arXiv subjects

Martin B. Plenio

Publications and source records attributed to Martin B. Plenio.

At least 181 records · Page 10Linked to original sources

arXiv2016

Universal Quantum Computing with Arbitrary Continuous-Variable Encoding

Implementing a qubit quantum computer in continuous-variable systems conventionally requires the engineering of specific interactions according to the encoding basis states. In this work, we present a unified formalism to conduct universal quantum computation with a fixed set of operations but arbitrary encoding. By storing a qubit in the parity of two or four qumodes, all computing processes can be implemented by basis state preparations, continuous-variable exponential-swap operations, and swap-tests. Our formalism inherits the advantages that the quantum information is decoupled from collective noise, and logical qubits with different encodings can be brought to interact without decoding. We also propose a possible implementation of the required operations by using interactions that are available in a variety of continuous-variable systems. Our work separates the `hardware' problem of engineering quantum-computing-universal interactions, from the `software' problem of designing encodings for specific purposes. The development of quantum computer architecture could hence be simplified.

quant-ph↗

arXiv2016

Necessary and sufficient condition for quantum adiabatic evolution by unitary control fields

We decompose the quantum adiabatic evolution as the products of gauge invariant unitary operators and obtain the exact nonadiabatic correction in the adiabatic approximation. A necessary and sufficient condition that leads to adiabatic evolution with geometric phases is provided and we determine that in the adiabatic evolution, while the eigenstates are slowly varying, the eigenenergies and degeneracy of the Hamiltonian can change rapidly. We exemplify this result by the example of the adiabatic evolution driven by parametrized pulse sequences. For driving fields that are rotating slowly with the same average energy and evolution path, fast modulation fields can have smaller nonadiabatic errors than obtained under the traditional approach with a constant amplitude.

quant-ph↗

arXiv2016

Positioning Nuclear Spins in Interacting Clusters for Quantum Technologies and Bio-imaging

We propose a method to measure the hyperfine vectors between a nitrogen-vacancy (NV) center and an environment of interacting nuclear spins. Our protocol enables the generation of tunable electron-nuclear coupling Hamiltonians while suppressing unwanted inter-nuclear interactions. In this manner, each nucleus can be addressed and controlled individually thereby permitting the reconstruction of the individual hyperfine vectors. With this ability the 3D-structure of spin ensembles and spins in bio-molecules can be identified without the necessity of varying the direction of applied magnetic fields. We demonstrate examples including the complete reconstruction of an interacting spin cluster in diamond and 3D imaging of all the nuclear spins in a bio-molecule.

quant-ph↗

arXiv2016

Delayed entanglement echo for individual control of a large number of nuclear spins

Methods for achieving quantum control and detection of individual nuclear spins by single electrons of solid-state defects play a central role for quantum information processing and nano-scale nuclear magnetic resonance (NMR). However, with standard techniques, no more than 8 nuclear spins have been resolved. Here we develop a method that improves significantly the ability to spectrally resolve nuclear spins and demonstrate its capabilities with detailed numerical simulations by using a nitrogen-vacancy (NV) centre as model system. Based on delayed entanglement control, a technique combining microwave and radio-frequency (rf) fields, nuclei with resonances in a broad frequency band can be unambiguously and individually addressed by the sensor electron. Additionally the spectral resolution can extend beyond the electron spin relaxation time by using a long-lived qubit memory. Our method greatly increases the number of useful register qubits accessible to a defect centre and improves the signals of nano-scale NMR.

quant-ph↗

arXiv2016

Laser cooling of high temperature oscillator by multi-level system

We study the laser cooling of a mechanical oscillator through the coupling with a dissipative three-level system. Under a background temperature beyond the Lamb-Dicke regime, we extend the standard cooling analysis by separately studying the classical motion and the quantum dynamics of the oscillator. In Ladder-system cooling, the cooling rate degrades by orders of magnitude at large classical motion. This phenomenon causes a critical transition of the final temperature at a hot background. In stark contrast, electromagnetic-induced-transparency (EIT) cooling with a $Λ$-system produces significant negative cooling rate at high motional excitation. At steady state, the oscillator could exhibit both cooling and lasing behaviours. We argue that a successful EIT cooling requires either a poor quality oscillator to suppress the lasing effect, or terminating the cooling process at a transient stage.

quant-ph↗

arXiv2016

Quantum Phase Transition in the Finite Jaynes-Cummings Lattice Systems

Phase transitions are commonly held to occur only in the thermodynamical limit of large number of system components. Here we exemplify at the hand of the exactly solvable Jaynes-Cummings (JC) model and its generalization to finite JC-lattices that finite component systems of coupled spins and bosons may exhibit quantum phase transitions (QPT). For the JC-model we find a continuous symmetry-breaking QPT, a photonic condensate with a macroscopic occupation as the ground state and a Goldstone mode as a low-energy excitation. For the two site JC-lattice we show analytically that it undergoes a Mott-insulator to superfluid QPT. We identify as the underlying principle of the emergence of finite size QPT the combination of increasing atomic energy and increasing interaction strength between the atom and the bosonic mode which allows for the exploration of an increasingly large portion of the infinite dimensional Hilbert space of the bosonic mode. This suggests that finite system phase transitions will be present in a broad range of physical systems.

quant-ph↗

arXiv2016

Converting Nonclassicality into Entanglement

Quantum mechanics exhibits a wide range of nonclassical features, of which entanglement in multipartite systems takes a central place. In several specific settings, it is well known that nonclassicality (e.g., squeezing, spin squeezing, coherence) can be converted into entanglement. In this work, we present a general framework, based on superposition, for structurally connecting and converting nonclassicality to entanglement. In addition to capturing the previously known results, this framework also allows us to uncover new entanglement convertibility theorems in two broad scenarios, one which is discrete and one which is continuous. In the discrete setting, the classical states can be any finite linearly independent set. For the continuous setting, the pertinent classical states are 'symmetric coherent states,' connected with symmetric representations of the group SU(K). These results generalize and link convertibility properties from the resource theory of coherence, spin coherent states, and optical coherent states, while also revealing important connections between local and nonlocal pictures of nonclassicality.

quant-ph↗

arXiv2016

Quantum metrology enhanced by repetitive quantum error correction

The accumulation of quantum phase in response to a signal is the central mechanism of quantum sensing, as such, loss of phase information presents a fundamental limitation. For this reason approaches to extend quantum coherence in the presence of noise are actively being explored. Here we experimentally protect a room-temperature hybrid spin register against environmental decoherence by performing repeated quantum error correction whilst maintaining sensitivity to signal fields. We use a long-lived nuclear spin to correct multiple phase errors on a sensitive electron spin in diamond and realize magnetic field sensing beyond the timescales set by natural decoherence. The universal extension of sensing time, robust to noise at any frequency, demonstrates the definitive advantage entangled multi-qubit systems provide for quantum sensing and offers an important complement to quantum control techniques. In particular, our work opens the door for detecting minute signals in the presence of high frequency noise, where standard protocols reach their limits.

quant-ph↗

arXiv2016

Dynamical error bounds for continuum discretisation via Gauss quadrature rules, -- a Lieb-Robinson bound approach

Instances of discrete quantum systems coupled to a continuum of oscillators are ubiquitous in physics. Often the continua are approximated by a discrete set of modes. We derive analytical error bounds on expectation values of system observables that have been time evolved under such discretised Hamiltonians. These bounds take on the form of a function of time and the number of discrete modes, where the discrete modes are chosen according to Gauss quadrature rules. The derivation makes use of tools from the field of Lieb-Robinson bounds and the theory of orthonormal polynominals.

quant-ph↗

arXiv2016

Optically induced dynamic nuclear spin polarisation in diamond

The sensitivity of Magnetic Resonance Imaging (MRI) depends strongly on nuclear spin polarisation and, motivated by this observation, dynamical nuclear spin polarisation has recently been applied to enhance MRI protocols (Kurhanewicz, J., et al., Neoplasia 13, 81 (2011)). Nuclear spins associated with the 13 C carbon isotope (nuclear spin I = 1/2) in diamond possess uniquely long spin lattice relaxation times (Reynhardt, E.C. and G.L. High, Prog. in Nuc. Mag. Res. Sp. 38, 37 (2011)) If they are present in diamond nanocrystals, especially when strongly polarised, they form a promising contrast agent for MRI. Current schemes for achieving nuclear polarisation, however, require cryogenic temperatures. Here we demonstrate an efficient scheme that realises optically induced 13 C nuclear spin hyperpolarisation in diamond at room temperature and low ambient magnetic field. Optical pumping of a Nitrogen-Vacancy (NV) centre creates a continuously renewable electron spin polarisation which can be transferred to surrounding 13 C nuclear spins. Importantly for future applications we also realise polarisation protocols that are robust against an unknown misalignment between magnetic field and crystal axis.

quant-ph↗

arXiv2015

Quantum Phase Transition and Universal Dynamics in the Rabi model

We consider the Rabi Hamiltonian which exhibits a quantum phase transition (QPT) despite consisting only of a single-mode cavity field and a two-level atom. We prove QPT by deriving an exact solution in the limit where the atomic transition frequency in unit of the cavity frequency tends to infinity. The effect of a finite transition frequency is studied by analytically calculating finite-frequency scaling exponents as well as performing a numerically exact diagonalization. Going beyond this equilibrium QPT setting, we prove that the dynamics under slow quenches in the vicinity of the critical point is universal, that is, the dynamics is completely characterized by critical exponents. Our analysis demonstrates that the Kibble-Zurek mechanism can precisely predict the universal scaling of residual energy for a model without spatial degrees of freedom. Moreover, we find that the onset of the universal dynamics can be observed even with a finite transition frequency.

quant-ph↗

arXiv2015

Proposal for high-fidelity quantum simulation using a hybrid dressed state

A fundamental goal of quantum technologies concerns the exploitation of quantum coherent dynamics for the realisation of novel quantum applications such as quantum computing, quantum simulation, and quantum metrology. A key challenge on the way towards these goals remains the protection of quantum coherent dynamics from environmental noise. Here, we propose a concept of hybrid dressed state from a pair of continuously driven systems. It allows sufficiently strong driving fields to suppress the effect of environmental noise, while at the same time being insusceptible to both the amplitude and phase noise in the continuous driving fields. This combination of robust features significantly enhances coherence times under realistic conditions, and at the same time provides new flexibility in Hamiltonian engineering that otherwise is not achievable. We demonstrate theoretically applications of our scheme for noise resistant analog quantum simulation in the well studied physical systems of nitrogen-vacancy centers in diamond and of trapped ions. The scheme may also be exploited for quantum computation and quantum metrology.

quant-ph↗

arXiv2015

Enhancing light-harvesting power with coherent vibrational interactions: a quantum heat engine picture

Recent evidence suggests that quantum effects may have functional importance in biological light-harvesting systems. Along with delocalized electronic excitations, it is now suspected that quantum coherent interactions with certain near-resonant vibrations may contribute to light-harvesting performance. However, the actual quantum advantage offered by such coherent vibrational interactions has not yet been established. We investigate a quantum design principle, whereby coherent exchange of single energy quanta between electronic and vibrational degrees of freedom can enhance a light-harvesting system's power above what is possible by thermal mechanisms alone. We present a prototype quantum heat engine which cleanly illustrates this quantum design principle, and quantify its quantum advantage using thermodynamic measures of performance. We also demonstrate the principle's relevance in parameter regimes connected to natural light-harvesting structures.

physics.chem-ph↗

arXiv2015

Formation of helical ion chains

We study the nonequilibrium dynamics of the linear to zigzag structural phase transition exhibited by an ion chain confined in a trap with periodic boundary conditions. The transition is driven by reducing the transverse confinement at a finite quench rate, which can be accurately controlled. This results in the formation of zigzag domains oriented along different transverse planes. The twists between different domains can be stabilized by the topology of the trap and under laser cooling the system has a chance to relax to a helical chain with nonzero winding number. Molecular dynamics simulations are used to obtain a large sample of possible trajectories for different quench rates. The scaling of the average winding number with different quench rates is compared to the prediction of the Kibble-Zurek theory, and a good quantitative agreement is found.

quant-ph↗

arXiv2015

Filter design for hybrid spin gates

The impact of control sequences on the environmental coupling of a quantum system can be described in terms of a filter. Here we analyze how the coherent evolution of two interacting spins subject to periodic control pulses, at the example of a nitrogen vacancy center coupled to a nuclear spin, can be described in the filter framework in both the weak and the strong coupling limit. A universal functional dependence around the filter resonances then allows for tuning the coupling type and strength. Originally limited to small rotation angles, we show how the validity range of the filter description can be extended to the long time limit by time-sliced evolution sequences. Based on that insight, the construction of tunable, noise decoupled, conditional gates composed of alternating pulse sequences is proposed. In particular such an approach can lead to a significant improvement in fidelity as compared to a strictly periodic control sequence. Moreover we analyze the decoherence impact, the relation to the filter for classical noise known from dynamical decoupling sequences, and we outline how an alternating sequence can improve spin sensing protocols.

quant-ph↗

arXiv2015

Optical signatures of quantum delocalization over extended domains in photosynthetic membranes

The prospect of coherent dynamics and excitonic delocalization across several light-harvesting structures in photosynthetic membranes is of considerable interest, but challenging to explore experimentally. Here we demonstrate theoretically that the excitonic delocalization across extended domains involving several light-harvesting complexes can lead to unambiguous signatures in the optical response, specifically, linear absorption spectra. We characterize, under experimentally established conditions of molecular assembly and protein-induced inhomogeneities, the optical absorption in these arrays from polarized and unpolarized excitation, and demonstrate that it can be used as a diagnostic tool to determine the coherent coupling among iso-energetic light-harvesting structures. The knowledge of these couplings would then provide further insight into the dynamical properties of transfer, such as facilitating the accurate determination of Förster rates.

physics.chem-ph↗

arXiv2015

Accelerated 2D magnetic resonance spectroscopy of single spins using matrix completion

Two dimensional nuclear magnetic resonance (NMR) spectroscopy is one of the major tools for analysing the chemical structure of organic molecules and proteins. Despite its power, this technique requires long measurement times, which, particularly in the recently emerging diamond based single molecule NMR, limits its application to stable samples. Here we demonstrate a method which allows to obtain the spectrum by collecting only a small fraction of the experimental data. Our method is based on matrix completion which can recover the full spectral information from randomly sampled data points. We confirm experimentally the applicability of this technique by performing two dimensional electron spin echo envelope modulation (ESEEM) experiments on a two spin system consisting of a single nitrogen vacancy (NV) centre in diamond coupled to a single 13C nuclear spin. We show that the main peaks in the spectrum can be obtained with only 10 % of the total number of the data points. We believe that our results reported here can find an application in all types of two dimensional spectroscopy, as long as the measured matrices have a low rank.

quant-ph↗

arXiv2015

Vibronic origin of long-lived coherence in an artificial molecular light harvester

Natural and artificial light harvesting processes have recently gained new interest. Signatures of long lasting coherence in spectroscopic signals of biological systems have been repeatedly observed, albeit their origin is a matter of ongoing debate, as it is unclear how the loss of coherence due to interaction with the noisy environments in such systems is averted. Here we report experimental and theoretical verification of coherent exciton-vibrational (vibronic) coupling as the origin of long-lasting coherence in an artificial light harvester, a molecular J-aggregate. In this macroscopically aligned tubular system, polarization controlled 2D spectroscopy delivers an uncongested and specific optical response as an ideal foundation for an in-depth theoretical description. We derive analytical expressions that show under which general conditions vibronic coupling leads to prolonged excited-state coherence.

physics.chem-ph↗