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Martin Hrtoň

Publications and source records attributed to Martin Hrtoň.

15 recordsLinked to original sources

Inverse designed full-Stokes polarimetric metasurface with simultaneous wavefront sensing for visible light

Metasurfaces have emerged as a powerful platform for compact optical sensors by replacing bulky lenses with flat arrays of subwavelength nanostructures. In precision optical metrology, the simultaneous mapping of a beam's polarization state and wavefront is crucial for real-time diagnostics of stress-induced birefringence and surface flatness. To achieve this in a compact footprint, existing metasurfaces typically partition their aperture into discrete zones, which inherently restricts the light-gathering efficiency and numerical aperture of the system. Here we demonstrate an inverse-designed metasurface that integrates full-Stokes polarimetry and Shack-Hartmann wavefront sensing within a single, continuous aperture in the visible spectrum. By leveraging an adjoint optimization approach to independently control the geometry and rotation of each nanostructure, we break the aperture-sharing paradigm and utilize the entire pixel area for all channels. When coupled with a shallow neural network to automate peak identification and correct for hardware non-idealities, our device yields a mean polarization reconstruction error of only 0.046 across 100 test states on the Poincaré sphere, while simultaneously maintaining the precise focal-spot tracking required for sensitive wavefront tilt detection. This work highlights the capacity of inverse design to generate multifunctional, non-intuitive flat optics that outperforms its traditional counterparts.

physics.optics↗

Optimal conditions for detecting optical dichroism at the nanoscale by electron energy-loss spectroscopy

The emergence of optical circular dichroism in chiral nanoscale and molecular systems provides not only a way for analyzing the sample chirality itself but also additional degrees of freedom in manipulating light. Such manipulation can be reached even at the nanoscale level; however, probing and understanding the properties of optical fields well below the diffraction limit requires an adequate technique. Electron energy-loss spectroscopy (EELS) with orbital angular momentum (OAM)-based electron state sorting has been suggested as a suitable candidate, but to date, no conclusive experiments have been performed. We, therefore, theoretically explore the emergence of dichroism in EELS for a canonical single-twist helix nanostructure and present a detailed analysis of the optimal parameters to obtain a robust signal. Our work offers novel insights into the interpretation and volatility of the OAM-resolved EELS signal, which can inspire and guide future experimental efforts.

cond-mat.mes-hall↗

SpinWaveToolkit: Python package for (semi-)analytical calculations in the field of spin-wave physics

We present an open-source Python package, SpinWaveToolkit (SWT), for (semi-)analytical modeling of spin-wave dynamics in thin ferromagnetic films and exchange-coupled magnetic bilayers. SWT combines analytical models based on the Kalinikos-Slavin theory with a semi-analytical dynamic-matrix approach, enabling the calculation of dispersion relations, group velocities, decay lengths, mode profiles, and static equilibrium magnetization states. In addition, SWT implements a quantitative model of micro-focused Brillouin light scattering (BLS) that incorporates vectorial optical focusing, spin-wave Bloch functions, magneto-optical coupling, and Green-function propagation to simulate experimentally measured BLS spectra. The package is validated against finite-element dynamic-matrix simulations performed with TetraX for Damon-Eshbach, backward-volume, forward-volume, and oblique-field geometries, showing excellent agreement while reducing computation times by nearly two orders of magnitude in comparison to the numerical simulations. Thanks to the easiness of the use and fast calculation times, SWT can be used not only for exploratory mapping of the parameter space, but also for the fitting of the measured dispersion relations and related parameters. Thus, it provides a versatile and efficient framework for experiment design, interpretation, and parameter optimization for magnonics research.

cond-mat.mes-hall↗

Establishing a library of metasurface building blocks through coherence-controlled holographic microscopy

Digital holographic microscopy is a powerful tool for characterizing transparent and reflective phase objects. Its ability to reconstruct amplitude and phase can also offer great insight into wavefront shaping and design of all-dielectric optical metasurfaces. While metasurfaces have reached widespread popularity, their design is often based purely on the results of numerical simulations which can overlook many of the real-world fabrication imperfections. Being able to verify the real phase response of a fabricated device is of great utility for high-performance devices. Here, we use holographic microscopy to validate metalibraries of rectangular TiO2 and Si building blocks. Illumination effects are studied for wavelengths from 600 to 740 nm and linear polarization rotating within the full range of unique states (0 to 180deg). Finally, by varying the numerical aperture of the condenser lens from 0.05 to 0.5 we also study the effects of an off-axis illumination. Comparing the experimental results with simulations from finite-difference time-domain and rigorous coupled-wave analysis, we highlight the limitations of these theoretical predictions and underscore the utility of an experimentally established library of building blocks. We demonstrate that our proposed method of holographic microscopy is both practical and effective for creating a metalibrary that accounts for all fabrication and material imperfections, which is crucial for designing high-efficiency metasurfaces.

physics.optics↗

Modeling of the micro-focused Brillouin light scattering spectra

Although micro-focused Brillouin light scattering (BLS) has been used for more than twenty years, it lacks a complete theoretical description. This complicates the analysis of experimental data and significantly limits the information that can be obtained. To fill this knowledge gap, we have developed a semi-analytical model based on the mesoscopic continuous medium approach. The model consists of the following steps: calculation of the incident electric field and the dynamic susceptibility, calculation of the induced polarisation, and calculation of the emitted electric field and its propagation towards the detector. We demonstrate the model on the examples of the measurements of thermal and coherently excited spin waves. However, the used approach is general and can describe any micro-focused Brillouin light scattering experiment. The model can also bring new analytical approaches to mechanobiology experiments or to characterization of acoustic wave based devices.

cond-mat.mes-hall↗

Mie-enhanced micro-focused Brillouin light scattering with wavevector resolution

Magnons, the quanta of spin waves, are magnetic excitations of matter spanning through the entire crystal's Brillouin zone and covering a wide range of frequencies ranging from sub-gigahertz to hundreds of terahertz. Magnons play a crucial role in many condensed matter phenomena, such as the reduction of saturation magnetization with increasing temperature or Bose-Einstein condensation. However, current experimental techniques cannot resolve magnons with wavevectors between 30 and 300$\,$rad$\,μ$m$^{-1}$. In this letter, we address this gap by tailoring the light in Brillouin light scattering process with dielectric periodic nanoresonators and thus gaining access to the previously unmeasurable spin waves with full wavevector resolution using table-top optical setup. Filling this gap can stimulate further experimental investigations of the fundamental phenomena associated with magnons but also stimulate the application of magnonics in computational and microwave devices. In addition, the same methodology can be applied to other excitations of matter, such as phonons, opening up new possibilities in e.g. mechanobiological studies.

cond-mat.mes-hall↗

Exploring single-photon recoil on free electrons

Recent advancements in time-resolved electron and photon detection enable novel correlative measurements of electrons and their associated cathodoluminescence (CL) photons within a transmission electron microscope. These studies are pivotal for understanding the underlying physics in coherent CL processes. We present experimental investigations of energy-momentum conservation and the corresponding dispersion relation on the single particle level, achieved through coincidence detection of electron-photon pairs. This not only enables unprecedented clarity in detecting weak signals otherwise obscured by non-radiative processes but also provides a new experimental pathway to investigate momentum-position correlations to explore entanglement within electron-photon pairs.

quant-ph↗

Phase-resolved optical characterization of nanoscale spin waves

We study theoretically and experimentally the process of Brillouin light scattering on an array of silicon disks on a thin Permalloy layer. We show that phase-resolved Brillouin light scattering microscopy performed on an array of weakly interacting dielectric nanoresonators can detect nanoscale waves and measure their dispersion. In our experiment, we were able to map the evolution of the phase of the spin wave with a wavelength of 209 nm with a precision of 6 nm. These results demonstrate the feasibility of all-optical phase-resolved characterization of nanoscale spin waves.

physics.optics↗

Observing high-k magnons with Mie-resonance-enhanced Brillouin light scattering

Magnonics is a prospective beyond CMOS technology which uses magnons, the quanta of spin waves, for low-power information processing. Many magnonic concepts and devices were recently demonstrated at macro- and microscale, and now these concepts need to be realized at nanoscale. Brillouin light scattering spectroscopy and microscopy (BLS) has become a standard technique for spin wave visualization and characterization, and enabled many pioneering magnonic experiments. However, due to its fundamental limit in maximum detectable magnon momentum, the conventional BLS cannot be used to detect nanoscale spin waves. Here we show that optically induced Mie resonances in dielectric nanoparticles can be used to extend the range of accessible spin wave wavevectors beyond the BLS fundamental limit. The method is universal and can be used in many magnonic experiments dealing with thermally excited as well as coherently excited high-momentum, short-wavelength spin waves. This discovery significantly extends the usability and relevance of the BLS technique for nanoscale magnonic research.

cond-mat.mes-hall↗

Fabrication and micro-Raman spectroscopy of arrays of copper phthalocyanine molecular-magnet microdisks

Phthalocyanines as organic semiconductors and molecular magnets provide plenty of industrial or high-tech applications from dyes and pigments up to gas sensors, molecular electronics, spintronics and quantum computing. Copper phthalocyanine (CuPc) belongs among the most used phthalocyanines, typically in the form of powder or films but self-grown nanowires are also known. Here we describe an opposite, i.e., top-down approach based on fabrication of ordered arrays of CuPc microstructures (microdisks) using electron beam lithography and other steps. Among critical points of this approach belongs a choice of a proper resist and a solvent. Fabricated CuPc microdisks have a diameter of 5 $μ$m and heights from 7 up to 70 nm. Micro-Raman spectroscopy of the films and microdisks reveals a crystalline $β$ phase associated with a paramagnetic form. Additional measurements with an increasing laser power show a significant shift ($Δω$ ~ 7.1 cm$^{-1}$ ) and broadening of a peak at 1532 rel$\cdot$cm$^{-1}$ corresponding to the phonon B1g mode. The observed smooth changes exclude a phase transition and confirm the thermally stable polymorph. Our versatile fabrication technique using the common lithographic resist brings new possibilities for the fabrication of various micro/nanostructures such as micromagnets, heterostructures or organic electronic devices.

physics.app-ph↗

Full-range optical imaging of planar collagen fiber orientation using polarized light microscopy

A novel method for automated assessment of directions of collagen fibers in soft tissues is presented. It is based on multiple rotated images obtained via polarized light microscope with perpendicular and inclined polarizers and thus it breaks the limitation of 90° periodicity of polarized light intensity and evaluates the fiber orientation over the whole 180° range accurately and quickly. After having verified the method, we used histological specimens of porcine Achilles tendon and aorta to validate the proposed algorithm and to lower the number of rotated images needed for evaluation. Our algorithm is capable to analyze 5.10^5 pixels in one micrograph in a few seconds and is thus a powerful and cheap tool for histological image analysis of such samples promising a broad application.

physics.med-ph↗

Optically tunable Mie-resonance VO2 nanoantennas for metasurfaces in the visible

Metasurfaces are ultrathin nanostructured surfaces that can allow arbitrary manipulation of light. Implementing dynamic tunability into their design could allow the optical functions of metasurfaces to be rapidly modified at will. The most pronounced and robust tunability of optical properties is provided by phase-change materials such as vanadium dioxide (VO2) and germanium antimony telluride (GST), but their implementations have been limited only to near-infrared wavelengths. Here, we demonstrate that VO2 nanoantennas with widely tunable Mie resonances can be utilized for designing tunable metasurfaces in the visible range. In contrast to the dielectric-metallic phase transition-induced tunability in previous demonstrations, we show that dielectric Mie resonances in VO2 nanoantennas offer remarkable scattering and extinction modulation depths (5-8 dB and 1-3 dB, respectively) for tunability in the visible. Moreover, these strong resonances are optically switchable using a continuous-wave laser. Our results establish VO2 nanostructures as low-loss building blocks of optically tunable metasurfaces.

physics.optics↗

Independent engineering of individual plasmon modes in plasmonic dimers with conductive and capacitive coupling

We revisit plasmonic modes in nanoparticle dimers with conductive or insulating junction resulting in conductive or capacitive coupling. In our study which combines electron energy loss spectroscopy, optical spectroscopy, and numerical simulations, we show coexistence of strongly and weakly hybridized modes. While the properties of the former ones strongly depend on the nature of the junction, the properties of the latter ones are nearly unaffected. This opens up a prospect for independent engineering of different plasmonic modes in a single plasmonic antenna. In addition, we show that Babinet's principle allows to engineer the near field of plasmonic modes independent of their energy. Finally, we demonstrate that combined electron energy loss imaging of a plasmonic antenna and its Babinet-complementary counterpart allows to reconstruct the distribution of both electric and magnetic near fields of localised plasmonic resonances supported by the antenna as well as charge and current antinodes of related charge oscillations.

physics.app-ph↗

Plasmonic antennas with electric, magnetic, and electromagnetic hot spots based on Babinet's principle

We theoretically study plasmonic antennas featuring areas of extremely concentrated electric or magnetic field, known as hot spots. We combine two types of electric-magnetic complementarity to increase the degree of freedom for the design of the antennas: bow-tie and diabolo duality and Babinet's principle. We evaluate the figures of merit for different plasmon-enhanced optical spectroscopy methods: field enhancement, decay rate enhancement, and quality factor of the plasmon resonances. The role of Babinet's principle in interchanging electric and magnetic field hot spots and its consequences for practical antenna design are discussed. In particular, diabolo antennas exhibit slightly better performance than bow-ties in terms of larger field enhancement and larger Q factor. For specific resonance frequency, diabolo antennas are considerably smaller than bow-ties which makes them favourable for the integration into more complex devices but also makes their fabrication more demanding in terms of spatial resolution. Finally, we propose Babinet-type dimer antenna featuring electromagnetic hot spot with both the electric and magnetic field components treated on equal footing.

physics.app-ph↗

Geometric-phase microscopy for high-resolution quantitative phase imaging of plasmonic metasurfaces with sensitivity down to a single nanoantenna

Optical metasurfaces have emerged as a new generation of building blocks for multi-functional optics. Design and realization of metasurface elements place ever-increasing demands on accurate assessment of phase alterations introduced by complex nanoantenna arrays, a process referred to as quantitative phase imaging. Despite considerable effort, the widefield (non-scanning) phase imaging that would approach resolution limits of optical microscopy and indicate the response of a single nanoantenna still remains a challenge. Here, we report on a new strategy in incoherent holographic imaging of metasurfaces, in which unprecedented spatial resolution and light sensitivity are achieved by taking full advantage of the polarization selective control of light through the geometric (Pancharatnam-Berry) phase. The measurement is carried out in an inherently stable common-path setup composed of a standard optical microscope and an add-on imaging module. Phase information is acquired from the mutual coherence function attainable in records created in broadband spatially incoherent light by the self-interference of scattered and leakage light coming from the metasurface. In calibration measurements, the phase was mapped with the precision and spatial background noise better than 0.01 rad and 0.05 rad, respectively. The imaging excels at the high spatial resolution that was demonstrated experimentally by the precise amplitude and phase restoration of vortex metalenses and a metasurface grating with 833 lines/mm. Thanks to superior light sensitivity of the method, we demonstrated, for the first time to our knowledge, the widefield measurement of the phase altered by a single nanoantenna, while maintaining the precision well below 0.15 rad.

physics.optics↗