arXiv subjects

Martial Ducloy

Publications and source records attributed to Martial Ducloy.

At least 19 recordsLinked to original sources

arXiv2024

Doppler-free selective reflection spectroscopy of electric-quadrupole transitions

Electric-dipole-forbidden transitions play an important role as in quantum sensing, quantum information, and fundamental test in physics. As such, the development of novel and sensitive spectroscopic methods is of major interest. Here, we present a Doppler-free selective reflection experiment on the 6S1/2 --> 5D5/2 electric-quadrupole transition of cesium vapor at the vicinity of a sapphire window. This is achieved by a precision experiment overcoming limitations due to the small signal amplitude of forbidden transitions. Narrow sub-Doppler lines allow for a collisional broadening measurement on the electric-quadrupole line. The interaction of cesium atoms with the sapphire surface of the cell is evidenced, but, due to its weak contribution, a quantitative analysis remains challenging. Nevertheless, our experiment paves the way for further studies of the Casimir-Polder interaction between exotic excited-state atoms and dielectric surfaces.

physics.atom-ph↗

arXiv2022

An excited atom interacting with a Chern insulator: towards a far-field resonant Casimir-Polder repulsion

We consider the resonant Casimir-Polder interaction of an excited alkali-type atom which has a single (electric dipole) transition with a Chern insulator. The Chern insulator has a nonzero, time reversal symmetry breaking Hall conductance, leading to an additional contribution to the resonant Casimir-Polder interaction which depends on the coupling between the Hall conductance and the circular polarization state of the atomic transition. We find that the resonant Casimir-Polder shift can be significantly enhanced for de-excitation frequencies near values associated with the van Hove singularities of the Chern insulator. Furthermore, we find that the resonant Casimir-Polder force can become monotonically decaying and repulsive for a relatively large atom-surface distance, if the atomic dipole transition is right circularly polarized and the Chern number of the Chern insulator is $-1$ or the atomic dipole transition is left circularly polarized and the Chern number is $1$.

quant-ph↗

arXiv2021

Atom-surface physics: A review

An atom in front of a surface is one of the simplest and fundamental problem in physics. Yet, it allows testing quantum electrodynamics, while providing potential platforms and interfaces for quantum technologies. Despite, its simplicity, combined with strong scientific and technological interests, atom-surface physics, at its fundamental level, remains largely unexplored mainly because of challenges associated with precise control of the atom-surface distance. Nevertheless, substantial breakthroughs have been made over the last two decades. With the development of cold and quantum atomic gases, one has gained further control on atom-surface position, naturally leading to improved precision in the Casimir-Polder interaction measurement. Advances have also been reported in finding experimental knobs to tune and even reverse the Casimir-Polder interaction strength. So far, this has only been achieved for atoms in short-lived excited states, however, the rapid progresses in material sciences, e.g. metamaterials and topological materials have inspired new ideas for controlling the atom-surface interaction in long-lived states. In addition, combining nano-photonic and atom-surface physics is now envisioned for applications in quantum information processing. The first purpose of this review is to give a general overview on the latest experimental developments in atom-surface physics. The second main objective is to sketch a vision of the future of the field, mainly inspired by the abundant theoretical works and proposals available now in the literature.

physics.atom-ph↗

arXiv2020

Plasmono-Atomic Interactions on a Fiber Tip

Light-atom interaction can be engineered by interfacing atoms with various specially designed media and optical fibers are convenient platforms for realization of compact interfaces. Here, we show that an optical fiber sensor bearing a plasmonic metasurface at its tip can be used to detect modifications of the Doppler-free hyperfine atomic spectra induced by coupling between atomic and plasmonic excitations. We observed the inversion of the phase modulation reflectivity spectra of Cesium vapor in presence of the metamaterial. This work paves the way for future compact hybrid atomic devices with a cleaved tip as substrate platform to host various two-dimensional materials.

physics.atom-ph↗

arXiv2019

Coupling of atomic quadrupole transitions with resonant surface plasmons

We report on the coupling of an electric quadrupole transition in atom with plasmonic excitation in a nanostructured metallic metamaterial. The quadrupole transition at 685 nm in the gas of Cesium atoms is optically pumped, while the induced ground state population depletion is probed with light tuned on the strong electric dipole transition at 852 nm. We use selective reflection to resolve the Doppler-free hyperfine structure of Cesium atoms. We observed a strong modification of the reflection spectra at the presence of metamaterial and discuss the role of the spatial variation of the surface plasmon polariton on the quadrupole coupling.

physics.atom-ph↗

arXiv2018

Tailoring optical metamaterials to tune the atom-surface Casimir-Polder interaction

Metamaterials are fascinating tools that can structure not only surface plasmons and electromagnetic waves but also electromagnetic vacuum fluctuations. The possibility of shaping the quantum vacuum is a powerful concept that ultimately allows engineering the interaction between macroscopic surfaces and quantum emitters such as atoms, molecules or quantum dots. The long-range atom-surface interaction, known as Casimir-Polder interaction, is of fundamental importance in quantum electrodynamics but also attracts a significant interest for platforms that interface atoms with nanophotonic devices. Here we perform a spectroscopic selective reflection measurement of the Casimir-Polder interaction between a Cs(6P_{3/2}) atom and a nanostructured metallic planar metamaterial. We show that by engineering the near-field plasmonic resonances of the metamaterial, we can successfully tune the Casimir-Polder interaction, demonstrating both a strong enhancement and reduction with respect to its non-resonant value. We also show an enhancement of the atomic spontaneous emission rate due to its coupling with the evanescent modes of the nanostructure. Probing excited state atoms next to nontrivial tailored surfaces is a rigorous test of quantum electrodynamics. Engineering Casimir-Polder interactions represents a significant step towards atom trapping in the extreme near field, possibly without the use of external fields.

physics.atom-ph↗

arXiv2018

Retardation effects in spectroscopic measurements of the Casimir-Polder interaction

Spectroscopy is a unique experimental tool for measuring the fundamental Casimir-Polder interaction between excited state atoms, or other polarizable quantum objects, and a macroscopic surface. Spectroscopic measurements probe atoms at nanometric distances away from the surface where QED retardation is usually negligible and the atom-surface interaction is proportional to the inverse cube of the separation distance, otherwise known as the van der Waals regime. Here we focus on selective reflection, one of the main spectroscopic probes of Casimir-Polder interactions. We calculate for the first time selective reflection spectra using the full, distance dependent, Casimir-Polder energy shift and linewidth. We demonstrate that retardation can have significant effects, in particular for experiments with low-lying energy states. We also show that the effective probing depth of selective reflection spectroscopy depends on the transition linewidth. Our analysis allows us to calculate selective reflection spectra with composite surfaces, such as metasurfaces, dielectric stacks, or even bi-dimensional materials.

physics.atom-ph↗

arXiv2016

Doppler-free approach to optical pumping dynamics in the $6S_{1/2}- 5D_{5/2}$ electric quadrupole transition of Cesium vapor

The $6S_{1/2}-5D_{5/2}$ electric quadrupole transition is investigated in Cesium vapor at room temperature via nonlinear Doppler-free 6P-6S-5D three-level spectroscopy. Frequency-resolved studies of individual E2 hyperfine lines allow one to analyze optical pumping dynamics, polarization selection rules and line intensities. It opens the way to studies of transfer of light orbital angular momentum to atoms, and the influence of metamaterials on E2 line spectra.

physics.atom-ph↗

arXiv2016

Atomic Response in the Near-field of Nanostructured Plasmonic Metamaterial

We report on reflection spectra of caesium atoms in close vicinity of a nanostructured metallic meta-surface. We show that the hyperfine sub-Doppler spectrum of the $6S_{1/2} - 6P_{3/2}$ resonance transition at 852 nm is strongly affected by the coupling to the plasmonic resonance of the nanostructure. Fine tuning of dispersion and positions of the atomic lines in the near-field of plasmonic metamaterials could have uses and implications for the atom-based metrology, sensing and the development of atom-on-a-chip devices.

cond-mat.mes-hall↗

arXiv2014

Casimir-Polder forces in the presence of thermally excited surface modes

The temperature dependence of the Casimir-Polder interaction addresses fundamental issues for understanding vacuum and thermal fluctuations. It is highly sensitive to surface waves which, in the near field, govern the thermal emission of a hot surface. Here we use optical reflection spectroscopy to monitor the atom-surface interaction between a Cs*(7D3/2) atom and a hot sapphire surface at a distance ~ 100 nm. In our experiments, that explore a large range of temperatures (500-1000K) the hot surface is at thermal equilibrium with the vacuum. The observed increase of the interaction with temperature, by up to 50 %, relies on the coupling between atomic virtual transitions in the infrared range and thermally excited surface-polariton modes. We extrapolate our findings to a broad distance range, from the isolated free atom to the short distances relevant to physical chemistry. Our work also opens the prospect of controlling atom surface interactions by engineering thermal fields.

physics.atom-ph↗

arXiv2014

Experimental observations of temperature effects in the near-field regime of the Casimir-Polder interaction

We investigate the temperature dependence of the Casimir-Polder interaction in the electrostatic limit. This unusual phenomenon relies on the coupling between a virtual atomic transition and a thermal excitation of surface polariton modes. We first focus on the scenario where a Cs(8P3/2) atom is next to a CaF2 or a BaF2 surface. Our theoretical predictions show a strong temperature dependence of the van der Waals coefficient at experimentally accessible conditions. A series of spectroscopic measurements performed in a specially designed Cs vapour cell containing a CaF2 tube is presented. Our results illustrate the sensitivity of atom surface-interaction experiments to the quality and chemical stability of the surface material and emphasize the need of using more durable materials, such as sapphire. We finally discuss selective reflection experiments on Cs(7D3/2) in an all-sapphire cell that clearly demonstrate a temperature dependent van der Waals coefficient.

physics.atom-ph↗

arXiv2012

Mapping of focused Laguerre-Gauss beams: The interplay between spin and orbital angular momentum and its dependence on detector characteristics

We show that propagating optical fields bearing an axial symmetry are not truly hollow in spite of a null electric field on-axis. The result, obtained by general arguments based upon the vectorial nature of electromagnetic fields, is of particular significance in the situation of an extreme focusing, when the paraxial approximation no longer holds. The rapid spatial variations of fields with a "complicated" spatial structure are extensively analyzed in the general case and for a Laguerre-Gauss beam 2 as well, notably for beams bearing a |l| = 2 orbital angular momentum for which a magnetic field and a gradient of the electric field are present on-axis. We thus analyze the behavior of a atomic size light-detector, sensitive as well to quadrupole electric transitions and to magnetic dipole transitions, and apply it to the case of Laguerre-Gauss beam. We detail how the mapping of such a beam depends on the nature and on the specific orientation of the detector. We show also that the interplay of mixing of polarization and topological charge, respectively associated to spin and orbital momentum when the paraxial approximation holds, modifies the apparent size of the beam in the focal plane. This even leads to a breaking of the cylindrical symmetry in the case of a linearly polarized transverse electric field.

physics.atom-ph↗

arXiv2011

Engineering of radiation of optically active molecules with chiral nano-meta-particles

The radiation of optically active (chiral) molecule placed near chiral nanoparticle is investigated. The optimal conditions for engineering of radiation of optically active (chiral) molecules with the help of chiral nanoparticles are derived. It is shown that for this purpose, the substance of the chiral particle must have both ε_and μ_negative (double negative material (DNG)) or negative μ_and positive ε_(μ_negative material (MNG)). Our results pave the way to an effective engineering of radiation of "left" and "right" molecules and to creating pure optical devices for separation of drugs enantiomers.

physics.optics↗

arXiv2009

Temperature dependence of the dielectric permittivity of CaF2, BaF2 and Al2O3: application to the prediction of a temperature dependent van der Waals surface interaction exerted onto a neighbouring Cs (8P{3/2}) atom

The temperature behaviour in the range 22\degree C to 500\degree C of the dielectric permittivity in the infrared range is investigated for CaF2, BaF2 and Al2O3 through reflectivity measurements. The dielectric permittivity is retrieved by fitting reflectivity spectra with a model taking into account multiphonon contributions. The results extrapolated from the measurements are applied to predict a temperature-dependent atom-surface van der Waals interaction. We specifically consider as the atom of interest Cs (8P3/2), the most relevant virtual couplings of which, fall in the range of thermal radiation and are located in the vicinity of the reststrahlen band of fluoride materials.

cond-mat.mtrl-sci↗

arXiv2007

Selective reflection spectroscopy of a vapour at a calcium fluoride interface

Fluoride materials exhibit surface resonances located in the thermal infrared. This makes them interesting to search for a fundamental temperature dependence of the atom-surface interaction, originating in the near-field thermal emissivity of the surface. Preliminary selective reflection experiments performed on a special Cs vapour cell that includes a CaF2 interface show a temperature dependence, yet to be analyzed

physics.atom-ph↗

arXiv2007

Selective Reflection Spectroscopy at the Interface between a Calcium Fluoride Window and Cs Vapour

A special vapour cell has been built, that allows the measurement of the atom-surface van der Waals interaction exerted by a CaF2 window at the interface with Cs vapour. Mechanical and thermal fragility of fluoride windows make common designs of vapour cells unpractical, so that we have developed an all-sapphire sealed cell with an internal CaF2 window. Although impurities were accidentally introduced when filling-up the prototype cell, leading to a line-broadening and shift, the selective reflection spectrum on the Cs D1 line (894 nm) makes apparent the weak van der Waals surface interaction. The uncertainties introduced by the effects of these impurities in the van der Waals measurement are nearly eliminated when comparing the selective reflection signal at the CaF2 interface of interest, and at a sapphire window of the same cell. The ratio of the interaction respectively exerted by a sapphire interface and a CaF2 interface is found to be 0.55 $\pm$ 0.25, in good agreement with the theoretical evaluation of ~0.67.

physics.atom-ph↗

arXiv2007

Theoretical study of dark resonances in micro-metric thin cells

We investigate theoretically dark resonance spectroscopy for a dilute atomic vapor confined in a thin (micro-metric) cell. We identify the physical parameters characterizing the spectra and study their influence. We focus on a Hanle-type situation, with an optical irradiation under normal incidence and resonant with the atomic transition. The dark resonance spectrum is predicted to combine broad wings with a sharp maximum at line-center, that can be singled out when detecting a derivative of the dark resonance spectrum. This narrow signal derivative, shown to broaden only sub-linearly with the cell length, is a signature of the contribution of atoms slow enough to fly between the cell windows in a time as long as the characteristic ground state optical pumping time. We suggest that this dark resonance spectroscopy in micro-metric thin cells could be a suitable tool for probing the effective velocity distribution in the thin cell arising from the atomic desorption processes, and notably to identify the limiting factors affecting desorption under a grazing incidence.

quant-ph↗

arXiv2007

Testing the distance-dependence of the van der Waals interaction between an atom and a surface through spectroscopy in a vapor nanocell

This paper presents our current measurements in a vapor nanocell aiming at a test of the distance-dependence of the atom-surface interaction, when simple asymptotic descriptions may turn to be not valid. A state-of-the-art of atom-surface interaction measurements is provided as an introduction, along with the comparison with the theory of the van der Waals (or Casimir-Polder) interaction; it is followed by a presentation of the most salient features of nanocell spectroscopy

physics.atom-ph↗