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Mark B. Lundeberg

Publications and source records attributed to Mark B. Lundeberg.

14 recordsLinked to original sources

Thermodynamic reciprocity in scanning photocurrent maps

Scanning photocurrent maps in inhomogeneous materials contain nontrivial patterns, which often can only be understood with a full model of device geometry and nonuniformities. We remark on the consequences of Onsager reciprocity to the photocurrent in linear response, with immediate applications in photovoltaic and photothermoelectric effects. In particular with photothermoelectric effects, we find that the ampere-per-watt responsivity is exactly governed by Peltier-induced temperature shifts in the same device when time-reversed and voltage-biased. We show, with the example of graphene, that this principle aids in understanding and modelling of photocurrent maps.

cond-mat.mes-hall

Dissociation of two-dimensional excitons in monolayer WSe2

Two-dimensional (2D) semiconducting materials are promising building blocks for optoelectronic applications, many of which require efficient dissociation of excitons into free electrons and holes. However, the strongly bound excitons arising from the enhanced Coulomb interaction in these monolayers suppresses the creation of free carriers. Here, we probe and identify the main exciton dissociation mechanism through time- and spectrally-resolved photocurrent measurements in a monolayer WSe2 p-n junction. We find that under static in-plane electric field, excitons dissociate at a rate corresponding to the one predicted for the tunnel ionization of 2D Wannier-Mott excitons. This study is essential for the understanding of the optoelectronic photoresponse in of 2D semiconductors, and offers design rules for the realization of efficient photodetectors, valley-dependent optoelectronics and novel quantum coherent phases.

cond-mat.mes-hall

Probing the Ultimate Plasmon Confinement Limits with a Van der Waals heterostructure

The ability to confine light into tiny spatial dimensions is important for applications such as microscopy, sensing and nanoscale lasers. While plasmons offer an appealing avenue to confine light, Landau damping in metals imposes a trade-off between optical field confinement and losses. We show that a graphene-insulator-metal heterostructure can overcome that trade-off, and demonstrate plasmon confinement down to the ultimate limit of the lengthscale of one atom. This is achieved by far-field excitation of plasmon modes squeezed into an atomically thin hexagonal boron nitride dielectric h-BN spacer between graphene and metal rods. A theoretical model which takes into account the non-local optical response of both graphene and metal is used to describe the results. These ultra-confined plasmonic modes, addressed with far-field light excitation, enables a route to new regimes of ultra-strong light-matter interactions.

cond-mat.mes-hall

Electrical 2π phase control of infrared light in a 350nm footprint using graphene plasmons

Modulating the amplitude and phase of light is at the heart of many applications such as wavefront shaping, transformation optics, phased arrays, modulators and sensors. Performing this task with high efficiency and small footprint is a formidable challenge. Metasurfaces and plasmonics are promising , but metals exhibit weak electro-optic effects. Two-dimensional materials, such as graphene, have shown great performance as modulators with small drive voltages. Here we show a graphene plasmonic phase modulator which is capable of tuning the phase between 0 and 2π in situ. With a footprint of 350nm it is more than 30 times smaller than the 10.6$μ$m free space wavelength. The modulation is achieved by spatially controlling the plasmon phase velocity in a device where the spatial carrier density profile is tunable. We provide a scattering theory for plasmons propagating through spatial density profiles. This work constitutes a first step towards two-dimensional transformation optics for ultra-compact modulators and biosensing.

physics.app-ph

Electrical detection of hyperbolic phonon-polaritons in heterostructures of graphene and boron nitride

Light properties in the mid-infrared can be controlled at a deep subwavelength scale using hyperbolic phonons-polaritons (HPPs) of hexagonal boron nitride (h-BN). While propagating as waveguided modes HPPs can concentrate the electric field in a chosen nano-volume. Such a behavior is at the heart of many applications including subdiffraction imaging and sensing. Here, we employ HPPs in heterostructures of h-BN and graphene as new nano-optoelectronic platform by uniting the benefits of efficient hot-carrier photoconversion in graphene and the hyperbolic nature of h-BN. We demonstrate electrical detection of HPPs by guiding them towards a graphene pn-junction. We shine a laser beam onto a gap in metal gates underneath the heterostructure, where the light is converted into HPPs. The HPPs then propagate as confined rays heating up the graphene leading to a strong photocurrent. This concept is exploited to boost the external responsivity of mid-infrared photodetectors, overcoming the limitation of graphene pn-junction detectors due to their small active area and weak absorption. Moreover this type of detector exhibits tunable frequency selectivity due to the HPPs, which combined with its high responsivity paves the way for efficient high-resolution mid-infrared imaging.

physics.app-ph

Ultra-confined acoustic THz graphene plasmons revealed by photocurrent nanoscopy

Terahertz (THz) fields are widely applied for sensing, communication and quality control. In future applications, they could be efficiently confined, enhanced and manipulated - well below the classical diffraction limit - through the excitation of graphene plasmons (GPs). These possibilities emerge from the strongly reduced GP wavelength, lp, compared to the photon wavelength, l0, which can be controlled by modulating the carrier density of graphene via electrical gating. Recently, GPs in a graphene-insulator-metal configuration have been predicted to exhibit a linear dispersion (thus called acoustic plasmons) and a further reduced wavelength, implying an improved field confinement, analogous to plasmons in two-dimensional electron gases (2DEGs) near conductive substrates. While infrared GPs have been visualised by scattering-type scanning near-field optical microscopy (s-SNOM), the real-space imaging of strongly confined THz plasmons in graphene and 2DEGs has been elusive so far - only GPs with nearly free-space wavelength have been observed. Here we demonstrate real-space imaging of acoustic THz plasmons in a graphene photodetector with split-gate architecture. To that end, we introduce nanoscale-resolved THz photocurrent near-field microscopy, where near-field excited GPs are detected thermoelectrically rather than optically. The on-chip GP detection simplifies GP imaging, as sophisticated s-SNOM detection schemes can be avoided. The photocurrent images reveal strongly reduced GP wavelengths (lp = l0/66), a linear dispersion resulting from the coupling of GPs with the metal gate below the graphene, and that plasmon damping at positive carrier densities is dominated by Coulomb impurity scattering. Acoustic GPs could thus strongly benefit the development of deep subwavelength-scale THz devices.

cond-mat.mes-hall

Mid-infrared pyro-resistive graphene detector on LiNbO3

Mid-infrared (mid-IR) photo-detection has been recently growing in importance because of its multiple applications, including vibrational spectroscopy and thermal imaging. We propose and demonstrate a novel pyro-resistive photo-detection platform that combines a ferroelectric substrate (a z-cut LiNbO3 crystal) and a graphene layer transferred on top of its surface with electrical connections. Upon strong light absorption in the LiNbO3 substrate and the subsequent temperature increase, via the pyroelectric effect, polarization (bound) charges form at the crystal surface. These causes doping into graphene which in turn changes its carrier density and conductivity. In this way, by monitoring the graphene electrical resistance one can measure the incident optical power. . Detectivities of about 10^5 cm sqrt(Hz)/W in the 6 to 10 microns wavelength region are demonstrated.We explain the underlying physical mechanism of the pyro-resistive photo-detection and propose a model that reproduces accurately the experimental results. We also show that up to two orders of magnitude larger detectivity can be achieved by optimising the geometry and operating in vacuum, thus opening the path to a new class of mid-IR photo-detectors that can challenge classical HgCdTe devices, especially in real applications where cooling is to be avoided and low cost is crucial.

physics.ins-det

Super-Planckian electron cooling in a van der Waals stack

Radiative heat transfer (RHT) between macroscopic bodies at separations that are much smaller than the thermal wavelength is ruled by evanescent electromagnetic modes and can be orders of magnitude more efficient than its far-field counterpart, which is described by the Stefan-Boltzmann law. In this Letter we present a microscopic theory of RHT in van der Waals stacks comprising graphene and a natural hyperbolic material, i.e. hexagonal boron nitride (hBN). We demonstrate that RHT between hot carriers in graphene and hyperbolic phonon-polaritons in hBN is extremely efficient at room temperature, leading to picosecond time scales for the carrier cooling dynamics.

cond-mat.mes-hall

Thermoelectric detection of propagating plasmons in graphene

Controlling, detecting and generating propagating plasmons by all-electrical means is at the heart of on-chip nano-optical processing. Graphene carries long-lived plasmons that are extremely confined and controllable by electrostatic fields, however electrical detection of propagating plasmons in graphene has not yet been realized. Here, we present an all-graphene mid-infrared plasmon detector, where a single graphene sheet serves simultaneously as the plasmonic medium and detector. Rather than achieving detection via added optoelectronic materials, as is typically done in other plasmonic systems, our device converts the natural decay product of the plasmon---electronic heat---directly into a voltage through the thermoelectric effect. We employ two local gates to fully tune the thermoelectric and plasmonic behaviour of the graphene. High-resolution real-space photocurrent maps are used to investigate the plasmon propagation and interference, decay, thermal diffusion, and thermoelectric generation.

cond-mat.mes-hall

Near-field photocurrent nanoscopy on bare and encapsulated graphene

Opto-electronic devices utilizing graphene have already demonstrated unique capabilities, which are much more difficult to realize with conventional technologies. However, the requirements in terms of material quality and uniformity are very demanding. A major roadblock towards high-performance devices are the nanoscale variations of graphene properties, which strongly impact the macroscopic device behaviour. Here, we present and apply opto-electronic nanoscopy to measure locally both the optical and electronic properties of graphene devices. This is achieved by combining scanning near-field infrared nanoscopy with electrical device read-out, allowing infrared photocurrent mapping at length scales of tens of nanometers. We apply this technique to study the impact of edges and grain boundaries on spatial carrier density profiles and local thermoelectric properties. Moreover, we show that the technique can also be applied to encapsulated graphene/hexagonal boron nitride (h-BN) devices, where we observe strong charge build-up near the edges, and also address a device solution to this problem. The technique enables nanoscale characterization for a broad range of common graphene devices without the need of special device architectures or invasive graphene treatment.

cond-mat.mes-hall

Highly confined low-loss plasmons in graphene-boron nitride heterostructures

Graphene plasmons were predicted to possess ultra-strong field confinement and very low damping at the same time, enabling new classes of devices for deep subwavelength metamaterials, single-photon nonlinearities, extraordinarily strong light-matter interactions and nano-optoelectronic switches. While all of these great prospects require low damping, thus far strong plasmon damping was observed, with both impurity scattering and many-body effects in graphene proposed as possible explanations. With the advent of van der Waals heterostructures, new methods have been developed to integrate graphene with other atomically flat materials. In this letter we exploit near-field microscopy to image propagating plasmons in high quality graphene encapsulated between two films of hexagonal boron nitride (h-BN). We determine dispersion and particularly plasmon damping in real space. We find unprecedented low plasmon damping combined with strong field confinement, and identify the main damping channels as intrinsic thermal phonons in the graphene and dielectric losses in the h-BN. The observation and in-depth understanding of low plasmon damping is the key for the development of graphene nano-photonic and nano-optoelectronic devices.

cond-mat.mes-hall

Defect-mediated spin relaxation and dephasing in graphene

A principal motivation to develop graphene for future devices has been its promise for quantum spintronics. Hyperfine and spin-orbit interactions are expected to be negligible in single-layer graphene. Spin transport experiments, on the other hand, show that graphene's spin relaxation is orders of magnitude faster than predicted. We present a quantum interference measurement that disentangles sources of magnetic and non-magnetic decoherence in graphene. Magnetic defects are shown to be the primary cause of spin relaxation, while spin-orbit interaction is undetectably small.

cond-mat.mes-hall

Rippled Graphene in an In-Plane Magnetic Field: Effects of a Random Vector Potential

We report measurements of the effects of a random vector potential generated by applying an in-plane magnetic field to a graphene flake. Magnetic flux through the ripples cause orbital effects: phase-coherent weak localization is suppressed, while quasi-random Lorentz forces lead to anisotropic magnetoresistance. Distinct signatures of these two effects enable an independent estimation of the ripple amplitude and correlation length.

cond-mat.mes-hall

Spin-resolved Quantum Interference in Graphene

The unusual electronic properties of single-layer graphene make it a promising material system for fundamental advances in physics, and an attractive platform for new device technologies. Graphene's spin transport properties are expected to be particularly interesting, with predictions for extremely long coherence times and intrinsic spin-polarized states at zero field. In order to test such predictions, it is necessary to measure the spin polarization of electrical currents in graphene. Here, we resolve spin transport directly from conductance features that are caused by quantum interference. These features split visibly in an in-plane magnetic field, similar to Zeeman splitting in atomic and quantum dot systems. The spin-polarized conductance features that are the subject of this work may, in the future, lead to the development of graphene devices incorporating interference-based spin filters.

cond-mat.mes-hall