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Marin Soljačić

Publications and source records attributed to Marin Soljačić.

At least 91 records · Page 5Linked to original sources

Automated Discovery and Optimization of 3D Topological Photonic Crystals

Topological photonic crystals have received considerable attention for their ability to manipulate and guide light in unique ways. They are typically designed by hand based on careful analysis of their bands and mode profiles, but recent theoretical advances have revealed new and powerful insights into the connection between band symmetry, connectivity, and topology. Here we propose a combined global and local optimization framework that integrates a flexible symmetry-constrained level-set parameterization with standard gradient-free optimization algorithms to optimize topological photonic crystals, a problem setting where the objective function may be highly non-convex and non-continuous. Our framework can be applied to any symmetry-identifiable band topology, and we demonstrate its applicability to several prominent kinds of three-dimensional band topology, namely $Γ$-enforced nodal lines, Weyl points, and Chern insulators. Requiring no prior examples of topological photonic crystals or prior knowledge on the connection between structure and band topology, our approach indicates a path towards the automated discovery of novel topological photonic crystal designs.

physics.optics↗

Non-Abelian nonsymmorphic chiral symmetries

The Hofstadter model exemplifies a large class of physical systems characterized by particles hopping on a lattice immersed in a gauge field. Recent advancements on various synthetic platforms have enabled highly-controllable simulations of such systems with tailored gauge fields featuring complex spatial textures. These synthetic gauge fields could introduce synthetic symmetries that do not appear in electronic materials. Here, in an SU(2) non-Abelian Hofstadter model, we theoretically show the emergence of multiple nonsymmorphic chiral symmetries, which combine an internal unitary anti-symmetry with fractional spatial translation. Depending on the values of the gauge fields, the nonsymmorphic chiral symmetries can exhibit non-Abelian algebra and protect Kramer quartet states in the bulk band structure, creating general four-fold degeneracy at all momenta. These nonsymmorphic chiral symmetries protect double Dirac semimetals at zero energy, which become gapped into quantum confined insulating phases upon introducing a boundary. Moreover, the parity of the system size can determine whether the resulting insulating phase is trivial or topological. Our work indicates a pathway for creating topology via synthetic symmetries emergent from synthetic gauge fields.

cond-mat.mes-hall↗

Free-electron-light interactions in nanophotonics

When impinging on optical structures or passing in their vicinity, free electrons can spontaneously emit electromagnetic radiation, a phenomenon generally known as cathodoluminescence. Free-electron radiation comes in many guises: Cherenkov, transition, and Smith-Purcell radiation, but also electron scintillation, commonly referred to as incoherent cathodoluminescence. While those effects have been at the heart of many fundamental discoveries and technological developments in high-energy physics in the past century, their recent demonstration in photonic and nanophotonic systems has attracted a lot of attention. Those developments arose from predictions that exploit nanophotonics for novel radiation regimes, now becoming accessible thanks to advances in nanofabrication. In general, the proper design of nanophotonic structures can enable shaping, control, and enhancement of free-electron radiation, for any of the above-mentioned effects. Free-electron radiation in nanophotonics opens the way to promising applications, such as widely-tunable integrated light sources from x-ray to THz frequencies, miniaturized particle accelerators, and highly sensitive high-energy particle detectors. Here, we review the emerging field of free-electron radiation in nanophotonics. We first present a general, unified framework to describe free-electron light-matter interaction in arbitrary nanophotonic systems. We then show how this framework sheds light on the physical underpinnings of many methods in the field used to control and enhance free-electron radiation. Namely, the framework points to the central role played by the photonic eigenmodes in controlling the output properties of free-electron radiation (e.g., frequency, directionality, and polarization). [... see full abstract in paper]

physics.optics↗

DiffCSE: Difference-based Contrastive Learning for Sentence Embeddings

We propose DiffCSE, an unsupervised contrastive learning framework for learning sentence embeddings. DiffCSE learns sentence embeddings that are sensitive to the difference between the original sentence and an edited sentence, where the edited sentence is obtained by stochastically masking out the original sentence and then sampling from a masked language model. We show that DiffSCE is an instance of equivariant contrastive learning (Dangovski et al., 2021), which generalizes contrastive learning and learns representations that are insensitive to certain types of augmentations and sensitive to other "harmful" types of augmentations. Our experiments show that DiffCSE achieves state-of-the-art results among unsupervised sentence representation learning methods, outperforming unsupervised SimCSE by 2.3 absolute points on semantic textual similarity tasks.

cs.CL↗

Equivariant Contrastive Learning

In state-of-the-art self-supervised learning (SSL) pre-training produces semantically good representations by encouraging them to be invariant under meaningful transformations prescribed from human knowledge. In fact, the property of invariance is a trivial instance of a broader class called equivariance, which can be intuitively understood as the property that representations transform according to the way the inputs transform. Here, we show that rather than using only invariance, pre-training that encourages non-trivial equivariance to some transformations, while maintaining invariance to other transformations, can be used to improve the semantic quality of representations. Specifically, we extend popular SSL methods to a more general framework which we name Equivariant Self-Supervised Learning (E-SSL). In E-SSL, a simple additional pre-training objective encourages equivariance by predicting the transformations applied to the input. We demonstrate E-SSL's effectiveness empirically on several popular computer vision benchmarks, e.g. improving SimCLR to 72.5% linear probe accuracy on ImageNet. Furthermore, we demonstrate usefulness of E-SSL for applications beyond computer vision; in particular, we show its utility on regression problems in photonics science. Our code, datasets and pre-trained models are available at https://github.com/rdangovs/essl to aid further research in E-SSL.

cs.CV↗

Meta-Learning and Self-Supervised Pretraining for Real World Image Translation

Recent advances in deep learning, in particular enabled by hardware advances and big data, have provided impressive results across a wide range of computational problems such as computer vision, natural language, or reinforcement learning. Many of these improvements are however constrained to problems with large-scale curated data-sets which require a lot of human labor to gather. Additionally, these models tend to generalize poorly under both slight distributional shifts and low-data regimes. In recent years, emerging fields such as meta-learning or self-supervised learning have been closing the gap between proof-of-concept results and real-life applications of machine learning by extending deep-learning to the semi-supervised and few-shot domains. We follow this line of work and explore spatio-temporal structure in a recently introduced image-to-image translation problem in order to: i) formulate a novel multi-task few-shot image generation benchmark and ii) explore data augmentations in contrastive pre-training for image translation downstream tasks. We present several baselines for the few-shot problem and discuss trade-offs between different approaches. Our code is available at https://github.com/irugina/meta-image-translation.

cs.CV↗

Discovering Sparse Interpretable Dynamics from Partial Observations

Identifying the governing equations of a nonlinear dynamical system is key to both understanding the physical features of the system and constructing an accurate model of the dynamics that generalizes well beyond the available data. We propose a machine learning framework for discovering these governing equations using only partial observations, combining an encoder for state reconstruction with a sparse symbolic model. Our tests show that this method can successfully reconstruct the full system state and identify the underlying dynamics for a variety of ODE and PDE systems.

cs.LG↗

Location and topology of the fundamental gap in photonic crystals

The fundamental, or first, band gap is of unmatched importance in the study of photonic crystals. Here, we address precisely where this gap can be opened in the band structure of three-dimensional photonic crystals. Although strongly constrained by symmetry, this problem cannot be addressed directly with conventional band-symmetry analysis due to the existence of a photonic polarization vortex at zero frequency. We develop an approach for overcoming the associated symmetry singularity by incorporating fictitious, auxiliary longitudinal modes. Our strategy also enables us to extend recent developments in symmetry-based topological analysis to the fundamental gap of three-dimensional photonic crystals. Exploiting this, we systematically study the topology of the minimal fundamental gaps. This reveals the existence of topological gap-obstructions that push the fundamental gap higher than what a conventional analysis would suggest. Our work demonstrates that topology can play a crucial role in the opening of the fundamental photonic gap and informs future theoretical and experimental searches for conventional and topological band gaps in three-dimensional photonic crystals.

physics.optics↗

End-to-end metasurface inverse design for single-shot multi-channel imaging

We introduce end-to-end metaoptics inverse design for multi-channel imaging: reconstruction of depth, spectral and polarization channels from a single-shot monochrome image. The proposed technique integrates a single-layer metasurface frontend with an efficient Tikhonov reconstruction backend, without any additional optics except a grayscale sensor. Our method yields multi-channel imaging by spontaneous demultiplexing: the metaoptics front-end separates different channels into distinct spatial domains whose locations on the sensor are optimally discovered by the inverse-design algorithm. We present large-area metasurface designs, compatible with standard lithography, for multi-spectral imaging, depth-spectral imaging, and ``all-in-one'' spectro-polarimetric-depth imaging with robust reconstruction performance ($\lesssim 10\%$ error with 1\% detector noise). In contrast to neural networks, our framework is physically interpretable and does not require large training sets. It can be used to reconstruct arbitrary three-dimensional scenes with full multi-wavelength spectra and polarization textures.

physics.optics↗

A general framework for scintillation in nanophotonics

Bombardment of materials by high-energy particles (e.g., electrons, nuclei, X- and $γ$-ray photons) often leads to light emission, known generally as scintillation. Scintillation is ubiquitous and enjoys widespread applications in many areas such as medical imaging, X-ray non-destructive inspection, night vision, electron microscopy, and high-energy particle detectors. A large body of research focuses on finding new materials optimized for brighter, faster, and more controlled scintillation. Here, we develop a fundamentally different approach based on integrating nanophotonic structures into scintillators to enhance their emission. To start, we develop a unified and ab initio theory of nanophotonic scintillators that accounts for the key aspects of scintillation: the energy loss by high-energy particles, as well as the light emission by non-equilibrium electrons in arbitrary nanostructured optical systems. This theoretical framework allows us, for the first time, to experimentally demonstrate nearly an order-of-magnitude enhancement of scintillation, in both electron-induced, and X-ray-induced scintillation. Our theory also allows the discovery of structures that could eventually achieve several orders-of-magnitude scintillation enhancement. The framework and results shown here should enable the development of a new class of brighter, faster, and higher-resolution scintillators with tailored and optimized performances - with many potential applications where scintillators are used.

physics.optics↗

Observation of enhanced free-electron radiation from photonic flatband resonances

Flatbands emerge from a myriad of structures such as Landau levels, Lieb and Kagome lattices, linegraphs, and more recently moire superlattices. They enable unique properties including slow light in photonics, correlated phases in electronics, and supercollimation in both systems. Despite these intense parallel efforts, flatbands have never been shown to affect the core light-matter interaction between electrons and photons, which is limited by a dimensionality mismatch. Here, we reveal that a photonic flatband can overcome this mismatch between localized electrons and extended photons and thus remarkably boost their light-matter interaction. We design flatband resonances in a silicon-on-insulator photonic crystal slab to control and enhance the radiation emission from free electrons by tuning their trajectory and velocity. In particular, we record a 100-fold radiation enhancement from the conventional diffraction-enabled Smith-Purcell radiation, and show the potential of our approach to achieve $10^6$-fold enhancements and beyond. The enhancement also enables us to perform polarization shaping of free electron radiation from multiple flatbands and demonstrate an approach to measure photonic bands via angle-resolved electron-beam measurements. Our results suggest flatbands as ideal test beds for strong light-electron interaction in various systems, with particular relevance for efficient and compact free-electron light sources and accelerators.

physics.optics↗

Towards 3D-Printed Inverse-Designed Metaoptics

Optical metasurfaces have been heralded as the platform to integrate multiple functionalities in a compact form-factor, potentially replacing bulky components. A central stepping stone towards realizing this promise is the demonstration of multifunctionality under several constraints (e.g. at multiple incident wavelengths and/or angles) in a single device -- an achievement being hampered by design limitations inherent to single-layer planar geometries. Here, we propose a general framework for the inverse design of volumetric 3D metaoptics via topology optimization, showing that even few-wavelength thick devices can achieve high-efficiency multifunctionality. We embody our framework in multiple closely-spaced patterned layers of a low-index polymer. We experimentally demonstrate our approach with an inverse-designed 3d-printed light concentrator working at five different non-paraxial angles of incidence. Our framework paves the way towards realizing multifunctional ultra-compact 3D nanophotonic devices.

physics.optics↗

A Brewster route to Cherenkov detectors

The Cherenkov effect enables a valuable tool, known as the Cherenkov detector, to identify high-energy particles via the measurement of the Cherenkov cone. However, the sensitivity and momentum coverage of such detectors are intrinsically limited by the refractive index of the host material. Especially, identifying particles with energy above multiple gigaelectronvolts requires host materials with a near-unity refractive index, which are often limited to large and bulky gas chambers. Overcoming this fundamental material limit is important for future particle detectors yet remains a long-standing scientific challenge. Here, we propose a different paradigm for Cherenkov detectors that utilizes the broadband angular filter made from stacks of variable one-dimensional photonic crystals. Owing to the Brewster effect, the angular filter is transparent only to Cherenkov photons from a precise incident angle, and particle identification is achieved by mapping each Cherenkov angle to the peak-intensity position of transmitted photons in the detection plane. This unique property of the angular filter is exceptionally beneficial to Cherenkov detection as it enables the realization of a non-dispersive pseudo refractive index over the entire visible spectrum. Moreover, such a pseudo refractive index can be flexibly tuned to arbitrary values, including those close to unity. Our angular-selective Brewster paradigm offers a feasible solution to implement compact and highly sensitive Cherenkov detectors especially in beam lines and it can cover a wide momentum range using readily available dielectric materials.

physics.optics↗

Three-dimensional non-Abelian generalizations of the Hofstadter model: spin-orbit-coupled butterfly trios

We theoretically introduce and study a three-dimensional Hofstadter model with linearly varying non-Abelian gauge potentials along all three dimensions. The model can be interpreted as spin-orbit coupling among a trio of Hofstadter butterfly pairs since each Cartesian surface ($xy$, $yz$, or $zx$) of the model reduces to a two-dimensional non-Abelian Hofstadter problem. By evaluating the commutativity among arbitrary loop operators around all axes, we derive its genuine (necessary and sufficient) non-Abelian condition, namely, at least two out of the three hopping phases should be neither 0 nor $π$. Under different choices of gauge fields in either the Abelian or the non-Abelian regime, both weak and strong topological insulating phases are identified in the model.

cond-mat.mes-hall↗

Quantum Surface-Response of Metals Revealed by Acoustic Graphene Plasmons

A quantitative understanding of the electromagnetic response of materials is essential for the precise engineering of maximal, versatile, and controllable light--matter interactions. Material surfaces, in particular, are prominent platforms for enhancing electromagnetic interactions and for tailoring chemical processes. However, at the deep nanoscale, the electromagnetic response of electron systems is significantly impacted by quantum surface-response at material interfaces, which is challenging to probe using standard optical techniques. Here, we show how ultra-confined acoustic graphene plasmons (AGPs) in graphene--dielectric--metal structures can be used to probe the quantum surface-response functions of nearby metals, here encoded through the so-called Feibelman $d$-parameters. Based on our theoretical formalism, we introduce a concrete proposal for experimentally inferring the low-frequency quantum response of metals from quantum shifts of the AGPs' dispersion, and demonstrate that the high field confinement of AGPs can resolve intrinsically quantum mechanical electronic length-scales with subnanometer resolution. Our findings reveal a promising scheme to probe the quantum response of metals, and further suggest the utilization of AGPs as plasmon rulers with ångström-scale accuracy.

cond-mat.mes-hall↗

Two photon emission from superluminal and accelerating index perturbations

Sources of photons with controllable quantum properties such as entanglement and squeezing are desired for applications in quantum information, metrology, and sensing. However, fine-grained control over these properties is hard to achieve, especially for two-photon sources. Here, we propose a new mechanism for generating entangled and squeezed photon pairs using superluminal and/or accelerating modulations of the refractive index in a medium. By leveraging time-changing dielectric media, where quantum vacuum fluctuations of the electromagnetic field can be converted into photon pairs, we show that energy- and momentum-conservation in multi-mode systems give rise to frequency and angle correlations of photon pairs which are controlled by the trajectory of the index modulation. These radiation effects are two-photon analogues of Cherenkov and synchrotron radiation by moving charged particles such as free electrons. We find the particularly intriguing result that synchrotron-like radiation into photon pairs exhibits frequency correlations which can enable the realization of a heralded single photon frequency comb. We conclude with a general discussion of experimental viability, showing how solitons, ultrashort pulses, and nonlinear waveguides may enable pathways to realize this two-photon emission mechanism. For completeness, we discuss in the Supplementary Information how these effects, sensitive to the local density of photonic states, can be strongly enhanced using photonic nanostructures. As an example, we show that index modulations propagating near the surface of graphene produce entangled pairs of graphene plasmons with high efficiency, leading to additional experimental opportunities.

physics.optics↗

Casimir light in dispersive nanophotonics

Time-varying optical media, whose dielectric properties are actively modulated in time, introduce a host of novel effects in the classical propagation of light, and are of intense current interest. In the quantum domain, time-dependent media can be used to convert vacuum fluctuations (virtual photons) into pairs of real photons. We refer to these processes broadly as ``dynamical vacuum effects'' (DVEs). Despite interest for their potential applications as sources of quantum light, DVEs are generally very weak, providing many opportunities for enhancement through modern techniques in nanophotonics, such as using media which support excitations such as plasmon and phonon polaritons. Here, we present a theory of DVEs in arbitrary nanostructured, dispersive, and dissipative systems. A key element of our framework is the simultaneous incorporation of time-modulation and ``dispersion'' through time-translation-breaking linear response theory. We propose a highly efficient scheme for generating entangled surface polaritons based on time-modulation of the optical phonon frequency of a polar insulator. We show that the high density of states, especially in hyperbolic polaritonic media, may enable high-efficiency generation of entangled phonon-polariton pairs. More broadly, our theoretical framework enables the study of quantum light-matter interactions in time-varying media, such as spontaneous emission, and energy level shifts.

physics.optics↗

Control of quantum electrodynamical processes by shaping electron wavepackets

Fundamental quantum electrodynamical (QED) processes such as spontaneous emission and electron-photon scattering encompass a wealth of phenomena that form one of the cornerstones of modern science and technology. Conventionally, calculations in QED and in other field theories assume that incoming particles are single-momentum states. The possibility that coherent superposition states, i.e. "shaped wavepackets", will alter the result of fundamental scattering processes is thereby neglected, and is instead assumed to sum to an incoherent (statistical) distribution in the incoming momentum. Here, we show that free-electron wave-shaping can be used to engineer quantum interferences that alter the results of scattering processes in QED. Specifically, the interference of two or more pathways in a QED process (such as photon emission) enables precise control over the rate of that process. As an example, we apply our concept to Bremsstrahlung, a ubiquitous phenomenon that occurs, for instance, in X-ray sources for state-of-the-art medical imaging, security scanning, materials analysis, and astrophysics. We show that free electron wave-shaping can be used to tailor both the spatial and the spectral distribution of emitted photons, enhancing their directionality and monochromaticity, and adding more degrees of freedom that make emission processes like Bremsstrahlung more versatile. The ability to tailor the spatiotemporal attributes of photon emission via quantum interference provides a new degree of freedom in shaping radiation across the entire electromagnetic spectrum. More broadly, the ability to tailor general QED processes through the shaping of free electrons opens up new avenues of control in processes ranging from optical excitation processes (e.g., plasmon and phonon emission) in electron microscopy to free electron lasing in the quantum regime.

quant-ph↗