arXiv subjects

Markus Allgaier

Publications and source records attributed to Markus Allgaier.

18 recordsLinked to original sources

arXiv2026

High-performance source of indistinguishable polarization-entangled photons with a local oscillator reference for quantum networking

Optical quantum networking protocols impose stringent requirements on the states produced by sources of entanglement. We demonstrate a free-space, compact, source of indistinguishable pairs of polarization entangled photons, with an integrated local oscillator reference as a significant step towards this goal. This source achieves $(99.11 \pm 0.01) \%$ polarization entanglement visibility, $(96.3 \pm 0.6) \%$ successive-photon Hong-Ou-Mandel interference visibility, $(68.0 \pm 0.1$) \% heralded efficiency as detected, and $(88.6 \pm 0.2) \%$ interference visibility with a local oscillator. This simultaneous achievement of state-of-the-art metrics demonstrates an adaptable platform for quantum networking.

quant-ph↗

arXiv2026

State Engineering via Nonlinear Interferometry with Linear Spectral Phases

Many protocols within quantum cryptography, communications, and computing require the ability to generate entangled states as well as spectral qudits. Nonlinear interferometry is a viable way to engineer these complex quantum states of light. However, it is difficult to achieve a high level of control over spectral correlations. Here, we present a protocol utilizing a nonlinear interferometer with linear spectral phases that can generate both high-dimensional spectral qudits and high-dimensional entangled states. We model the effect of loss and loss of overlap on interference visibility and thereby on the states generated.

quant-ph↗

arXiv2023

Interferometric imaging using shared quantum entanglement

Quantum entanglement-based imaging promises significantly increased resolution by extending the spatial separation of optical collection apertures used in very-long-baseline interferometry for astronomy and geodesy. We report a table-top entanglement-based interferometric imaging technique that utilizes two entangled field modes serving as a phase reference between two apertures. The spatial distribution of a simulated thermal light source is determined by interfering light collected at each aperture with one of the entangled fields and performing joint measurements. This experiment demonstrates the ability of entanglement to implement interferometric imaging.

quant-ph↗

arXiv2022

Tailored frequency conversion makes infrared light visible for streak cameras

Streak cameras are one of the most common and convenient devices to measure pulsed emission e.g. from semiconductor lightsources with picosecond time resolution. However, they are most sensitive in the visible range and possess low or negligible efficiency in the infrared and telecom regime. In this work, we present a frequency conversion based on sum-frequency generation that converts infrared to visible signals while preserving their temporal properties, making them detectable with a streak camera. We demonstrate and verify the functionality of our device by converting the emission from a quantum dot laser.

physics.optics↗

arXiv2022

Smartphone-based measurements of the optical properties of snow

Snow is a highly complex medium composed of ice crystals of various shapes and sizes. Knowledge of its intrinsic optical properties such as the scattering and absorption coefficient is tantamount to radiative transfer models in climate research. The absorption coefficient, in particular, allows us to access information about light-absorbing particles contained in the snow. In contrast to snow's apparent properties like the albedo, measuring the intrinsic properties is challenging. Here, we present a simple apparatus that can measure bulk optical properties of snow using readily available components and a smartphone camera, and a robust diffuse-optical framework for data analysis. We demonstrate the instrument both on scattering phantoms with known scattering and absorption coefficient as well as in the field. Its low cost, simplicity and portability uniquely qualify this setup for large-scale field work, undergraduate education and citizen science.

physics.ins-det↗

arXiv2022

Direct measurement of optical properties of glacier ice using a photon-counting diffuse LiDAR

The production of meltwater from glacier ice, which is exposed at the margins of land ice during the summer, is responsible for a large proportion of glacier mass loss. The rate of meltwater production from glacier ice is especially sensitive to its physical structure and chemical composition which combine to determine the albedo of glacier ice. However, the optical properties of near-surface glacier ice are not well known since most prior work has focused on ice made in the laboratory or from deep cores. Here, we demonstrate a measurement technique based on diffuse propagation of nanosecond-duration laser pulses in near-surface glacier ice that enables the independent measurement of the scattering and absorption coefficients, allowing for a complete description of the processes governing radiative transfer. We employ a photon-counting detector to overcome the high losses associated with diffuse optics. The instrument is highly portable and rugged, making it optimally suited for deployment in remote regions. A set of measurements taken on Collier Glacier, Oregon, serves as a demonstration of the technique. These measurements provide insight into both physical structure and composition of near-surface glacier ice and open new avenues for the analysis of light-absorbing impurities and remote sensing of the cryosphere.

physics.optics↗

arXiv2021

Diffuse optics for glaciology

Optical probing of glaciers has the potential for tremendous impact on environmental science. However, glacier ice is turbid, which prohibits the use of most established optical measurements for determining a glacier's interior structure. Here, we propose a method for determining the depth, scattering and absorption length based upon diffuse propagation of short optical pulses. Our model allows us to extract several characteristics of the glacier. Performing Monte Carlo simulations implementing Mie scattering and mixed boundary conditions, we show that the proposed approach should be feasible with current technology. The results suggest that optical properties and geometry of the glacier can be extracted from realistic measurements, which could be implemented with low cost and small footprint.

physics.optics↗

arXiv2021

Quantifying the enhancement of two-photon absorption due to spectral-temporal entanglement

When a low flux of time-frequency-entangled photon pairs (EPP) illuminates a two-photon transition, the rate of two-photon absorption (TPA) can be enhanced considerably by the quantum nature of photon number correlations and frequency correlations. We present a quantum-theoretic derivation of entangled TPA (ETPA) and calculate an upper bound on the amount of quantum enhancement that is possible in such systems. The derived bounds indicate that in order to observe ETPA the experiments would need to operate at a combination of significantly higher rates of EPP illumination, molecular concentrations, and conventional TPA cross sections than are achieved in typical experiments.

quant-ph↗

arXiv2020

Experimental feasibility of molecular two-photon absorption with isolated time-frequency-entangled photon pairs

Entangled photon pairs have been promised to deliver a substantial quantum advantage for two-photon absorption spectroscopy. However, recent work has challenged the previously reported magnitude of quantum enhancement in two-photon absorption. Here, we present an experimental comparison of sum-frequency generation and molecular absorption, each driven by isolated photon pairs. We establish an upper bound on the enhancement for entangled-two-photon absorption in Rhodamine-6G, which lies well below previously reported values.

quant-ph↗

arXiv2020

Two-photon absorption of time-frequency-entangled photon pairs by molecules: the roles of photon-number correlations and spectral correlations

While two-photon absorption (TPA) and other forms of nonlinear interactions of molecules with isolated time-frequency-entangled photon pairs (EPP) have been predicted to display a variety of fascinating effects, their potential use in practical quantum-enhanced molecular spectroscopy requires close examination. This paper presents a detailed theoretical study of quantum-enhanced TPA by both photon-number correlations and spectral correlations, including an account of the deleterious effects of dispersion. While such correlations in EPP created by spontaneous parametric down conversion can increase the TPA rate significantly in the regime of extremely low optical flux, we find that for typical molecules in solution this regime corresponds to such low TPA event rates as to be unobservable in practice. Our results support the usefulness of EPP spectroscopy in atomic or other narrow-linewidth systems, while questioning the efficacy of such approaches for broadband systems including molecules in solution.

quant-ph↗

arXiv2020

Temporal mode transformations by sequential time and frequency phase modulation for applications in quantum information science

Controlling the temporal mode shape of quantum light pulses has wide ranging application to quantum information science and technology. Techniques have been developed to control the bandwidth, allow shifting in the time and frequency domains, and perform mode-selective beam-splitter-like transformations. However, there is no present scheme to perform targeted multimode unitary transformations on temporal modes. Here we present a practical approach to realize general transformations for temporal modes. We show theoretically that any unitary transformation on temporal modes can be performed using a series of phase operations in the time and frequency domains. Numerical simulations show that several key transformations on temporal modes can be performed with greater than 95% fidelity using experimentally feasible specifications.

physics.optics↗

arXiv2018

Pulse shaping using dispersion-engineered difference frequency generation

The temporal-mode (TM) basis is a prime candidate to perform high-dimensional quantum encoding. Quantum frequency conversion has been employed as a tool to perform tomographic analysis and manipulation of ultrafast states of quantum light necessary to implement a TM-based encoding protocol. While demultiplexing of such states of light has been demonstrated in the Quantum Pulse Gate (QPG), a multiplexing device is needed to complete an experimental framework for TM encoding. In this work we demonstrate the reverse process of the QPG. A dispersion-engineered difference frequency generation in non-linear optical waveguides is employed to imprint the pulse shape of the pump pulse onto the output. This transformation is unitary and can be more efficient than classical pulse shaping methods. We experimentally study the process by shaping the first five orders of Hermite-Gauss modes of various bandwidths. Finally, we establish and model the limits of practical, reliable shaping operation.

quant-ph↗

arXiv2018

Tomography and Purification of the Temporal-Mode Structure of Quantum Light

High-dimensional quantum information processing promises capabilities beyond the current state of the art, but addressing individual information-carrying modes presents a significant experimental challenge. Here we demonstrate effective high-dimensional operations in the time-frequency domain of non-classical light. We generate heralded photons with tailored temporal-mode structures through ultrafast pulse shaping of a parametric downconversion pump. We then implement a quantum pulse gate, enabled by dispersion-engineered sum-frequency generation, to project onto programmable temporal modes, reconstructing the quantum state in seven dimensions. We also manipulate the time-frequency structure by selectively removing temporal modes, explicitly demonstrating the effectiveness of engineered nonlinear processes for mode-selective manipulation of quantum states.

quant-ph↗

arXiv2017

Temporal-mode measurement tomography of a quantum pulse gate

Encoding quantum information in the photon temporal mode (TM) offers a robust platform for high-dimensional quantum protocols. The main practical challenge, however, is to design a device that operates on single photons in specific TMs and all coherent superpositions. The quantum pulse gate (QPG) is a mode-selective sum-frequency generation designed for this task. Here, we perform a full modal characterisation of a QPG using weak coherent states in well-defined TMs. We reconstruct a full set of measurement operators, which show an average fidelity of 0.85 to a theoretically ideal device when operating on a 7-dimensional space. Then we use these characterised measurement operators of the QPG to calibrate the device. Using the calibrated device and a tomographically complete set of measurements, we show that the QPG can perform high-dimensional TM state tomography with 0.99 fidelity.

quant-ph↗

arXiv2017

Streak-camera measurements of single photons at telecom wavelength

Up to this point streak-cameras have been a powerful tool for temporal characterization of ultrafast light pulses even at the single photon level. However, the low signal-to-noise ratio in the infrared range prevents measurement on weak light sources in the telecom regime. We present an approach to circumvent this problem. The method utilizes an up-conversion process in periodically poled waveguides in Lithium Niobate. We convert single photons from a parametric down-conversion source in order to reach the point of maximum detection efficiency of commercially available streak-cameras. We explore phase-matching configurations to investigate the up-conversion scheme in real-world applications.

quant-ph↗

arXiv2017

Fast time-domain measurements on telecom single photons

Direct measurements on the temporal envelope of quantum light are a challenging task and not many examples are known since most classical pulse characterisation methods do not work on the single photon level. Knowledge of both spectrum and timing can however give insights on properties that cannot be determined by the spectrum alone. While temporal measurements on single photons on timescales of tens of picoseconds are possible with superconducting photon detectors and picosecond measurements have been performed using streak cameras, there are no commercial single photon sensitive devices with femtosecond resolution available. While time-domain sampling using sum-frequency generation has been already exploited for such measurement, inefficient conversion has necessitated long integration times to build the temporal profile. We demonstrate a highly efficient waveguided sum-frequency generation process in Lithium Niobate to measure the temporal envelope of single photons with femtosecond resolution with short enough acquisition time to provide a live-view of the measurement. We demonstrate the measurement technique and combine it with spectral measurements using a dispersive fiber time-of-flight spectrometer to determine upper and lower bounds for the spectral purity of heralded single photons. The approach complements the joint spectral intensity measurements as a measure on the purity can be given without knowledge of the spectral phase.

quant-ph↗

arXiv2016

Highly efficient frequency conversion with bandwidth compression of quantum light

Hybrid quantum networks rely on efficient interfacing of dissimilar quantum nodes, since elements based on parametric down-conversion sources, quantum dots, color centres or atoms are fundamentally different in their frequencies and bandwidths. While pulse manipulation has been demonstrated in very different systems, to date no interface exists that provides both an efficient bandwidth compression and a substantial frequency translation at the same time. Here, we demonstrate an engineered sum-frequency-conversion process in Lithium Niobate that achieves both goals. We convert pure photons at telecom wavelengths to the visible range while compressing the bandwidth by a factor of 7.47 under preservation of non-classical photon-number statistics. We achieve internal conversion efficiencies of 75.5%, significantly outperforming spectral filtering for bandwidth compression. Our system thus makes the connection between previously incompatible quantum systems as a step towards usable quantum networks.

quant-ph↗

arXiv2015

Regular modes of a mixed dynamical based optical fiber

A multimode optical fiber with a truncated transverse cross section acts as a powerful versatile support to investigate the wave features of complex ray dynamics. In this paper, we concentrate on the case of a geometry inducing a mixed dynamics. We highlight the properties of regular modes associated to stable periodic orbits such as an enhanced intensity localization and report unexpected attributes such as the statistics of the Inverse Participation Ratio that present features analogous to those of Anderson localized modes. Our study is supported by both numerical and experimental results.

physics.optics↗