arXiv subjects

Mario Schwarz

Publications and source records attributed to Mario Schwarz.

7 recordsLinked to original sources

arXiv2026

Procurement and Purification of Liquid Argon for the LEGEND-200 Experiment

LEGEND-200 requires high-purity liquid argon for effective background discrimination. In this paper, we present the design, construction, and performance of a dedicated liquid argon purification system, along with the procurement and purification of liquid argon for filling the LEGEND-200 cryostat to its total capacity of 91 t. The purifier is based on copper catalyst and molecular sieve to remove oxygen and water. Starting with liquid argon of 5.5 quality, featuring an effective scintillation light triplet lifetime $\tau_t$ of about 0.9 $\mu$s, we achieved a final purity corresponding to $\tau_t$ = 1.3 $\mu$s. After complete filling of the LEGEND-200 cryostat, the measured effective triplet lifetime was 1.16 $\mu$s. The notable reduction is caused by a residual nitrogen impurity introduced by an accidentally spoiled liquid argon delivery. An excessive nitrogen influx was prevented by the LEGEND Liquid Argon Monitoring Apparatus (LLAMA), which served as one of the three independent purity monitors during the filling campaign.

physics.ins-det↗

arXiv2025

First operation of poly(ethylene naphthalate) enclosures for high-purity germanium detectors in liquid argon for $^{42}$K/$^{42}$Ar mitigation

Commercial argon contains cosmogenic $^{42}$Ar whose progeny $^{42}$K is a critical background component for the Large Enriched Germanium Experiment for Neutrinoless $\beta \beta$ Decay (LEGEND). LEGEND operates High-Purity Germanium (HPGe) detectors bare in liquid argon. $^{42}$K is attracted by the HPGe detectors' electric fields, and drifts toward the germanium surface, where it undergoes beta decay. LEGEND-1000 will mitigate $^{42}$K-induced background by using underground-sourced argon, depleted in cosmogenic isotopes. If underground argon is not available, mitigation techniques must be employed. Poly(ethylene naphthalate) (PEN) enclosures were proposed to hinder the ion drift, decrease the beta-particle's energy, and produce scintillation light. In this paper, we report on operating two HPGe detectors, both bare and PEN-enclosed, in $^{42}$Ar-enriched liquid argon, and find no evidence for deterioration of energy stability or resolution due to the enclosures. We monitor the beta and gamma rates of $^{42}$K, find complex time-dependencies extending to roughly 30 days after applying the HPGe detectors' high-voltage, and qualitatively demonstrate the $^{42}$K suppression capabilities of enclosures.

physics.ins-det↗

arXiv2025

$^{42}$Ar Production and Injection to a Liquid Argon Environment for Background Mitigation Studies

Atmosphere-sourced argon contains traces of $^{42}$Ar, whose $\beta^-$-decaying progeny $^{42}$K represents a significant intrinsic background for rare-event experiments using liquid argon (LAr) as detector or shielding medium. Understanding and mitigating this background is crucial for current and future large-scale detectors in neutrino and dark-matter physics. To enable controlled studies of $^{42}$K behavior and suppression techniques, $^{42}$Ar was produced by irradiating natural argon with 34 MeV $^{7}$Li$^{3+}$ ions at the Maier-Leibnitz-Laboratorium tandem accelerator, using beam currents of $101 \pm 5$ nA and $140 \pm 5$ nA, yielding $476 \pm 9$ Bq within two weeks, corresponding to a production rate of $\sim 1 \times 10^{6}$ atoms$\,$s$^{-1}$. The activated argon was injected into the one-ton SCARF cryostat, where two HPGe detectors monitored the subsequent $^{42}$K activity build-up. A time-dependent model describing $^{42}$Ar mixing and $^{42}$K equilibration in LAr yielded characteristic mixing time constants between one and two days. The established production and injection capability provides a reproducible platform for high-statistics $^{42}$K background studies, essential for developing and validating suppression strategies for next-generation LAr-based rare-event experiments such as LEGEND-1000.

physics.ins-det↗

arXiv2024

The MONUMENT Experiment: Ordinary Muon Capture studies for 0$\nu\beta\beta$ decay

The MONUMENT experiment measures ordinary muon capture (OMC) on isotopes relevant for neutrinoless double-beta (0$\nu\beta\beta$) decay and nuclear astrophysics. OMC is a particularly attractive tool for improving the theoretical description of 0$\nu\beta\beta$ decay. It involves similar momentum transfers and allows testing the virtual transitions involved in 0$\nu\beta\beta$ decay against experimental data. During the 2021 campaign, MONUMENT measured OMC on $^{76}$Se and $^{136}$Ba, the isotopes relevant for next-generation 0$\nu\beta\beta$ decay searches, like LEGEND and nEXO. The experimental setup has been designed to accurately extract the total and partial muon capture rates, which requires precise reconstruction of energies and time-dependent intensities of the OMC-related $\gamma$ rays. The setup also includes a veto counter system to allow selecting a clean sample of OMC events. This work provides a detailed description of the MONUMENT setup operated during the 2021 campaign, its two DAQ systems, calibration and analysis approaches, and summarises the achieved detector performance. Future improvements are also discussed.

nucl-ex↗

arXiv2023

A liquid-phase loop-mode argon purification system

Noble gas and liquid detectors rely on high chemical purity for successful operation. While gaseous purification has emerged as a reliable method of producing high-purity noble fluids, the requirement for large mass flows drives the development of liquid-phase purification. We constructed a medium-scale liquid argon (LAr) purification system based on a copper catalyst and 4 A molecular sieve capable of purifying 1 t of commercial LAr 5.0 to a long effective triplet lifetime of $\tau_3 \sim 1.3 \mu$s. We further demonstrate that a quenched effective triplet lifetime of $\tau_3 \sim 1 \mu$s, due to contamination by air, can be recovered in loop-mode purification to $\tau_3 \sim 1.3 \mu$s after > 20 volume exchanges.

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arXiv2019

Modeling of GERDA Phase II data

The GERmanium Detector Array (GERDA) experiment at the Gran Sasso underground laboratory (LNGS) of INFN is searching for neutrinoless double-beta ($0νββ$) decay of $^{76}$Ge. The technological challenge of GERDA is to operate in a "background-free" regime in the region of interest (ROI) after analysis cuts for the full 100$\,$kg$\cdot$yr target exposure of the experiment. A careful modeling and decomposition of the full-range energy spectrum is essential to predict the shape and composition of events in the ROI around $Q_{ββ}$ for the $0νββ$ search, to extract a precise measurement of the half-life of the double-beta decay mode with neutrinos ($2νββ$) and in order to identify the location of residual impurities. The latter will permit future experiments to build strategies in order to further lower the background and achieve even better sensitivities. In this article the background decomposition prior to analysis cuts is presented for GERDA Phase II. The background model fit yields a flat spectrum in the ROI with a background index (BI) of $16.04^{+0.78}_{-0.85} \cdot 10^{-3}\,$cts/(kg$\cdot$keV$\cdot$yr) for the enriched BEGe data set and $14.68^{+0.47}_{-0.52} \cdot 10^{-3}\,$cts/(kg$\cdot$keV$\cdot$yr) for the enriched coaxial data set. These values are similar to the one of Gerda Phase I despite a much larger number of detectors and hence radioactive hardware components.

nucl-ex↗

arXiv2018

Measurements of the Lifetime of Orthopositronium in the LAB-Based Liquid Scintillator of JUNO

Electron antineutrinos are detected in organic liquid scintillator based neutrino experiments by means of the inverse beta decay, producing both a positron and a neutron. The positron may form a bound state together with an electron, called positronium (Ps). The longer-lived spin state of Ps, orthopositronium (o-Ps) has a lifetime of about $3\,\mathrm{ns}$ in organic liquid scintillators (LS). Its formation changes the time distribution of photon emission, which affects positron reconstruction algorithms and allows the application of pulse shape discrimination (PSD) to distinguish electron from positron events. In this work, we measured the lifetime $τ_2$ of o-Ps in the linear alkylbenzene (LAB) based LS of the JUNO (Jiangmen Underground Neutrino Observatory) experiment including wavelength shifters, obtaining $τ_2 = 2.97\,\mathrm{ns} \pm 0.04\,\mathrm{ns}$. Due to systematics, which are not yet completely understood, we are not able to give a final result for the o-Ps formation probability $I_2$. We use a novel type of setup, which allows a better background suppression as compared to commonly used PALS (positron annihilation lifetime spectroscopy) measurements.

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