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Martin Trulsson

Publications and source records attributed to Martin Trulsson.

At least 19 recordsLinked to original sources

Non-Local Particle Flows Become Local When Considering Dissipative Stress

Dense granular and suspension flows under inhomogeneous shear exhibit persistent particle motion in regions where the local yield criterion is subcritical, an apparent breakdown of locality that has motivated the development of a generation of nonlocal rheological models. Using particle-resolved simulations of frictionless dense suspensions in two-dimensional Kolmogorov flow, we show that two independent considerations together account for this signature. First, replacing the conventional shear stress by a shear-rate-weighted dissipative stress $\tau_W=\langle \tau \dot \gamma \rangle/\langle \dot \gamma \rangle$, which isolates the component of stress that performs irreversible work, restores the homogeneous $\mu(J)$ law throughout the bulk of the flow, with the inferred friction remaining strictly above yield. Second, a simple geometric mixing-length construction, applied with conventional stresses and requiring no fluctuation input, accounts for the residual sub-yielding within a sub-diameter layer at flow reversals. Each approach is based on a different philosophy and mechanism, and together they suggest that much of the apparent non-locality in this geometry and frictionless case is an artefact of how stress is measured and averaged rather than an intrinsic breakdown of local rheology.

cond-mat.soft

Mapping the limits of equilibrium in sheared granular liquid crystals

Athermal elongated particles are well-known to follow Jeffery orbits when sheared in viscous fluids. It is less clear if similar orbits appear in dense granular flows. We show that when sheared for long enough, sufficiently elongated frictionless granular rods, rather than following noisy Jeffery-like orbits, exist in a quasi-equilibrium state, whose orientational statistics are quantitatively described by classical liquid crystal theory, where the noise is provided by collisions due to shear. At the same time, we demonstrate a systematic breakdown of this equilibrium analogy at two distinct limits: at low aspect ratios, where the equilibrium theory incorrectly predicts an isotropic state, and as inter-particle friction is introduced, where the system moves from steric screening to frictional gearing. Even within this frictionally geared state, the rotational dynamics remain distinct from classical Jeffery orbits. We link this frictional breakdown directly to the system being driven far from equilibrium, as quantified by an effective Ericksen number that compares non-equilibrium rotational driving to steric ordering. Our results provide a quantitative map of the transition from a quasi-equilibrium to a far-from-equilibrium steady state in a dense, driven system, defining the limits of applicability for thermal liquid crystal theory in athermal matter.

cond-mat.soft

Shear flow of frictional spheroids: Comparison between elongated and flattened particles

The rheology of dense granular shear flows is influenced by friction and particle shape. We investigate numerically the impact of non-spherical particle geometries under shear on packing fraction, stress ratios, velocity fluctuations, force distribution, and dissipation mechanisms, for a wide range of inertial numbers, friction coefficients and aspect ratios. We obtain a regime diagram for the dissipation which shows that lentil-like (oblate) particles exhibit an extended sliding regime compared to rice-like (prolate) particles with the same degree of eccentricity. Additionally, we identify non-monotonic behaviour of slightly aspherical particles at low friction, linking it to their higher fluctuating rotational kinetic energy. We find that angular velocity fluctuations are generally reduced when particles align with the flow, except in highly frictional rolling regimes, where fluctuations collapse onto a power-law distribution and motion becomes less correlated. Moreover, for realistic friction coefficients power dissipation tends to concentrate along the major axis aligned with the flow, where slip events are more frequent. We also show that flat particles develop stronger fabric anisotropy than elongated ones, influencing macroscopic stress transmission. These findings provide new insights into the role of particle shape in granular mechanics, with implications for both industrial and geophysical applications.

cond-mat.soft

Shear jamming transition in alternating shear rotation for frictional and frictionless suspensions

Alternating shear rotations in dense suspensions have recently shown the ability to reduce both viscosity and dissipation per strain (at a fixed global shear rate). Here, we study alternating shear rotation, with extensive numerical simulations, at various angles and up to their corresponding jamming points. For increasing shear rotation angles, we find that the jamming point is continuously shifted to higher packing fractions for frictional particles, while it remains constant for frictionless particles. As a consequence, the alternating shear rotation is unable to reduce the dissipation per strain for suspensions composed of frictionless particles. We detail the individual contributions, hydrodynamic or contact, to the shear stress, being uncharted for this protocol. As the angle of rotation increases, the average contact stress decreases. However, we find that the hydrodynamics shows the opposite trend, instead increasing with increasing angle. Hence, hydrodynamic stress will dominate up to much higher packing fractions as the angle of rotation increases. In addition, we report how the microstructure varies and establish a one-to-one mapping between the contact number and its contribution to the total stress for both frictionless and frictional particles.

cond-mat.soft

Dense Suspensions in Rotary Shear

We introduce a novel unsteady shear protocol, which we name Rotary Shear (RS), where the flow and vorticity directions are continuously rotated around the velocity gradient direction by imposing two out-of-phase oscillatory shear (OS) in orthogonal directions. We perform numerical simulations of dense suspensions of rigid non-Brownian spherical particles at volume fractions ($\phi$) between 0.40 and 0.55 subject to this new RS protocol and compare to the classical OS protocol. We find that the suspension viscosity displays a similar non-monotonic response as the strain amplitude ($\gamma_0$) is increased: a minimum viscosity is found at an intermediate, volume-fraction dependent strain amplitude. However, the suspension dynamics is different in the new protocol. Unlike the OS protocol, suspensions under RS do not show self-adsorbing states at any $\gamma_0$ and do not undergo the reversible-irreversible transition: the stroboscropic particle dynamics are always diffusive, which we attribute to the fact that the RS protocol is irreversible. To validate this hypothesis, we introduce a reversible-RS (RRS) protocol, a combination of RS and OS, where we rotate the shear direction (as in RS) until it is instantaneously reversed (as in OS), and find the resulting rheology and dynamics to be closer to OS. Detailed microstructure analysis shows that both the OS and RRS protocols result in a contact-free, isotropic to an in-contact, anisotropic microstructure at the dynamically reversible-to-irreversible transition. The RS protocol does not render such a transition, and the dynamics remain diffusive with an in-contact, anisotropic microstructure for all strain amplitudes.

cond-mat.soft

Optimum dissipation by cruising in dense suspensions

Dense suspensions tend to shear jam at large packing fractions. However, it has recently been shown that various oscillation protocols can unjam as well as reduce viscosity and dissipation. In this numerical work, we ask ourselves what is the optimum shear protocol in terms of dissipation. We show that many cruising protocols' dissipation are similar to shear protocols with a steady primary shear and superimposed cross oscillations, even though the latter's viscosity reduction is more considerable. Furthermore, we find that alternating between primary and perpendicular oscillations yields a much higher dissipation than the two protocols mentioned above, yet has similar viscosity as the cross-oscillatory one. While self-organization has been shown to minimize viscosity, our findings challenge the idea that random organization is the underlying mechanism for reducing dissipation. Instead, shear ``fragility'' combined with geometry seems to be the key ingredients, which explains the counter-intuitive decoupling of the minima of viscosity and dissipation for the cruising protocol. This work paves the way for a new class of highly-energy efficient flow protocols.

cond-mat.soft

Orientational arrest in dense suspensions of elliptical particles under oscillatory shear flows

We study the rheological response of dense suspensions of elliptical particles, with an aspect ratio equal to 3, under oscillatory shear flows and imposed pressure by numerical simulations. Like for the isotropic particles, we find that the oscillatory shear flows respect the Cox-Merz rule at large oscillatory strains but differ at low strains, with a lower viscosity than the steady shear and higher shear jamming packing fractions. However, unlike the isotropic cases (i.e., discs and spheres), frictionless ellipses get dynamically arrested in their initial orientational configuration at small oscillatory strains. We illustrate this by starting at two different configurations with different nematic order parameters and the average orientation of the particles. Surprisingly, the overall orientation in the frictionless case is uncoupled to the rheological response close to jamming, and the rheology is only controlled by the average number of contacts and the oscillatory strain. Having larger oscillatory strains or adding friction does, however, help the system escape these orientational arrested states, which are evolving to a disordered state independent of the initial configuration at low strains and ordered ones at large strains.

cond-mat.soft

Ion and site correlations of charge regulating surfaces: a simple and accurate theory

Charge regulation is a fundamental mechanism in most chemical, geochemical, and biochemical systems. Various minerals surfaces and proteins are well-known to change their charge state as a function of the activity of the hydronium ions, i.e., the pH. Besides being modulated by the pH, the charge state is sensitive to salt concentration and composition due to screening and ion correlations. Given the importance of electrostatic interactions, a reliable and straightforward theory of charge regulation would be of utmost importance. This paper presents such a theory that accounts for salt screening, site and ion correlations. Our approach shows an impeccable agreement compared to Monte Carlo simulations and experiments of 1:1 and 2:1 salts. We furthermore disentangle the relative importance of site-site, ion-ion and ion-site correlations. Contrary to previous claims, we find that ion-site correlations are subdominant to the two other correlation terms.

cond-mat.soft

Oscillatory shear flows of dense suspensions at imposed pressure: Rheology and micro-structure

Oscillatory shear has been widely used to study the rheological properties of suspensions under unsteady shear. Furthermore, recent works have shown that oscillatory flows can improve the flowability of dense suspensions. While most studies have been done under constant volume we here study oscillatory shear flows of a two-dimensional suspensions using a normal pressure-controlled set-up. To characterise the rheology, we introduce both a complex macroscopic friction coefficient $μ^{*}$, following the convention of the complex viscosity $η^{*}$, and a shear-rate averaged viscous number $J'$. The rheology and microstructure of dense suspensions are studied by systematically varying both the strain magnitude $γ_0$ and $J'$ using numerical simulations. We study both suspensions composed of frictional ($μ_p=0.4$) or frictionless ($μ_p=0$) particles and find that the critical values, as $J' \to 0$, of both the complex macroscopic friction and the number of contacts, both total and sliding, decrease with decreasing $γ_0$. For suspensions composed of frictional particles we also find that the critical (i.e.~the shear jamming) packing fraction $ϕ_c$ increase with decreasing $γ_0$. In both cases, frictional and frictionless, we find that the rheological response approaching the shear jamming turns from a viscous to an elastic response as $γ_0$ is lowered below $\sim0.33$.

cond-mat.soft

Directional shear-jamming

In this work we, study shear reversals of dense non-Brownian suspensions composed of cohesionless elliptical particles. By numerical simulations, we show that a new fragility appears for frictionless ellipses in the flowing states, where particles can flow indefinitely in one direction at applied shear stresses but shear-jams in the other direction upon shear stress reversal. This new fragility, absent in the isotropic particle case, is linked to the directional order of the elongated particles at steady shear and its reorientation at shear stress reversal, which forces the suspensions to pass through a more disordered state with an increased number of contacts in which it might get arrested.

cond-mat.soft

Strong-coupling theory of counterions with hard cores between symmetrically charged walls

By a combination of Monte Carlo simulations and analytical calculations, we investigate the effective interactions between highly charged planar interfaces, neutralized by mobile counterions (salt-free system). While most previous analysis have focused on point-like counterions, we treat them as charged hard spheres. We thus work out the fate of like-charge attraction when steric effects are at work. The analytical approach partitions counterions in two sub-populations, one for each plate, and integrates out one sub-population to derive an effective Hamiltonian for the remaining one. The effective Hamiltonian features plaquette four-particle interactions, and it is worked out by computing a Gibbs-Bogoliubov inequality for the free energy. At the root of the treatment is the fact that under strong electrostatic coupling, the system of charges forms an ordered arrangement, that can be affected by steric interactions. Fluctuations around the reference positions are accounted for. To dominant order at high coupling, it is found that steric effects do not significantly affect the interplate effective pressure, apart at small distances where hard sphere overlap are unavoidable, and thus rule out configurations.

cond-mat.soft

Extended $μ(J)$-rheology for dense suspensions at oscillatory shear flows

Recent studies have highlighted that oscillatory and time-dependent shear flows might help increase flowability of dense suspensions. While most focus has been on cross-flows we here study a simple two-dimensional suspensions where we apply simultaneously oscillatory and stationary shear along the same direction. We first show that the viscosities in this set-up significantly decrease with an increasing magnitude of the oscillations, contrary to previous claims. The decrease can be attributed to the large decrease in the number of contacts and an altered microstructure as the magnitude of the oscillation is increased. As a sub-result we find both an extension to the $μ(J)$-rheology, a constitutive relationship between the shear stresses and the shear rate, valid for pure oscillatory flows and with a higher shear-jammed packing fraction for suspensions composed of frictional particles compared to steady-shear conditions.

cond-mat.soft

Local Rheology Relation with Variable Yield Stress Ratio across Dry, Wet, Dense, and Dilute Granular Flows

Dry, wet, dense, and dilute granular flows have been previously considered fundamentally different and thus described by distinct, and in many cases incompatible, rheologies. We carry out extensive simulations of granular flows, including wet and dry conditions, various geometries and driving mechanisms (boundary driven, fluid driven, and gravity driven), many of which are not captured by standard rheology models. For all simulated conditions, except for fluid-driven and gravity-driven flows close to the flow threshold, we find that the Mohr-Coulomb friction coefficient $μ$ scales with the square root of the local Péclet number $\mathrm{Pe}$ provided that the particle diameter exceeds the particle mean free path. With decreasing $\mathrm{Pe}$ and granular temperature gradient $M$, this general scaling breaks down, leading to a yield condition with a variable yield stress ratio characterized by $M$.

cond-mat.soft

Discontinuous shear thickening of dense suspensions under confining pressure

We use 2D numerical simulations to study dense suspensions of non-Brownian hard particles using the Critical Load Model (CLM) under constant confining pressures. This simple model shows discontinuous shear thickening (DST) as the tangential forces get activated upon increased shear stresses. By parameterizing a simple binary system of frictional and non-frictional particles of different proportions we show that the jamming packing fraction, at which the viscosity diverges, is controlled by the fraction of frictional contacts. The viscosity of dense suspensions can thereby be expressed as a function of the fraction of frictional contacts as well as the packing fraction of solid particles. In addition, we show that there exists a simple relationship between the fraction of frictional contacts and the two control parameters (under confining pressure): the viscous number J and the ratio between the repulsive barrier force and confining pressure. Under confining pressures the viscosity curves are found to depend on the shear protocol, with the possibility of yielding negative dynamic compressibility.

cond-mat.soft

Non-local rheology in dense granular flows -- Revisiting the concept of fluidity

The aim of this article is to discuss the concepts of non-local rheology and fluidity, recently introduced to describe dense granular flows. We review and compare various approaches based on different constitutive relations and choices for the fluidity parameter, focusing on the kinetic elasto-plastic model introduced by Bocquet et al. [Phys. Rev. Lett 103, 036001 (2009)] for soft matter, and adapted for granular matter by Kamrin et al. [Phys. Rev. Lett. 108, 178301 (2012)], and the gradient expansion of the local rheology $μ(I)$ that we have proposed [Phys. Rev. Lett. 111, 238301 (2013)]. We emphasise that, to discriminate between these approaches, one has to go beyond the predictions derived from linearisation around a uniform stress profile, such as that obtained in a simple shear cell. We argue that future tests can be based on the nature of the chosen fluidity parameter, and the related boundary conditions, as well as the hypothesis made to derive the models and the dynamical mechanisms underlying their dynamics.

cond-mat.soft

Microrheology to probe non-local effects in dense granular flows

A granular material is observed to flow under the Coulomb yield criterion as soon as this criterion is satisfied in a remote but contiguous region of space. We investigate this non-local effect using discrete element simulations, in a geometry similar, in spirit, to the experiment of Reddy et al. (Phys. Rev. Lett., 106 (2011) 108301): a micro-rheometer is introduced to determine the influence of a distant shear band on the local rheological behaviour. The numerical simulations recover the dominant features of this experiment: the local shear rate is proportional to that in the shear band and decreases (roughly) exponentially with the distance to the yield conditions. The numerical results are in quantitative agreement with the predictions of the non-local rheology proposed by (Phys. Rev. Lett., 111 (2013) 238301) and derived from a gradient expansion of the rheology $μ[I]$. The consequences of these findings for the dynamical mechanisms controlling non-locality are finally discussed.

cond-mat.soft

A new dipolar potential for numerical simulations of polar fluids on the $4\mathrm{D}$ hypersphere

We present a new method for Monte Carlo or Molecular Dynamics numerical simulations of three dimensional polar fluids. The simulation cell is defined to be the surface of the northern hemisphere of a four-dimensional (hyper)sphere. The point dipoles are constrained to remain tangent to the sphere and their interactions are derived from the basic laws of electrostatics in this geometry. The dipole-dipole potential has two singularities which correspond to the following boundary conditions : when a dipole leaves the northern hemisphere at some point of the equator, it reappears at the antipodal point bearing the same dipole moment. We derive all the formal expressions needed to obtain the thermodynamic and structural properties of a polar liquid at thermal equilibrium in actual numerical simulation. We notably establish the expression of the static dielectric constant of the fluid as well as the behavior of the pair correlation at large distances. We report and discuss the results of extensive numerical Monte Carlo simulations for two reference states of a fluid of dipolar hard spheres and compare these results with previous methods with a special emphasis on finite size effects.

cond-mat.soft

A non-local rheology for granular flows across yield conditions

The rheology of dense granular flows is studied numerically in a shear cell controlled at constant pressure and shear stress, confined between two granular shear flows. We show that a liquid state can be achieved even far below the yield stress, whose flow can be described with the same rheology as above the yield stress. A non-local constitutive relation is derived from dimensional analysis through a gradient expansion and calibrated using the spatial relaxation of velocity profiles observed under homogeneous stresses. Both for frictional and frictionless grains, the relaxation length is found to diverge as the inverse square-root of the distance to the yield point, on both sides of that point.

cond-mat.soft