arXiv subjects

Mark Linne

Publications and source records attributed to Mark Linne.

5 recordsLinked to original sources

arXiv2025

Spatial phase coherence in femtosecond coherent Raman scattering

Conventional femtosecond coherent laser spectroscopy predominantly focuses on the temporal phase coherence through time- or frequency-resolved methods. In this work, we suggest an alternative experimental framework based on spatial phase coherence. The intrinsic spectral dispersion of wavevectors in femtosecond pulses and sample dimensions exceeding the laser wavelength create a compelling basis to establish spatial phase coherence as a novel and robust foundation for femtosecond laser spectroscopy. Using rotational Raman coherence in gas molecules as a case study, we analyze the transverse spatial distribution of the third-order signal generated by a rotational wave-packet. Our findings reveal apparent temporal shifts and distortions in time-resolved signals that arise in conventional measurements lacking sensitivity to spatial phase coherence. Moreover, we demonstrate that spatial phase coherence can serve as a useful tool for thermometric applications, showcasing its sensitivity to temperature variations. These discoveries open new avenues in femtosecond laser spectroscopy, including an alternative single-shot detection scheme, a new form of Raman coherence imaging and molecular species quantification during overlapping fractional revivals.

physics.optics↗

arXiv2023

Assessment and Application of Wavelet-based Optical Flow Velocimetry (wOFV) to Wall-Bounded Turbulent Flows

The performance of a wavelet-based optical flow velocimetry (wOFV) algorithm to extract high accuracy and high resolution velocity fields from particle images in wall-bounded turbulent flows is assessed. wOFV is first evaluated using synthetic particle images generated from a channel flow DNS of a turbulent boundary layer. The sensitivity of wOFV to the regularization parameter (lambda) is quantified and results are compared to PIV. Results on synthetic particle images indicated different sensitivity to under-regularization or over-regularization depending on which region of the boundary layer is analyzed. Synthetic data revealed that wOFV can modestly outperform PIV in vector accuracy across a broad lambda range. wOFV showed clear advantages over PIV in resolving the viscous sublayer and obtaining highly accurate estimates of the wall shear stress. wOFV was also applied to experimental data of a developing turbulent boundary layer. Overall, wOFV revealed good agreement with both PIV and PIV + PTV. However, wOFV was able to successfully resolve the wall shear stress and correctly normalize the boundary layer streamwise velocity to wall units where PIV and PIV + PTV showed larger deviations. Analysis of the turbulent velocity fluctuations revealed spurious results for PIV in close proximity to the wall, leading to significantly exaggerated and non-physical turbulence intensity. PIV + PTV showed a minor improvement in this aspect. wOFV did not exhibit this same effect, revealing that it is more accurate in capturing small-scale turbulent motion in the vicinity of boundaries. The enhanced vector resolution of wOFV enabled improved estimation of instantaneous derivative quantities and intricate flow structure both closer to the wall. These aspects show that, within a reasonable lambda range, wOFV can improve resolving the turbulent motion occurring in the vicinity of physical boundaries.

physics.flu-dyn↗

arXiv2022

Revisiting N$_2$-N$_2$ collisional linewidth models for S-branch rotational Raman scattering

This paper presents an evaluation of two commonly accepted Raman linewidth models typically used to fit CARS model parameters to data; the Modified Exponential Gap (MEG) and the Energy Corrected Sudden (ECS) models. The adjustable parameters in each model have been fit to published experimental linewidths, and comparisons are made to the various publications that have already provided similar adjustable constants. The approaches presented in the literature are discussed as are differences with the findings presented here.

physics.data-an↗

arXiv2020

Optimising hybrid rotational femtosecond/picosecond coherent anti-Stokes Raman spectroscopy (HR-CARS) in nitrogen at high pressures and temperatures

We demonstrate the use of hybrid rotational femtosecond/picosecond (fs/ps) coherent anti-Stokes Raman spectroscopy (HR-CARS) as a technique for temperature measurements in nitrogen gas at high pressures and temperatures. A broadband pulse shaper-adjusted 42 fs pulse interacts with a narrow-bandwidth, frequency-upconverted 5.5 ps pulse in a cell containing nitrogen at pressures of 1-70 atm and temperatures of 300-1000 K. A computational code is used to model spectra and fit experimental results to obtain best-fit temperatures. We demonstrate good qualitative fits as well as good accuracy and precision between thermocouple measured and best-fit temperatures over the explored pressure and temperature regimes. The overall average percentage temperature difference between thermocouple measurements and best-fit temperatures is -0.3% with a standard deviation of 7.1%, showing the suitability of HR-CARS for characterising high pressure and temperature environments.

physics.optics↗

arXiv2020

Dual-probe 1-d hybrid fs/ps rotational CARS for simultaneous single-shot temperature, pressure, and O2/N2 measurements

We employ dual-probe 1-d fs/ps hybrid rotational coherent anti-Stokes Raman spectroscopy to investigate simultaneous temperature, pressure, and O2/N2 measurements for gas-phase diagnostics. The dual-probe HRCARS technique allows for simultaneous measurements from the time and frequency-domain. A novel approach for measuring pressure, which offers high accuracy (<1%) and precision (0.42%) is presented. The technique is first demonstrated in a chamber for a range of pressures (1-1.5 bar). This technique shows an impressive capability of resolving 1-d pressure gradients arising from a N2 jet impinging on a surface, both in laminar and turbulent conditions. The technique is shown to be capable of resolving single-shot pressure gradients (0.04 bar/mm) originating from kinetic energy conversion to pressure, and resolves characteristic O2/N2 structures from laminar and turbulent mixing.

physics.optics↗