arXiv subjects

Mark P. Croce

Publications and source records attributed to Mark P. Croce.

6 recordsLinked to original sources

arXiv2022

Quantification of 242Pu with a Microcalorimeter Gamma Spectrometer

We report measurements of the 103-keV and 159-keV gamma ray signatures of 242Pu using microcalorimetry. This is the first observation of these gamma rays in a non-destructive measurement of an unprepared sample, and so represents an important advance in nuclear material accountancy. The measurement campaign also serves as the first demonstration of a field campaign with a portable microcalorimeter gamma-ray spectrometer. For the 103-keV gamma ray we report an improved centroid energy and emission probability.

physics.ins-det↗

arXiv2021

New Experimentally Observable Gamma-ray Emissions from 241Am Nuclear Decay

With the high resolution of microcalorimeter detectors, previously unresolvable gamma-ray lines are now clearly resolvable. A careful measurement of Am-241 decay with a large array of gamma-ray microcalorimeters has revealed never before seen or predicted gamma lines at 207.72 +/- 0.02 keV and 208.21 +/- 0.01 keV. These results were made possible by new microwave-multiplexing readout to increase the array size and improved analysis algorithms to eliminate spectral artifacts. We suggest nuclear levels from which these gamma-rays might originate and calculate branching ratios for these transitions from measurements of both mixed Pu-Am standards and a pure Am-241 source. These results have implications for nuclear material safeguards and accounting, particularly for microcalorimeter gamma spectrometers, which are now being adopted in nuclear safeguards analytical laboratories.

nucl-ex↗

arXiv2021

First Measurements of Nuclear Detonation Debris with Decay Energy Spectroscopy

We report the first isotopic composition measurements of trinitite, nuclear detonation debris from the Trinity test, using the novel forensics technique of decay energy spectroscopy (DES). DES measures the unique total decay energy (Q value) of each alpha-decaying isotope in a small radioactive sample embedded in a microcalorimeter detector. We find that DES can measure the major alpha-decaying isotopes in small particles of trinitite with no dissolution or chemical processing. These first measurements demonstrate the potential of DES to provide a radiometric isotopic characterization method with sensitivity and precision to complement traditional forensics techniques.

physics.ins-det↗

arXiv2021

Measurement of Ac227 Impurity in Ac225 using Decay Energy Spectroscopy

225Ac is a valuable medical radionuclide for targeted alpha therapy, but 227Ac is an undesirable byproduct of an accelerator-based synthesis method under investigation. Sufficient detector sensitivity is critical for quantifying the trace impurity of 227Ac, with the 227Ac/225Ac activity ratio predicted to be approximately 0.15% by end-of-bombardment (EOB). Superconducting transition edge sensor (TES) microcalorimeters offer high resolution energy spectroscopy using the normal-to-superconducting phase transition to measure small change in temperature. By embedding 225Ac production samples in a gold foil thermally coupled to a TES microcalorimeter we can measure the decay energies of the radionuclides embedded with high resolution and efficiency. This technique, known as decay energy spectroscopy (DES), collapses several peaks from alpha decays into single Q-value peaks. In practice there are more complex factors in the interpretation of data using DES, which we will discuss herein. Using this technique we measured the EOB 227Ac impurity to be (0.142 +/- 0.005)% for a single production sample. This demonstration has shown that DES can distinguish closely related isotopic features and is a useful tool for quantitative measures.

physics.ins-det↗

arXiv2020

Improved Plutonium and Americium Photon Branching Ratios from Microcalorimeter Gamma Spectroscopy

Photon branching ratios are critical input data for activities such as nuclear materials protection and accounting because they allow material compositions to be extracted from measurements of gamma-ray intensities. Uncertainties in these branching ratios are often a limiting source of uncertainty in composition determination. Here, we use high statistics, high resolution (~60-70eV full-width-at-half-maximum at 100 keV) gamma-ray spectra acquired using microcalorimeter sensors to substantially reduce the uncertainties for 11 plutonium (238Pu,239Pu,241Pu) and 241Am branching ratios important for material control and accountability and nuclear forensics in the energy range of 125 keV to 208 keV. We show a reduction in uncertainty of over a factor of three for one branching ratio and a factor of 2{3 for four branching ratios.

nucl-ex↗

arXiv2018

First Calorimetric Measurement of Electron Capture in ${}^{193}$Pt with a Transition Edge Sensor

The neutrino mass can be extracted from a high statistics, high resolution calorimetric spectrum of electron capture in ${}^{163}$Ho. In order to better understand the shape of the calorimetric electron capture spectrum, a second isotope was measured with a close to ideal absorber-source configuration. ${}^{193}$Pt was created by irradiating a ${}^{192}$Pt-enriched platinum foil in a nuclear reactor. This Pt-in-Pt absorber was designed to have a nearly ideal absorber-source configuration. The measured ${}^{193}$Pt calorimetric electron-capture spectrum provides an independent check on the corresponding theoretical calculations, which have thus far been compared only for ${}^{163}$Ho. The first experimental and theoretically-calculated spectra from this ${}^{193}$Pt-in-Pt absorber are presented and overlaid for preliminary comparison of theory with experiment.

physics.atom-ph↗