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Mario Krenn

Publications and source records attributed to Mario Krenn.

At least 73 records · Page 4Linked to original sources

Experimental High-Dimensional Entanglement by Path Identity

Versatile and high-brightness sources of high-dimensional entangled photon pairs are important for emerging quantum technologies such as secure quantum communication. Here, we experimentally demonstrate a new scalable method to create photon pairs carrying orbital angular momentum that are entangled in arbitrarily high dimensions. Our method relies on indistinguishable photon pairs created coherently in different sources. We demonstrate the creation of three-dimensionally entangled states and show how to incrementally increase the dimensionality of entanglement. The generated states retain their quality even in higher dimensions. In addition, the modular structure of our approach allows for generalization to various degrees of freedom and even implementation in integrated compact devices. We therefore expect that future quantum technologies and fundamental tests of nature in higher dimensions will benefit from this novel approach.

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Quantum Experiments and Graphs III: High-Dimensional and Multi-Particle Entanglement

Quantum entanglement plays an important role in quantum information processes, such as quantum computation and quantum communication. Experiments in laboratories are unquestionably crucial to increase our understanding of quantum systems and inspire new insights into future applications. However, there are no general recipes for the creation of arbitrary quantum states with many particles entangled in high dimensions. Here, we exploit a recent connection between quantum experiments and graph theory and answer this question for a plethora of classes of entangled states. We find experimental setups for Greenberger-Horne-Zeilinger states, W states, general Dicke states, and asymmetrically high-dimensional multipartite entangled states. This result sheds light on the producibility of arbitrary quantum states using photonic technology with probabilistic pair sources and allows us to understand the underlying technological and fundamental properties of entanglement.

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Quantum Experiments and Graphs II: Quantum Interference, Computation and State Generation

We present a conceptually new approach to describe state-of-the-art photonic quantum experiments using Graph Theory. There, the quantum states are given by the coherent superpositions of perfect matchings. The crucial observation is that introducing complex weights in graphs naturally leads to quantum interference. The new viewpoint immediately leads to many interesting results, some of which we present here. Firstly, we identify a new and experimentally completely unexplored multiphoton interference phenomenon. Secondly, we find that computing the results of such experiments is #P-hard, which means it is a classically intractable problem dealing with the computation of a matrix function Permanent and its generalization Hafnian. Thirdly, we explain how a recent no-go result applies generally to linear optical quantum experiments, thus revealing important insights to quantum state generation with current photonic technology. Fourthly, we show how to describe quantum protocols such as entanglement swapping in a graphical way. The uncovered bridge between quantum experiments and Graph Theory offers a novel perspective on a widely used technology, and immediately raises many follow-up questions.

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Arbitrary d-dimensional Pauli X-Gates of a flying Qudit

High-dimensional degrees of freedom of photons can encode more quantum information than their two-dimensional counterparts. While the increased information capacity has advantages in quantum applications (such as quantum communication), controlling and manipulating these systems has been challenging. Here we show a method to perform lossless arbitrary high-dimensional Pauli-X gates for single photon. The X-gate consists of a cyclic permutation of qudit basis vectors, and, together with the Z gate, forms the basis for performing arbitrary transformations. We propose an implementation of such gates on the orbital angular momentum of photons. The proposed experimental setups only use two basic optical elements such as mode-sorters and mode-shifters -- thus could be implemented in any system where these experimental tools are available. Furthermore the number of involved interferometers scales logarithmically with the dimension, which is important for practical implementation.

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Gouy Phase Radial Mode Sorter for Light: Concepts and Experiments

We present an in principle lossless sorter for radial modes of light, using accumulated Gouy phases. The experimental setups have been found by a computer algorithm, and can be intuitively understood in a geometric way. Together with the ability to sort angular-momentum modes, we now have access to the complete 2-dimensional transverse plane of light. The device can readily be used in multiplexing classical information. On a quantum level, it is an analog of the Stern-Gerlach experiment -- significant for the discussion of fundamental concepts in quantum physics. As such, it can be applied in high-dimensional and multi-photonic quantum experiments.

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On Small Beams with Large Topological Charge II: Photons, Electrons and Gravitational Waves

Beams of light with a large topological charge significantly change their spatial structure when they are focused strongly. Physically, it can be explained by an emerging electromagnetic field component in the direction of propagation, which is neglected in the simplified scalar wave picture in optics. Here we ask: Is this a specific photonic behavior, or can similar phenomena also be predicted for other species of particles? We show that the same modification of the spatial structure exists for relativistic electrons as well as for focused gravitational waves. However, this is for different physical reasons: For electrons, which are described by the Dirac equation, the spatial structure changes due to a Spin-Orbit coupling in the relativistic regime. In gravitational waves described with linearized general relativity, the curvature of space-time between the transverse and propagation direction leads to the modification of the spatial structure. Thus, this universal phenomenon exists for both massive and massless elementary particles with Spin 1/2, 1 and 2. It would be very interesting whether other types of particles such as composite systems (neutrons or C$_{60}$) or neutrinos show a similar behaviour and how this phenomenon can be explained in a unified physical way.

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Active learning machine learns to create new quantum experiments

How useful can machine learning be in a quantum laboratory? Here we raise the question of the potential of intelligent machines in the context of scientific research. A major motivation for the present work is the unknown reachability of various entanglement classes in quantum experiments. We investigate this question by using the projective simulation model, a physics-oriented approach to artificial intelligence. In our approach, the projective simulation system is challenged to design complex photonic quantum experiments that produce high-dimensional entangled multiphoton states, which are of high interest in modern quantum experiments. The artificial intelligence system learns to create a variety of entangled states, and improves the efficiency of their realization. In the process, the system autonomously (re)discovers experimental techniques which are only now becoming standard in modern quantum optical experiments - a trait which was not explicitly demanded from the system but emerged through the process of learning. Such features highlight the possibility that machines could have a significantly more creative role in future research.

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Quantum Experiments and Graphs: Multiparty States as coherent superpositions of Perfect Matchings

We show a surprising link between experimental setups to realize high-dimensional multipartite quantum states and Graph Theory. In these setups, the paths of photons are identified such that the photon-source information is never created. We find that each of these setups corresponds to an undirected graph, and every undirected graph corresponds to an experimental setup. Every term in the emerging quantum superposition corresponds to a perfect matching in the graph. Calculating the final quantum state is in the complexity class #P-complete, thus cannot be done efficiently. To strengthen the link further, theorems from Graph Theory -- such as Hall's marriage problem -- are rephrased in the language of pair creation in quantum experiments. We show explicitly how this link allows to answer questions about quantum experiments (such as which classes of entangled states can be created) with graph theoretical methods, and potentially simulate properties of Graphs and Networks with quantum experiments (such as critical exponents and phase transitions).

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Twisted Photons: New Quantum Perspectives in High Dimensions

Quantum information science and quantum information technology have seen a virtual explosion world-wide. It is all based on the observation that fundamental quantum phenomena on the individual particle or system-level lead to completely novel ways of encoding, processing and transmitting information. Quantum mechanics, a child of the first third of the 20th century, has found numerous realizations and technical applications, much more than was thought at the beginning. Decades later, it became possible to do experiments with individual quantum particles and quantum systems. This was due to technological progress, and for light in particular, the development of the laser. Hitherto, nearly all experiments and also nearly all realizations in the fields have been performed with qubits, which are two-level quantum systems. We suggest that this limitation is again mainly a technological one, because it is very difficult to create, manipulate and measure more complex quantum systems. Here, we provide a specific overview of some recent developments with higher-dimensional quantum systems. We mainly focus on Orbital Angular Momentum (OAM) states of photons and possible applications in quantum information protocols. Such states form discrete higher-dimensional quantum systems, also called qudits. Specifically, we will first address the question what kind of new fundamental properties exist and the quantum information applications which are opened up by such novel systems. Then we give an overview of recent developments in the field by discussing several notable experiments over the past 2-3 years. Finally, we conclude with several important open questions which will be interesting for investigations in the future.

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Experimental GHZ Entanglement beyond Qubits

The Greenberger-Horne-Zeilinger (GHZ) argument provides an all-or-nothing contradiction between quantum mechanics and local-realistic theories. In its original formulation, GHZ investigated three and four particles entangled in two dimensions only. Very recently, higher dimensional contradictions especially in three dimensions and three particles have been discovered but it has remained unclear how to produce such states. In this article we experimentally show how to generate a three-dimensional GHZ state from two-photon orbital-angular-momentum entanglement. The first suggestion for a setup which generates three-dimensional GHZ entanglement from these entangled pairs came from using the computer algorithm Melvin. The procedure employs novel concepts significantly beyond the qubit case. Our experiment opens up the possibility of a truly high-dimensional test of the GHZ-contradiction which, interestingly, employs non-Hermitian operators.

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Quantifying high dimensional entanglement with two mutually unbiased bases

We derive a framework for quantifying entanglement in multipartite and high dimensional systems using only correlations in two unbiased bases. We furthermore develop such bounds in cases where the second basis is not characterized beyond being unbiased, thus enabling entanglement quantification with minimal assumptions. Furthermore, we show that it is feasible to experimentally implement our method with readily available equipment and even conservative estimates of physical parameters.

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Quantum gate description for induced coherence without induced emission and related phenomena

We introduce unitary quantum gates for photon pair creation in spontaneous parametric down-conversion nonlinear crystals (NLs) and for photon path alignment. These are the two key ingredients for the method of "induced coherence without induced emission" and many ensuing variations thereof. The difficulty in doing so stems from an apparent mixing of the mode picture (such as the polarization of photons) and the Fock picture (such as the existence of the photons). We illustrate utility of these gates by obtaining quantum circuits for the experimental setups of the frustrated generation of photon pairs, identification of a point-like object with undetected photons, and creation of a Bell state. We also introduce an effective nonunitary description for the action of NLs in experiments where all the NLs are pumped coherently. As an example, by using this simplifying picture, we show how NLs can be used to create superposition of given quantum states in a modular fashion.

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Generation of the Complete Four-dimensional Bell Basis

The Bell basis is a distinctive set of maximally entangled two-particle quantum states that forms the foundation for many quantum protocols such as teleportation, dense coding and entanglement swapping. While the generation, manipulation, and measurement of two-level quantum states is well understood, the same is not true in higher dimensions. Here we present the experimental generation of a complete set of Bell states in a four-dimensional Hilbert space, comprising of 16 orthogonal entangled Bell-like states encoded in the orbital angular momentum of photons. The states are created by the application of generalized high-dimensional Pauli gates on an initial entangled state. Our results pave the way for the application of high-dimensional quantum states in complex quantum protocols such as quantum dense coding.

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High-Dimensional Single-Photon Quantum Gates: Concepts and Experiments

Transformations on quantum states form a basic building block of every quantum information system. From photonic polarization to two-level atoms, complete sets of quantum gates for a variety of qubit systems are well known. For multi-level quantum systems beyond qubits, the situation is more challenging. The orbital angular momentum modes of photons comprise one such high-dimensional system for which generation and measurement techniques are well-studied. However, arbitrary transformations for such quantum states are not known. Here we experimentally demonstrate a four-dimensional generalization of the Pauli X-gate and all of its integer powers on single photons carrying orbital angular momentum. Together with the well-known Z-gate, this forms the first complete set of high-dimensional quantum gates implemented experimentally. The concept of the X-gate is based on independent access to quantum states with different parities and can thus be easily generalized to other photonic degrees-of-freedom, as well as to other quantum systems such as ions and superconducting circuits.

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Entanglement by Path Identity

Quantum entanglement is one of the most prominent features of quantum mechanics and forms the basis of quantum information technologies. Here we present a novel method for the creation of quantum entanglement in multipartite and high-dimensional systems. The two ingredients are 1) superposition of photon pairs with different origins and 2) aligning photons such that their paths are identical. We explain the experimentally feasible creation of various classes of multiphoton entanglement encoded in polarization as well as in high-dimensional Hilbert spaces -- starting only from non-entangled photon pairs. For two photons, arbitrary high-dimensional entanglement can be created. The idea of generating entanglement by path identity could also apply to other quantum entities than photons. We discovered the technique by analyzing the output of a computer algorithm. This shows that computer designed quantum experiments can be inspirations for new techniques.

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Quantum communication with photons

The secure communication of information plays an ever increasing role in our society today. Classical methods of encryption inherently rely on the difficulty of solving a problem such as finding prime factors of large numbers and can, in principle, be cracked by a fast enough machine. The burgeoning field of quantum communication relies on the fundamental laws of physics to offer unconditional information security. Here we introduce the key concepts of quantum superposition and entanglement as well as the no-cloning theorem that form the basis of this field. Then, we review basic quantum communication schemes with single and entangled photons and discuss recent experimental progress in ground and space-based quantum communication. Finally, we discuss the emerging field of high-dimensional quantum communication, which promises increased data rates and higher levels of security than ever before. We discuss recent experiments that use the orbital angular momentum of photons for sharing large amounts of information in a secure fashion.

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Quantum optical rotatory dispersion

The phenomenon of molecular optical activity manifests itself as the rotation of the plane of linear polarization when light passes through chiral media. Measurements of optical activity and its wavelength dependence, optical rotatory dispersion, can reveal information about intricate properties of molecules, such as the 3D arrangement of atoms comprising a molecule. Given a limited probe power, quantum metrology offers the possibility to outperform classical measurements. This holds particular appeal when samples may be damaged by high powers, a potential concern for chiroptical studies. Here we show the first experiment in which multi-wavelength polarization-entangled photon pairs are used to measure the optical activity and optical rotatory dispersion exhibited by a solution of chiral molecules. Our work paves the way for quantum-enhanced measurements of chirality, with potential applications in chemistry, biology, materials science, and the pharmaceutical industry. The scheme we employ for probing the wavelength dependence allows to surpass the information extracted per photon in a classical measurement, and can also be used for more general differential measurements.

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Orbital angular momentum of photons and the entanglement of Laguerre-Gaussian modes

The identification of orbital angular momentum (OAM) as a fundamental property of a beam of light nearly twenty-five years ago has led to an extensive body of research around this topic. The possibility that single photons can carry OAM has made this degree of freedom an ideal candidate for the investigation of complex quantum phenomena and their applications. Research in this direction has ranged from experiments on complex forms of quantum entanglement to the interaction between light and quantum states of matter. Furthermore, the use of OAM in quantum information has generated a lot of excitement, as it allows for encoding large amounts of information on a single photon. Here we explain the intuition that led to the first quantum experiment with OAM fifteen years ago. We continue by reviewing some key experiments investigating fundamental questions on photonic OAM and the first steps into applying these properties in novel quantum protocols. In the end, we identify several interesting open questions that could form the subject of future investigations with OAM.

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