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Mario Cuoco

Publications and source records attributed to Mario Cuoco.

At least 19 recordsLinked to original sources

Raman signatures of a non-reciprocal magnetic phase transition in Ca$_2$RuO$_4$

The magnetic behavior of Ca$_2$RuO$_4$ represents a unique puzzle due to the interplay of strong electronic correlations, magneto-elastic interactions, and large spin-orbit coupling. At low temperatures, an anomalous Mott insulating state emerges, characterized by a complex antiferromagnetic order with a collective amplitude excitation of the magnetic moment which has been discussed in analogy with the Higgs mode. We report here evidence of a magnetic first-order phase transition driven by an out-of-plane magnetic field along the crystallographic $c$-axis of Ca$_2$RuO$_4$. Raman measurements in magnetic field reveal the emergence of mode of magnetic origin and a concomitant modification of the coupling between a phonon and the Higgs amplitude mode. Both the Raman features are characterized by a non-reciprocal hysteresis in magnetic field. Surprisingly, the observed phase transition does not affect the Raman scattering from the in-plane magnons, indicating that the dipolar antiferromagnetic order is preserved. This is consistent with the onset of a new quadrupolar field-controlled state, whose fluctuations structure can trigger an hybridization between the lattice and the magnetic Higgs mode resulting in the observed Raman features.

cond-mat.str-el

Spin selectivity induced by non-collinear spins in Rashba wires

We report a previously overlooked general mechanism to obtain highly efficient spin selectivity in conventional time-reversal symmetric one-dimensional systems without invoking phase decoherence. We reveal that Rashba quantum wires featuring non-collinear spin states at the Fermi level inherently possess spin-selective transport properties. We show that this spin noncollinearity can be systematically designed and engineered by introducing an additional pseudospin degree of freedom - such as valley, sublattice, or orbital angular momentum - into spin-orbit coupled systems. By applying this framework to multi-subband semiconducting quantum wires and oxide nanowires, we establish a generalized route toward quantum-coherent spin selectivity up to 10 %. Our findings offer practical design principles for spin-selective transport devices.

cond-mat.mes-hall

Transverse Magnetic Response from Orbitally Polarized Cooper Pairs in Elemental Superconductors

We demonstrate how crystalline symmetry lowering, as for instance through strain, allows elemental superconductors such as vanadium and niobium to realize spin-singlet orbitally polarized Cooper pairs composed of electrons with identical orbital moments. Using superconducting density functional theory, we show that lowering of trigonal symmetry to $C_s$, thus keeping only a single mirror plane, activates interorbital pairing in bulk and (111) surfaces, with a pronounced surface enhancement. In a magnetic field, the resulting orbitally polarized superconducting state leads to a novel transverse magnetic response. For in--plane field orientations that break the remaining mirror symmetry, a sizable orbital magnetization emerges perpendicular to the applied field. We show that this effect is a direct consequence of equal--orbital-moment Cooper pairing, providing an experimentally accessible signature of this state. Our results establish strained elemental superconductors as a minimal material platform for superconducting orbitronics.

cond-mat.supr-con

Curvature-induced nonlinear anomalous Hall effect in thin magnetic shells

Optoelectronic and nonlinear transport experiments probe the quantum geometric tensor of Bloch states, whose real and imaginary components -- the quantum metric and the Berry curvature -- are typically constrained by symmetry. Here, we show that geometric bending provides a route to engineer such responses in centrosymmetric ferromagnets. Curvature-induced strain gradients across the shell thickness break inversion symmetry and activate an orbital Rashba coupling. In the presence of in-plane magnetization and spin-orbit coupling, this generates spin textures with a nontrivial quantum geometry, leading to an intrinsic nonlinear anomalous Hall effect (NAHE) governed by the quantum metric and maximized when the magnetization aligns with the applied electric field. When geometric deformations further break twofold rotational symmetry around the out-of-plane axis, an additional NAHE emerges, maximal for magnetization perpendicular to the driving electric field and governed by the Berry curvature dipole, thus giving access to the imaginary component of the quantum geometric tensor. These results establish curved ferromagnetic shells as a platform for engineering anisotropic nonlinear transport and for selectively probing both components of the quantum geometric tensor.

cond-mat.mes-hall

A Kapitza Pendulum Route to Supercurrent Tunnel Diodes

Superconducting diodes that support nonreciprocal supercurrent flow in principle constitute attractive, non-dissipative, circuit elements for superconducting electronics. But their realization faces fundamental challenges, as conventional Josephson tunnel junctions are inherently reciprocal. Existing approaches to break reciprocity typically involve magnetism or spin-orbit coupling, which often increase device complexity and limit reproducibility. Here, we demonstrate an alternative dynamical route to supercurrent nonreciprocity based on parametric driving. By applying a frequency-modulated supercurrent amplitude we show that effective higher-order, nonharmonic terms are generated in the current-phase relation. Leveraging mathematical equivalences with the Kapitza pendulum, we show that these terms dynamically break reciprocity. This establishes the concept of a Kapitza supercurrent diode and demonstrates that nonreciprocal superconducting transport can be engineered by nonequilibrium driving conventional Josephson tunnel junctions. We propose two implementations of the Kapitza supercurrent diode - via gate-controlled superconducting interferometers or flux-driven double-loop SQUIDs - to achieve nonreciprocal supercurrent transport within experimentally accessible frequencies $\omega/2\pi \sim 1$-$10\,\mathrm{GHz}$.

cond-mat.supr-con

Competing magnetic states in a non-coplanar Kagome magnet

Non-collinear Kagome antiferromagnets (AFMs) Mn3X (X = Sn, Ga, Ge, Ir, Pt) can generate an anomalous Hall effect (AHE) despite vanishing net magnetization, enabled by broken time-reversal and inversion symmetries. However, strong in-plane anisotropy has limited studies of the AFM-AHE and electronic applications to coplanar spin configurations. Non-coplanar spin textures in these systems have been realized only in low temperature spin-glass states or at interfaces with heavy metals. Here, we report an intrinsic non-coplanar spin configuration persisting up to 400 K in cubic-phase Mn3Ge, originating from coexisting symmetric and antisymmetric exchange interactions. Competing magnetic states associated with this non-coplanar spin configuration give rise to an unconventional AHE with a magnetic-field-induced sign reversal and a hump-like feature. Our findings establish a platform for non-coplanar magnetism in AFM spintronics.

cond-mat.mtrl-sci

Unveiling Hidden Magnons with Anomalous Rotational Symmetry

Correlated materials with competing spin-orbit and crystal-field interactions can host composite spin-orbital magnons that are highly susceptible to structural and electronic perturbations, enabling the control of magnetic dynamics beyond spin-only physics. Using Raman spectroscopy on Ca$_2$RuO$_4$, we show that the partial substitution of Ru with Mn reconstructs the magnon spectrum and reveals one-magnon modes that are hidden in the undoped state. We demonstrate that the transition-metal substitution activates otherwise symmetry-forbidden magnon modes through mirror-symmetry breaking of the underlying spin-orbital configuration. This effect can be theoretically explained by the local structural distortions induced in the RuO$_6$ octahedra near the dopant, that enable the observation of mixed-parity one-magnon modes. These excitations display a distinctive polarization dependence, with a lowering from fourfold to twofold rotational symmetry arising from the mixed-parity character of the coupled magnons and interference between resonant and nonresonant scattering channels. Our results show that spin-orbit-lattice entanglement provides a route to tailoring collective magnetic excitations and their polarization response in spin-orbit-coupled correlated systems.

cond-mat.str-el

Probing the quantum metric of 3D topological insulators

The surface states of 3D topological insulators possess geometric structures that imprint distinctive signatures on electronic transport. A prime example is the Berry curvature, which controls, for instance, electric frequency doubling via its higher order moments. In addition to the Berry curvature, topological surface states are expected to exhibit a nontrivial quantum metric, which plays a key role in governing nonlinear magnetotransport. However, its manifestation has yet to be experimentally observed and controlled in 3D topological insulators. Here, we provide evidence for a nonlinear response activated by the quantum metric of the topological surface states of Sb$_2$Te$_3$. We measure a time-reversal odd, nonlinear magnetoresistance that is independent from the temperature and the scattering time below 30 K, and is thus of intrinsic geometrical origin. This quantum metric magnetoresistance can be controlled by tuning the contributions of the top and bottom topological surface states by voltage gating. Our measurements thus demonstrate the existence and tunability of quantum geometry-induced transport in topological phases of matter and provide strategies for designing novel functionalities in topological devices.

cond-mat.mes-hall

Inducing ferromagnetism by structural engineering in a strongly spin-orbit coupled oxide

Magnetic materials with strong spin-orbit coupling (SOC) are essential for the advancement of spin-orbitronic devices, as they enable efficient spin-charge conversion, complex magnetic structures, spin-valley physics, topological phases and other exotic phenomena. 5d transition-metal oxides such as SrIrO3 feature large SOC, but usually show paramagnetic behavior due to broad bands and a low density of states at the Fermi level, accompanied by a relatively low Coulomb repulsion. Here, we unveil ferromagnetism in 5d SrIrO3 thin films grown on SrTiO3 (111). Through substrate-induced structural engineering, a zigzag stacking of three-unit-cell thick layers along the [111] direction is achieved, stabilizing a ferromagnetic state at the interfaces. Magnetotransport measurements reveal an anomalous Hall effect below ~30 K and hysteresis in the Hall conductivity below 7 K, indicating ferromagnetic ordering. X-ray magnetic circular dichroism further supports these results. Theoretical analysis suggests that the structural engineering of the IrO6 octahedral network enhances the density of states at the Fermi level and thus stabilizes Stoner ferromagnetism. This work highlights the potential of structurally engineered 5d oxides for spin-orbitronic devices, where efficient control of SOC-induced magnetic phases by electric currents can lead to lower energy consumption and improved performance in next-generation device technologies.

cond-mat.mtrl-sci

Sign competing sources of Berry curvature and anomalous Hall conductance humps in topological ferromagnets

The use of Berry-phase concepts has established a strong link between the anomalous Hall effect (AHE) and the topological character of the Hall currents. However, the occurrence of sign competition in the Berry curvature often hinders the topological origin of the observed anomalous Hall effects. Here, we study a two-dimensional topological ferromagnet with coupled spin and orbital degrees of freedom to assess the anomalous Hall effects in the presence of sign-competing sources of Berry curvature. We show that 2D itinerant topological ferromagnets described by t2g electronic states can generally lead to topological metallic bands marked by a non-zero Chern number. We find that the resulting Berry curvature at the Fermi level exhibits a characteristic anisotropic profile with a non-monotonous angular dependence when the magnetization is reversed. The sign change of the intrinsic contribution to the anomalous Hall conductance can occur together with topological transitions or be driven by the population imbalance of the topological bands. The breaking of the inversion symmetry introduces the orbital Rashba coupling in the system. The interplay between the orbital Rashba and sign competing sources of Berry curvature leads to anomalies in the anomalous Hall conductance at values of magnetic fields for which the magnetization switches its orientation. The humps in topological ferromagnets arise when the anomalous Hall conductivity is small in absolute value and they can be detected only close to the sign-change of the AHE and far from half-filling. This study could be relevant for the family of the topological 2D ferromagnets as well as Weyl ferromagnets, and can particularly account for the variety of unconventional behaviors observed in ultrathin films of SrRuO$_3$.

cond-mat.str-el

Triplet superconductivity by the orbital Rashba effect at surfaces of elemental superconductors

It is often assumed that in a superconductor without spin-triplet pairing, the formation of unconventional spin-triplet densities requires the spin-orbit interaction in combination with either broken inversion symmetry or broken time-reversal symmetry. Here, we show from first principles the existence of supercurrent-driven spin triplet densities on the surface of a variety of simple superconducting materials without spin-orbit coupling. We are able to attribute this phenomenon to the superconducting non-relativistic orbital Rashba Edelstein effect. Furthermore, we find that the spin-orbit induced spin moment is one order of magnitude smaller than the orbital moment, and has a vanishing effect on the total magnitude of the induced triplet density. Our findings imply the existence of a route to generate spin-currents without the use of heavy metals. Additionally, as an orbital moment can couple directly to a magnetic field, it shows that orbital physics is the dominant term that drives the superconducting diode effect.

cond-mat.supr-con

Insulator-to-Metal Transition via Magnetic Reconstruction at Oxide Interfaces

Ultrathin two-dimensional (2D) electronic systems at the interfaces of layered materials are highly desirable platforms for exploring of novel quantum phenomena and developing advanced device applications. Here, we investigate ultrathin heterostructures composed of SrIrO3 (SIO) and SrRuO3 (SRO) layers to uncover their emergent properties. Strikingly, despite the fact that both individual layers are antiferromagnetic insulators, the interfaced heterostructure exhibits emergent metallicity. Through transport measurements, magnetic characterization, and angle-resolved photoemission spectroscopy (ARPES), we analyze the underlying mechanisms governing this insulator-to-metal transition. Our findings reveal that the transition is driven by interface-induced magnetic reconstruction, which is further corroborated by density functional theory (DFT) calculations. The staggered Dzyaloshinskii-Moriya interaction at the SIO/SRO interface is identified as the key driving force for this spin reorganization, as it stabilizes ferromagnetism in the coupled antiferromagnetic insulating layers. These findings highlight the significant potential of engineering interfacial magnetic interactions as a powerful approach to generate and control emergent electronic properties, paving the way for novel functionalities that are unattainable in individual ultrathin films.

cond-mat.mes-hall

Robust spin splitting and fermiology in a layered altermagnet

Altermagnetism defies conventional classifications of collinear magnetic phases, standing apart from ferromagnetism and antiferromagnetism with its unique combination of spin-dependent symmetries, net-zero magnetization, and anomalous Hall transport. Although altermagnetic states have been realized experimentally, their integration into functional devices has been hindered by the structural rigidity and poor tunability of existing materials. First, through cobalt intercalation of the superconducting 2H-NbSe$_2$ polymorph, we induce and stabilize a robust altermagnetic phase and using both theory and experiment, we directly observe the lifting of Kramers degeneracy. Additionally, we present spectroscopic insight into a previously hinted low-temperature phase, and provide evidence of its electronic origin. While shedding light on overlooked aspects of altermagnetism, these findings open pathways to spin-based technologies and lay a foundation for advancing the emerging field of altertronics.

cond-mat.str-el

Topological phase transitions in superconductors with chiral symmetry

We study topological transitions in one dimensional superconductors that can harbor multiple edge Majorana bound states protected by chiral symmetry. The chiral symmetry arises due to the structure of the internal spin degrees of freedom of the superconductor and it can be guided by the coupling of the superconductor with sources of time-reversal symmetry breaking. We then consider distinct regions of the phase diagram in the parameters space that are marked by gapless excitations in the spectrum and evaluate the conditions for inducing a topological transition. We show that for gapless chiral symmetric superconductors one can identify a class of physical perturbations that enable a gap opening in the spectrum, without breaking chirality, and turn the system into a topological state. This type of superconductor is dubbed marginal topological superconductor because an infinitesimally small perturbation is able to induce a transition into a topological nontrivial phase. To explicitly demonstrate and evaluate the character of the transitions from gapless to topological gapfull phases we explore different physical cases including p-wave superconductor in the presence of an applied magnetic field or proximity-coupled to a ferromagnet, and s-wave superconductor in a noncollinear magnetic ordering.

cond-mat.supr-con

Anomalous spin-optical helical effect in Ti-based kagome metal

The kagome lattice stands as a rich platform for hosting a wide array of correlated quantum phenomena, ranging from charge density waves and superconductivity to electron nematicity and loop current states. Direct detection of loop currents in kagome systems has remained a formidable challenge due to their intricate spatial arrangements and the weak magnetic field signatures they produce. This has left their existence and underlying mechanisms a topic of intense debate. In this work, we uncover a hallmark reconcilable with loop currents: spin handedness-selective signals that surpass conventional dichroic, spin, and spin-dichroic responses. We observe this phenomenon in the kagome metal CsTi$_3$Bi$_5$ and we call it the anomalous spin-optical helical effect. This effect arises from the coupling of light' s helicity with spin-orbital electron correlations, providing a groundbreaking method to visualize loop currents in quantum materials. Our discovery not only enriches the debate surrounding loop currents but also paves the way for new strategies to exploit the electronic phases of quantum materials via light-matter interaction.

cond-mat.str-el

Filtering Spin and Orbital Moment in Centrosymmetric Systems

The control of spin and orbital angular momentum without relying on magnetic materials is commonly accomplished by breaking of inversion symmetry, which enables charge-to-spin conversion and spin selectivity in electron transfer processes occurring in chiral media. In contrast to this perspective, we show that orbital moment filtering can be accomplished in centrosymmetric systems: the electron states can be selectively manipulated allowing for the preferential transfer of electrons with a particular orbital momentum orientation. We find that orbital moment filtering is indeed efficiently controlled through orbital couplings that break both mirror and rotational symmetries. We provide the symmetry conditions required for the electron transmission to achieve orbital filtering and relate them to the orientation of the orbital moment. The presence of atomic spin-orbit interaction in the centrosymmetric transmission medium leads to the selective filtering of spin and orbital moments. Our findings allow to identify optimal regimes for having highly efficient simultaneous spin and orbital moment filtering.

cond-mat.other

Imaging orbital Rashba induced charge transport anisotropy

Identifying orbital textures and their effects on the electronic properties of quantum materials is a critical element in developing orbitronic devices. However, orbital effects are often entangled with the spin degree of freedom, making it difficult to uniquely identify them in charge transport phenomena. Here, we present a combination of scanning superconducting quantum interference device (SQUID) current imaging, global transport measurements, and theoretical analysis, that reveals a direct contribution of orbital textures to the linear charge transport of 2D systems. Specifically, we show that in the LaAlO$_3$/SrTiO$_3$ interface, which lacks both rotation and inversion symmetries, an anisotropic orbital Rashba coupling leads to conductivity anisotropy in zero magnetic field. We experimentally demonstrate this result by locally measuring the conductivity anisotropy, and correlating its appearance to the non-linear Hall effect, showing that the two phenomena have a common origin. Our results lay the foundations for an all--electrical probing of orbital currents in two-dimensional systems.

cond-mat.mes-hall

Supercurrent Diode Effect in Josephson Interferometers with Multiband Superconductors

We investigate nonreciprocal supercurrent phenomena in superconducting quantum interference devices (SQUIDs) that integrate Josephson junctions with single and multiband order parameters, which may exhibit time-reversal symmetry breaking. Our results show that the magnetic field can independently control both the amplitude and direction of supercurrent rectification, depending on the multiband characteristics of the superconductors involved. We analyze the effects of zero and antiphase ({\pi}) pairing among different bands on the development of nonreciprocal effects and find that the rectification is not influenced by {\pi}-pairing. Furthermore, we demonstrate that incorporating multiband superconductors that break time-reversal symmetry produces significant signatures in rectification. The rectification exhibits an even parity dependence on the magnetic field and the average rectification amplitude across quantum flux multiples does not equal zero. These findings indicate that magnetic flux pumping can be accomplished with time-reversal symmetry broken multiband superconductors by adjusting the magnetic field. Overall, our findings provide valuable insights for identifying and utilizing phases with broken time-reversal symmetry in multiband superconductors.

cond-mat.supr-con