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Markus Gräfe

Publications and source records attributed to Markus Gräfe.

At least 19 recordsLinked to original sources

Phase estimation in spontaneous nonlinear interferometry for enhanced quantum imaging

Bicolor quantum imaging can reach, in principle, phase supersensitivity approaching the Heisenberg limit using squeezed light from high-gain parametric down-conversion, but established quantum-imaging setups typically operate in the low-gain, spontaneous regime, where such scaling is inaccessible. Here, we show experimentally and theoretically that a symmetric nonlinear interferometer, even in the spontaneous regime, retains a phase-sensitivity advantage over configurations where entanglement is not exploited as a quantum-metrological resource, although the achievable phase sensitivity remains shot-noise-limited. This advantage appears as a shift of the optimal working point toward the dark fringe, the low-gain signature of the mechanism underlying high-gain supersensitivity. We derive design choices for phase-optimized nonlinear interferometers accordingly, favoring configurations that exploit entanglement as a metrological resource and specifying their optimal operating point.

quant-ph

Below-shot-noise capacity in phase estimation using nonlinear interferometers

Over the past decade, several schemes for imaging and sensing based on nonlinear interferometers have been proposed and demonstrated experimentally. These interferometers exhibit two main advantages. First, they enable probing a sample at a chosen wavelength while detecting light at a different wavelength with high efficiency (bicolor quantum imaging and sensing with undetected light). Second, they can show quantum-enhanced sensitivities below the shot-noise limit, potentially reaching Heisenberg-limited precision in parameter estimation. Here, we compare three quantum-imaging configurations using only easily accessible intensity-based measurements for phase estimation: a Yurke-type SU(1,1) interferometer, a Mandel-type induced-coherence interferometer, and a hybrid scheme that continuously interpolates between them. While an ideal Yurke interferometer can exhibit Heisenberg scaling, this advantage is known to be fragile under realistic detection constraints and in the presence of loss. We demonstrate that differential intensity detection in the Mandel interferometer provides the highest and most robust phase sensitivity among the considered schemes, reaching but not surpassing the shot-noise limit, even in the presence of loss. Intensity measurements in a Yurke-type configuration can achieve genuine sub-shot-noise sensitivity under balanced losses and moderate gain; however, their performance degrades in realistic high-gain regimes. Consequently, in this regime, the Mandel configuration with differential detection outperforms the Yurke-type setup and constitutes the most robust approach for phase estimation.

quant-ph

Quantum scanning synthetic optical holography

Synthetic optical holography (SOH) introduced holographic reconstruction into scanning optical microscopy, enabling quantitative phase imaging with sequential acquisition and point detection. Here, we extend this concept to the quantum regime by implementing SOH within quantum imaging with undetected light (QIUL). By integrating a controlled synthetic phase carrier into a scanning QIUL implementation, we retrieve amplitude and phase images of objects probed by mid-infrared (MIR) photons while detecting only their visible partners. We demonstrate the method on binary, transparent, and biological samples, showing complex-field reconstruction in a scanning quantum imaging system. This approach decouples spatial resolution from photon-pair spatial correlations and establishes a route toward diffraction-limited, label-free MIR phase imaging with visible-wavelength detection.

physics.optics

Advances in Position-Momentum Entanglement: A Versatile Tool for Quantum Technologies

Position-momentum entanglement is a versatile high-dimensional resource in quantum optics. From fundamental tests of reality to applications in quantum technologies, spatial entanglement has experienced significant growth in recent years. In this review, we explore these advances, beginning with the generation of spatial entanglement, followed by various types of measurements for certifying entanglement, and concluding with different quantum-based applications. We conclude the review with a discussion and outlook of the field.

quant-ph

Vectorial field reconstruction without detecting the field

Vector beams, whose polarization varies across the transverse profile, are a central resource in structured-light optics and quantum photonics. Their characterization, however, becomes challenging when the field lies in a spectral region for which efficient spatially resolving detectors are unavailable. Here we demonstrate the spatially resolved reconstruction of an undetected vector beam by exploiting induced coherence in a nonlinear interferometer. In this effect, indistinguishability between two down-conversion pathways allows information encoded in an undetected field to be read out through interference of its detected partner. A telecom-wavelength idler field acquires a spatially varying polarization transformation but is never directly detected. Instead, its local polarization information is inferred from single-photon interference in the visible signal field, enabled by momentum correlations of the photon pair. Using phase-shifting and off-axis quantum holography with two polarization projections, we reconstruct the horizontal and vertical amplitudes and their relative phase across the beam profile, thereby recovering the full vectorial structure of the undetected field. We experimentally retrieve the polarization texture of an $m=2$ vector beam and compare multi-shot and single-shot reconstruction strategies. Our results extend imaging with undetected light from scalar objects to vectorial optical fields and open a route to polarization-sensitive sensing and state reconstruction in spectral regions that are difficult to access directly.

physics.optics

Noise resilient real-time phase imaging via undetected light

Quantum imaging with undetected light has recently emerged as a technique in which quantum correlations and nonlinear interferometry are combined to decouple illumination and detection paths. This approach has been more recently extended and combined with digital phase-shifting holography and off-axis holography to extract both the amplitude and phase information of a sample relying on single-photon interference. Despite these advantages, implementing the technique in real-world scenarios where the observed system is subject to environmental noise and dynamic variations remains challenging. The primary limitation lies in the inability of quantum imaging systems to retrieve object information in real time under high-noise conditions. Here, we experimentally demonstrate real-time amplitude and phase imaging in noisy environments, building upon our previous implementation of quantum off-axis holography. Our results demonstrate real-time imaging at acquisition rates up to 4~Hz, even when the noise level exceeds the signal by an order of magnitude.

physics.optics

Certifying spatial entanglement between non-degenerate photon pairs with a camera

We investigate transverse spatial entanglement between photon pairs of different wavelengths using a camera-based coincidence technique. By adapting the correlation measurements to the photons frequencies, we certify the presence of entanglement between the pairs through violation of an Einstein-Podolsky-Rosen criterion. Additionally, we examine how parameters such as pump waist and crystal length influence these correlations. Our results highlight key differences from the frequency-degenerate case, showing that an adapted theoretical analysis is essential to avoid significant misestimations and to reliably certify entanglement.

quant-ph

Rubidium-Doped KTiOPO$_4$ Waveguides as a Dual-Type Photon Pair Source

We investigate the dual generation of type-0 and type-II spontaneous parametric down conversions (SPDCs) within a single periodically poled rubidium-doped KTiOPO$_4$ (PPRKTP) waveguide. By coupling a 45 degree linearly polarized pump laser into the waveguide, both SPDC processes are concurrently excited: the type-0 SPDC process is facilitated via third-order quasi-phase matching (QPM) utilizing the nonlinear coefficient $d_{33}$ , while the type-II SPDC process employs first-order QPM with the nonlinear coefficient $d_{24}$. This dual-SPDC scheme holds potential for applications in quantum communication protocols targeting the telecommunication wavelength.

quant-ph

Non-degenerate SPDC photon-pair source for UV-A illumination

We present a frequency-correlated non-degenerate photon-pair source consisting of a second-order nonlinear crystal that generates ultraviolet UV-A and infrared light via spontaneous parametric down-conversion. Quantum imaging and sensing techniques like quantum imaging with undetected light and quantum ghost imaging leverage on wavelength correlations between down-converted photon pairs to decouple sensing and detection wavelengths, thereby exploiting established camera technology within the visible spectrum. Our results open up novel quantum sensing application scenarios in the ultraviolet domain, with potential implications for advancements in biomedical and non-destructive testing fields.

quant-ph

Visibility Stokes parameters as a foundation for quantum information science with undetected photons

The framework of measurement operators plays a fundamental role in extracting information about quantum systems. Recently, techniques based on induced coherence have been developed to access the same information for undetected photons. However, there has been a lack of consistent reformulation of quantum operators for these techniques. In this work, we introduce a set of parameters that quantify the polarization of undetected photons based on measured visibilities. Given their similarity to classical counterparts, we refer to them as visibility Stokes parameters. We apply these parameters and the corresponding quantum operators to the problem of quantum state tomography, thoroughly analyzing the environment of undetected photons and its role in the reconstruction process. Because these parameters provide a more intuitive and consistent understanding of the measurement process, we believe that some established quantum information protocols could be adapted for undetected photons.

quant-ph

Mid-infrared quantum scanning microscopy via visible light beyond spatial correlations

The mid-infrared (MIR) region of the electromagnetic spectrum spans from 2- to 25-$μ\mathrm{m}$, serving as a valuable tool for accessing rich chemical information. Functional groups, lipids, and other complex molecules can be analyzed by optical absorption measurements due to their vibrational modes in the MIR spectral region. Over the past few decades, this field has faced challenges due to difficulties in generating MIR light and the limited maturity of detection systems in this spectral range. Quantum imaging with undetected light (QIUL) provides a spectrally tuneable photon-pair source, in which the sample can be illuminated with MIR light while visible (VIS) light is employed for detection and image reconstruction, overcoming the detection limitations and benefiting from the rich chemical information of the MIR spectral region. All previous QIUL implementations are based on spatial correlations, which are never perfect and thus hindered the imaging performance. In this work, we implement a raster-scanning QIUL method that is independent of the strength of the spatial correlations and achieves a spatial resolution beyond the limitations of these correlations.

physics.optics

Benchmarking of Fluorescence Lifetime Measurements using Time-Frequency Correlated Photons

The investigation of fluorescence lifetime became an important tool in biology and medical science. So far, established methods of fluorescence lifetime measurements require the illumination of the investigated probes with pulsed or amplitude-modulated light. In this paper, we examine the limitations of an innovative method of fluorescence lifetime using the strong time-frequency correlation of entangled photons generated by a continuous-wave source. For this purpose, we investigate the lifetime of IR-140 to demonstrate the functional principle and its dependencies on different experimental parameters. We also compare this technique with state-of-the-art FLIM and observed an improved figure-of-merit. Finally, we discuss the potential of a quantum advantage.

quant-ph

Enhancing entangled two-photon absorption of Nile Red via temperature-controlled SPDC

Entangled two-photon absorption can enable a linear scaling of fluorescence emission with the excitation power. In comparison to classical two-photon absorption with a quadratic scaling, this can allow fluorescence imaging or photolithography with high axial resolution at minimal exposure intensities. However, most experimental studies on two-photon absorption were not able to show an unambiguous proof of fluorescence emission driven by entangled photon pairs. On the other hand, existing theoretical models struggle to accurately predict the entangled two-photon absorption behavior of chemically complex dyes. In this paper, we introduce an approach to simulate entangled two-photon absorption in common fluorescence dyes considering their chemical properties. Our theoretical model allows a deeper understanding of experimental results and thus the occurrence of entangled two-photon absorption. In particular, we found a remarkable dependency of the absorption probability on the phase-matching temperature of the nonlinear material. Further, we compared results of our theoretical approach to experimental data for Nile Red.

quant-ph

Synthetic Quantum Holography with Undetected Light

Utilizing nonlinear interferometers for sensing with undetected light enables new sensing and imaging techniques in spectral ranges that are difficult to detect. To enhance this method for future applications, it is advantageous to extract both amplitude and phase information of an object. This study introduces two approaches for synthetic quantum holography with undetected light, which allows for obtaining an object's amplitude and phase information in a nonlinear interferometer by capturing only a single image. One method is based on quasi-phase-shifting holography using superpixel structures displayed on a spatial light modulator. The other method relies on synthetic off-axis holography implemented through a linear phase gradient on a spatial light modulator. Both approaches are experimentally analyzed for applicability and compared against available multi-acquisition methods.

physics.optics

Polarization-entangled photon pair source using beam displacers and thin crystals

We present an experimental implementation of a polarization-entangled photon pair source based on beam displacers. The down-converted photons are emitted via spontaneous parametric down-conversion in a non-degenerate and type-0 process. We obtain a state fidelity of $F=0.975\pm0.004$ and violate a Clauser-Horne-Shimony-Holt inequality with $S=2.75\pm0.01$. Our source also uses thin crystals for applications in quantum imaging, taking advantage of the large number of spatial modes. We estimate that our source could produce 550$\pm$12 spatial modes.

quant-ph

Off-axis holographic imaging with undetected light

Quantum imaging with undetected light (QIUL) can retrieve amplitude and phase information of an object by exploiting the quantum correlations of photon-pairs generated through spontaneous parametric down conversion (SPDC), where the illumination and detection can be carried at very distinct wavelength ranges. This fact allows to benefit from a mature detection technology in the visible spectral range, while probing the object at a more exotic wavelength. Here we experimentally implement a QIUL approach with Fourier off-axis holography in a hybrid-type induced-coherence non-linear interferometer. Our approach reconstructs the amplitude and phase information of an object with a single shot in a wide-field configuration, being an alternative in front of techniques that require multiple acquisition frames, such as phase-shifting holography.

physics.optics

Quantum Imaging Beyond the Standard-Quantum Limit and Phase Distillation

Quantum sensing using non-linear interferometers offers the possibility of bicolour imaging, using light that never interacted with the object of interest, and provides a way to achieve phase supersensitivity, i.e. a Heisenberg-type scaling of the phase uncertainty. Such a scaling behaviour is extremely susceptible to noise and only arises at specific phases that define the optimal working point of the device. While phase-shifting algorithms are to some degree robust against the deleterious effects induced by noise they extract an image by tuning the interferometer phase over a broad range, implying an operation beyond the working point. In our theoretical study, we investigate both the spontaneous and the high-gain regime of operation of a non-linear interferometer. In fact, in the spontaneous regime using a distillation technique and operating at the working point leads to a qualitatively similar behaviour. In the high-gain regime, however, typical distillation techniques inherently forbid a scaling better than the standard-quantum limit, as a consequence of the photon statistics of squeezed vacuum. In contrast, an operation at the working point still may lead to a sensitivity below shot noise, even in the presence of noise. Therefore, this procedure opens the perspective of bicolour imaging with a better than shot-noise phase uncertainty by working in the vicinity of the working point. Our results transfer quantum imaging distillation in a noisy environment to the high-gain regime with the ultimate goal of harnessing its full potential by combining bicolour imaging and phase supersensitivity.

quant-ph

Spectral Properties of Transverse Laguerre-Gauss Modes in Parametric Down-Conversion

The first color photos of the parametric down-conversion (PDC) emission cone illustrate the correlation of longitudinal- and transverse momentum in the process, i.e., wavelength-dependent emission angle of PDC photons. However, current experiments and applications are more conveniently described in terms of discrete mode sets, with the most suitable choice depending on the propagation symmetries of the experimental setting. Remarkably, despite the fact that experiments with PDC sources are becoming ever more demanding, e.g. in terms of brightness or state fidelity, a description of spectral-spatial coupling in parametric downconversion for the case of discrete modal decompositions remains elusive. We present a comprehensive study, in theory and experiment, of the spectral dependence of the transverse Laguerre-Gauss modes in parametric downconversion. Moreover, we show how the spectral and spatial coupling can be harnessed to tune the purity of the well-known orbital angular momentum entanglement. This work has implications for efficient collection of entangled photons in a transverse single mode, quantum imaging, and engineering pure states for high-dimensional quantum information processing.

quant-ph