arXiv subjects

Martin Frimmer

Publications and source records attributed to Martin Frimmer.

At least 37 records · Page 2Linked to original sources

arXiv2022

Scalable all-optical cold damping of levitated nanoparticles

The field of levitodynamics has made significant progress towards controlling and studying the motion of a levitated nanoparticle. Motional control relies on either autonomous feedback via a cavity or measurement-based feedback via external forces. Recent demonstrations of measurement-based ground-state cooling of a single nanoparticle employ linear velocity feedback, also called cold damping, and require the use of electrostatic forces on charged particles via external electrodes. Here we introduce a novel all-optical cold damping scheme based on spatial modulation of the trap position that is scalable to multiple particles. The scheme relies on using programmable optical tweezers to provide full independent control over trap frequency and position of each tweezer. We show that the technique cools the center-of-mass motion of particles down to $17\,$mK at a pressure of $2 \times 10^{-6}\,$mbar and demonstrate its scalability by simultaneously cooling the motion of two particles. Our work paves the way towards studying quantum interactions between particles, achieving 3D quantum control of particle motion without cavity-based cooling, electrodes or charged particles, and probing multipartite entanglement in levitated optomechanical systems.

physics.optics↗

arXiv2022

Optimal orientation detection of an anisotropic dipolar scatterer

The angular orientation of an anisotropic scatterer with cylindrical symmetry in a linearly polarized light field represents an optomechanical librator. Here, we propose and theoretically analyze an optimal measurement scheme for the two angular degrees of freedom of such a librator. The imprecision-backaction product of this scheme reaches the Heisenberg uncertainty limit. Furthermore, we propose and analyze a realistic measurement scheme and show that, in the absence of spinning motion around the symmetry axis, measurement-based ground-state cooling of the rotational degrees of freedom of an anisotropic point scatterer levitated in an optical trap is feasible.

physics.optics↗

arXiv2022

Ponderomotive squeezing of light by a levitated nanoparticle in free space

A mechanically compliant element can be set into motion by the interaction with light. In turn, this light-driven motion can give rise to ponderomotive correlations in the electromagnetic field. In optomechanical systems, cavities are often employed to enhance these correlations up to the point where they generate quantum squeezing of light. In free-space scenarios, where no cavity is used, observation of squeezing remains possible but challenging due to the weakness of the interaction, and has not been reported so far. Here, we measure the ponderomotively squeezed state of light scattered by a nanoparticle levitated in a free-space optical tweezer. We observe a reduction of the optical fluctuations by up to $25$~\% below the vacuum level, in a bandwidth of about $15$~kHz. Our results are well explained by a linearized dipole interaction between the nanoparticle and the electromagnetic continuum. These ponderomotive correlations open the door to quantum-enhanced sensing and metrology with levitated systems, such as force measurements below the standard quantum limit.

quant-ph↗

arXiv2021

Controlling spatial coherence with an optical complex medium

Control over optical spatial coherence is a key requirement in diverse applications including imaging, optical trapping, and communications. Current approaches to controlling spatial coherence are constrained by speed or limited to a single pair of optical fields. Here, we propose a method to achieve single-shot control of the spatial coherence between an arbitrary number of fields. Our method employs a multi-port linear optical device, which we realize by shaping the wavefront of the input light fields and transmitting them through a complex medium. To demonstrate the capabilities of our method, we experimentally realize a 3x3-port system and use it to generate three output beams with desired mutual correlations.

physics.optics↗

arXiv2021

Quantum control of a nanoparticle optically levitated in cryogenic free space

Tests of quantum mechanics on a macroscopic scale require extreme control over mechanical motion and its decoherence. Quantum control of mechanical motion has been achieved by engineering the radiation-pressure coupling between a micromechanical oscillator and the electromagnetic field in a resonator. Furthermore, measurement-based feedback control relying on cavity-enhanced detection schemes has been used to cool micromechanical oscillators to their quantum ground states. In contrast to mechanically tethered systems, optically levitated nanoparticles are particularly promising candidates for matter-wave experiments with massive objects, since their trapping potential is fully controllable. In this work, we optically levitate a femto-gram dielectric particle in cryogenic free space, which suppresses thermal effects sufficiently to make the measurement backaction the dominant decoherence mechanism. With an efficient quantum measurement, we exert quantum control over the dynamics of the particle. We cool its center-of-mass motion by measurement-based feedback to an average occupancy of 0.65 motional quanta, corresponding to a state purity of 43%. The absence of an optical resonator and its bandwidth limitations holds promise to transfer the full quantum control available for electromagnetic fields to a mechanical system. Together with the fact that the optical trapping potential is highly controllable, our experimental platform offers a route to investigating quantum mechanics at macroscopic scales.

quant-ph↗

arXiv2021

Raman Sideband Thermometry of Single Carbyne Chains

We demonstrate Raman sideband thermometry of single carbyne chains confined in double-walled carbon nanotubes. Our results show that carbyne's record-high Raman scattering cross section enables anti-Stokes Raman measurements at the single chain level. Using laser irradiation as a heating source, we exploit the temperature dependence of the anti-Stokes/Stokes ratio for local temperature sensing. Due to its molecular size and its large Raman cross section carbyne is an efficient probe for local temperature monitoring, with applications ranging from nanoelectronics to biology.

cond-mat.mes-hall↗

arXiv2021

Kovacs memory effect with an optically levitated nanoparticle

The understanding of the dynamics of nonequilibrium cooling and heating processes at the nanoscale is still an open problem. These processes can follow surprising relaxation paths due to, e.g., memory effects, which significantly alter the expected equilibration routes. The Kovacs effect can take place when a thermalization process is suddenly interrupted by a change of the bath temperature, leading to a non-monotonic dependence of the energy of the system. Here, we demonstrate that the Kovacs effect can be observed in the thermalization of the center of mass motion of a levitated nanoparticle. The temperature is controlled during the experiment through an external source of white gaussian noise. We describe our experiments in terms of the dynamics of a Brownian particle in a harmonic trap without any fitting parameter, suggesting that the Kovacs effect canappear in a large variety of systems.

cond-mat.mes-hall↗

arXiv2021

Observation of radiation torque shot noise on an optically levitated nanodumbbell

According to quantum theory, measurement and backaction are inextricably linked. In optical position measurements, this backaction is known as radiation pressure shot noise. In analogy, a measurement of the orientation of a mechanical rotor must disturb its angular momentum by radiation torque shot noise. In this work, we observe the shot-noise torque fluctuations arising in a measurement of the angular orientation of an optically levitated nanodumbbell. We feedback cool the dumbbell's rotational motion and investigate its reheating behavior when released from feedback. In high vacuum, the heating rate due to radiation torque shot noise dominates over the thermal and technical heating rates in the system.

physics.optics↗

arXiv2020

Escape dynamics of active particles in multistable potentials

Rare transitions between long-lived metastable states underlie a great variety of physical, chemical and biological processes. Our quantitative understanding of reactive mechanisms has been driven forward by the insights of transition state theory. In particular, the dynamic framework developed by Kramers marks an outstanding milestone for the field. Its predictions, however, do not apply to systems driven by non-conservative forces or correlated noise histories. An important class of such systems are active particles, prominent in both biology and nanotechnology. Here, we trap a silica nanoparticle in a bistable potential. To emulate an active particle, we subject the particle to an engineered external force that mimics self-propulsion. We investigate the active particle's transition rate between metastable states as a function of friction and correlation time of the active force. Our experiments reveal the existence of an optimal correlation time where the transition rate is maximized. This novel \emph{active turnover} is reminiscent of the much celebrated Kramers turnover despite its fundamentally different origin. Our observations are quantitatively supported by a theoretical analysis of a one-dimensional model. Besides providing a deeper understanding of the escape dynamics of active particles in multistable potentials, our work establishes a new, versatile experimental platform to study particle dynamics in non-equilibrium settings.

cond-mat.soft↗

arXiv2020

Cooling mechanical oscillators by coherent control

In optomechanics, electromagnetic fields are harnessed to control a single mode of a mechanically compliant system, while other mechanical degrees of freedom remain unaffected due to the modes' mutual orthogonality and high quality factor. Extension of the optical control beyond the directly addressed mode would require a controlled coupling between mechanical modes. Here, we introduce an optically controlled coupling between two oscillation modes of an optically levitated nanoparticle. We sympathetically cool one oscillation mode by coupling it coherently to the second mode, which is feedback cooled. Furthermore, we demonstrate coherent energy transfer between mechanical modes and discuss its application for ground-state cooling.

quant-ph↗

arXiv2020

Optically levitated rotor at its thermal limit of frequency stability

Optically levitated rotors are prime candidates for torque sensors whose precision is limited by the fluctuationsof the rotation frequency. In this work we investigate an optically levitated rotor at its fundamental thermal limitof frequency stability, where rotation-frequency fluctuations arise solely due to coupling to the thermal bath.

physics.optics↗

arXiv2020

Raman Scattering Cross Section of Confined Carbyne

We experimentally quantify the Raman scattering from individual carbyne chains confined in double-walled carbon nanotubes. We find that the resonant differential Raman cross section of confined carbyne is on the order of $10^{-22}$ cm$^{2}\,$sr$^{-1}$ per atom, making it the strongest Raman scatterer ever reported.

cond-mat.mes-hall↗

arXiv2019

Rapid flipping of parametric phase states

Since the invention of the solid-state transistor, the overwhelming majority of computers followed the von Neumann architecture that strictly separates logic operations and memory. Today, there is a revived interest in alternative computation models accompanied by the necessity to develop corresponding hardware architectures. The Ising machine, for example, is a variant of the celebrated Hopfield network based on the Ising model. It can be realized with artifcial spins such as the `parametron' that arises in driven nonlinear resonators. The parametron encodes binary information in the phase state of its oscillation. It enables, in principle, logic operations without energy transfer and the corresponding speed limitations. In this work, we experimentally demonstrate flipping of parametron phase states on a timescale of an oscillation period, much faster than the ringdown time τthat is often (erroneously) deemed a fundamental limit for resonator operations. Our work establishes a new paradigm for resonator-based logic architectures.

physics.app-ph↗

arXiv2019

Motional Sideband Asymmetry of a Nanoparticle Optically Levitated in Free Space

The hallmark of quantum physics is Planck's constant $h$, whose finite value entails the quantization that gave the theory its name. The finite value of $h$ gives rise to inevitable zero-point fluctuations even at vanishing temperature. The zero-point fluctuation of mechanical motion becomes smaller with growing mass of an object, making it challenging to observe at macroscopic scales. Here, we transition a dielectric particle with a diameter of 136 nm from the classical realm to the regime where its zero-point motion emerges as a sizeable contribution to its energy. To this end, we optically trap the particle at ambient temperature in ultrahigh vacuum and apply active feedback cooling to its center-of-mass motion. We measure an asymmetry between the Stokes and anti-Stokes sidebands of photons scattered by the levitated particle, which is a signature of the particle's quantum ground state of motion.

physics.optics↗

arXiv2019

Optimal Position Detection of a Dipolar Scatterer in a Focused Field

We theoretically analyze the problem of detecting the position of a classical dipolar scatterer in a strongly focused optical field. We suggest an optimal measurement scheme and show that it resolves the scatterer's position in three dimensions at the Heisenberg limit of the imprecision-backaction product. We apply our formalism to levitated-optomechanics experiments and show that backscattering detection provides sufficient information to feedback-cool the particle's motion along the optical axis to a phonon occupancy below unity under realistic experimental conditions.

physics.optics↗

arXiv2018

Cold Damping of an Optically Levitated Nanoparticle to micro-Kelvin Temperatures

We implement a cold damping scheme to cool one mode of the center-of-mass motion of an optically levitated nanoparticle in ultrahigh vacuum from room temperature to a record-low temperature of 100 micro-Kelvin. The measured temperature dependence on feedback gain and thermal decoherence rate is in excellent agreement with a parameter-free model. We determine the imprecision-backaction product for our system and provide a roadmap towards ground-state cooling of optically levitated nanoparticles.

physics.optics↗

arXiv2018

GHz Rotation of an Optically Trapped Nanoparticle in Vacuum

We report on rotating an optically trapped silica nanoparticle in vacuum by transferring spin angular momentum of light to the particle's mechanical angular momentum. At sufficiently low damping, realized at pressures below $10^{-5}$ mbar, we observe rotation frequencies of single 100 nm particles exceeding 1 GHz. We find that the steady-state rotation frequency scales linearly with the optical trapping power and inversely with pressure, consistent with theoretical considerations based on conservation of angular momentum. Rapidly changing the polarization of the trapping light allows us to extract the pressure-dependent response time of the particle's rotational degree of freedom.

physics.optics↗

arXiv2018

Measuring the Internal Temperature of a Levitated Nanoparticle in High Vacuum

The interaction of an object with its surrounding bath can lead to a coupling between the object's internal degrees of freedom and its center-of-mass motion. This coupling is especially important for nanomechanical oscillators, which are amongst the most promising systems for preparing macroscopic objects in quantum mechanical states. Here we exploit this coupling to derive the internal temperature of a levitated nanoparticle from measurements of its center-of-mass dynamics. For a laser-trapped silica particle in high vacuum we find an internal temperature of $1000(60)\,\mathrm{K}$. The measurement and control of the internal temperature of nanomechanical oscillators is of fundamental importance because blackbody emission sets limits to the coherence of macroscopic quantum states.

physics.ins-det↗