelving effects are extensively discussed. The influence of differing approaches for the processing of the single-ion quantum jump data on the lifetime values is shown. Comparison with recent measurements shows excellent agreement when evaluated from a given method.

physics.atom-ph↗