arXiv subjects

Markus Münzenberg

Publications and source records attributed to Markus Münzenberg.

At least 19 recordsLinked to original sources

arXiv2026

Non-Volatile Vortex MTJs with Opto-Electrical and Spin-Diode Nonlinearities as Multifunctional Neuromorphic Platforms

The human brain achieves exceptional energy efficiency by co-locating memory and processing, yet reproducing this principle in hardware remains challenging because many neuromorphic devices require standby power, offer limited programmability, or separate state storage from nonlinear computation. Here we demonstrate a multifunctional spintronic platform based on storage-layer-enabled vortex magnetic tunnel junctions (MTJs) that unifies non-volatile weight storage, optoelectrically driven nonlinear computation, and multilevel readout within a single nanopillar. A thermally programmable FM/AFM storage layer retains analog synaptic weights with zero standby power and enables non-volatile tuning of the vortex gyrotropic resonance over ${\sim}15$~MHz. Under optoelectrical operation, combined laser heating and dc bias drive the junction into the bias-enhanced tunnel magneto-Seebeck (bTMS) regime, where the thermoelectric response exhibits a pronounced cubic nonlinearity providing a compact, hardware-native transfer function for weighted analog computation. The electrical and thermoelectric channels switch at matched coercive fields but with distinct amplitudes, yielding an effective four-level readout space. Crossbar-array simulations parameterized by measured device response maps evaluate two neuromorphic modes -- a bTMS mode (optical input, dc-bias weights) and a spin-diode mode (RF-frequency input, RF-power weights) -- achieving image-classification accuracies of $95.4\%$ and $94.9\%$, comparable to a digital single-layer network with sigmoid activations. Smaller 600~nm devices consistently outperform larger ones, identifying nonlinear-response engineering as a key device-level lever. Because bTMS and spin-diode rectification coexist in the same junction, a combined regime could enable nonlinear multi-input interactions, including quadratic cross-terms, within a single nanoscale element.

physics.app-ph↗

arXiv2026

Femtosecond all-optical coherent control of spin polarization in altermagnets

Altermagnets constitute an emerging materials platform for spintronic technologies by combining compensated magnetic order with ferromagnet-like spin-split electronic bands. Here, we investigate the proposed d-wave altermagnetic material RuO2 using circularly polarized ultrashort laser pulses. Time-resolved magneto-optical Kerr effect measurements, which are intrinsically sensitive to surface and interface states, reveal the ultrafast spin response of RuO2. In contrast to the demagnetization dynamics characteristic of conventional ferromagnets, we observe a distinct coherent contribution to the complex Kerr rotation that appears during the light-matter interaction and lasts for about 200 fs. Similar signatures have been associated with spin-momentum locking and directional band splitting in spin-split surface states of topological insulators as well as spin-orbit-coupled semiconductors. They are governed by a finite Raman coherence time. We interpret this coherent response as evidence for transient spin-polarized surface states in RuO2, consistent with the emergence of altermagnetic surface states that are directly relevant to spin-polarized transport at surfaces and interfaces.

cond-mat.other↗

arXiv2025

Bulk spin-orbit torque-driven spin Hall nano-oscillators using PtBi alloys

Spin-orbit-torque-driven auto-oscillations in spin Hall nano-oscillators (SHNOs) offer a transformative pathway toward energy-efficient, nanoscale microwave devices for next-generation neuromorphic computing and high-frequency technologies. A key requirement for achieving robust, sustained oscillations is reducing the threshold current ($I_{\text{th}}$), strongly governed by spin Hall efficiency ($θ_{\text{SH}}$). However, conventional strategies to enhance $θ_{\text{SH}}$ face trade-offs, including high longitudinal resistivity, interfacial effects, and symmetry-breaking torques that limit performance. Here, we demonstrate a substantial enhancement of the bulk spin Hall effect in PtBi alloys, achieving over a threefold increase in $θ_{\text{SH}}$, from 0.07 in pure Pt to 0.24 in Pt$_{94.0}$Bi$_{6.0}$ and 0.19 in Pt$_{91.3}$Bi$_{8.7}$, as extracted from DC-bias spin-torque ferromagnetic resonance. The enhanced $θ_{\text{SH}}$ originates from bulk-dominated, extrinsic side-jump scattering across all PtBi compositions. Correspondingly, we observe a 42\% and 32\% reduction in $I_{\text{th}}$ in 100 nm SHNOs based on Co$_{40}$Fe$_{40}$B$_{20}$(3 nm)/Pt$_{94.0}$Bi$_{6.0}$(4 nm) and Co$_{40}$Fe$_{40}$B$_{20}$(3 nm)/Pt$_{91.3}$Bi$_{8.7}$(4 nm), respectively. Structural characterization reveals reduced Pt crystallinity, along with emergence of preferred crystallographic orientations upon introducing higher Bi concentrations. Together, these results position PtBi alloys as a compelling alternative to conventional 5$d$ transition metals, enabling enhanced $θ_{\text{SH}}$ and significantly lower $I_{\text{th}}$, thus opening new avenues for energy-efficient neuromorphic computing and magnetic random access memory.

cond-mat.mes-hall↗

arXiv2025

Femtosecond photocurrents by the Dresselhaus bulk spin-galvanic effect in an inversion-asymmetric ferromagnet

We study ultrafast photocurrents in thin films of a model ferromagnetic metal with broken bulk inversion symmetry, the half-metallic Heusler compound NiMnSb, following excitation with an optical pump pulse with photon energy 1.55 eV. Remarkably, in terms of the direction of the sample magnetization M, all photocurrents are found to be a superposition of a component with Rashba- and Dresselhaus-type symmetry. We explain the Dresselhaus bulk photocurrent as follows: Pump-induced electron heating induces an excess of spin μ_s||M, which transfers spin angular momentum into states with Dresselhaus-type spin-momentum locking. The resulting charge current relaxes on a time scale of 10 fs by momentum relaxation and, thus, follows μ_s quasi-instantaneously. The relaxation of μ_s is governed by the cooling of the electrons and not by the significantly slower spin-lattice relaxation of half-metals. Our findings add the Dresselhaus spin-galvanic effect (SGE) to the set of ultrafast spin-charge-conversion phenomena. They indicate a route to more efficient spintronic terahertz emitters and detectors based on the volume scaling of the bulk SGE.

cond-mat.mtrl-sci↗

arXiv2025

Hybrid Opto-Electrical Excitation of Spin-Transfer Torque Nano-Oscillators for Advanced Computing

Neuromorphic computing, inspired by the brain's parallel and energy-efficient processing, offers a transformative approach to artificial intelligence. In this study, we fabricated optimized spin-transfer torque nano-oscillators (STNOs) and investigated their dynamic behaviors using a hybrid excitation scheme combining AC laser illumination and DC bias currents. Laser-induced thermal gradients generate pulsed thermoelectric voltages ($V_{\text{AC}}$) via the Tunnel Magneto-Seebeck (TMS) effect, while the addition of bias currents enhances this response, producing both $V_{\text{AC}}$ and a DC component ($V_{\text{DC}}$). Magnetic field sweeps reveal distinct switching between parallel (P) and antiparallel (AP) magnetization states in both voltage components, supporting multistate memory applications. Millivolt-range thermovoltage signals in open-circuit conditions demonstrate CMOS compatibility, enabling simplified, scalable neuromorphic systems. Under biased conditions, enhanced thermovoltage outputs exhibit intriguing phenomena, including spikes correlated with Barkhausen jumps and double-switching behavior, offering insights into magnetization dynamics and vortex transitions. These features resemble neural spiking behavior, suggesting applications in spiking neural networks, reservoir computing, multistate logic, analog computing, and high-resolution sensing. By bridging spintronic phenomena with practical applications, this work provides a versatile platform for next-generation AI technologies and adaptive computing architectures.

physics.optics↗

arXiv2024

Accessing ultrafast spin-transport dynamics in copper using broadband terahertz spectroscopy

We study the spatiotemporal dynamics of ultrafast electron spin transport across nanometer-thick copper layers using broadband terahertz spectroscopy. Our analysis of temporal delays, broadening and attenuation of the spin-current pulse revealed ballistic-like propagation of the pulse peak, approaching the Fermi velocity, and diffusive features including a significant velocity dispersion. A comparison to the frequency-dependent Ficks law identified the diffusion-dominated transport regime for distances larger than 2 nm. The findings lie the groundwork for designing future broadband spintronic devices.

cond-mat.mes-hall↗

arXiv2023

Tunable ultrabroadband hybrid THz emitter combining a spintronic THz source and a GaSe crystal

Linear terahertz time-domain spectroscopy (THz-TDS) is a sensitive probe for material characterization including thickness measurements of thin layers. These applications critically rely on a sufficiently large bandwidth, which is not straightforwardly available in typical THz-TDS systems. Here, we introduce a hybrid THz-emitter concept based on a spintronic THz emitter that is deposited onto a thin freestanding GaSe nonlinear crystal. By tuning the parameters of this hybrid emitter, we generate an ultrabroadband spectrum covering the full range from 1 to 40 THz without any gaps at high spectral amplitudes, resulting in ultrashort THz-pulse durations of only 32 fs. Finally, we demonstrate the straightforward tunability of the carrier-envelope phase from unipolar or bipolar THz pulses with ultrashort duration.

physics.optics↗

arXiv2023

Comparative Analysis of THz Signal Emission from SiO$_2$/CoFeB/Metal Heterostructures: Wideband and High-Frequency THz Signal Advantage of PtBi-based Emitter

Spintronic THz emitters have attracted much attention due to their desirable properties, such as affordability, ultra-wideband capability, high efficiency, and tunable polarization. In this study, we investigate the characteristics of THz signals, including their frequency, bandwidth, and amplitude, emitted from a series of heterostructures with ferromagnetic (FM) and nonmagnetic (NM) materials. The FM layer consists of a wedge-shaped CoFeB layer with a thickness of 0 to 5 nm, while the NM materials include various metals such as Pt, Au, W, Ru, Pt$_{\%92}$Bi$_{\%8}$, and Ag$_{\%90}$Bi$_{\%10}$ alloys. Our experiments show that the emitter with Pt-NM layer has the highest amplitude of the emitted THz signal. However, the PtBi-based emitter exhibits a higher central THz peak and wider bandwidth, making it a promising candidate for broadband THz emitters. These results pave the way for further exploration of the specific compositions of Pt$_{1-x}$Bi$_{x}$ for THz emitter design, especially with the goal of generating higher frequency and wider bandwidth THz signals. These advances hold significant potential for applications in various fields such as high-resolution imaging, spectroscopy, communications, medical diagnostics, and more.

physics.optics↗

arXiv2023

Enhancing Spin Transfer Torque in Magnetic Tunnel Junction Devices: Exploring the Influence of Capping Layer Materials and Thickness on Device Characteristics

We have developed and optimized two categories of spin transfer torque magnetic tunnel junctions (STT-MTJs) that exhibit a high tunnel magnetoresistance (TMR) ratio, low critical current, high outputpower in the micro watt range, and auto-oscillation behavior. These characteristics demonstrate the potential of STT-MTJs for low-power, high-speed, and reliable spintronic applications, including magnetic memory, logic, and signal processing. The only distinguishing factor between the two categories, denoted as A-MTJs and B-MTJs, is the composition of their free layers, 2 CoFeB/0.21 Ta/6 CoFeSiB for A-MTJs and 2 CoFeB/0.21 Ta/7 NiFe for B-MTJs. Our study reveals that B-MTJs exhibit lower critical currents for auto-oscillation than A-MTJs. We found that both stacks have comparable saturation magnetization and anisotropy field, suggesting that the difference in auto-oscillation behavior is due to the higher damping of A-MTJs compared to B-MTJs. To verify this hypothesis, we employed the all-optical time-resolved magneto-optical Kerr effect (TRMOKE) technique, which confirmed that STT-MTJs with lower damping exhibited auto-oscillation at lower critical current values. Additionally, our study aimed to optimize the STT-MTJ performance by investigating the impact of the capping layer on the device's response to electronic and optical stimuli.

physics.optics↗

arXiv2022

Identification and characterization of various plastics using THz-spectroscopy

THz spectroscopy has reached imaging capability with a spatial resolution of a few micrometres. This property enables measurements and imaging of biological samples like cells. THz photons have very low photon energies in the millielectronvolt range. These energies interact mainly with vibrations in the molecules. Therefore, the investigated samples are neither ionized nor their DNA damaged, making this the perfect method for application on living cell tissue. In the future, material databases with absorption spectra will empower this method to distinguish even artificial particles like microplastics inside biological tissue. Current research aims at the impact of plastic nanoparticles on cell tissue considering various aspects. One of them is the investigation of the potential harm, the interaction of these particles with human body cells can cause, as these highly abundant particles are found anywhere in the environment. THz absorption spectroscopy offers the opportunity to investigate the polymers and identify them using their specific absorption lines as a fingerprint. In this publication, we study different polymers and analyse their particular fingerprints in the THz frequency spectrum from 0.1 up to 4 THz using a commercially available THz spectrometer. With this work we are contributing to the development, using THz waves for imaging, by identifying the fingerprints of the four most used plastics by humankind. At the end of this development, we envision a method to investigate the influence of nanometre-sized plastic particles on the human body and other biological organisms.

cond-mat.soft↗

arXiv2022

Interface-Assisted Room-Temperature Magnetoresistance in Cu-Phenalenyl-based Magnetic Tunnel Junctions

Delocalized carbon-based radical species with unpaired spin, such as phenalenyl (PLY) radical, opened avenues for developing multifunctional organic spintronic devices. Here we develop a novel technique based on a three-dimensional shadow mask and the in-situ deposition to fabricate PLY-, Cu-PLY-, and Zn-PLY-based organic magnetic tunnel junctions (OMTJs) with area 3x8 μm2 and improved morphology. The nonlinear and weakly temperature-dependent current-voltage (I-V) characteristics in combination with the low organic barrier height suggest tunneling as the dominant transport mechanism in the structurally and dimensionally optimized OMTJs. Cu-PLY-based OMTJs, show a significant magnetoresistance up to 14 percent at room temperature due to the formation of hybrid states at the metal-molecule interfaces called spinterface, which reveals the importance of spin-dependent interfacial modification in OMTJs design. In particular, Cu-PLY OMTJs shows a stable voltage-driven resistive switching response that suggests their use as a new viable and scalable platform for building molecular scale quantum memristors and processors.

cond-mat.mtrl-sci↗

arXiv2022

Coupling broadband terahertz dipoles to microscale resonators

Spintronic emitters are a unique class of terahertz (THz) sources due to their quasi-two-dimensional geometry and thereby their capability to couple to resonator near fields. Global excitation of the emitters often obstructs the intricate details of the coupling mechanisms between local THz dipoles and the individual modes of resonator structures. Here, we demonstrate the spatial mapping of the coupling strength between a local terahertz source on a spintronic emitter and far-field light mediated by a structured metallic environment. For a bow-tie geometry, experimental results are reproduced by a numerical model providing insights into the microscopic coupling mechanisms. The broad applicability of the technique is showcased by extracting the THz mode structure in split-ring resonator metasurfaces and linear arrays. With these developments, planar THz sources with tailored spectral and angular emission profiles are accessible.

physics.optics↗

arXiv2022

Second Harmonic Generation from Grating-Coupled Hybrid Plasmon-Phonon Polaritons

Polaritons can provide strong optical field enhancement allowing to boost light-matter interaction. Here, we experimentally observe enhancement of mid-infrared second-harmonic generation (SHG) using grating-coupled surface phonon polaritons of the 6H-SiC surface. In our experiment, we measure the SHG along the polariton dispersion by changing the incidence angle of the excitation beam. We observe hybridization between the propagating surface phonon polaritons and localized plasmon resonances in the gold grating, evidenced by the modification of the polariton dispersion as we change the area ratio of grating and substrate. Design options for engineering the plasmon-phonon polariton hybridization are discussed. Overall, we find a rather low yield of polariton-enhanced SHG in this geometry compared to prism-coupling and nanostructures, and discuss possible origins.

physics.optics↗

arXiv2022

Magnetic domain scanning imaging using phase-sensitive THz-pulse detection

In our study, we determine the alignment of magnetic domains in a CoFeB layer using THz radiation. We generate THz-pulses by fs-laser-pulses in magnetized CoFeB/Pt heterostructures, based on spin currents. An LT-GaAs Auston switch detects the radiation phase-sensitively and allows to determine the magnetization alignment. Our scanning technique with motorized stages with step sizes in the sub-micrometer range, allows to image two dimensional magnetic structures. Theoretically the resolution is restricted to half of the wavelength if focusing optics in the far-field limit are used. By applying near-field imaging, the spatial resolution is enhanced to the single digit micrometer range. For this purpose, spintronic emitters in diverse geometric shapes, e.g. circles, triangles, squares, and sizes are prepared to observe the formation of magnetization patterns. The alignment of the emitted THz radiation can be influenced by applying unidirectional external magnetic fields. We demonstrate how magnetic domains with opposite alignment and different shapes divided by domain walls are created by demagnetizing the patterns using minor loops and imaged using phase sensitive THz radiation detection. For analysis, the data is compared to Kerr microscope images. The possibility to combine this method with THz range spectroscopic information of magnetic texture or antiferromagnets in direct vicinity to the spintronic emitter, makes this detection method interesting for much wider applications probing THz excitation in spin systems with high resolution beyond the Abbe diffraction limit, limited solely by the laser excitation area.

physics.optics↗

arXiv2021

Spintronic emitters for super-resolution in THz-spectral imaging

THz-spectroscopy is an attractive imaging tool for scientific research, especially in life science, offering non-destructive interaction with matter due to its low photon energies. However, wavelengths above $100μm$ principally limit its spatial resolution in the far-field by diffraction to this regime, making it not sufficient to image biological cells in the micrometer scale. Therefore, super-resolution imaging techniques are required to overcome this restriction. Near-field-imaging using spintronic emitters offers the most feasible approach because of its simplicity and potential for wide-ranging applications. In our study, we investigate THz-radiation generated by fs-laser-pulses in CoFeB/Pt heterostructures, based on spin currents, detected by commercial LT-GaAs Auston switches. The spatial resolution is evaluated applying a 2D scanning technique with motorized stages allowing scanning steps in the sub-micrometer range. By applying near-field imaging we can increase the spatial resolution to the dimensions of the laser spot size in the micrometer scale. For this purpose, the spintronic emitter is directly evaporated on a gold test pattern separated by a 300 nm spacer layer. Moving these structures with respect to the femtosecond laser spot which generates the THz radiation allows for resolution determination using the knife-edge method. We observe a full-width half-maximum THz beam diameter of $4.9(4)μ$m at 1 THz. The possibility to deposit spintronic emitter heterostructures on simple glass substrates makes them an interesting candidate for near-field imaging for a large number of applications.

physics.optics↗

arXiv2021

Frequency-independent terahertz anomalous Hall effect in DyCo$_{5}$, Co$_{32}$Fe$_{68}$ and Gd$_{27}$Fe$_{73}$ thin films from DC to 40 THz

The anomalous Hall effect (AHE) is a fundamental spintronic charge-to-charge-current conversion phenomenon and closely related to spin-to-charge-current conversion by the spin Hall effect. Future high-speed spintronic devices will crucially rely on such conversion effects at terahertz (THz) frequencies. Here, we reveal that the AHE remains operative from DC up to 40 THz with a flat frequency response in thin films of three technologically relevant magnetic materials: DyCo$_{5}$, Co$_{32}$Fe$_{68}$ and Gd$_{27}$Fe$_{73}$. We measure the frequency-dependent conductivity-tensor elements $σ_{xx}$ and $σ_{yx}$ and find good agreement with DC measurements. Our experimental findings are fully consistent with ab-initio calculations of $σ_{yx}$ for CoFe and highlight the role of the large Drude scattering rate (~100 THz) of metal thin films, which smears out any sharp spectral features of the THz AHE. Finally, we find that the intrinsic contribution to the THz AHE dominates over the extrinsic mechanisms for the Co$_{32}$Fe$_{68}$ sample. The results imply that the AHE and related effects such as the spin Hall effect are highly promising ingredients of future THz spintronic devices reliably operating from DC to 40 THz and beyond.

cond-mat.mtrl-sci↗

arXiv2021

Observation of multi-skyrmion objects created by size and density control in Ta/CoFeB/MgO films

Magnetic skyrmions are chiral spin textures with a nontrivial topology that offer a potential for future magnetic memory and storage devices. The controlled formation and adjustment of size and density of magnetic skyrmions in Ta/CoFeB/MgO trilayers is demonstrated. It is the ideal candidate for the use as a bottom electrode integration into CoFeB/MgO/CoFeB magnetic tunnel junctions. Varying the CoFeB thickness close to the out-of-plane to in-plane magnetic phase transition, we find that subtle energy contributions enable the skyrmion formation in a narrow thickness window, corresponding to only around 10 pm variation in CoFeB thickness. Using magneto-optical imaging with quantitative image processing, variations in skyrmion diameter and distribution below the Abbe limit can be analyzed. We demonstrate a high degree of diameter and density control. Zero-field stable skyrmions can be set with proper magnetic field initialization. This demonstrated tunability and degree of comprehension of skyrmion formation, paves the way for future skyrmion based magnetic memory. Moreover, we demonstrate a controlled merging of individual skyrmions to complex topological objects. We compare our results with the baby-Skyrme model, developed to describe the soliton nature, for any topological charge n, and demonstrate the ability to form multi-skyrmion objects. These objects will be interesting for fundamental mathematical studies of the topological behavior of solitons in the future.

cond-mat.mes-hall↗

arXiv2021

The impact of metallic contacts on spin-polarized photocurrents in topological insulator $\text{Bi}_2\text{Se}_3$ nanowires

Recently, a new quantum phase, the topological insulator, has been vividly investigated in a variety of materials. Its unique bandstructure allows for optical generation and control of spin-polarized currents based on the circular photogalvanic effect. In this paper, we generate and distinguish the different photocurrent contributions via the the polarization of the driving light wave. We discuss the helicity-dependent spin-polarized current and the polarization independent thermoelectric current as spatially resolved maps, focusing on the influence of the topological insulator/metallic contact interface. We observe for both current contributions a significant enhancement of the current values at the topological insulator/metallic contact interface and moreover a dipole-like distribution of the spin-polarized current close to the contacts. We discuss the general behavior of the thermovoltage as a three-material Seebeck effect and explain the enhanced values by the acceleration of the photoelectrons generated in the space charge region of the topological insulator/metallic contact interface. Furthermore, we interpret the temperature gradient together with the spin Nernst effect as a possible origin for the enhancement and dipole-like distribution of the spin-polarized current.

cond-mat.mes-hall↗