arXiv subjects

Mark E. Siemens

Publications and source records attributed to Mark E. Siemens.

23 records · Page 2Linked to original sources

arXiv2018

Diagonal Slice Four-Wave Mixing: Natural Separation of Coherent Broadening Mechanisms

We present an ultrafast coherent spectroscopy data acquisition scheme that samples slices of the time domain used in multidimensional coherent spectroscopy to achieve faster data collection than full spectra. We derive analytical expressions for resonance lineshapes using this technique that completely separate homogeneous and inhomogeneous broadening contributions into separate projected lineshapes for arbitrary inhomogeneous broadening. These lineshape expressions are also valid for slices taken from full multidimensional spectra and allow direct measurement of the parameters contributing to the lineshapes in those spectra as well as our own.

physics.ins-det↗

arXiv2017

Efficient Modal Decomposition of Vortex Beams via Holographically Reconstructed Phase

We use phase-shifting digital holography to measure the amplitude and phase of twisted light. In our experiment, a spatial light modulator generates the studied vortex beams in addition to a co-propagating reference beam with a controllable relative phase. We show complex field measurements for single and superposition Laguerre Gaussian (LG) modes, demonstrate full modal decompositions into LG and orbital angular momentum (OAM) power spectral bases, provide error analysis and demonstrate high insensitivity to detector misalignment to show the robustness of the technique. This enables rapid determination of OAM spectra with low uncertainty, allowing us to report the first vortex beams with 99.9% purity.

physics.optics↗

arXiv2017

The Angular Momentum of Topologically Structured Darkness

We theoretically analyze and experimentally measure the extrinsic angular momentum contribution of topologically structured darkness found within fractional vortex beams, and show that this structured darkness can be explained by evanescent waves at phase discontinuities in the generating optic. We also demonstrate the first direct measurement of the intrinsic orbital angular momentum of light with both intrinsic and extrinsic angular momentum, and explain why the total orbital angular momenta of fractional vortices do not match the winding number of their generating phases.

physics.optics↗

arXiv2016

The Centroid Shifts of Light Beams Reflected from Multi-Layers and the Effects of Angular Momentum Manifestations

Laguerre-Gaussian (LG) beams reflected from a multi-layered dielectric experience a shift in their centroid that is different than that from a single interface. This has been previously investigated for linearly polarized beams and, to a much lesser extent, beams with spin angular momentum. Here a combination of perturbation and computational analyses is used to provide a unified quantification of these shifts in layered dielectrics with two parallel interfaces. The approach is then extended to consider the qualitatively new behavior that results when the light is endowed with an intrinsic orbital angular momentum--i.e. vortex beams. Destructive interference causes singular lateral shifts in the centroid of the reflected vortex beam for which spin alone produces only a mild modulation. In the case of total internal reflection, both spin and intrinsic orbital angular momentum contribute to an enhancement of these lateral shifts as the interlayer thickness is decreased. This is just the opposite of the trend associated with longitudinal shifts. Two geometries are considered: air/glass/air and glass/air/glass multi-layers. A commonly available glass is used to show that vortex beams can result in centroid shifts on the order of microns for beams with a significant reflection coefficient.

physics.optics↗

arXiv2016

Efficient Thermal Conductance in Organometallic Perovskite CH3NH3PbI3 Films

Perovskite-based optoelectronic devices have shown great promise for solar conversion and other optoelectronic applications, but their long-term performance instability is regarded as a major obstacle to their widespread deployment. Previous works have shown that the ultralow thermal conductivity and inefficient heat spreading might put an intrinsic limit on the lifetime of perovskite devices. Here, we report the observation of a remarkably efficient thermal conductance, with conductivity of 11.2 +/- 0.8 W m^-1 K^-1 at room temperature, in densely-packed perovskite CH3NH3PbI3 films, via noncontact time-domain thermal reflectance measurements. The temperature-dependent experiments suggest the important roles of organic cations and structural phase transitions, which are further confirmed by temperature-dependent Raman spectra. The thermal conductivity at room temperature observed here is over one order of magnitude larger than that in the early report, suggesting that perovskite device performance will not be limited by thermal stability.

cond-mat.mtrl-sci↗