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Marin Bukov

Publications and source records attributed to Marin Bukov.

At least 37 records · Page 2Linked to original sources

Geometric Floquet theory

We derive Floquet theory from quantum geometry. We identify quasienergy folding as a consequence of a broken gauge group of the adiabatic gauge potential $U(1){\mapsto}\mathbb{Z}$. Fixing instead the gauge freedom using the parallel-transport gauge uniquely decomposes Floquet dynamics into a purely geometric and a purely dynamical evolution. The dynamical average-energy operator provides an unambiguous sorting of the quasienergy spectrum, identifying a Floquet ground state and suggesting a way to define the filling of Floquet-Bloch bands. We exemplify the features of geometric Floquet theory using an exactly solvable XY model and a non-integrable kicked Ising chain. We elucidate the geometric origin of inherently nonequilibrium effects, like the $π$-quasienergy splitting in discrete time crystals or $π$-edge modes in anomalous Floquet topological insulators. The spectrum of the average-energy operator is a susceptible indicator for both heating and spatiotemporal symmetry-breaking transitions. Last, we demonstrate that the periodic lab frame Hamiltonian generates transitionless counterdiabatic driving for Floquet eigenstates. This work directly bridges seemingly unrelated areas of nonequilibrium physics.

quant-ph↗

Learning to stabilize nonequilibrium phases of matter with active feedback using partial information

We investigate the role of information in active feedback control of quantum many-body systems using reinforcement learning. Active feedback breaks detailed balance, enabling the engineering of steady states and dynamical phases of matter otherwise inaccessible in equilibrium. We train reinforcement learning agents using partial state information to prevent entanglement spreading in (1+1)-dimensional stabilizer circuits with up to 128 qubits. We find that, above a critical information threshold, learned near-optimal strategies are non-greedy, stochastic, and reduce volume-law entangled steady states to area-law scaling. The agents achieve this by placing a series of bottlenecks that induce pyramidal structures in the long-time spatial entanglement distribution, which effectively split the system and reduce the maximum accessible entanglement. Crucially, learned strategies are inherently out of equilibrium and require real-time active feedback; we find that the learned behavior cannot be replaced by simple human-designed control rules. This work establishes the foundations for classically implemented, information-driven individual control of many interacting quantum degrees of freedom, demonstrating the capabilities of reinforcement learning to stabilize and uncover novel critical properties of many-body nonequilibrium steady states.

quant-ph↗

Floquet-engineered Emergent Massive Nambu-Goldstone Modes

We present a general framework to implement massive Nambu-Goldstone quasi-particles in driven many-body systems. The underlying mechanism leverages an explicit Lie group structure imprinted into an effective Hamiltonian that governs the dynamics of slow degrees of freedom; the resulting emergent continuous symmetry is weakly explicitly broken, giving rise to a massive Nambu-Goldstone mode, with a spectral mass gap scaling linearly with the drive period. We discuss explicit and experimentally implementable realizations, such as Heisenberg-like spin models that support gapped spin-wave excitations. We provide a protocol to certify the existence of the massive Nambu-Goldstone mode from the dynamics of specific observables, and analyse the dispersion spectrum and their lifetime in the presence of weak explicit symmetry breaking.

quant-ph↗

Nanoscale engineering and dynamical stabilization of mesoscopic spin textures

Thermalization phenomena, while ubiquitous in quantum systems, have traditionally been viewed as obstacles to be mitigated. In this study, we demonstrate the ability, instead, to harness thermalization to dynamically engineer and stabilize structured quantum states in a mesoscopically large ensemble of spins. Specifically, we showcase the capacity to generate, control, stabilize, and read out 'shell-like' spin texture with interacting $ {}^{ 13}\mathrm{C}$ nuclear spins in diamond, wherein spins are polarized oppositely on either side of a critical radius. The texture spans several nanometers and encompasses many hundred spins. We capitalize on the thermalization process to impose a quasi-equilibrium upon the generated texture; as a result, it is highly stable, immune to spin diffusion, and endures over multiple-minute long periods -- over a million times longer than the intrinsic interaction scale of the spins. Additionally, the texture is created and interrogated without locally controlling or probing the nuclear spins. These features are accomplished using an electron spin as a nanoscale injector of spin polarization, and employing it as a source of spatially varying dissipation, allowing for serial readout of the emergent spin texture. Long-time stabilization is achieved via prethermalization to a Floquet-induced Hamiltonian under the electronic gradient field. Our work presents a new approach to robust nanoscale spin state engineering and paves the way for new applications in quantum simulation, quantum information science, and nanoscale imaging.

quant-ph↗

Engineering Hierarchical Symmetries

The capacity to custom tailor the properties of quantum matter and materials is a central requirement for enlarging their range of possible functionalities. A particularly promising route is the use of driving protocols to engineer specific desired properties with a high degree of control and flexibility. Here, we present such a program for the tunable generation of sequences of symmetries on controllable timescales. Concretely, our general driving protocol for many-body systems generates a sequence of prethermal regimes, each exhibiting a lower symmetry than the preceding one. We provide an explicit construction of effective Hamiltonians exhibiting these symmetries, which imprints emergent quasiconservation laws hierarchically, enabling us to engineer the respective symmetries and concomitant orders in nonequilibrium matter. We provide explicit examples, including spatiotemporal and topological phenomena, as well as a spin chain realizing the symmetry ladder $\text{SU(2)}{\rightarrow}\text{U(1)} {\rightarrow} \mathbb{Z}_2{\rightarrow} E$. Our results have direct applications in experiments with quantum simulators.

quant-ph↗

Counterdiabatic Driving for Periodically Driven Systems

Periodically driven systems have emerged as a useful technique to engineer the properties of quantum systems, and are in the process of being developed into a standard toolbox for quantum simulation. An outstanding challenge that leaves this toolbox incomplete is the manipulation of the states dressed by strong periodic drives. The state-of-the-art in Floquet control is the adiabatic change of parameters. Yet, this requires long protocols conflicting with the limited coherence times in experiments. To achieve fast control of nonequilibrium quantum matter, we generalize the notion of variational counterdiabatic driving away from equilibrium focusing on Floquet systems. We derive a nonperturbative variational principle to find local approximations to the adiabatic gauge potential for the effective Floquet Hamiltonian. It enables transitionless driving of Floquet eigenstates far away from the adiabatic regime. We discuss applications to two-level, Floquet band, and interacting periodically driven models. The developed technique allows us to capture nonperturbative photon resonances and obtain high-fidelity protocols that respect experimental limitations like the locality of the accessible control terms.

quant-ph↗

Probing topological phases in a perturbed Kane-Mele model via RKKY interaction: Application to monolayer jacutingaite Pt$_2$HgSe$_3$

Quantum spin Hall insulators (QSHIs) are promising for spintronics, leveraging strong spin-orbit coupling for efficient spin manipulation via electrical and optical methods, with potential applications in memory storage, quantum computing, and spin-based logic. While the Kane-Mele model effectively captures the low-energy physics of these materials, the impact of perturbations driving phase transitions is less well understood. Developing approaches to describe these phases is crucial. Here, we study the noncollinear Ruderman-Kittel-Kasuya-Yosida (RKKY) interaction between two magnetic impurities in a \textit{perturbed} Kane-Mele model with strong spin-orbit coupling, relevant to monolayer jacutingaite Pt$_2$HgSe$_3$ as a prominent QSHI. By analyzing RKKY interactions, we reveal distinct, relative (rather than absolute) signatures of the different phase transitions induced by static and dynamic perturbations based on their impact on magnetic impurities. We then employ these perturbations to switch between ferromagnetic and antiferromagnetic or clockwise and counterclockwise magnetic interactions for control processes. Our results offer a practical way to track topological phases via magnetic properties.

cond-mat.mes-hall↗

Adaptive Trotterization for time-dependent Hamiltonian quantum dynamics using piecewise conservation laws

Digital quantum simulation relies on Trotterization to discretize time evolution into elementary quantum gates. On current quantum processors with notable gate imperfections, there is a critical tradeoff between improved accuracy for finer timesteps, and increased error rate on account of the larger circuit depth. We present an adaptive Trotterization algorithm to cope with time-dependent Hamiltonians, where we propose a concept of piecewise "conserved" quantities to estimate errors in the time evolution between two (nearby) points in time; these allow us to bound the errors accumulated over the full simulation period. They reduce to standard conservation laws in the case of time-independent Hamiltonians, for which we first developed an adaptive Trotterization scheme [PRX Quantum 4, 030319]. We validate the algorithm for a time-dependent quantum spin chain, demonstrating that it can outperform the conventional Trotter algorithm with a fixed step size at a controlled error.

quant-ph↗

Reinforcement learning pulses for transmon qubit entangling gates

The utility of a quantum computer depends heavily on the ability to reliably perform accurate quantum logic operations. For finding optimal control solutions, it is of particular interest to explore model-free approaches, since their quality is not constrained by the limited accuracy of theoretical models for the quantum processor - in contrast to many established gate implementation strategies. In this work, we utilize a continuous-control reinforcement learning algorithm to design entangling two-qubit gates for superconducting qubits; specifically, our agent constructs cross-resonance and CNOT gates without any prior information about the physical system. Using a simulated environment of fixed-frequency, fixed-coupling transmon qubits, we demonstrate the capability to generate novel pulse sequences that outperform the standard cross-resonance gates in both fidelity and gate duration, while maintaining a comparable susceptibility to stochastic unitary noise. We further showcase an augmentation in training and input information that allows our agent to adapt its pulse design abilities to drifting hardware characteristics, importantly with little to no additional optimization. Our results exhibit clearly the advantages of unbiased adaptive-feedback learning-based optimization methods for transmon gate design.

quant-ph↗

Learning effective Hamiltonians for adaptive time-evolution quantum algorithms

Digital quantum simulation of many-body dynamics relies on Trotterization to decompose the target time evolution into elementary quantum gates operating at a fixed equidistant time discretization. Recent advances have outlined protocols enabling more efficient adaptive Trotter protocols, which have been shown to exhibit a controlled error in the dynamics of local observables and correlation functions. However, it has remained open to which extent the errors on the actual generator of the dynamics, i.e., the target many-body Hamiltonian, remain controlled. Here, we propose to use quantum Hamiltonian learning to numerically obtain the effective Hamiltonian and apply it on the recently introduced ADA-Trotter algorithm as a concrete demonstration. Our key observation is that deviations from the target generator remain bounded on all simulation times. This result suggests that the ADA-Trotter not only generates reliable digital quantum simulation of local dynamics, but also controllably approximates the global quantum state of the target system. Our proposal is sufficiently general and readily applicable to other adaptive time-evolution algorithms.

quant-ph↗

Experimental observation of a time rondeau crystal: Temporal Disorder in Spatiotemporal Order

Our understanding of phases of matter relies on symmetry breaking, one example being water ice whose crystalline structure breaks the continuous translation symmetry of space. Recently, breaking of time translation symmetry was observed in systems not in thermal equilibrium. The associated notion of time crystallinity has led to a surge of interest, raising the question about the extent to which highly controllable quantum simulators can generate rich and tunable temporal orders, beyond the conventional classification of order in static systems. Here, we investigate different kinds of partial temporal orders, stabilized by non-periodic yet structured drives, which we call rondeau order. Using a $^{13}$C-nuclear-spin diamond quantum simulator, we report the first experimental observation of a -- tunable degree of -- short-time disorder in a system exhibiting long-time stroboscopic order. This is based on a novel spin control architecture that allows us to implement a family of drives ranging from structureless via structured random to quasiperiodic and periodic drives. Leveraging a high throughput read-out scheme, we continuously observe the spin polarization over 105 pulses to probe rondeau order, with controllable lifetimes exceeding 4 seconds. Using the freedom in the short-time temporal disorder of rondeau order, we show the capacity to encode information in the response of observables. Our work broadens the landscape of observed nonequilibrium temporal order, paving the way for new applications harnessing driven quantum matter.

quant-ph↗

Spin high-harmonic generation through terahertz laser-driven phonons

In the realm of open quantum systems, steady states and high-harmonic generation (HHG) existing far from equilibrium have become core pillars of ultrafast science. Most solid-state research explores charge HHG with limited investigations into spin degrees of freedom. In this study, we theoretically address spin HHG in the steady state resulting from the terahertz laser-driven spin-phonon coupling in a dissipative dimerized spin-1/2 chain. Instead of directly driving spins using time-dependent magnetic fields, we employ the magnetophononic mechanism, where the laser first drives the lattice, and then the excited lattice subsequently drives the spins. We investigate the role of various model parameters for optimizing HHG. Increasing the laser's amplitude amplifies spin HHG beyond the perturbative regime, enhancing both harmonic amplitudes and orders. We find that configuring the drive frequency far below the spin band yields the highest harmonic order. Additionally, we provide a theory matching the numerical results under weak spin-phonon coupling and propose an experimental procedure to probe the emission spectrum of spin HHG.

cond-mat.str-el↗

Ultrafast dynamics of a fermion chain in a terahertz field-driven optical cavity

We study the effect of a terahertz field-driven single cavity mode for ultrafast control of a fermion chain with dissipation-induced nonlinearity and quadratic coupling to an infrared-active phonon mode. Without photon loss from the cavity, we uncover a first-order phase transition in the nonequilibrium steady state only for the lower phonon-polariton, accompanied by polaritons whose frequency response is asymmetric with respect to the photon frequency due to the direct laser-induced dressing effect on the photon. A weak laser field fails to induce the phase transition but renders the polaritons symmetrical. Finally, we show that sufficiently strong photon loss from the cavity eliminates the polaritons and the associated phase transition. The experimental feasibility of these phenomena is also proposed.

cond-mat.str-el↗

Beyond Fermi's golden rule with the statistical Jacobi approximation

Many problems in quantum dynamics can be cast as the decay of a single quantum state into a continuum. The time-dependent overlap with the initial state, called the fidelity, characterizes this decay. We derive an analytic expression for the fidelity after a quench to an ergodic Hamiltonian. The expression is valid for both weak and strong quenches, and timescales before finiteness of the Hilbert space limits the fidelity. It reproduces initial quadratic decay and asymptotic exponential decay with a rate which, for strong quenches, differs from Fermi's golden rule. The analysis relies on the statistical Jacobi approximation (SJA), which was originally applied in nearly localized systems, and which we here adapt to well-thermalizing systems. Our results demonstrate that the SJA is predictive in disparate regimes of quantum dynamics.

quant-ph↗

Prethermalization in periodically-driven nonreciprocal many-body spin systems

We analyze a new class of time-periodic nonreciprocal dynamics in interacting chaotic classical spin systems, whose equations of motion are conservative (phase-space-volume-preserving) yet possess no symplectic structure. As a result, the dynamics of the system cannot be derived from any time-dependent Hamiltonian. In the high-frequency limit, we find that the magnetization dynamics features a long-lived metastable plateau, whose duration is controlled by the fourth power of the drive frequency. However, due to the lack of an effective Hamiltonian, the prethermal state the system evolves into cannot be understood within the framework of the canonical ensemble. We propose a Hamiltonian extension of the system using auxiliary degrees of freedom, in which the original spins constitute an open yet nondissipative subsystem. This allows us to perturbatively derive effective equations of motion that manifestly display symplecticity breaking at leading order in the inverse frequency. We thus extend the notion of prethermal dynamics, observed in the high-frequency limit of periodically-driven systems, to nonreciprocal systems.

cond-mat.stat-mech↗

Quantum many-body Jarzynski equality and dissipative noise on a digital quantum computer

The quantum Jarzynski equality and the Crooks relation are fundamental laws connecting equilibrium processes with nonequilibrium fluctuations. They are promising tools to benchmark quantum devices and measure free energy differences. While they are well established theoretically and also experimental realizations for few-body systems already exist, their experimental validity in the quantum many-body regime has not been observed so far. Here, we present results for nonequilibrium protocols in systems with up to sixteen interacting degrees of freedom obtained on trapped ion and superconducting qubit quantum computers, which test the quantum Jarzynski equality and the Crooks relation in the many-body regime. To achieve this, we overcome present-day limitations in the preparation of thermal ensembles and in the measurement of work distributions on noisy intermediate-scale quantum devices. We discuss the accuracy to which the Jarzynski equality holds on different quantum computing platforms subject to platform-specific errors. The analysis reveals the validity of Jarzynski's equality in a regime with energy dissipation, compensated for by a fast unitary drive. This provides new insights for analyzing errors in many-body quantum simulators.

cond-mat.stat-mech↗

Laser-enhanced magnetism in SmFeO$_3$

To coherently enhance inherent weak magnetic interactions in rare-earth orthoferrite SmFeO$_3$ as a functional material for spintronic applications, we simulate the dissipative spin dynamics that are linearly and quadratically coupled to laser-driven infrared-active phonons. When linear coupling dominates, we discover a magnetophononic dynamical first-order phase transition in the nonequilibrium steady state which can inhibit strong enhancement of magnetic interactions. By contrast, when quadratic spin-phonon coupling dominates, no phase transition exists at experimentally relevant parameters. By utilizing a chirp protocol, the phase transition can be engineered, enabling stronger magnetic interactions. We also discuss the route for experimental observation of our results.

cond-mat.mtrl-sci↗

Nonequilibrium phononic first-order phase transition in a driven fermion chain

We study the direct laser drive of infrared-active phonons that are quadratically coupled to a spinless fermion chain. Feedback is incorporated by phonon dressing of the electronic dispersion, which enables effective non-linearities in the phonon dynamics. We uncover a first-order phase transition in the phononic steady state in which hysteretic effects allow either large or small phonon occupation depending on the drive protocol. We discuss the implications of these findings for probing phase transitions in real driven materials.

cond-mat.str-el↗