arXiv subjects

Martin Kamp

Publications and source records attributed to Martin Kamp.

At least 37 records · Page 2Linked to original sources

arXiv2024

Epitaxial RuO$_2$ and IrO$_2$ films by pulsed laser deposition on TiO$_2$(110)

We present a systematic growth study of epitaxial RuO$_2$(110) and IrO$_2$(110) on TiO$_2$(110) substrates by pulsed laser deposition. We describe the main challenges encountered in the growth process, such as a deteriorating material flux due to laser induced target metallization or the delicate balance of under- vs over-oxidation of the 'stubborn' Ru and Ir metals. We identify growth temperatures and oxygen partial pressures of 700 K, $1\times 10^{-3}$ mbar for RuO$_2$ and 770 K, $5\times 10^{-4}$ mbar for IrO$_2$ to optimally balance between metal oxidation and particle mobility during nucleation. In contrast to IrO$_2$, RuO$_2$ exhibits layer-by-layer growth up to 5 unit cells if grown at high deposition rates. At low deposition rates, the large lattice mismatch between film and substrate fosters initial 3D island growth and cluster formation. In analogy to reports for RuO$_2$ based on physical vapor deposition, we find these islands to eventually merge and growth to continue in a step flow mode, resulting in highly crystalline, flat, stoichiometric films of RuO$_2$(110) (up to 30 nm thickness) and IrO$_2$(110) (up to 13 nm thickness) with well defined line defects.

cond-mat.mtrl-sci↗

arXiv2023

Time-bin entanglement at telecom wavelengths from a hybrid photonic integrated circuit

Mass-deployable implementations for quantum communication require compact, reliable, and low-cost hardware solutions for photon generation, control and analysis. We present a fiber-pigtailed hybrid photonic circuit comprising nonlinear waveguides for photon-pair generation and a polymer interposer reaching 68dB of pump suppression and photon separation with >25dB polarization extinction ratio. The optical stability of the hybrid assembly enhances the quality of the entanglement, and the efficient background suppression and photon routing further reduce accidental coincidences. We thus achieve a 96(-8,+3)% concurrence and a 96(-5,+2)% fidelity to a Bell state. The generated telecom-wavelength, time-bin entangled photon pairs are ideally suited for distributing Bell pairs over fiber networks with low dispersion.

quant-ph↗

arXiv2023

Fabrication of low-loss III-V Bragg-reflection waveguides for parametric down-conversion

Entangled photon pairs are an important resource for quantum cryptography schemes that go beyond point-to-point communication. Semiconductor Bragg-reflection waveguides are a promising photon-pair source due to mature fabrication, integrability, large transparency window in the telecom wavelength range, integration capabilities for electro-optical devices as well as a high second-order nonlinear coefficient. To increase performance we improved the fabrication of Bragg-reflection waveguides by employing fixed-beam-moving-stage optical lithography, low pressure and low chlorine concentration etching, and resist reflow. The reduction in sidewall roughness yields a low optical loss coefficient for telecom wavelength light of alpha_reflow = 0.08(6)mm^(-1). Owing to the decreased losses, we achieved a photon pair production rate of 8800(300)(mW*s*mm)^(-1) which is 15-fold higher than in previous samples.

physics.optics↗

arXiv2023

Saturation of the anomalous Hall effect at high magnetic fields in altermagnetic RuO2

Observations of the anomalous Hall effect in RuO$_2$ and MnTe have demonstrated unconventional time-reversal symmetry breaking in the electronic structure of a recently identified new class of compensated collinear magnets, dubbed altermagnets. While in MnTe the unconventional anomalous Hall signal accompanied by a vanishing magnetization is observable at remanence, the anomalous Hall effect in RuO$_2$ is excluded by symmetry for the Néel vector pointing along the zero-field [001] easy-axis. Guided by a symmetry analysis and ab initio calculations, a field-induced reorientation of the Néel vector from the easy-axis towards the [110] hard-axis was used to demonstrate the anomalous Hall signal in this altermagnet. We confirm the existence of an anomalous Hall effect in our RuO$_2$ thin-film samples whose set of magnetic and magneto-transport characteristics is consistent with the earlier report. By performing our measurements at extreme magnetic fields up to 68 T, we reach saturation of the anomalous Hall signal at a field $H_{\rm c} \simeq$ 55 T that was inaccessible in earlier studies, but is consistent with the expected Néel-vector reorientation field.

cond-mat.mes-hall↗

arXiv2023

Stabilizing an atomically thin quantum spin Hall insulator at ambient conditions: Graphene-intercalation of indenene

Atomic monolayers on semiconductor surfaces represent a new class of functional quantum materials at the ultimate two-dimensional limit, ranging from superconductors [1, 2] to Mott insulators [3, 4] and ferroelectrics [5] to quantum spin Hall insulators (QSHI) [6, 7]. A case in point is the recently discovered QSHI indenene [7, 8], a triangular monolayer of indium epitaxially grown on SiC(0001), exhibiting a $\sim$120meV gap and substrate-matched monodomain growth on the technologically relevant $μ$m scale [9]. Its suitability for room-temperature spintronics is countered, however, by the instability of pristine indenene in air, which destroys the system along with its topological character, nullifying hopes of ex-situ processing and device fabrication. Here we show how indenene intercalation into epitaxial graphene offers effective protection from the oxidizing environment, while it leaves the topological character fully intact. This opens an unprecedented realm of ex-situ experimental opportunities, bringing this monolayer QSHI within realistic reach of actual device fabrication and edge channel transport.

cond-mat.mtrl-sci↗

arXiv2022

Moiré pattern formation in epitaxial growth on a covalent substrate: Sb on InSb(111)A

Structural moiré superstructures arising from two competing lattices may lead to unexpected electronic behavior, such as superconductivity or Mottness. Most investigated moiré heterostructures are based on van der Waals (vdW) materials, as strong interface interactions typically lead to the formation of strained films or regular surface reconstructions. Here we successfully synthesize ultrathin Sb films, that are predicted to show thickness-dependent topological properties, on semi-insulating InSb(111)A. Despite the covalent nature of the substrate surface, we prove by scanning transmission electron microscopy (STEM) that already the first layer of Sb atoms grows completely unstrained, while azimuthally aligned. Rather than compensating the lattice mismatch of -6.4% by structural modifications, the Sb films form a pronounced moiré pattern as we evidence by scanning tunneling microscopy (STM) topography up to film thicknesses of several bilayers. Our model calculations based on density functional theory (DFT) assign the moiré pattern to a periodic surface corrugation. In agreement with DFT predictions, irrespective of the moiré modulation, the topological surface state known on thick Sb film is experimentally confirmed to persist down to low film thicknesses, and the Dirac point shifts towards lower binding energies with decreasing Sb thickness.

cond-mat.mtrl-sci↗

arXiv2022

Linear colossal magnetoresistance driven by magnetic textures in LaTiO3 thin films on SrTiO3

Linear magnetoresistance (LMR) is of particular interest for memory, electronics, and sensing applications, especially when it does not saturate over a wide range of magnetic fields. One of its principal origins is local mobility or density inhomogeneities, often structural, which in the Parish-Littlewood theory leads to an unsaturating LMR proportional to mobility. Structural disorder, however, also tends to limit the mobility and hence the overall LMR amplitude. An alternative route to achieve large LMR is via non-structural inhomogeneities which do not affect the zero field mobility, like magnetic domains. Here, linear positive magnetoresistance caused by magnetic texture is reported in \ch{LaTiO3}/\ch{SrTiO3} heterostructures. The LMR amplitude reaches up to 6500\% at 9T. This colossal value is understood by the unusual combination of a very high thin film mobility, up to 40 000 cm$^2$/V.s, and a very large coverage of low-mobility regions. These regions correlate with a striped magnetic structure, compatible with a spiral magnetic texture in the \ch{LaTiO3} film, revealed by low temperature Lorentz transmission electron microscopy. These results provide a novel route for the engineering of large-LMR devices.

cond-mat.mes-hall↗

arXiv2021

Simulation of X-ray diffraction in Mn$_x$Bi$_2$Te$_{3+x}$ epitaxic films

Disordered heterostructures stand as a general description for compounds that are part of homologous series such as bismuth chalcogenides. In device engineering, van der Waals epitaxy of these compounds is very promising for applications in spintronic and quantum computing. Structural analysis methods are essential to control and improve their synthesis in the form of thin films. Recently, X-rays tools have been proposed for structural modeling of disordered heterostructures [arXiv:2107.12280]. Here, we further evaluate the use of these tools to study the compound Mn$_x$Bi$_2$Te$_{3+x}$ in the grazing incidence region of the reflectivity curves, as well as the effect of thickness fluctuation in the wide angle region.

cond-mat.mtrl-sci↗

arXiv2021

X-ray diffraction tools for structural modeling of epitaxic films of an intrinsic antiferromagnetic topological insulator

Synthesis of new materials demands structural analysis tools suited to the particularities of each system. Van der Waals (vdW) materials are fundamental in emerging technologies of spintronics and quantum information processing, in particular topological insulators and, more recently, materials that allow the phenomenological exploration of the combination of non-trivial electronic band topology and magnetism. Weak vdW forces between atomic layers give rise to composition fluctuations and structural disorder that are difficult to control even in a typical binary topological insulators such as Bi2Te3. The addition of a third element as in MnBi2Te4 makes the epitaxy of these materials even more chaotic. In this work, statistical model structures of thin films on single crystal substrates are described. It allows the simulation of X-ray diffraction in disordered heterostructures, a necessary step towards controlling the epitaxial growth of these materials. On top of this, the diffraction simulation method described here can be readily applied as a general tool in the field of design new materials based on stacking of vdW bonded layers of distint elements.

cond-mat.mtrl-sci↗

arXiv2020

Understanding photoluminescence in semiconductor Bragg-reflection waveguides: Towards an integrated, GHz-rate telecom photon pair source

Compared to traditional nonlinear optical crystals, like BaB$_2$O$_4$, KTiOPO$_4$ or LiNbO$_3$, semiconductor integrated sources of photon pairs may operate at pump wavelengths much closer to the bandgap of the materials. This is also the case for Bragg-reflection waveguides (BRW) targeting parametric down-conversion (PDC) to the telecom C-band. The large nonlinear coefficient of the AlGaAs alloy and the strong confinement of the light enable extremely bright integrated photon pair sources. However, under certain circumstances, a significant amount of detrimental broadband photoluminescence has been observed in BRWs. We show that this is mainly a result of linear absorption near the core and subsequent radiative recombination of electron-hole pairs at deep impurity levels in the semiconductor. For PDC with BRWs, we conclude that devices operating near the long wavelength end of the S-band or the short C-band require temporal filtering shorter than 1 ns. We predict that shifting the operating wavelengths to the L-band and making small adjustments in the material composition will reduce the amount of photoluminescence to negligible values. Such measures enable us to increase the average pump power and/or the repetition rate, which makes integrated photon pair sources with on-chip multi-gigahertz pair rates feasible.

quant-ph↗

arXiv2020

Molecular beam epitaxy of the half-Heusler antiferromagnet CuMnSb

We report growth of CuMnSb thin films by molecular beam epitaxy on InAs(001) substrates. The CuMnSb layers are compressively strained ($0.6~\text{%}$) due to lattice mismatch. The thin films have a $ω$ full width half max of $7.7^{''}$ according to high resolution X-ray diffraction, and a root mean square roughness of $0.14~\text{nm}$ as determined by atomic force microscopy. Magnetic and electrical properties are found to be consistent with reported values from bulk samples. We find a Néel temperature of $62~\text{K}$, a Curie-Weiss temperature of $-65~\text{K}$ and an effective moment of $5.9~μ_{\text{B}}/\text{f.u.}$. Transport measurements confirm the antiferromagetic transition and show a residual resistivity at $4~\text{K}$ of $35~μΩ\cdot \text{cm}$.

cond-mat.mtrl-sci↗

arXiv2020

Four-wave mixing dynamics of a strongly coupled quantum-dot--microcavity system driven by up to 20 photons

The Jaynes-Cummings (JC) model represents one of the simplest ways in which single qubits can interact with single photon modes, leading to profound quantum phenomena like superpositions of light and matter states. One system, that can be described with the JC model, is a single quantum dot embedded in a micropillar cavity. In this joint experimental and theoretical study we investigate such a system using four-wave mixing (FWM) micro-spectroscopy. Special emphasis is laid on the dependence of the FWM signals on the number of photons injected into the microcavity. By comparing simulation and experiment, which are in excellent agreement with each other, we infer that up to ~20 photons take part in the observed FWM dynamics. Thus we verify the validity of the JC model for the system under consideration in this non-trivial regime. We find that the inevitable coupling between the quantum dot exciton and longitudinal acoustic phonons of the host lattice influences the real time FWM dynamics and has to be taken into account for a sufficient description of the quantum dot-microcavity system. Performing additional simulations in an idealized dissipation-less regime, we observe that the FWM signal exhibits quasi-periodic dynamics, analog to the collapse and revival phenomenon of the JC model. In these simulations we also see that the FWM spectrum has a triplet structure, if a large number of photons is injected into the cavity.

cond-mat.mes-hall↗

arXiv2020

Picosecond Ultrasonics with Miniaturized Semiconductor Lasers

There is a great desire to extend ultrasonic techniques to the imaging and characterization of nanoobjects. This can be achieved by picosecond ultrasonics, where by using ultrafast lasers it is possible to generate and detect acoustic waves with frequencies up to terahertz and wavelengths down to nanometers. In our work we present a picosecond ultrasonics setup based on miniaturized mode-locked semiconductor lasers, whose performance allows us to obtain the necessary power, pulse duration and repetition rate. Using such a laser, we measure the ultrasonic echo signal with picosecond resolution in a Al film deposited on a semiconductor substrate. We show that the obtained signal is as good as the signal obtained with a standard bulky mode-locked Ti-Sa laser. The experiments pave the way for designing integrated portable picosecond ultrasonic setups on the basis of miniaturized semiconductor lasers.

physics.app-ph↗

arXiv2020

Acoustic Phonon Sideband Dynamics During Polaron Formation in a Single Quantum Dot

When an electron-hole pair is optically excited in a semiconductor quantum dot the host crystal lattice needs to adapt to the presence of the generated charge distribution. Therefore the coupled exciton-phonon system has to establish a new equilibrium, which is reached in the form of a quasiparticle called polaron. Especially, when the exciton is abruptly generated on a timescale faster than the typical lattice dynamics, the lattice displacement cannot follow adiabatically. Consequently, a rich dynamics on the picosecond timescale of the coupled system is expected. In this study we combine simulations and measurements of the ultrafast, coherent, nonlinear optical response, obtained by four-wave mixing spectroscopy, to resolve the formation of this polaron. By detecting and investigating the phonon sidebands in the four-wave mixing spectra for varying pulse delays and different temperatures we have access to the influence of phonon emission and absorption processes which finally result in the emission of an acoustic wave packet out from the quantum dot.

cond-mat.mes-hall↗

arXiv2019

Optical Thouless conductance and level-spacing statistics in two-dimensional Anderson localizing systems

We experimentally investigate spectral statistics in Anderson localization in two-dimensional amorphous disordered media. Intensity distributions captured over an ultrabroad wavelength range of $\sim 600$~nm and averaged over numerous configurations provided the Ioffe-Regel parameter to be $\sim2.5$ over the investigated wavelength range. The spectra of the disordered structures provided access to several quasimodes, whose widths and separations allowed to directly estimate the optical Thouless conductance $g_{Th}$, consistently observed to be below unity. The probability distribution of $g_{Th}$ was measured to be a log-normal. Despite being in the Anderson localization regime, the spacings of energy levels of the system was seen to follow a near Wigner-Dyson function. Theoretical calculations based on the tight-binding model, modified to include coupling to a bath, yielded results that were in excellent agreement with experiments. From the model, the level-spacing behavior was attributed to the degree of localization obtained in the optical disordered system.

physics.optics↗

arXiv2019

Discrepant transport characteristics under Anderson localization at the two limits of disorder

Anderson localization is a striking phenomenon wherein transport of light is arrested due to the formation of disorder-induced resonances. Hitherto, Anderson localization has been demonstrated separately in two limits of disorder, namely, amorphous disorder and nearly-periodic disorder. However, transport properties in the two limits are yet unstudied, particularly in a statistically consistent manner. Here, we experimentally measure light transport across two-dimensional open mesoscopic structures, wherein the disorder systematically ranges from nearly-periodic to amorphous. We measure the generalized conductance, which quantifies the transport probability in the sample. Although localization was identified in both the limits, statistical measurements revealed a discrepant behavior in the generalized conductance fluctuations in the two disorder regimes. Under amorphous disorder, the generalized conductance remains below unity for any configuration of the disorder, attesting to the arrested nature of transport. Contrarily, at near-periodic disorder, the distribution of generalized conductance is heavy-tailed towards large conductance values, indicating that the overall transport is delocalized. Theoretical results from a model based on the tight-binding approximation, augmented to include open boundaries, are in excellent agreement with experiments, and also endorse the results over much larger ensembles. These results quantify the differences in the two disorder regimes, and advance the studies of disordered systems into actual consequences of Anderson localization in light transport.

physics.optics↗

arXiv2018

Rabi oscillations of a quantum dot exciton coupled to acoustic phonons: coherence and population readout

While the advanced coherent control of qubits is now routinely carried out in low frequency (GHz) systems like single spins, it is far more challenging to achieve for two-level systems in the optical domain. This is because the latter evolve typically in the THz range, calling for tools of ultrafast, coherent, nonlinear optics. Using four-wave mixing micro-spectroscopy, we here measure the optically driven dynamics of a single exciton quantum state confined in a semiconductor quantum dot. In a combined experimental and theoretical approach, we reveal the intrinsic Rabi oscillation dynamics by monitoring both central exciton quantities, i.e., its occupation and the microscopic coherence, as resolved by the four-wave mixing technique. In the frequency domain this oscillation generates the Autler-Townes splitting of the light-exciton dressed states, directly seen in the four-wave mixing spectra. We further demonstrate that the coupling to acoustic phonons strongly influences the FWM dynamics on the picosecond timescale, because it leads to transitions between the dressed states.

cond-mat.mes-hall↗

arXiv2018

High-concurrence time-bin entangled photon pairs from optimized Bragg-reflection waveguides

Semiconductor Bragg-reflection waveguides are well-established sources of correlated photon pairs as well as promising candidates for building up integrated quantum optics devices. Here, we use such a source with optimized non-linearity for preparing time-bin entangled photons in the telecommunication wavelength range. By taking advantage of pulsed state preparation and efficient free-running single-photon detection, we drive our source at low pump powers, which results in a strong photon-pair correlation. The tomographic reconstruction of the state's density matrix reveals that our source exhibits a high degree of entanglement. We extract a concurrence of $88.9\pm 1.8\%$ and a fidelity of $94.2 \pm 0.9\%$ with respect to a Bell state.

quant-ph↗