SearcharxivSearch

arXiv subjects

Martine Hennion

Publications and source records attributed to Martine Hennion.

2 recordsLinked to original sources

From chessboard of bipolarons of size 4a in cubic La7/8Sr1/8MnO3 to stripes of the same bipolarons in layered high Tc cuprates

The compound La1-xSrxMnO3 exhibits a charge order (CO) state at $x\approx 1/8$ and $T T_{co}$ which become ordered on a chessboard organized in a 3D-order state of ferromagnetically paired polarons at $T<T_{co}$. Applied to the CuO$_2$ planes of the cuprates of the "214" family, this model produces stripes of bipolarons intertwined with stripes of antiferromagnetically arranged spins, hole-poor, both of size $4a$, leading to a spin density wave with a wave vector $δ=1/8$, a charge density wave with $q=1/4$, the Yamada laws $δ(x)=x$ and $T_c\propto δ$ and a decrease of $T_c$ at x=1/8. This work invokes relevance of a bipolaronic origin of high $T_c$ superconductivity, in which bipolarons of size $4a$ can play a major role.

cond-mat.supr-con

Interacting chains of orbital polarons in "Colossal" magnetoresistive La1-xSrxMnO3 revealed by spin and lattice dynamics

The origin of the effect of colossal magneto-resistance (CMR) remains still unexplained. In this work we revisit the spin dynamics of the pseudo-cubic La1-xSrxMnO3 along the Mn-O-Mn bond direction at four x doping values (x < 0.5) and various temperatures and report a new lattice dynamics study at x0=0.2, representative of the optimal doping for CMR. We propose an interpretation of the spin dynamics in terms of orbital polarons. This picture is supported by the observation of a discrete magnetic energy spectrum Enmag (q) characteristic of the internal excitations of "orbital polarons" defined by Mn3+ neighbors surrounding a Mn4+ center with a hole. Because of its hopping, the hole mixes up dynamically all the possible orbital configurations of its surrounding Mn3+ sites with degenerate energies. The Enmag values indicate a lift of orbital degeneracy by phonon excitations. The number n varies with the spatial dimension D of the polaron and the q-range determines its size. At x=0.125 and x=0.3 the spectrum reveals 2D polarons coupled by exchange and 3D "free" polarons respectively, with sizes l=1.67a < 2a in all bond directions. At x0=0.2, the spin and the lattice dynamics provide evidence for chains of orbital polarons of size l=2a with a periodic distribution over ~ 3a and an interaction energy ~ 3 meV. At T < Tc the charges propagate together with the longitudinal acoustic phonons along the chains enhancing their ferromagnetic character. The phase separation between metallic and ferromagnetic chains in a non-metallic matrix may be crucial for CMR.

cond-mat.str-el