arXiv subjects

Markus Garst

Publications and source records attributed to Markus Garst.

At least 55 records · Page 3Linked to original sources

arXiv2015

Spin-orbit physics of j=1/2 Mott insulators on the triangular lattice

The Heisenberg-Kitaev (HK) model on the triangular lattice is conceptually interesting for its interplay of geometric and exchange frustration. HK models are also thought to capture the essential physics of the spin-orbital entanglement in effective $j=1/2$ Mott insulators studied in the context of various 5d transition metal oxides. Here we argue that the recently synthesized Ba$_3$IrTi$_2$O$_9$ is a prime candidate for a microscopic realization of the triangular HK model. We establish that an infinitesimal Kitaev exchange destabilizes the 120$^\circ$ order of the quantum Heisenberg model and results in the formation of an extended $\mathbb{Z}_2$-vortex crystal phase in the parameter regime most likely relevant to the real material. Using a combination of analytical and numerical techniques we map out the entire phase diagram of the model, which further includes various ordered phases as well as an extended nematic phase around the antiferromagnetic Kitaev point.

cond-mat.str-el↗

arXiv2014

Magnon-skyrmion scattering in chiral magnets

Chiral magnets support topological skyrmion textures due to the Dzyaloshinskii-Moriya spin-orbit interaction. In the presence of a sufficiently large applied magnetic field, such skyrmions are large amplitude excitations of the field-polarized magnetic state. We investigate analytically the interaction between such a skyrmion excitation and its small amplitude fluctuations, i.e., the magnons in a clean two-dimensional chiral magnet. The magnon spectrum is found to include two magnon-skyrmion bound states corresponding to a breathing mode and, for intermediate fields, a quadrupolar mode, which will give rise to subgap magnetic and electric resonances. Due to the skyrmion topology, the magnons scatter from a Aharonov-Bohm flux density that leads to skew and rainbow scattering, characterized by an asymmetric differential cross section with, in general, multiple peaks. As a consequence of the skew scattering, a finite density of skyrmions will generate a topological magnon Hall effect. Using the conservation law for the energy-momentum tensor, we demonstrate that the magnons also transfer momentum to the skyrmion. As a consequence, a magnon current leads to magnon pressure reflected in a momentum-transfer force in the Thiele equation of motion for the skyrmion. This force is reactive and governed by the scattering cross sections of the skyrmion; it causes not only a finite skyrmion velocity but also a large skyrmion Hall effect. Our results provide, in particular, the basis for a theory of skyrmion caloritronics for a dilute skyrmion gas in clean insulating chiral magnets.

cond-mat.str-el↗

arXiv2013

Critical speeding-up near the monopole liquid-gas transition in magnetoelectric spin-ice

Competing interactions in the so-called spin-ice compounds stabilize a frustrated ground-state with finite zero-point entropy and, interestingly, emergent magnetic monopole excitations. The properties of these monopoles are at the focus of recent research with particular emphasis on their quantum dynamics. It is predicted that each monopole also possesses an electric dipole moment, which allows to investigate their dynamics via the dielectric function ε(ν). Here, we report on broadband spectroscopic measurements of ε(ν) in Dy2Ti2O7 down to temperatures of 200mK with a specific focus on the critical endpoint present for a magnetic field along the crystallographic [111] direction. Clear critical signatures are revealed in the dielectric response when, similarly as in the liquid-gas transition, the density of monopoles changes in a critical manner. Surprisingly, the dielectric relaxation time τ exhibits a critical speeding-up with a significant enhancement of 1/τ as the temperature is lowered towards the critical temperature. Besides demonstrating the magnetoelectric character of the emergent monopole excitations, our results reveal unique critical dynamics near the monopole condensation transition.

cond-mat.str-el↗

arXiv2013

Specific heat of the skyrmion lattice phase and field-induced tricritical point in MnSi

We report high-precision measurements of the temperature and magnetic field dependence of the specific heat, C(T,H), across the magnetic phase diagram of MnSi. Clear anomalies establish the skyrmion lattice unambiguously as a thermodynamic phase. The evolution of the specific heat anomalies, the field dependence of the entropy released at the phase transitions, and the temperature versus field dependence of crossover lines provide striking evidence of a tricritical point at an internal magnetic field of 340mT and temperature of 28.5K. The existence of this tricritical point represents strong support of a helimagnetic Brazovskii transition, i.e., a fluctuation-induced first order transition at H = 0.

cond-mat.str-el↗

arXiv2013

Quantum criticality in itinerant metamagnets

Critical thermodynamics close to a metamagnetic quantum critical endpoint (QCEP) in a metal is discussed within the framework of spin-fluctuation theory. We analyze the effective potential for the Ising order parameter that is renormalized by spin-fluctuations and acquires a characteristic temperature dependence. The resulting magnetic field, H, and temperature, T, dependence of the magnetization, specific heat, thermal expansion, magnetostriction, susceptibility and the Grüneisen parameter are determined, and the crossover lines in the (H,T) phase diagram are specified. We point out that the metamagnetic QCEP is intrinsically unstable with respect to a magnetoelastic coupling.

cond-mat.str-el↗

arXiv2012

Quantum criticality with multiple dynamics

Quantum critical systems with multiple dynamics possess not only one but several time scales, tau_i ~ xi^(z_i), which diverge with the correlation length xi. We investigate how scaling predictions are modified for the simplest case of multiple dynamics characterized by two dynamical critical exponents, z_> and z_<. We argue that one should distinguish the case of coupled and decoupled multiple dynamic scaling depending on whether there exists a scaling exponent which depends on both z_i or not. As an example, we study generalized Phi^4-theories with multiple dynamics below their upper critical dimension, d+z_<<4. We identify under which condition coupled scaling is generated. In this case the interaction of quantum and classical fluctuations leads to an emergent dynamical exponent, z_e=z_>/(nu (z_>-z_<)+1).

cond-mat.str-el↗

arXiv2012

Mott metal-insulator transition on compressible lattices

The critical properties of the finite temperature Mott endpoint are drastically altered by a coupling to crystal elasticity, i.e., whenever it is amenable to pressure tuning. Similar as for critical piezoelectric ferroelectrics, the Ising criticality of the electronic system is preempted by an isostructural instability, and long-range shear forces suppress microscopic fluctuations. As a result, the endpoint is governed by Landau criticality. Its hallmark is thus a breakdown of Hooke's law of elasticity with a non-linear strain-stress relation characterized by a mean-field exponent. Based on a quantitative estimate, we predict critical elasticity to dominate the temperature range DeltaT/Tc ~ 8% close to the Mott endpoint of kappa-(BEDT-TTF)2X.

cond-mat.str-el↗

arXiv2012

Fluctuation-induced first-order phase transition in Dzyaloshinskii-Moriya helimagnets

Two centuries of research on phase transitions have repeatedly highlighted the importance of critical fluctuations that abound in the vicinity of a critical point. They are at the origin of scaling laws obeyed by thermodynamic observables close to second-order phase transitions resulting in the concept of universality classes, that is of paramount importance for the study of organizational principles of matter. Strikingly, in case such soft fluctuations are too abundant they may alter the nature of the phase transition profoundly; the system might evade the critical state altogether by undergoing a discontinuous first-order transition into the ordered phase. Fluctuation-induced first-order transitions have been discussed broadly and are germane for superconductors, liquid crystals, or phase transitions in the early universe, but clear experimental confirmations remain scarce. Our results from neutron scattering and thermodynamics on the model Dzyaloshinskii-Moriya (DM) helimagnet (HM) MnSi show that such a fluctuation-induced first-order transition is realized between its paramagnetic and HM state with remarkable agreement between experiment and a theory put forward by Brazovskii. While our study clarifies the nature of the HM phase transition in MnSi that has puzzled scientists for several decades, more importantly, our conclusions entirely based on symmetry arguments are also relevant for other DM-HMs with only weak cubic magnetic anisotropies. This is in particular noteworthy in light of a wide range of recent discoveries that show that DM helimagnetism is at the heart of problems such as topological magnetic order, multiferroics, and spintronics.

cond-mat.str-el↗

arXiv2012

Rotating skyrmion lattices by spin torques and field or temperature gradients

Chiral magnets like MnSi form lattices of skyrmions, i.e. magnetic whirls, which react sensitively to small electric currents j above a critical current density jc. The interplay of these currents with tiny gradients of either the magnetic field or the temperature can induce a rotation of the magnetic pattern for j>jc. Either a rotation by a finite angle of up to 15 degree or -- for larger gradients -- a continuous rotation with a finite angular velocity is induced. We use Landau-Lifshitz-Gilbert equations extended by extra damping terms in combination with a phenomenological treatment of pinning forces to develop a theory of the relevant rotational torques. Experimental neutron scattering data on the angular distribution of skyrmion lattices suggests that continuously rotating domains are easy to obtain in the presence of remarkably small currents and temperature gradients.

cond-mat.str-el↗

arXiv2011

Current induced rotational torques in the skyrmion lattice phase of chiral magnets

In chiral magnets without inversion symmetry, the magnetic structure can form a lattice of magnetic whirl lines, a two-dimensional skyrmion lattice, stabilized by spin-orbit interactions in a small range of temperatures and magnetic fields. The twist of the magnetization within this phase gives rise to an efficient coupling of macroscopic magnetic domains to spin currents. We analyze the resulting spin-transfer effects, and, in particular, focus on the current induced rotation of the magnetic texture by an angle. Such a rotation can arise from macroscopic temperature gradients in the system as has recently been shown experimentally and theoretically. Here we investigate an alternative mechanism, where small distortions of the skyrmion lattice and the transfer of angular momentum to the underlying atomic lattice play the key role. We employ the Landau-Lifshitz-Gilbert equation and adapt the Thiele method to derive an effective equation of motion for the rotational degree of freedom. We discuss the dependence of the rotation angle on the orientation of the applied magnetic field and the distance to the phase transition.

cond-mat.str-el↗

arXiv2011

Dislocation-mediated melting of one-dimensional Rydberg crystals

We consider cold Rydberg atoms in a one-dimensional optical lattice in the Mott regime with a single atom per site at zero temperature. An external laser drive with Rabi frequency Ωand laser detuning Δ, creates Rydberg excitations whose dynamics is governed by an effective spin-chain model with (quasi) long-range interactions. This system possesses intrinsically a large degree of frustration resulting in a ground-state phase diagram in the (Δ,Ω) plane with a rich topology. As a function of Δ, the Rydberg blockade effect gives rise to a series of crystalline phases commensurate with the optical lattice that form a so-called devil's staircase. The Rabi frequency, Ω, on the other hand, creates quantum fluctuations that eventually lead to a quantum melting of the crystalline states. Upon increasing Ω, we find that generically a commensurate-incommensurate transition to a floating Rydberg crystal occurs first, that supports gapless phonon excitations. For even larger Ω, dislocations within the floating Rydberg crystal start to proliferate and a second, Kosterlitz-Thouless-Nelson-Halperin-Young dislocation-mediated melting transition finally destroys the crystalline arrangement of Rydberg excitations. This latter melting transition is generic for one-dimensional Rydberg crystals and persists even in the absence of an optical lattice. The floating phase and the concomitant transitions can, in principle, be detected by Bragg scattering of light.

cond-mat.quant-gas↗

arXiv2011

Quantum phase transition in quantum wires controlled by an external gate

We consider electrons in a quantum wire interacting via a long-range Coulomb potential screened by a nearby gate. We focus on the quantum phase transition from a strictly one-dimensional to a quasi-one-dimensional electron liquid, that is controlled by the dimensionless parameter $n x_0$, where $n$ is the electron density and $x_0$ is the characteristic length of the transverse confining potential. If this transition occurs in the low-density limit, it can be understood as the deformation of the one-dimensional Wigner crystal to a zigzag arrangement of the electrons described by an Ising order parameter. The critical properties are governed by the charge degrees of freedom and the spin sector remains essentially decoupled. At large densities, on the other hand, the transition is triggered by the filling of a second one-dimensional subband of transverse quantization. Electrons at the bottom of the second subband interact strongly due to the diverging density of states and become impenetrable. We argue that this stabilizes the electron liquid as it suppresses pair-tunneling processes between the subbands that would otherwise lead to an instability. However, the impenetrable electrons in the second band are screened by the excitations of the first subband, so that the transition is identified as a Lifshitz transition of impenetrable polarons. We discuss the resulting phase diagram as a function of $n x_0$.

cond-mat.mes-hall↗

arXiv2011

Quantum phase transitions in the quasi-periodic kicked rotor

We present a microscopic theory of transport in quasi-periodically driven environments (`kicked rotors'), as realized in recent atom optic experiments. We find that the behavior of these systems depends sensitively on the value of Planck's constant $\tilde h$: for irrational values of $\tilde h/(4π)$ they fall into the universality class of disordered electronic systems and we derive the microscopic theory of the ensuing localization phenomena. In contrast, for rational values the rotor-Anderson insulator acquires an infinite (static) conductivity and turns into a `super-metal'. Signatures of the corresponding metal/super-metal transition are discussed.

nlin.CD↗

arXiv2010

Electron self-energy near a nematic quantum critical point

We consider an isotropic Fermi liquid in two dimensions near the n=2 Pomeranchuk instability in the charge channel. The order parameter is a quadrupolar stress tensor with two polarizations, longitudinal and transverse to the quadrupolar momentum tensor. Longitudinal and transverse bosonic modes are characterized by dynamical exponents z_parallel=3 and z_perp=2, respectively. Previous studies have found that such a system exhibits multiscale quantum criticality with two different energy scales omega ~ xi^{-z_{parallel,perp}}, where xi is the correlation length. We study the impact of the multiple energy scales on the electron Green function. The interaction with the critical z_parallel =3 mode is known to give rise to a local self-energy that develops a non-Fermi liquid form, Sigma(omega) ~ omega^{2/3} for frequencies larger than the energy scale omega ~ xi^{-3}. We find that the exchange of transverse z_perp=2 fluctuations leads to a logarithmically singular renormalizations of the quasiparticle residue Z and the vertex Gamma. We derive and solve renormalization group equations for the flow of Z and Gamma and show that the system develops an anomalous dimension at the nematic quantum-critical point (QCP). As a result, the spectral function at a fixed omega and varying k has a non-Lorentzian form. Away from the QCP, we find that the flow of Z is cut at the energy scale omega_{FL} ~ xi^{-1}, associated with the z=1 dynamics of electrons. The z_perp=2 energy scale, omega ~ xi^{-2}, affects the flow of Z only if one includes into the theory self-interaction of transverse fluctuations.

cond-mat.str-el↗

arXiv2009

Multiscale quantum criticality: Pomeranchuk instability in isotropic metals

As a paradigmatic example of multi-scale quantum criticality, we consider the Pomeranchuk instability of an isotropic Fermi liquid in two spatial dimensions, d=2. The corresponding Ginzburg-Landau theory for the quadrupolar fluctuations of the Fermi surface consists of two coupled modes, critical at the same point, and characterized by different dynamical exponents: one being ballistic with dynamical exponent z=2 and the other one is Landau-damped with z=3, thus giving rise to multiple dynamical scales. We find that at temperature T=0, the ballistic mode governs the low-energy structure of the theory as it possesses the smaller effective dimension d+z. Its self-interaction leads to logarithmic singularities, which we treat with the help of the renormalization group. At finite temperature, the coexistence of two different dynamical scales gives rise to a modified quantum-to-classical crossover. It extends over a parametrically large regime with intricate interactions of quantum and classical fluctuations leading to a universal T-dependence of the correlation length independent of the interaction amplitude. The multiple scales are also reflected in the phase diagram and in the critical thermodynamics. In particular, we find that the latter cannot be interpreted in terms of only a single dynamical exponent: whereas, e.g., the critical specific heat is determined by the z=3 mode, the critical compressibility is found to be dominated by the z=2 fluctuations.

cond-mat.str-el↗

arXiv2009

Dimensional crossover in quantum critical metallic magnets

Nearly magnetic metals often have layered lattice structures, consisting of coupled planes. In such a situation, physical properties will display, upon decreasing temperature or energy, a dimensional crossover from two-dimensional (2d) to three-dimensional (3d) behavior, which is particularly interesting near quantum criticality. Here we study this crossover in thermodynamics using a suitably generalized Landau-Ginzburg-Wilson approach to the critical behavior, combined with renormalization group techniques. We focus on two experimentally relevant cases: the crossover from a 2d to a 3d antiferromagnet, and the crossover from a 2d ferromagnet to a 3d antiferromagnet. We discuss the location of phase boundary and crossover lines and determine the crossover functions for important thermodynamic quantities. As naive scaling does not apply at and above the upper critical dimension, two crossover scales arise which can be associated with separate dimensional crossovers of classical and quantum fluctuations, respectively. In particular, we find an intermediate regime with novel power laws where the quantum fluctuations still have a 2d and the classical fluctuations already have a 3d character. For the ferromagnet-to-antiferromagnet crossover, the mismatch of the dynamical exponents between the 2d and 3d regimes leads to an even richer crossover structure, with an interesting 2d non-critical regime sandwiched between two critical regimes. For all cases, we find that thermal expansion and compressibility are particularly sensitive probes of the dimensional crossover. Finally, we relate our results to experiments on the quantum critical heavy-fermion metals CeCu(6-x)Au(x), YbRh(2)Si(2) and CeCoIn(5).

cond-mat.str-el↗

arXiv2008

Spin-spin correlations of the spin-ladder compound (C$_5$H$_{12}$N)$_2$CuBr$_4$ measured by magnetostriction and comparison to Quantum Monte Carlo results

Magnetostriction and thermal expansion of the spin-ladder compound piperidinium copper bromide (C$_5$H$_{12}$N)$_2$CuBr$_4$ are analyzed in detail. We find perfect agreement between experiments and the theory of a two-leg spin ladder Hamiltonian for more than a decade in temperature and in a wide range of magnetic fields. Relating the magnetostriction along different crystallographic directions to two static spin-spin correlation functions, which we compute with Quantum Monte Carlo, allows us to reconstruct the magnetoelastic couplings of (C$_5$H$_{12}$N)$_2$CuBr$_4$. We especially focus on the quantum critical behavior near the two critical magnetic fields $H_{c1}$ and $H_{c2}$, which is characterized by strong singularities rooted in the low dimensionality of the critical spin-system. Extending our discussion in Lorenz et al [Phys. Rev. Lett., 100, 067208 (2008)], we show explicitly that the thermal expansion near the upper critical field $H_{c2}$ is quantitatively described by a parameter-free theory of one-dimensional, non-relativistic Fermions. We also point out that there exists a singular quantum critical correction to the elastic moduli. This correction is proportional to the magnetic susceptibility $χ$ which diverges as $χ\sim 1/\sqrt{T}$ at the critical fields and thus leads to a strong softening of the crystal.

cond-mat.str-el↗

arXiv2006

Sign change of the Grueneisen parameter and magnetocaloric effect near quantum critical points

We consider the Grueneisen parameter and the magnetocaloric effect near a pressure and magnetic field controlled quantum critical point, respectively. Generically, the Grueneisen parameter (and the thermal expansion) displays a characteristic sign change close to the quantum-critical point signaling an accumulation of entropy. If the quantum critical point is the endpoint of a line of finite temperature phase transitions, T_c \propto (p_c-p)^Psi, then we obtain for p T_c, (2) a sign change in the Ginzburg regime of the classical transition, (3) possibly a peak at T_c, (4) a second increase Gamma \sim -T^{-1/(nu z)} below T_c for systems above the upper critical dimension and (5) a saturation of Gamma \propto 1/(p_c-p). We argue that due to the characteristic divergencies and sign changes the thermal expansion, the Grueneisen parameter and magnetocaloric effect are excellent tools to detect and identify putative quantum critical points.

cond-mat.str-el↗