arXiv subjects

Marko Lončar

Publications and source records attributed to Marko Lončar.

At least 19 recordsLinked to original sources

arXiv2026

Hysteresis and trap emission in dc-biased integrated lithium niobate electro-optic modulators

The electro-optic effect is crucially important for low power and efficient tuning of integrated photonic circuits. However, in electro-optic materials such as lithium niobate, dc biasing for an extended duration of time results in the emergence of numerous nonidealities, including hysteresis -- a persistent degradation of the magnitude and linearity of the dc electro-optic response. We show that electro-optic hysteresis can be reversed under both zero-bias and reverse-bias conditions, given sufficient time or reverse voltage and consistent with a defect model of the underlying physics. Specifically, we find that drift phenomena at short time scales can be explained by charge trapping dynamics near the contact junction, and thereby devise an active reset protocol that restores the magnitude of the response and partially restores the drift time scales.

physics.optics↗

arXiv2026

Increased cyclicity of atomic transitions via coherent interference of decay paths

Optical readout is a fundamental tool in atomic state measurement, yet the fidelity of optical readout is frequently limited by imperfect photon collection. This can be mitigated when readout occurs on a cycling transition which continuously fluoresces under resonant excitation, thus increasing signal and enabling single-shot readout. We present a method to extend the cyclicity of atomic transitions via coherent destructive interference between spurious decay paths. We describe the characteristics of atomic systems in which this method can be implemented and model several examples in which the number of emitted photons is increased by multiple orders of magnitude.

quant-ph↗

arXiv2026

A high-performance quantum pulse gate in thin-film lithium niobate

In this work, we demonstrate a quantum pulse gate (QPG) in thin-film lithium niobate. QPGs enable the selective manipulation and detection of temporal modes of quantum light and form the basis of numerous applications in photonic quantum technologies. To date, their widespread adaption is held back by two main limitations: restricted wavelength and polarization combinations of the involved fields and low normalized conversion efficiencies. We overcome these limitations through developing a QPG in thin-film lithium niobate. We design a waveguide geometry that provides the required dispersion properties for a highly efficient type-0 sum-frequency generation.We verify our design through mapping of the phase matching intensity, and demonstrate high-quality QPG operation by measuring a temporal-mode selectivity of (96.8$\pm$1.7)% on par with existing QPGs. Thanks to the strong confinement in thin-film lithium niobate, we succeed in demonstrating an internal conversion efficiency of (89.6$\pm$0.1)% for a pump power of only 20mW in front of our sample. This yields a lower-bound estimate for the normalized conversion efficiency of (1810$\pm$10)$\mathrm{W}^{-1}\mathrm{cm}^{-2}$, three orders of magnitude higher than in previous QPGs. Our results establish thin-film lithium niobate as ideal platform for high-performance QPGs and are a major step towards practical QPGs for photonic quantum technologies.

quant-ph↗

arXiv2026

Ultrafast programmable Bragg reflection in photonic integrated circuits

Distributed Bragg reflectors (DBRs) are foundational building blocks of classical and quantum photonic technologies. However, their optical responses are typically fixed upon fabrication, limiting circuit robustness, reconfigurability, and functionality in applications from high-speed communications to quantum computing. Here, we demonstrate photonic chip-based programmable DBRs at telecommunications wavelengths, which are formed by electro-optically inducing refractive index contrast between periodic ferroelectric domains in thin-film lithium niobate waveguides. We achieve voltage-controlled Bragg reflection from zero to near-unity, and gigahertz-speed reflectivity modulation. Our results bring DBRs into the ultrafast programmable regime, opening new opportunities in topological photonics, cavity quantum electrodynamics, integrated lasers, and optical interconnects. The interplay between nanoscale ferroelectric domain engineering and strong electro-optic nonlinearity establishes a new design strategy for nanophotonic devices, otherwise inaccessible in bulk media.

physics.optics↗

arXiv2026

Simulation-guided design of an integrated photonic cavity for frequency-multiplexed Spontaneous Parametric Down Conversion

Frequency-multiplexed entangled photon pair sources with narrow bandwidths and high pair generation efficiency are a key enabling technology for quantum networking. We present a simulation-based design study of an integrated photonic racetrack resonator source for spontaneous parametric down-conversion (SPDC) that simultaneously achieves all three properties. The central result is a simulated set of 90 doubly resonant signal/idler frequency-mode pairs with an effective Schmidt number of 89.62, average bandwidths of 1.08 GHz, a mean free spectral range of 51.9 GHz, and a total internal pair-generation-rate efficiency of 1.16 GHz/mW. Under deterministic wavelength-based splitting, the accessible frequency-state Schmidt number is reduced to 44.93. To support these predictions, we derive a closed-form analytical connection between classical cavity parameters (resonant frequencies, decay rates, coupling coefficients) and the quantum joint spectral amplitude and pair generation rate, extending the dispersive-medium quantization formalism of Raymer to the nonlinear optical cavity case. We demonstrate how classical electromagnetic field simulations can be combined with this analytical framework to predict quantum figures of merit for an integrated photonic source prior to fabrication. Fabrication and experimental validation are left for future work.

quant-ph↗

arXiv2026

Ultracoherent self-assembled diamond nanomechanics reveals superfluid dynamics

From gravitational-wave detection, protein force microscopy, to exploration of quantum-classical boundaries, many anticipated discoveries in fundamental science require improving measurement sensitivity limits. Through the fluctuation-dissipation theorem, mechanical dissipation sets the acoustic noise for this limit. Yet, even in high-purity crystals, the microscopic mechanisms responsible for the acoustic loss remain poorly understood. Tension-induced dissipation dilution offers a route to ultralow acoustic loss, but is challenging to implement in crystalline materials including single-crystal diamond. Here we realize a strain-engineered diamond nanomechanical platform using a liquid-assisted van der Waals self-assembly process that harnesses intrinsic surface forces to apply tensile stress exceeding 1 GPa. At cryogenic temperatures these resonators achieve quality factors beyond 10 billion (intrinsic material quality factors beyond 100 million). This exceptional coherence turns them into a sensitive probe for residual dissipation, elucidating three distinct two-level-system channels and one topological dissipation channel from a surface superfluid helium film. Our work shows how advancing mechanical coherence opens access to new regimes of physics in hybrid quantum systems, precision metrology, and condensed-matter physics.

cond-mat.mes-hall↗

arXiv2026

Generalized model of anisotropic thermo-optic response on thin-film lithium niobate platform

Thermo-optic (TO) control is crucial for thin-film lithium niobate (TFLN) photonic integrated circuits (PICs), offering a simple and practical method for low-frequency and DC tuning while remaining compatible with high-frequency electro-optic (EO) modulation. In x-cut TFLN, the TO response is inherently anisotropic, depending on both waveguide propagation angle and polarization due to the mode-specific overlap of the electric field with the ordinary and extraordinary refractive index axes of the crystal. Despite its significance, a systematic and quantitative analysis of this anisotropy has remained elusive. Here, we present the first generalized analytical model that describes the anisotropic TO response as a function of polarization and arbitrary waveguide orientation, and rigorously validate it through numerical simulations and experiments. This study provides foundational insight into anisotropic thermal tuning and enables new opportunities for engineering energy-efficient and scalable photonic design in next-generation TFLN PICs.

physics.optics↗

arXiv2025

Spectral-temporal processing using integrated recursive electro-optic circuit

Advances in integrated photonics have enabled unprecedented level of control of light, powering a wide range of photonic technologies from communications and computing to precision metrology and quantum information. However, the conventional on-chip optical signal processing approaches based on optical waveguides and cavities suffer from their large physical footprint and narrow operating bandwidth, respectively. To address this, we propose and experimentally demonstrate, using the thin film lithium niobate (TFLN) photonics, a modular, recursive optical signal processing framework. In our approach, fast electro-optic (EO) switch is used to either keep an optical packet inside the loop, with the processing element embedded within, or to release it from the loop and direct it towards the output waveguide. By configuring the switch on a timescale shorter than a time the photon spends traversing the loop, this architecture can achieve different optical pathlengths in a compact footprint without sacrificing optical bandwidth. As an example, we embed a phase-modulator (PM) inside the loop and demonstrate a frequency shift of optical packets up to 420 GHz, using only a 3 GHz sinusoidal microwave signal. By replacing the PM with chirped Bragg gratings (CBG), we demonstrate recursive delay line featuring large group delays of 28 ps/nm over a 30 nm optical bandwidth. Finally, by introducing asymmetric Mach-Zehnder interferometer (AMZI) inside the loop, we demonstrate a reconfigurable differentiation of the optical packet in time, up to an unprecedented fifth-order. Our results establish a powerful and scalable platform for multifunctional photonic processing, setting the stage for next-generation integrated systems with ultrahigh reconfigurability and spectral-temporal versatility.

physics.optics↗

arXiv2025

High Finesse Buckled Microcavities

Optical cavities are widely used in modern science and technology to enable a wide range of both quantum and classical applications. Recently, the growing demand for miniaturization and high performance has fueled the exploration of new fabrication methods beyond traditional polishing techniques and macroscopic mirrors. Visible and near-infrared (NIR) wavelengths are particularly important for quantum applications, where achieving low-loss resonators is also more challenging than in the telecom range, presenting unique challenges and opportunities for microscopic cavity systems. Here, we present a novel fabrication method for making NIR microcavities using buckled dielectric membrane mirrors, achieving a record finesse of 0.9 million at 780 nm. We demonstrated flexible device geometries, including singular mirrors and mirror arrays, featuring radii of curvature ranging from 1 mm to 10 mm. The fabrication process offers high uniformity, high yield, and robust performance across a wide range of cavity lengths. Additionally, we can produce easy-to-assemble microcavity packages, with a total volume of ~2 (4) $\,\mathrm{mm}^3\,$, featuring optical modes with a linewidth of 5.16 MHz (570 kHz) and a free spectral range of 3.18 THz (150 GHz). Our results extend the frontier of microcavity fabrication for classical and quantum photonic technologies.

physics.optics↗

arXiv2025

Strong-coupling and high-bandwidth cavity electro-optic modulation for advanced pulse-comb synthesis

Cavity electro-optic (EO) modulation plays a pivotal role in optical pulse and frequency comb synthesis, supporting a wide range of applications including communication, computing, ranging, and quantum information. The ever-growing demand for these applications has driven efforts in enhancing modulation coupling strength and bandwidth towards advanced pulse-comb synthesis. However, the effects of strong-coupling and high-bandwidth cavity EO modulation remain underexplored, due to the lack of a general, unified model that captures this extreme condition. In this work, we present a universal framework for pulse-comb synthesis under cavity EO modulation, where coupling strength and modulation bandwidth far exceed the cavity's free spectral range (FSR). We show that, under such intense and ultrafast driving conditions, EO-driven frequency combs and pulses exhibit rich higher-order nonlinear dynamics, including temporal pulse compression and comb generation with arbitrary pump detuning. Leveraging this framework, we reveal a direct link between the higher-order dynamics of EO pulse-comb generation and the band structure of synthetic dimension. Furthermore, we demonstrate arbitrary comb shaping via machine-learning-based inverse microwave drive design, achieving a tenfold enhancement in cavity electro-optic comb flatness by exploring the synergistic effects of high-bandwidth driving and detuning-induced frequency boundaries. Our findings push cavity electro-optic modulation into a new frontier, unlocking significant potential for universal and machine-learning-programmable electro-optic frequency combs, topological photonics, as well as photonic quantum computing in the strong-coupling and high-bandwidth regimes.

physics.optics↗

arXiv2025

All-mechanical coherence protection and fast control of a spin qubit

In a phononic quantum network, quantum information is stored and processed within stationary nodes defined by solid-state spins, and the information is routed between nodes by phonons. The phonon holds distinct advantages over its electromagnetic counterpart the photon, including smaller device footprints, reduced crosstalk, long coherence times at low temperatures, and strong interactions with both solid-state spins and electromagnetic waves. Enhanced interactions between a phononic cavity and a stationary qubit have been demonstrated in multiple platforms including superconducting qubits, spins in silicon carbide and spins in diamond. However, an outstanding issue is the compatibility between the spin's coupling to the resonant phononic cavity and the simultaneous use of pulse sequences to extend the coherence time of the spin by suppressing the low-frequency environmental noise. Here we demonstrate all-mechanical coherence protection of a solid-state spin qubit, where optical initialization, quantum operations, and readout are performed in a dressed basis that is highly immune to low-frequency noise and compatible with a phononic cavities. We additionally show record-high Rabi frequencies reaching 800 MHz, which allows for ultrafast quantum control. Our results establish a first step for high-fidelity, phonon-mediated quantum gates and represent a crucial advance toward robust on-chip quantum phononic networks.

quant-ph↗

arXiv2025

A sub-volt near-IR lithium tantalate electro-optic modulator

We demonstrate a low-loss integrated electro-optic Mach-Zehnder modulator in thin-film lithium tantalate at 737 nm, featuring a low half-wave voltage-length product of 0.65 V$\cdot$cm, an extinction ratio of 30 dB, low optical loss of 5.3 dB, and a detector-limited bandwidth of 20 GHz. A small $<2$ dB DC bias drift relative to quadrature bias is measured over 16 minutes using 4.3 dBm of on-chip power in ambient conditions, which outperforms the 8 dB measured using a counterpart thin-film lithium niobate modulator. Finally, an optical loss coefficient of 0.5 dB/cm for a thin-film lithium tantalate waveguide is estimated at 638 nm using a fabricated ring resonator.

physics.optics↗

arXiv2025

Cross-Polarized Stimulated Brillouin Scattering in Lithium Niobate Waveguides

We report on the experimental demonstration of cross-polarization backward stimulated Brillouin scattering (BSBS) in lithium niobate on insulator (LNOI) waveguides. Performing polarization-sensitive pump and probe measurements, we captured both intra- and intermodal scattering between counterpropagating fundamental optical modes. Remarkably, cross-polarization scattering achieved SBS gains that exceeded $G_{B}=$80m$^{-1}$W$^{-1}$. This substantial gain not only broadens the utility of polarization in SBS but also paves the way for high-performance devices, including ultranarrowband lasers, robust broadband nonreciprocal devices, RF filters, and microwave-to-optical converters.

physics.optics↗

arXiv2024

Integrated electro-optic digital-to-analog link for efficient computing and arbitrary waveform generation

The rapid growth in artificial intelligence and modern communication systems demands innovative solutions for increased computational power and advanced signaling capabilities. Integrated photonics, leveraging the analog nature of electromagnetic waves at the chip scale, offers a promising complement to approaches based on digital electronics. To fully unlock their potential as analog processors, establishing a common technological base between conventional digital electronic systems and analog photonics is imperative to building next-generation computing and communications hardware. However, the absence of an efficient interface has critically challenged comprehensive demonstrations of analog advantage thus far, with the scalability, speed, and energy consumption as primary bottlenecks. Here, we address this challenge and demonstrate a general electro-optic digital-to-analog link (EO-DiAL) enabled by foundry-based lithium niobate nanophotonics. Using purely digital inputs, we achieve on-demand generation of (i) optical and (ii) electronic waveforms at information rates up to 186 Gbit/s. The former addresses the digital-to-analog electro-optic conversion challenge in photonic computing, showcasing high-fidelity MNIST encoding while consuming 0.058 pJ/bit. The latter enables a pulse-shaping-free microwave arbitrary waveform generation method with ultrabroadband tunable delay and gain. Our results pave the way for efficient and compact digital-to-analog conversion paradigms enabled by integrated photonics and underscore the transformative impact analog photonic hardware may have on various applications, such as computing, optical interconnects, and high-speed ranging.

physics.optics↗

arXiv2024

High-power and narrow-linewidth laser on thin-film lithium niobate enabled by photonic wire bonding

Thin-film lithium niobate (TFLN) has emerged as a promising platform for the realization of high performance chip-scale optical systems, spanning a range of applications from optical communications to microwave photonics. Such applications rely on the integration of multiple components onto a single platform. However, while many of these components have already been demonstrated on the TFLN platform, to date, a major bottleneck of the platform is the existence of a tunable, high-power, and narrow-linewidth on-chip laser. Here, we address this problem using photonic wire bonding to integrate optical amplifiers with a thin-film lithium niobate feedback circuit, and demonstrate an extended cavity diode laser yielding high on-chip power of 78 mW, side mode suppression larger than 60 dB and wide wavelength tunability over 43 nm. The laser frequency stability over short timescales shows an ultra-narrow intrinsic linewidth of 550 Hz. Long-term recordings indicate a high passive stability of the photonic wire bonded laser with 58 hours of mode-hop-free operation, with a trend in the frequency drift of only 4.4 MHz/h. This work verifies photonic wire bonding as a viable integration solution for high performance on-chip lasers, opening the path to system level upscaling and Watt-level output powers.

physics.optics↗

arXiv2024

Entanglement of Nanophotonic Quantum Memory Nodes in a Telecom Network

A key challenge in realizing practical quantum networks for long-distance quantum communication involves robust entanglement between quantum memory nodes connected via fiber optical infrastructure. Here, we demonstrate a two-node quantum network composed of multi-qubit registers based on silicon-vacancy (SiV) centers in nanophotonic diamond cavities integrated with a telecommunication (telecom) fiber network. Remote entanglement is generated via the cavity-enhanced interactions between the SiV's electron spin qubits and optical photons. Serial, heralded spin-photon entangling gate operations with time-bin qubits are used for robust entanglement of separated nodes. Long-lived nuclear spin qubits are used to provide second-long entanglement storage and integrated error detection. By integrating efficient bi-directional quantum frequency conversion of photonic communication qubits to telecom frequencies (1350 nm), we demonstrate entanglement of two nuclear spin memories through 40 km spools of low-loss fiber and a 35 km long fiber loop deployed in the Boston area urban environment, representing an enabling step towards practical quantum repeaters and large-scale quantum networks.

quant-ph↗

arXiv2024

Stable electro-optic modulators using thin-film lithium tantalate

We demonstrate electro-optic modulators realized in low-loss thin-film lithium tantalate with superior DC-stability (<1 dB power fluctuation from quadrature with 12.1 dBm input) compared to equivalent thin-film lithium niobate modulators (5 dB fluctuation) over 46 hours.

physics.optics↗

arXiv2024

Frequency comb generation via synchronous pumped $χ^{(3)}$ resonator on thin-film lithium niobate

Resonator-based optical frequency comb generation is an enabling technology for a myriad of applications ranging from communications to precision spectroscopy. These frequency combs can be generated in nonlinear resonators driven using either continuous-wave (CW) light, which requires alignment of the pump frequency with the cavity resonance, or pulsed light, which also mandates that the pulse repetition rate and cavity free spectral range (FSR) are carefully matched. Advancements in nanophotonics have ignited interest in chip-scale optical frequency combs. However, realizing pulse-driven on-chip Kerr combs remains challenging, as microresonator cavities have limited tuning range in their FSR and resonance frequency. Here, we take steps to overcome this limitation and demonstrate broadband frequency comb generation using a $χ^{(3)}$ resonator synchronously pumped by a tunable femtosecond pulse generator with on-chip amplitude and phase modulators. Notably, employing pulsed pumping overcomes limitations in Kerr comb generation typically seen in crystalline resonators from stimulated Raman scattering.

physics.optics↗