arXiv subjects

Mark Oxborrow

Publications and source records attributed to Mark Oxborrow.

27 records · Page 2Linked to original sources

arXiv2021

Bench-top Cooling of a Microwave Mode using an Optically Pumped Spin Refrigerator

We experimentally demonstrate the temporary removal of thermal photons from a microwave mode at 1.45 GHz through its interaction with the spin-polarized triplet states of photo-excited pentacene molecules doped within a p-terphenyl crystal at room temperature. The crystal functions electromagnetically as a narrow-band cryogenic load, removing photons from the otherwise room-temperature mode via stimulated absorption. The noise temperature of the microwave mode dropped to $50^{+18}_{-32}$ K (as directly inferred by noise-power measurements) while the metal walls of the cavity enclosing the mode remained at room temperature. Simulations based on the same system's behavior as a maser (which could be characterized more accurately) indicate the possibility of the mode's temperature sinking to $\sim$10 K (corresponding to $\sim$140 microwave photons). These observations, when combined with engineering improvements to deepen the cooling, identify the system as a narrow-band yet extremely convenient platform -- free of cryogenics, vacuum chambers and strong magnets -- for realizing low-noise detectors, quantum memory and quantum-enhanced machines (such as heat engines) based on strong spin-photon coupling and entanglement at microwave frequencies.

quant-ph↗

arXiv2020

Room-temperature quasi-continuous-wave pentacene maser pumped by an invasive Ce:YAG luminescent concentrator

We present in this work a quasi-continuous-wave (CW) pentacene maser operating at 1.45 GHz in the Earth's magnetic field at room temperature with a duration of $\sim$4 ms and an output power of up to -25 dBm. The maser is optically pumped by a cerium-doped YAG (Ce:YAG) luminescent concentrator (LC) whose wedge-shaped output is embedded inside a 0.1% pentacene-doped para-terphenyl (Pc:Ptp) crystal. The pumped crystal is located inside a ring of strontium titanate (STO) that supports a TE$_{01δ}$ mode of high magnetic Purcell factor. Combined with simulations, our results indicate that CW operation of pentacene masers at room-temperature is perfectly feasible so long as excessive heating of the crystal is avoided.

physics.app-ph↗

arXiv2020

Pulsed Electron Spin Resonance of an Organic Microcrystal by Dispersive Readout

We establish a testbed system for the development of high-sensitivity Electron Spin Resonance (ESR) techniques for small samples at cryogenic temperatures. Our system consists of a Niobium Nitride thin-film planar superconducting microresonator designed to have a concentrated mode volume to couple to a small amount of paramagnetic material, and to be resilient to magnetic fields of up to 400 mT. At 65 mK we measure high-cooperativity coupling ($C \approx 19$) to an organic radical microcrystal containing $10^{12}$ spins in a pico-litre volume. We detect the spin-lattice decoherence rate via the dispersive frequency shift of the resonator. Techniques such as these could be suitable for applications in quantum information as well as for pulsed ESR interrogation of very few spins and could provide insights into the surface chemistry of, for example, the material defects in superconducting quantum processors.

quant-ph↗

arXiv2013

Slow noise processes in superconducting resonators

Slow noise processes, with characteristic timescales ~1s, have been studied in planar superconducting resonators. A frequency locked loop is employed to track deviations of the resonator centre frequency with high precision and bandwidth. Comparative measurements are made in varying microwave drive, temperature and between bare resonators and those with an additional dielectric layer. All resonators are found to exhibit flicker frequency noise which increases with decreasing microwave drive. We also show that an increase in temperature results in a saturation of flicker noise in resonators with an additional dielectric layer, while bare resonators stop exhibiting flicker noise instead showing a random frequency walk process.

cond-mat.supr-con↗

arXiv2011

Pound-locking for characterization of superconducting microresonators

We present a new application and implementation of the so-called Pound locking technique for the interrogation of superconducting microresonators. We discuss how by comparing against stable frequency sources this technique can be used to characterize properties of resonators that can not be accessed using traditional methods. Specifically, by analyzing the noise spectra and the Allan deviation we obtain valuable information about the nature of the noise in superconducting planar resonators. This technique also greatly improves the read-out accuracy and measurement throughput compared to conventional methods.

physics.ins-det↗

arXiv2010

Unprecedented High Long Term Frequency Stability with a Macroscopic Resonator Oscillator

This article reports on the long-term frequency stabilty characterisation of a new type of cryogenic sapphire oscillator using an autonomous pulse-tube cryocooler as its cold source. This new design enables a relative frequency stability of better than 4.5e-15 over one day of integration. This represents to our knowledge the best long-term frequency stability ever obtained with a signal source based on a macroscopic resonator.

physics.ins-det↗

arXiv2010

DC-powered Fe3+:sapphire Maser and its Sensitivity to Ultraviolet Light

The zero-field Fe3+:sapphire whispering-gallery-mode maser oscillator exhibits several alluring features: Its output is many orders of magnitude brighter than that of an active hydrogen maser and thus far less degraded by spontaneous-emission (Schawlow-Townes) and/or receiving-amplifier noise. Its oscillator loop is confined to a piece of mono-crystalline rock bolted into a metal can. Its quiet amplification combined with high resonator Q provide the ingredients for exceptionally low phase noise. We here concentrate on novelties addressing the fundamental conundrums and technical challenges that impede progress. (1) Roasting: The "mase-ability" of sapphire depends significantly on the chemical conditions under which it is grown and heat-treated. We provide some fresh details and nuances here. (2) Simplification: This paper obviates the need for a Ka-band synthesizer: it describes how a 31.3 GHz loop oscillator, operating on the preferred WG pump mode, incorporating Pound locking, was built from low-cost components. (3) "Dark Matter": A Siegman-level analysis of the experimental data determines the substitutional concentration of Fe3+ in HEMEX to be less than a part per billion prior to roasting and up to a few hundred ppb afterwards. Chemical assays, using different techniques (incl. glow discharge mass spectra spectroscopy and neutron activation analysis) consistently indicate, however, that HEMEX contains iron at concentrations of a few parts per million. Drawing from several forgotten-about/under-appreciated papers, this substantial discrepancy is addressed. (4) Excitons: Towards providing a new means of controlling the Fe3+:sapph. system, a cryogenic sapphire ring was illuminated, whilst masing, with UV light at wavelengths corresponding to known electronic and charge-transfer (thus valence-altering) transitions. Preliminary experiments are reported.

quant-ph↗

arXiv2007

Ex-house 2D finite-element simulation of the whispering-gallery modes of arbitrarily shaped axisymmetric electromagnetic resonators

It is described, explicitly, how a popular, commercially-available software package for solving partial-differential-equations (PDEs), as based on the finite-element method (FEM), can be configured to calculate the frequencies and fields of the whispering-gallery (WG) modes of axisymmetric dielectric resonators. The approach is traceable; it exploits the PDE-solver's ability to accept the definition of solutions to Maxwell's equations in so-called `weak form'. Associated expressions and methods for estimating a WG mode's volume, filling factor(s) and, in the case of closed(open) resonators, its wall (radiation) loss, are provided. As no transverse approxi-mation is imposed, the approach remains accurate even for so-called quasi-TM and -TE modes of low, finite azimuthal mode order. The approach's generality and utility are demonstrated by modeling several non-trivial structures: (i)two different optical microcavities [one toroidal made of silica, the other an AlGaAs microdisk]; (ii) a 3rd-order microwave Bragg cavity containing alumina layers (iii) two different cryogenic sapphire X-band microwave resonators. By fitting one of the latter to a set of measured resonance frequencies, the dielectric constants of sapphire at liquid-helium temperature have been estimated.

quant-ph↗

arXiv2007

Traceable 2D finite-element simulation of the whispering-gallery modes of axisymmetric electromagnetic resonators

This paper explains how a popular, commercially-available software package for solving partial-differential-equations (PDEs), as based on the finite-element method (FEM), can be configured to calculate, efficiently, the frequencies and fields of the whispering-gallery (WG) modes of axisymmetric dielectric resonators. The approach is traceable; it exploits the PDE-solver's ability to accept the definition of solutions to Maxwell's equations in so-called `weak form'. Associated expressions and methods for estimating a WG mode's volume, filling factor(s) and, in the case of closed(open) resonators, its wall(radiation) loss, are provided. As no transverse approximation is imposed, the approach remains accurate even for quasi-transverse magnetic/electric modes of low, finite azimuthal mode order. The approach's generality and utility are demonstrated by modeling several non-trivial structures: (i) two different optical microcavities [one toroidal made of silica, the other an AlGaAs microdisk]; (ii) a 3rd-order sapphire:air Bragg cavity; (iii) two different cryogenic sapphire WG-mode resonators; both (ii) and (iii) operate in the microwave X-band. By fitting one of (iii) to a set of measured resonance frequencies, the dielectric constants of sapphire at liquid-helium temperature have been estimated.

quant-ph↗