arXiv subjects

Marko Loncar

Publications and source records attributed to Marko Loncar.

At least 73 records · Page 4Linked to original sources

arXiv2018

Spectral alignment of single-photon emitters in diamond using strain gradient

Solid-state single-photon emitters are attractive for realization of integrated quantum systems due to their experimental convenience and scalability. Unfortunately, however, their complex mesoscopic environments cause photons from different emitters to be spectrally distinguishable. Here we demonstrate spectral alignment of two solid-state single-photon emitters by utilizing the strain gradient. Multiple germanium vacancy (GeV) color centers in diamond are created in fabricated diamond microcantilevers using focused ion beam implantation. The strain response of the electronic energy levels of the GeV is measured by inducing an electrically controlled strain in the device. Leveraging the large strain gradient, we tune two GeVs in the spot to emit at the same optical wavelength. Simultaneous resonant excitation of two spectrally aligned GeVs is demonstrated using a narrow linewidth laser. This strain gradient tuning can be used to realize spectrally identical quantum emitters for on-chip integrated quantum systems.

cond-mat.mes-hall↗

arXiv2018

Controlling the coherence of a diamond spin qubit through strain engineering

The uncontrolled interaction of a quantum system with its environment is detrimental for quantum coherence. In the context of solid-state qubits, techniques to mitigate the impact of fluctuating electric and magnetic fields from the environment are well-developed. In contrast, suppression of decoherence from thermal lattice vibrations is typically achieved only by lowering the temperature of operation. Here, we use a nano-electro-mechanical system (NEMS) to mitigate the effect of thermal phonons on a solid-state quantum emitter without changing the system temperature. We study the silicon-vacancy (SiV) colour centre in diamond which has optical and spin transitions that are highly sensitive to phonons. First, we show that its electronic orbitals are highly susceptible to local strain, leading to its high sensitivity to phonons. By controlling the strain environment, we manipulate the electronic levels of the emitter to probe, control, and eventually, suppress its interaction with the thermal phonon bath. Strain control allows for both an impressive range of optical tunability and significantly improved spin coherence. Finally, our findings indicate that it may be possible to achieve strong coupling between the SiV spin and single phonons, which can lead to the realisation of phonon-mediated quantum gates and nonlinear quantum phononics.

quant-ph↗

arXiv2018

Strain engineering of the silicon-vacancy center in diamond

We control the electronic structure of the silicon-vacancy (SiV) color-center in diamond by changing its static strain environment with a nano-electro-mechanical system. This allows deterministic and local tuning of SiV optical and spin transition frequencies over a wide range, an essential step towards multi-qubit networks. In the process, we infer the strain Hamiltonian of the SiV revealing large strain susceptibilities of order 1 PHz/strain for the electronic orbital states. We identify regimes where the spin-orbit interaction results in a large strain suseptibility of order 100 THz/strain for spin transitions, and propose an experiment where the SiV spin is strongly coupled to a nanomechanical resonator.

quant-ph↗

arXiv2017

An integrated diamond Raman laser pumped in the near-visible

Using a high-Q diamond microresonator (Q > 300,000) interfaced with high-power-handling directly-written doped-glass waveguides, we demonstrate a Raman laser in an integrated platform pumped in the near-visible. Both TM-to-TE and TE-to-TE lasing is observed, with a Raman lasing threshold as low as 20 mW and Stokes power of over 1 mW at 120 mW pump power. Stokes emission is tuned over a 150 nm (60 THz) bandwidth around 875 nm wavelength, corresponding to 17.5% of the center frequency.

physics.optics↗

arXiv2017

Monolithic Ultrahigh-Q Lithium Niobate Microring Resonator

We demonstrate an ultralow loss monolithic integrated lithium niobate photonic platform consisting of dry-etched subwavelength waveguides. We show microring resonators with a quality factor of 10$^7$ and waveguides with propagation loss as low as 2.7 dB/m.

physics.optics↗

arXiv2017

Strongly Cavity-Enhanced Spontaneous Emission from Silicon-Vacancy Centers in Diamond

Quantum emitters are an integral component for a broad range of quantum technologies including quantum communication, quantum repeaters, and linear optical quantum computation. Solid-state color centers are promising candidates for scalable quantum optics due to their long coherence time and small inhomogeneous broadening. However, once excited, color centers often decay through phonon-assisted processes, limiting the efficiency of single photon generation and photon mediated entanglement generation. Herein, we demonstrate strong enhancement of spontaneous emission rate of a single silicon-vacancy center in diamond embedded within a monolithic optical cavity, reaching a regime where the excited state lifetime is dominated by spontaneous emission into the cavity mode. We observe 10-fold lifetime reduction and 42-fold enhancement in emission intensity when the cavity is tuned into resonance with the optical transition of a single silicon-vacancy center, corresponding to 90% of the excited state energy decay occurring through spontaneous emission into the cavity mode. We also demonstrate the largest to date coupling strength ($g/2π=4.9\pm0.3 GHz$) and cooperativity ($C=1.4$) for color-center-based cavity quantum electrodynamics systems, bringing the system closer to the strong coupling regime.

quant-ph↗

arXiv2017

Efficient quantum microwave-to-optical conversion using electro-optic nanophotonic coupled-resonators

We propose a low noise, triply-resonant, electro-optic (EO) scheme for quantum microwave-to-optical conversion based on coupled nanophotonics resonators integrated with a superconducting qubit. Our optical system features a split resonance - a doublet - with a tunable frequency splitting that matches the microwave resonance frequency of the superconducting qubit. This is in contrast to conventional approaches where large optical resonators with free-spectral range comparable to the qubit microwave frequency are used. In our system, EO mixing between the optical pump coupled into the low frequency doublet mode and a resonance microwave photon results in an up-converted optical photon on resonance with high frequency doublet mode. Importantly, the down-conversion process, which is the source of noise, is suppressed in our scheme as the coupled-resonator system does not support modes at that frequency. Our device has at least an order of magnitude smaller footprint than the conventional devices, resulting in large overlap between optical and microwave fields and large photon conversion rate ($g/2π$) in the range of $\sim$5-15 kHz. Owing to large $g$ factor and doubly-resonant nature of our device, microwave-to-optical frequency conversion can be achieved with optical pump powers in the range of tens of microwatts, even with moderate values for optical $\it{Q}$ ($\sim 10^6$) and microwave $Q$ ($ \sim10^4$). The performance metrics of our device, with substantial improvement over the previous EO-based approaches, promise a scalable quantum microwave-to-optical conversion and networking of superconducting processors via optical fiber communication.

quant-ph↗

arXiv2017

Robust nano-fabrication of an integrated platform for spin control in a tunable microcavity

Coupling nitrogen-vacancy centers in diamond to optical cavities is a promising way to enhance the efficiency of diamond based quantum networks. An essential aspect of the full toolbox required for the operation of these networks is the ability to achieve microwave control of the electron spin associated with this defect within the cavity framework. Here, we report on the fabrication of an integrated platform for microwave control of an NV center electron spin in an open, tunable Fabry-Perot microcavity. A critical aspect of the measurements of the cavity's finesse reveals that the presented fabrication process does not compromise its optical properties. We provide a method to incorporate a thin diamond slab into the cavity architecture and demonstrate control of the NV center spin. These results show the promise of this design for future cavity-enhanced NV center spin-photon entanglement experiments.

quant-ph↗

arXiv2017

Metasurface-assisted phase-matching-free second harmonic generation in lithium niobate waveguides

The phase-matching condition is a key aspect in nonlinear wavelength conversion processes, which requires the momenta of the photons involved in the processes to be conserved. Conventionally, nonlinear phase matching is achieved using either birefringent or periodically poled nonlinear crystals, which requires careful dispersion engineering and are usually narrowband. In recent years, metasurfaces consisting of densely packed arrays of optical antennas have been demonstrated to provide an effective optical momentum to bend light in arbitrary ways. Here, we demonstrate that gradient metasurface structures consisting of phased array antennas are able to circumvent the phase-matching requirement in on-chip nonlinear wavelength conversion. We experimentally demonstrate phase-matching-free second harmonic generation over many coherent lengths in thin film lithium niobate waveguides patterned with the gradient metasurfaces. Efficient second-harmonic generation (1660% W-1cm-2) in the metasurface-based devices was observed over a wide range of pump wavelengths (1580-1650 nm).

physics.optics↗

arXiv2017

Competition between Raman and Kerr effects in microresonator comb generation

We investigate the effects of Raman and Kerr gain in crystalline microresonators and determine the conditions required to generate modelocked frequency combs. We show theoretically that strong, narrowband Raman gain determines a maximum microresonator size allowable to achieve comb formation. We verify this condition experimentally in diamond and silicon microresonators and show that there exists a competition between Raman and Kerr effects that leads to the existence of two different comb states.

physics.optics↗

arXiv2017

Nanophotonic Lithium Niobate Electro-optic Modulators

Modern communication networks require high performance and scalable electro-optic modulators that convert electrical signals to optical signals at high speed. Existing lithium niobate modulators have excellent performance but are bulky and prohibitively expensive to scale up. Here we demonstrate scalable and high-performance nanophotonic electro-optic modulators made of single-crystalline lithium niobate microring resonators and micro-Mach-Zehnder interferometers. We show a half-wave electro-optic modulation efficiency of 1.8V$\cdot$cm and data rates up to 40 Gbps.

physics.optics↗

arXiv2016

Large-scale quantum-emitter arrays in atomically thin semiconductors

The flourishing field of two-dimensional (2D) nanophotonics has generated much excitement in the quantum technologies community after the identification of quantum emitters (QEs) in layered materials (LMs). LMs offer many advantages as platforms for quantum circuits, such as integration within hybrid technologies, valley degree of freedom and strong spin-orbit coupling. QEs in LMs, however, suffer from uncontrolled occurrences, added to the uncertainty over their origin, which has been linked to defects and strain gradients. Here, we report a scalable method to create arrays of single-photon emitting QEs in tungsten diselenide (WSe2) and tungsten disulphide (WS2) using a nanopatterned silica substrate. We obtain devices with QE numbers in the range of hundreds, limited only by the flake size, and a QE yield approaching unity. The overall quality of these deterministic QEs surpasses that of their randomly appearing counterparts, with spectral wanderings of around 0.1 meV, an order of magnitude lower than previous reports. Our technique solves the scalability challenge for LM-based quantum photonic devices.

cond-mat.mes-hall↗

arXiv2015

On-Chip Diamond Raman Laser

Synthetic single-crystal diamond has recently emerged as a promising platform for Raman lasers at exotic wavelengths due to its giant Raman shift, large transparency window and excellent thermal properties yielding a greatly enhanced figure-of-merit compared to conventional materials. To date, diamond Raman lasers have been realized using bulk plates placed inside macroscopic cavities, requiring careful alignment and resulting in high threshold powers (~W-kW). Here we demonstrate an on-chip Raman laser based on fully-integrated, high quality-factor, diamond racetrack micro-resonators embedded in silica. Pumping at telecom wavelengths, we show Stokes output discretely tunable over a ~100nm bandwidth around 2-μm with output powers >250 μW, extending the functionality of diamond Raman lasers to an interesting wavelength range at the edge of the mid-infrared spectrum. Continuous-wave operation with only ~85 mW pump threshold power in the feeding waveguide is demonstrated along with continuous, mode-hop-free tuning over ~7.5 GHz in a compact, integrated-optics platform.

physics.optics↗

arXiv2015

Percolation lithography: Tuning and freezing disorder in 3D photonic crystals using partial wetting and drying

Although complex, hierarchical nanoscale geometries with tailored degrees of disorder are commonly found in biological systems, few simple self-assembly routes to fabricating synthetic analogues have been identified. We present two techniques that exploit basic capillary phenomena to finely control disorder in porous 3D photonic crystals, leading to complex and hierarchical geometries. In the first, we exposed the structures to mixtures of ethanol and water that partially wet their pores, where small adjustments to the ethanol content controlled the degree of partial wetting. In the second, we infiltrated the structures with thin films of volatile alkanes and observed a sequence of partial infiltration patterns as the liquid evaporated. In both cases, macroscopic symmetry breaking was driven by subtle sub-wavelength variations in the pore geometry that directed site-selective infiltration of liquids. The resulting patterns, well described by percolation theory, had significant effects on the photonic structures' optical properties, including the wavelength-dependence and angular dependence of scattering. Incorporating cross-linkable resins into our liquids, we were able create permanent photonic structures with these properties by freezing in place the filling patterns at arbitrary degrees of partial wetting and intermediate stages of drying. These techniques illustrate the versatility of interfacial phenomena in directing and tuning self-assembly of aperiodic structures.

physics.optics↗

arXiv2015

Cavity-enhanced second harmonic generation via nonlinear-overlap optimization

We describe an approach based on topology optimization that enables automatic discovery of wavelength-scale photonic structures for achieving high-efficiency second-harmonic generation (SHG). A key distinction from previous formulation and designs that seek to maximize Purcell factors at individual frequencies is that our method not only aims to achieve frequency matching (across an entire octave) and large radiative lifetimes, but also optimizes the equally important nonlinear--coupling figure of merit $\barβ$, involving a complicated spatial overlap-integral between modes. We apply this method to the particular problem of optimizing micropost and grating-slab cavities (one-dimensional multilayered structures) and demonstrate that a variety of material platforms can support modes with the requisite frequencies, large lifetimes $Q > 10^4$, small modal volumes $\sim (λ/n)^3$, and extremely large $\barβ \gtrsim 10^{-2}$, leading to orders of magnitude enhancements in SHG efficiency compared to state of the art photonic designs. Such giant $\barβ$ alleviate the need for ultra-narrow linewidths and thus pave the way for wavelength-scale SHG devices with faster operating timescales and higher tolerance to fabrication imperfections.

physics.optics↗

arXiv2014

Classical and fluctuation-induced electromagnetic interactions in micronscale systems: designer bonding, antibonding, and Casimir forces

Whether intentionally introduced to exert control over particles and macroscopic objects, such as for trapping or cooling, or whether arising from the quantum and thermal fluctuations of charges in otherwise neutral bodies, leading to unwanted stiction between nearby mechanical parts, electromagnetic interactions play a fundamental role in many naturally occurring processes and technologies. In this review, we survey recent progress in the understanding and experimental observation of optomechanical and quantum-fluctuation forces. Although both of these effects arise from exchange of electromagnetic momentum, their dramatically different origins, involving either real or virtual photons, lead to different physical manifestations and design principles. Specifically, we describe recent predictions and measurements of attractive and repulsive optomechanical forces, based on the bonding and antibonding interactions of evanescent waves, as well as predictions of modified and even repulsive Casimir forces between nanostructured bodies. Finally, we discuss the potential impact and interplay of these forces in emerging experimental regimes of micromechanical devices.

physics.optics↗

arXiv2014

Superconducting Nanowire Single Photon Detector on Diamond

Superconducting nanowire single photon detectors (SNSPDs) are fabricated directly on diamond substrates and their optical and electrical properties are characterized. Dark count performance and photon count rates are measured at varying temperatures for 1310nm and 632nm photons. The procedure to prepare diamond substrate surfaces suitable for the deposition and patterning of thin film superconducting layers is reported. Using this approach, diamond substrates with less than 300pm RMS surface roughness are obtained.

physics.optics↗

arXiv2013

High-efficiency degenerate four wave-mixing in triply resonant nanobeam cavities

We demonstrate high-efficiency, degenerate four-wave mixing in triply resonant Kerr $χ^(3)$ photonic crystal (PhC) nanobeam cavities. Using a combination of temporal coupled mode theory and nonlinear finite-difference time-domain (FDTD) simulations, we study the nonlinear dynamics of resonant four-wave mixing processes and demonstrate the possibility of observing high-efficiency limit cycles and steady-state conversion corresponding to $\approx 100$% depletion of the pump light at low powers, even including effects due to losses, self- and cross-phase modulation, and imperfect frequency matching. Assuming operation in the telecom range, we predict close to perfect quantum efficiencies at reasonably low $\sim$ 50 mW input powers in silicon micrometer-scale cavities.

physics.optics↗