arXiv subjects

Mark G. Blamire

Publications and source records attributed to Mark G. Blamire.

9 recordsLinked to original sources

arXiv2021

Thermal annealing enhancement of Josephson critical currents in ferromagnetic CoFeB

The electrical and structural properties of Co40Fe40B20 (CoFeB) alloy are tunable with thermal annealing. This is key in the optimization of CoFeB-based spintronic devices, where the advantageously low magnetic coercivity, high spin polarization, and controllable magnetocrystalline anisotropy are utilised. So far, there has been no report on superconducting devices based on CoFeB. Here, we report Nb/CoFeB/Nb Josephson devices and demonstrate an enhancement of the critical current by up to 700% following thermal annealing due to increased structural ordering of the CoFeB. The results demonstrate that CoFeB is a promising material for the development of superconducting spintronic devices.

cond-mat.supr-con↗

arXiv2021

Spin-orbit coupling suppression and singlet-state blocking of spin-triplet Cooper pairs

An inhomogeneous magnetic exchange field at a superconductor/ferromagnet interface converts spin-singlet Cooper pairs to a spin-aligned (i.e. spin-polarized) triplet state. Although the decay envelope of such triplet pairs within ferromagnetic materials is well studied, little is known about their decay in non-magnetic metals and superconductors, and in particular in the presence of spin-orbit coupling (SOC). Here we investigate devices in which triplet supercurrents are injected into the s-wave superconductor Nb. In the normal state of Nb, triplet supercurrents decay over a distance of 5 nm, which is an order of magnitude smaller than the decay of spin singlet pairs due to the SOC interacting with the spin associated with triplet pairs. In the superconducting state of Nb, triplet supercurrents are not able to couple with the singlet wavefunction and thus blocked by the absence of available equilibrium states in the singlet gap. The results offer new insight into the dynamics between s-wave singlet and s-wave triplet states.

cond-mat.supr-con↗

arXiv2019

Tunable pure spin supercurrents and the demonstration of a superconducting spin-wave device

Recent ferromagnetic resonance experiments and theory of Pt/Nb/Ni8Fe2 proximity-coupled structures strongly suggest that spin-orbit coupling (SOC) in Pt in conjunction with a magnetic exchange field in Ni8Fe2 are the essential ingredients to generate a pure spin supercurrent channel in Nb. Here, by substituting Pt for a perpendicularly magnetized Pt/Co/Pt spin-sink, we are able to demonstrate the role of SOC, and show that pure spin supercurrent pumping efficiency across Nb is tunable by controlling the magnetization direction of Co. By inserting a Cu spacer with weak SOC between Nb and Pt/(Co/Pt) spin-sink, we also prove that Rashba type SOC is key for forming and transmitting pure spin supercurrents across Nb. Finally, by engineering these properties within a single multilayer structure, we demonstrate a prototype superconducting spin-wave (SW) device in which lateral SW propagation is gateable via the opening or closing of a vertical pure spin supercurrent channel in Nb.

cond-mat.mes-hall↗

arXiv2019

Abrikosov vortex nucleation and its detrimental effect on superconducting spin pumping in Pt/Nb/Ni80Fe20/Nb/Pt proximity structures

We report Abrikosov vortex nucleation in Pt/Nb/Ni80Fe20/Nb/Pt proximity-coupled structures under oblique ferromagnetic resonance (FMR) that turns out to be detrimental to superconducting spin pumping. By measuring an out-of-plane field-angle θH dependence and comparison with Pt-absent control samples, we show that as θH increases, the degree of enhancement (suppression) of spin pumping efficiency in the superconducting state for the Pt-present (Pt-absent) sample diminishes and it reverts to the normal state value at θH = 90°. This can be explained in terms of a substantial out-of-plane component of the resonance field for the Ni80Fe20 layer (with in-plane magnetization anisotropy and high aspect ratio) that approaches the upper critical field of the Nb, turning a large fraction of the singlet superconductor volume into the normal state.

cond-mat.mes-hall↗

arXiv2019

Effect of Meissner screening and trapped magnetic flux on magnetization dynamics in thick Nb/Ni80Fe20/Nb trilayers

We investigate the influence of Meissner screening and trapped magnetic flux on magnetization dynamics for a Ni80Fe20 film sandwiched between two thick Nb layers (100 nm) using broadband (5-20 GHz) ferromagnetic resonance (FMR) spectroscopy. Below the superconducting transition Tc of Nb, significant zero-frequency line broadening (5-6 mT) and DC resonance field shift (50 mT) to a low field are both observed if the Nb thickness is comparable to the London penetration depth of Nb films (>= 100 nm). We attribute the observed peculiar behaviors to the increased incoherent precession near the Ni80Fe20/Nb interface and the effectively focused magnetic flux in the middle Ni80Fe20 caused by strong Meissner screening and (defect-)trapped flux of the thick adjacent Nb layers. This explanation is supported by static magnetic properties of the samples and comparison with FMR data on thick Nb/Ni80Fe20 bilayers. Great care should therefore be taken in the analysis of FMR response in ferromagnetic Josephson structures with thick superconductors, a fundamental property for high-frequency device applications of spin-polarized supercurrents.

cond-mat.mes-hall↗

arXiv2017

Magnetization-control and transfer of spin-polarized Cooper pairs into a half-metal manganite

The pairing state and critical temperature (T$_c$) of a thin s-wave superconductor (S) on two or more ferromagnets (F) are controllable through the magnetization-alignment of the F layers. Magnetization misalignment can lead to spin-polarized triplet pair creation, and since such triplets are compatible with spin-polarized materials they are able to pass deeply into the F layers and so, cause a decrease in T$_c$. Various experiments on S/F$_1$/F$_2$ "triplet spin-valves" have been performed with the most pronounced suppression of T$_c$ reported in devices containing the half-metal ferromagnet (HMF) CrO$_2$ (F$_2$) albeit using out-of-plane magnetic fields to tune magnetic non-collinearity [Singh et al., Phys. Rev. X 5, 021019 (2015)]. Routine transfer of spin-polarized triplets to HMFs is a major goal for superconducting spintronics so as to maximize triplet-state spin-polarization. However, CrO$_2$ is chemically unstable and out-of-plane fields are undesirable for superconductivity. Here, we demonstrate magnetization-tuneable pair conversion and transfer of spin-polarized triplet pairs to the chemically stable mixed valence manganite La$_{2/3}$Ca$_{1/3}$MnO$_3$ in a pseudo spin-valve device using in-plane magnetic fields. The results match microscopic theory and offer full control over the pairing state.

cond-mat.supr-con↗

arXiv2015

Magnetic field-enhanced spin filtering in rare-earth mononitride tunnel junctions

Spin filter tunnel junctions are based on selective tunneling of up and down spin electrons controlled through exchange splitting of the band structure of a ferromagnetic insulator. Therefore, spin filter efficiency can be tuned by adjusting exchange strength of the tunnel barrier. We have observed that magnetic field and bias voltage (current) can be used to regulate exchange strength and consequently spin-filter efficiency in tunnel junctions with ferromagnetic DyN and GdN tunnel barrier. In tunnel junctions with DyN barrier we obtained $\sim$37$\%$ spin polarization of tunneling electrons at 11 K due to a small exchange splitting ($ E_{ex}$) $\approx$5.6 meV of the barrier height ($Φ_0$) $\approx$60 meV. Huge spin-filter efficiency $\sim$97$\%$ was found for tunnel junctions with GdN barrier due to larger $E_{ex}$ $\approx$47 meV. In the presence of an applied magnetic field, barrier height can further split due to magnetic field dependent exchange splitting $ E_{ex}(H)$. The spin filter efficiency in DyN tunnel junctions can be increased up to $\sim$87$\%$ with magnetic field. Electric and magnetic field tuned spin-filter efficiency of these tunnel junctions gives opportunity for practical application of these devices with additional functionality.

cond-mat.mes-hall↗

arXiv2011

Depairing critical current achieved in superconducting thin films with through-thickness arrays of artificial pinning centers

Large area arrays of through-thickness nanoscale pores have been milled into superconducting Nb thin films via a process utilizing anodized aluminum oxide thin film templates. These pores act as artificial flux pinning centers, increasing the superconducting critical current, Jc, of the Nb films. By optimizing the process conditions including anodization time, pore size and milling time, Jc values approaching and in some cases matching the Ginzburg-Landau depairing current of 30 MA/cm^2 at 5 K have been achieved - a Jc enhancement over as-deposited films of more than 50 times. In the field dependence of Jc, a matching field corresponding to the areal pore density has also been clearly observed. The effect of back-filling the pores with magnetic material has then been investigated. While back-filling with Co has been successfully achieved, the effect of the magnetic material on Jc has been found to be largely detrimental compared to voids, although a distinct influence of the magnetic material in producing a hysteretic Jc versus applied field behavior has been observed. This behavior has been tested for compatibility with currently proposed models of magnetic pinning and found to be most closely explained by a model describing the magnetic attraction between the flux vortices and the magnetic inclusions.

cond-mat.supr-con↗

arXiv2009

Superconductor-ferromagnet nanocomposites created by co-deposition of niobium and dysprosium

We have created superconductor-ferromagnet composite films in order to test the enhancement of critical current density, Jc, due to magnetic pinning. We co-sputter the type-II superconductor niobium (Nb) and the low-temperature ferromagnet dysprosium (Dy) onto a heated substrate; the immiscibility of the two materials leads to a phase-separated composite of magnetic regions within a superconducting matrix. Over a range of compositions and substrate temperatures, we achieve phase separation on scales from 5 nm to 1 micron. The composite films exhibit simultaneous superconductivity and ferromagnetism. Transport measurements show that while the self-field Jc is reduced in the composites, the in-field Jc is greatly enhanced up to the 3 T saturation field of Dy. In one instance, the phase separation orders into stripes, leading to in-plane anisotropy in Jc.

cond-mat.supr-con↗