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Markus Stöcker

Publications and source records attributed to Markus Stöcker.

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Ultra-slow orbital and spin dynamics in an electrically tunable quantum dot molecule

Tunnel-coupled optically active quantum dot molecules (QDMs), have the potential to operate as spin-photon-interfaces with coupled spins that interact with two different photon frequencies at the same time. A prerequisite is to deterministically prepare two (electron or hole) spins in the QDM and be able to electrically tune the orbital state couplings. Here, we demonstrate the sequential optical charging of a single QDM with two electron spins while simultaneously maintaining the ability to widely tune orbital couplings using static electric fields and optically drive the system for quantum light generation. We optically prepare one- and two-spin states, initialize via optical pumping and explore orbital and spin relaxation dynamics for one and two-spin states as a function of the energy detuning and hybridization of orbital states. For two-spin states, remarkably long S-T relaxation times are observed extending beyond $\sim 100\mu s$ with strong dependence on the relative energy of ground and excited two-spin states. Qualitative agreement is observed with $\mathbf{k \cdot p}$ calculations of phonon-mediated spin-relaxation. Our results provide new quantitative understanding of the dynamics of one and two-spin states and confirm their suitability of QDMs for creating multidimensional photonic cluster states by exploiting tunable spin-spin exchange couplings at zero magnetic fields combined with optical driving.

cond-mat.mes-hall

Resonant and Anti-resonant Exciton-Phonon Coupling in Quantum Dot Molecules

Optically active quantum dot molecules (QDMs) can host multi-spin quantum states with the potential for the deterministic generation of photonic graph states with tailored entanglement structures. Their usefulness for the generation of such non-classical states of light is determined by orbital and spin decoherence mechanisms, particularly phonon-mediated processes dominant at energy scales up to a few millielectronvolts. Here, we directly measure the spectral function of orbital phonon relaxation in a QDM and benchmark our findings against microscopic kp theory. Our results reveal phonon-mediated relaxation rates exhibiting pronounced resonances and anti-resonances, with rates ranging from several ten ns$^{-1}$ to tens of $μ$s$^{-1}$. Comparison with a kinetic model reveals the voltage (energy) dependent phonon coupling strength and fully explains the interplay between phonon-assisted relaxation and radiative recombination. These anti-resonances can be leveraged to increase the lifetime of energetically unfavorable charge configurations needed for realizing efficient spin-photon interfaces and multi-dimensional cluster states.

cond-mat.mes-hall

Deep-Learning-Based Radio-Frequency Side-Channel Attack on Quantum Key Distribution

Quantum key distribution (QKD) protocols are proven secure based on fundamental physical laws, however, the proofs consider a well-defined setting and encoding of the sent quantum signals only. Side channels, where the encoded quantum state is correlated with properties of other degrees of freedom of the quantum channel, allow an eavesdropper to obtain information unnoticeably as demonstrated in a number of hacking attacks on the quantum channel. Yet, also classical radiation emitted by the devices may be correlated, leaking information on the potential key, especially when combined with novel data analysis methods. We here demonstrate a side-channel attack using a deep convolutional neural network to analyze the recorded classical, radio-frequency electromagnetic emissions. Even at a distance of a few centimeters from the electronics of a QKD sender employing frequently used electronic components we are able to recover virtually all information about the secret key. Yet, as shown here, countermeasures can enable a significant reduction of both the emissions and the amount of secret key information leaked to the attacker. Our analysis methods are independent of the actual device and thus provide a starting point for assessing the presence of classical side channels in QKD devices.

quant-ph