arXiv subjects

Marta Fajardo

Publications and source records attributed to Marta Fajardo.

9 recordsLinked to original sources

arXiv2026

Reexamination of collisional ionization cross sections including double photoionization processes

Collisional ionization (CI) cross sections in dense plasmas remain difficult to constrain due to uncertainties in plasma conditions and the overlapping spectral signatures of competing atomic processes. The use of x-ray free electron lasers (XFELs) to both heat and probe solid-density targets has significantly advanced the field by eliminating assumptions about ion density. However, questions remain regarding collisional cross sections, suprathermal electron evolution and competing atomic processes. In this work, we revisit experimental data from XFEL-heated aluminum, previously analyzed using collisional radiative models that did not treat the degenerate electron distribution and atomic processes self consistently. We present a new analysis using BibBarT which dynamically evolves non-thermal electron populations and explicitly includes degeneracy effects. Furthermore, we incorporate an important atomic process recently observed in plasma state that mimic signatures of CI, shake-off. Our results show that including shake-off processes improves agreement with observed emission features, and lowering recombination rates further improves the agreement with data -- indicating a possible overestimate of three-body recombination in these conditions.

physics.plasm-ph↗

arXiv2026

Space-time beams with tunable orbital group velocity toward plasma superradiance

Light springs are space-time beams that have a helical wavepacket. Due to this special property, light springs result into a rotating pulse when intercepting a plane lying orthogonal to their propagation direction. Associated to this, we introduce here the orbital group velocity, an additional tunable property of light springs. The orbital group velocity quantifies the speed of the light spring intensity rotation, distinctly from the conventional longitudinal group velocity, which describes the motion of the wavepacket envelope along its propagation axis. We demonstrate experimentally by tunable Fourier synthesis that the orbital group velocity can assume sub- and superluminal values, thus becoming a new platform for synthetic motion studies and control of laser-matter interactions. Particularly, in the superluminal regime, when interacting with a thin overdense plasma, we reveal by particle-in-cell simulations that the light spring unlocks superradiant radiation, due to the coherent excitation of the electrons in the plasma acting as a quasiparticle. This superradiant source inherits the ultrafast temporal dynamics of the light springs while emitting in the terahertz region, thus creating a new source of terahertz radiation controlled by the properties of spatiotemporal coupling of the laser. Therefore, spatiotemporal tuning of light springs is at the frontier of controlling laser-matter interaction and generating new tunable sources of radiation.

physics.optics↗

arXiv2025

High-aspect-ratio silica meta-optics for high-intensity structured light

Structured light and high-intensity ultrafast lasers are two rapidly advancing frontiers in photonics, yet their intersection remains largely unexplored. While ultrafast lasers continue to push the boundaries of peak intensities, structured light has enabled unprecedented control over light's spatial, temporal, and polarization properties. However, the lack of robust optical devices capable of bridging structured light with the high-intensity domain has constrained progress in combining these directions. Here, we demonstrate high-aspect-ratio silica meta-optics, which close this gap by combining silica's extraordinary damage resistance with the advanced phase and polarization control offered by metasurfaces. By leveraging anisotropic etching techniques, we fabricate nanopillars exceeding 3 $\mu$m in height with aspect ratios up to 14, enabling precise manipulation of complex light fields at intensities far beyond the thresholds of conventional metasurfaces. We showcase their functionality in generating vortex beams and achieving polarization manipulation with large phase retardance at challenging long-visible wavelengths. High-aspect-ratio silica meta-optics unlock structured laser-matter interactions in extreme regimes, that will surpass plasma ionization thresholds and enable applications such as relativistic particle acceleration and high-harmonic generation with structured beams, for both tabletop ultrafast systems and large-scale laser facilities.

physics.optics↗

arXiv2025

Relaxation pathways in X-ray Free Electron Laser heated Iron

Non-thermal photo-ionized plasmas are now established in the laboratory, and require models that treat the atomic processes and electron distribution self-consistently. We investigate the effects of inelastic thermalization in iron under intense X-ray irradiation using the atomic model BigBarT, suited for the self-consistent evolution of the electron continuum, including degeneracy effects. Our study focuses particularly on collisional $M$-shell ionization, which we identify as the dominant relaxation process of the non-thermal electrons. We show that $M$-shell satellite intensities are sensitive to non-thermal ionization, providing a potential method to refine collisional cross sections that are otherwise difficult to compute due to their proximity to the continuum and the associated plasma screening effects.

physics.plasm-ph↗

arXiv2025

Incoherent Diffraction Imaging with a Pseudo-Thermal Light Source

Incoherent Diffraction Imaging - IDI - is a diffraction-based imaging technique that has been recently proposed to exploit the partial coherence of incoherently scattered light to retrieve structural information from the scattering centers. Similar to the stellar intensity interferometry of Hanbury Brown and Twiss, the signal builds up on the second-order spatial correlations of the emitted light. The complex spatial distribution of the target is thereby encoded in the spatial intensity fluctuations of the scattered light. The first experimental realisations of this imaging technique have been realised using the fluorescence excited by an ultra-short X-ray pulse at Free Electron Laser (FEL) facilities. Here, we propose an alternative set-up based on a table-top Pseudo-Thermal Light Source. This set-up allows us to explore IDI under a wide range of physically relevant conditions as well as to benchmark numerical and analytical models currently used to determine the imaging capabilities of this technique.

physics.optics↗

arXiv2022

Self-probed ptychography from semiconductor high-harmonic generation

We demonstrate a method to image an object using a self-probing approach based on semiconductor high-harmonic generation. On one hand, ptychography enables high-resolution imaging from the coherent light diffracted by an object. On the other hand, high-harmonic generation from crystals is emerging as a new source of extreme-ultraviolet ultrafast coherent light. We combine these two techniques by performing ptychography measurements with nano-patterned crystals serving as the object as well as the generation medium of the harmonics. We demonstrate that this strong field in situ approach can provide structural information about the object. With the future developments of crystal high harmonics as a compact short-wavelength light source, our demonstration can be an innovative approach for nanoscale imaging of photonic and electronic devices in research and industry.

physics.optics↗

arXiv2021

The data-driven future of high energy density physics

The study of plasma physics under conditions of extreme temperatures, densities and electromagnetic field strengths is significant for our understanding of astrophysics, nuclear fusion and fundamental physics. These extreme physical systems are strongly non-linear and very difficult to understand theoretically or optimize experimentally. Here, we argue that machine learning models and data-driven methods are in the process of reshaping our exploration of these extreme systems that have hitherto proven far too non-linear for human researchers. From a fundamental perspective, our understanding can be helped by the way in which machine learning models can rapidly discover complex interactions in large data sets. From a practical point of view, the newest generation of extreme physics facilities can perform experiments multiple times a second (as opposed to ~daily), moving away from human-based control towards automatic control based on real-time interpretation of diagnostic data and updates of the physics model. To make the most of these emerging opportunities, we advance proposals for the community in terms of research design, training, best practices, and support for synthetic diagnostics and data analysis.

physics.plasm-ph↗

arXiv2021

Non-linear propagation effects of intense femtosecond pulses on low order harmonics in solids

The non-linear propagation of the intense near-infrared (NIR) driving field in wide bandgap materials pose a challenge and an opportunity to control the spectral properties of high harmonic generation (HHG) in solids. Here, we have investigated the non-linear propagation effects of the ultrafast intense near-infrared (NIR) driving field at 800 nm of 40 fs pulse duration operating at a repetition rate of 1 kHz focused on the wide bandgap dielectrics such as MgO, Chromium (Cr) doped MgO (Cr: MgO), Sapphire (Sa) crystals and fused silica (FS). Furthermore, we have generated second and third harmonic (TH) in these materials to explore the non-linear response at a strong field. To quantify the non-linear propagation effects, low-order harmonics have been generated in reflection and compared with the harmonics generated in transmission. We observe spectral shifts and broadening of the driving field spectrum which is imprinted on the harmonics. We attribute these effects to strong photoionization, generation of free-carrier density and self-phase modulation effects. We have also studied the polarization dependence of second harmonic generation (SHG) and TH in FS. The linear polarization dependence of below bandgap harmonics in FS and Sa generated in reflection demonstrated the sharp anisotropy than in transmission. This work shows the sensitivity to control the spectral profile of harmonics by manipulating the driving field, showing the possibility of new tailored solid-state XUV sources for optical diagnostics.

physics.optics↗

arXiv2020

Controlling the nonlinear optical properties of MgO by tailoring the electronic structure

The study of the non-linear response of matter to high electric fields has recently encompassed harmonic generation in solids at near-infrared (NIR) driving wavelengths. Interest has been driven by the prospect of ultrafast signal processing and all-optical mapping of electron wave-functions in solids. Engineering solid-state band structures to control the non-linear process has already been highlighted theoretically. Here, we show experimentally for the first time that second harmonic generation (SHG) can be enhanced by doping crystals of magnesium oxide (MgO) with chromium (Cr) atoms. We show that the degree of enhancement depends non-linearly on dopant concentration. The SHG efficiency is shown to increase when Cr dopants are introduced into pure MgO. A physical picture of the effect of Cr dopants is aided by density functional theory (DFT) calculations of the electronic structure for pure and doped samples. This work shows an unambiguous enhancement of the SHG efficiency by modifying the electronic structure. The observed effects are consistent with an electronic structure that facilitates the surface induced SHG and demonstrates a minimal angular dependence. This work highlights the potential of manipulating the electronic structure of solids to control or test theories of their non-linear optical response.

physics.optics↗