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Martin Kamp

Publications and source records attributed to Martin Kamp.

At least 73 records · Page 4Linked to original sources

Experimental realization of a polariton beam amplifier

In this report we demonstrate a novel concept for a planar cavity polariton beam amplifier using non-resonant excitation. In contrast to resonant excitation schemes, background carriers are injected which form excitons, providing both gain and a repulsive potential for a polariton condensate. Using an attractive potential environment induced by a locally elongated cavity layer, the repulsive potential of the injected background carriers is compensated and a significant amplification of polariton beams is achieved without beam distortion.

cond-mat.mes-hall↗

Highly indistinguishable on-demand resonance fluorescence photons from a deterministic quantum dot micropillar device with 75 $\%$ extraction efficiency

The implementation and engineering of bright and coherent solid state quantum light sources is key for the realization of both on chip and remote quantum networks. Despite tremendous efforts for more than 15 years, the combination of these two key prerequisites in a single, potentially scalable device is a major challenge. Here, we report on the observation of bright and coherent single photon emission generated via pulsed, resonance fluorescence conditions from a single quantum dot (QD) deterministically centered in a micropillar cavity device via cryogenic optical lithography. The brightness of the QD fluorescence is greatly enhanced on resonance with the fundamental mode of the pillar, leading to an overall device efficiency of $η=(74\pm4)~\%$ for a single photon emission as pure as $g^{(2)}(0)=0.0092\pm0.0004$. The combination of large Purcell enhancement and resonant pumping conditions allows us to observe a two-photon wave packet overlap up to $ν=(88\pm3)~\%$

quant-ph↗

Deterministic generation of bright single resonance fluorescence photons from a Purcell-enhanced quantum dot-micropillar system

We report on the observation of bright emission of single photons under pulsed resonance fluorescence conditions from a single quantum dot (QD) in a micropillar cavity. The brightness of the QD fluorescence is greatly enhanced via the coupling to the fundamental mode of a micropillar, allowing us to determine a single photon extraction efficiency of $(20.7\pm0.8)~\%$ per linear polarization basis. This yields an overall extraction efficiency of $(41.4\pm1.5)~\%$ in our device. We observe the first Rabi-oscillation in a weakly coupled quantum dot-micropillar system under coherent pulsed optical excitation, which enables us to deterministically populate the excited QD state. In this configuration, we probe the single photon statistics of the device yielding $g^{(2)}(0)=0.072\pm0.011$ at a QD-cavity detuning of $75~μ$eV.

quant-ph↗

Observation of resonance fluorescence and the Mollow-triplet from a coherently driven site-controlled quantum dot

Resonant excitation of solid state quantum emitters has the potential to deterministically excite a localized exciton while ensuring a maximally coherent emission. In this work, we demonstrate the coherent coupling of an exciton localized in a lithographically positioned, site-controlled semiconductor quantum dot to an external resonant laser field. For strong continuous-wave driving we observe the characteristic Mollow triplet and analyze the Rabi splitting and sideband widths as a function of driving strength and temperature. The sideband widths increase linearly with temperature and the square of the driving strength, which we explain via coupling of the exciton to longitudinal acoustic phonons. We also find an increase of the Rabi splitting with temperature, which indicates a temperature induced delocalization of the excitonic wave function resulting in an increase of the oscillator strength. Finally, we demonstrate coherent control of the exciton excited state population via pulsed resonant excitation and observe a damping of the Rabi oscillations with increasing pulse area, which is consistent with our exciton-photon coupling model. We believe that our work outlines the possibility to implement fully scalable platforms of solid state quantum emitters. The latter is one of the key prerequisites for more advanced, integrated nanophotonic quantum circuits.

quant-ph↗

A charged quantum dot micropillar system for deterministic light matter interactions

Quantum dots (QDs) are semiconductor nanostructures in which a three dimensional potential trap produces an electronic quantum confinement, thus mimicking the behaviour of single atomic dipole-like transitions. However unlike atoms, QDs can be incorporated into solid state photonic devices such as cavities or waveguides that enhance the light-matter interaction. A near unit efficiency light-matter interaction is essential for deterministic, scalable quantum information (QI) devices. In this limit, a single photon input into the device will undergo a large rotation of the polarization of the light field due to the strong interaction with the QD. In this paper we measure a macroscopic ($\sim6^o$) phase shift of light as a result of the interaction with a negatively charged QD coupled to a low quality-factor (Q$\sim290$) pillar microcavity. This unexpectedly large rotation angle demonstrates this simple low Q-factor design would enable near deterministic light-matter interactions.

quant-ph↗

Ghost Branch Photoluminescence From a Polariton Fluid Under Nonresonant Excitation

An expanding polariton condensate is investigated under pulsed nonresonant excitation with a small laser pump spot. Far above the condensation threshold we observe a pronounced increase in the dispersion curvature with a subsequent linearization of the spectrum and strong luminescence from a ghost branch orthogonally polarized with respect to the linearly polarized condensate emission. The presence of the ghost branch has been confirmed in time-resolved measurements. The dissipative and nonequilibrium effects in the photoluminescence of polariton condensates and their excitations are discussed.

cond-mat.mes-hall↗

Quantum dot micropillar cavities with quality factors exceeding 250,000

We report on the spectroscopic investigation of quantum dot - micropillar cavities with unprecedented quality factors. We observe a pronounced dependency of the quality factor on the measurement scheme, and find that significantly larger quality factors can be extracted in photoreflectance compared to photoluminescence measurements. While the photoluminescence spectra of the microcavity resonances feature a Lorentzian lineshape and Q-factors up to 184,000, the reflectance spectra have a Fano-shaped asymmetry and feature significantly higher Q-factors in excess of 250,000 resulting from a full saturation of the embedded emitters. The very high quality factors in our cavities promote strong light-matter coupling with visibilities exceeding 0.5 for a single QD coupled to the cavity mode.

quant-ph↗

Cavity-enhanced simultaneous dressing of quantum dot exciton and biexciton states

We demonstrate the simultaneous dressing of both vacuum-to-exciton and exciton-to-biexciton transitions of a single semiconductor quantum dot in a high-Q micropillar cavity, using photoluminescence spectroscopy. Resonant two-photon excitation of the biexciton is achieved by spectrally tuning the quantum dot emission with respect to the cavity mode. The cavity couples to both transitions and amplifies the Rabi-frequency of the likewise resonant cw laser, driving the transitions. We observe strong-field splitting of the emission lines, which depend on the driving Rabi field amplitude and the cavity-laser detuning. A dressed state theory of a driven 4-level atom correctly predicts the distinct spectral transitions observed in the emission spectrum, and a detailed description of the emission spectra is further provided through a polaron master equation approach which accounts for cavity coupling and acoustic phonon interactions of the semiconductor medium.

quant-ph↗

All-optical flow control of a polariton condensate using non-resonant excitation

The precise adjustment of the polariton condensate flow under incoherent excitation conditions is an indispensable prerequisite for polariton-based logic gate operations. In this report, an all-optical approach for steering the motion of a polariton condensate using only non-resonant excitation is demonstrated. We create arbitrarily shaped functional potentials by means of a spatial light modulator, which allow for tailoring the condensate state and guiding a propagating condensate along reconfigurable pathways. Additional numerical simulations confirm the experimental observations and elucidate the interaction effects between background carriers and polariton condensates.

cond-mat.mes-hall↗

Two-photon interference from a quantum dot--microcavity: Persistent pure-dephasing and suppression of time-jitter

We demonstrate the emission of highly indistinguishable photons from a quasi-resonantly pumped coupled quantum dot--microcavity system operating in the regime of cavity quantum electrodynamics. Changing the sample temperature allows us to vary the quantum dot--cavity detuning, and on spectral resonance we observe a three-fold improvement in the Hong--Ou--Mandel interference visibility, reaching values in excess of 80\%. Our measurements off-resonance allow us to investigate varying Purcell enhancements, and to probe the dephasing environment at different temperatures and energy scales. By comparison with our microscopic model, we are able to identify pure-dephasing and not time-jitter as the dominating source of imperfections in our system.

quant-ph↗

Electrically-driven optical antennas

Unlike radiowave antennas, optical nanoantennas so far cannot be fed by electrical generators. Instead, they are driven by light or via optically active materials in their proximity. Here, we demonstrate direct electrical driving of an optical nanoantenna featuring an atomic-scale feed gap. Upon applying a voltage, quantum tunneling of electrons across the feed gap creates broadband quantum shot noise. Its optical frequency components are efficiently converted into photons by the antenna. We demonstrate that the properties of the emitted photons are fully controlled by the antenna architecture, and that the antenna improves the quantum efficiency by up to two orders of magnitude with respect to a non-resonant reference system. Our work represents a new paradigm for interfacing electrons and photons at the nanometer scale, e.g. for on-chip wireless data communication, electrically driven single- and multiphoton sources, as well as for background-free linear and nonlinear spectroscopy and sensing with nanometer resolution.

physics.optics↗

Temperature-dependent Mollow triplet spectra from a single quantum dot: Rabi frequency renormalisation and sideband linewidth insensitivity

We investigate temperature-dependent resonance fluorescence spectra obtained from a single self-assembled quantum dot. A decrease of the Mollow triplet sideband splitting is observed with increasing temperature, an effect we attribute to a phonon-induced renormalisation of the driven dot Rabi frequency. We also present first evidence for a non-perturbative regime of phonon coupling, in which the expected linear increase in sideband linewidth as a function of temperature is cancelled by the corresponding reduction in Rabi frequency. These results indicate that dephasing in semiconductor quantum dots may be less sensitive to changes in temperature than expected from a standard weak-coupling analysis of phonon effects.

cond-mat.mes-hall↗

Nonlinear spectroscopy of exciton-polaritons in a GaAs-based microcavity

We present a systematic investigation of two-photon excitation processes in a GaAs-based microcavity in the strong-coupling regime. We observe second harmonic generation resonant to the upper and lower polariton level, which exhibits a strong dependence on the photonic fraction of the corresponding polariton. In addition we have performed two-photon excitation spectroscopy to identify $2p$ exciton states which are crucial for the operation as a terahertz lasing device, which was suggested recently [A. V. Kavokin et al., Phys. Rev. Lett. \textbf{108}, 197401 (2012)]. However, no distinct signatures of a $2p$ exciton state could be identified, which indicates a low two-photon pumping efficiency.

cond-mat.mes-hall↗

Creation of orbital angular momentum states with chiral polaritonic lenses

Controlled transfer of orbital angular momentum to exciton-polariton Bose-Einstein condensate spontaneously created under incoherent, off-resonant excitation conditions is a long-standing challenge in the field of microcavity polaritonics. We demonstrate, experimentally and theoretically, a simple and efficient approach to generation of nontrivial orbital angular momentum states by using optically-induced potentials -- chiral polaritonic lenses.

cond-mat.quant-gas↗

Deterministic and Robust Generation of Single Photons On a Chip with 99.5% Indistinguishability Using Rapid Adiabatic Passage

We demonstrate deterministic and robust generation of pulsed resonance fluorescence single photons from a single InGaAs quantum dot using the method of rapid adiabatic passage. Comparative study is performed with transform-limited, negatively chirped and positively chirped pulses, identifying the last one to be the most robust against fluctuation of driving strength. The generated single photons are background free, have a vanishing two-photon emission probability of 0.3% and a raw (corrected) two-photon Hong-Ou-Mandel interference visibility of 97.9% (99.5%), reaching a precision that places single photons at the threshold for fault-tolerant surface-code quantum computing. The single-photon source can be readily scaled up to multi-photon entanglement and used for quantum metrology, boson sampling and linear optical quantum computing.

quant-ph↗

Gallium Arsenide (GaAs) Quantum Photonic Waveguide Circuits

Integrated quantum photonics is a promising approach for future practical and large-scale quantum information processing technologies, with the prospect of on-chip generation, manipulation and measurement of complex quantum states of light. The gallium arsenide (GaAs) material system is a promising technology platform, and has already successfully demonstrated key components including waveguide integrated single-photon sources and integrated single-photon detectors. However, quantum circuits capable of manipulating quantum states of light have so far not been investigated in this material system. Here, we report GaAs photonic circuits for the manipulation of single-photon and two-photon states. Two-photon quantum interference with a visibility of 94.9 +/- 1.3% was observed in GaAs directional couplers. Classical and quantum interference fringes with visibilities of 98.6 +/- 1.3% and 84.4 +/- 1.5% respectively were demonstrated in Mach-Zehnder interferometers exploiting the electro-optic Pockels effect. This work paves the way for a fully integrated quantum technology platform based on the GaAs material system.

quant-ph↗

Influence of interactions with non-condensed particles on the coherence of a 1D polariton condensate

One-dimensional polariton condensates (PoCos) in a photonic wire are generated through non-resonant laser excitation, by which also a reservoir of background carriers is created. Interaction with this reservoir may affect the coherence of the PoCo, which is studied here by injecting a condensate locally and monitoring the coherence along the wire. While the incoherent reservoir is mostly present within the excitation laser spot, the condensate can propagate ballistically through the wire. Photon correlation measurements show that far from the laser spot the second order correlation function approaches unity value, as expected for the coherent condensed state. When approaching the spot, however, the correlation function increases up to values of 1.2 showing the addition of noise to the emission due to interaction with the reservoir. This finding is substantiated by measuring the first order coherence by a double slit experiment, which shows a reduced visibility of interference at the excitation laser spot.

cond-mat.mes-hall↗

Zero Dimensional Polariton Laser in a Sub-Wavelength Grating Based Vertical Microcavity

Semiconductor exciton-polaritons in planar microcavities form coherent two-dimensional condensates in non-equilibrium. However, coupling of multiple lower-dimensional polariton quantum systems, critically needed for polaritonic quantum device applications and novel cavity-lattice physics, has been limited due to the conventional cavity structures. Here we demonstrate full confinement of the polaritons non-destructively using a hybrid cavity made of a single-layer sub-wavelength grating mirror and a distributed Bragg reflector. Single-mode polariton lasing was observed at a chosen polarization. Incorporation of a designable slab mirror into the conventional vertical cavity, when operating in the strong-coupling regime, enables confinement, control and coupling of polariton gasses in a scalable fashion. It may open a door to experimental implementation of polariton-based quantum photonic devices and coupled cavity quantum electrodynamics systems.

cond-mat.quant-gas↗