arXiv subjects

Masahiro Ohkuma

Publications and source records attributed to Masahiro Ohkuma.

7 recordsLinked to original sources

arXiv2026

Diamond quantum-sensing platform with integrated boron-doped diamond microwave antenna and thermometer

Wide-field nitrogen-vacancy (NV) magnetic imaging at cryogenic temperatures requires microwave excitation and reliable knowledge of the temperature near the sensing region. Here, we report an integrated diamond quantum-sensing platform combining an ensemble of NV centers with a boron-doped diamond (BDD) microwave antenna and thermometer formed on the same diamond substrate. The BDD antenna provides microwave excitation for optically detected magnetic resonance measurements, and the BDD thermometer monitors the thermal environment near the NV sensing region. The BDD thermometer detected laser-induced local heating that was not clearly resolved by a stage-mounted thermometer. Using this platform, we imaged the temperature-dependent Meissner response of multiple cuprate superconductors while recording the temperature. These results demonstrate that the integrated BDD--NV platform provides a practical approach for cryogenic wide-field magnetic imaging with integrated microwave delivery and local thermometry.

physics.app-ph↗

arXiv2026

Wide-field NV magnetometry under simultaneous high-pressure and high-temperature conditions

We demonstrate wide-field optically detected magnetic resonance (ODMR) under simultaneous high-pressure and high-temperature conditions using nitrogen-vacancy (NV) centers. Although NV-center magnetometry has been widely used for spatially resolved magnetic-field imaging, its application to extreme environments combining pressure and temperature remains challenging. In this work, we show that ODMR can be observed at 5 GPa and 500 K, demonstrating the feasibility of NV spin readout under such combined extreme conditions. We further perform wide-field ODMR of iron at 7 GPa and 500 K, where the stray magnetic field from the sample is spatially visualized through the pressure cell. These results establish NV-center magnetometry as a promising platform for imaging magnetic phenomena in materials under high-pressure and high-temperature environments.

physics.app-ph↗

arXiv2026

Probing the Meissner effect in single crystals of $\mathbf{Bi_2Sr_2Ca_2Cu_3O_{10+δ}}$ via wide-field quantum microscopy under high pressure

We investigated the pressure dependence of the superconducting transition temperature ($T_{\rm c}$) in optimally doped Bi$_2$Sr$_2$Ca$_2$Cu$_3$O$_{10+δ}$ (Bi-2223) single crystals using different pressure-transmitting media. Previous high-pressure studies have reported conflicting behaviors, ranging from a resurgence of $T_{\rm c}$ of optimally doped Bi-2223 in fluid media to an insulating-like transition in solid media. However, a direct comparison of the effects of different pressure-transmitting media is lacking. Here, we employed wide-field quantum microscopy based on nitrogen-vacancy centers to probe the magnetic response under high pressure, utilizing cBN and KBr as media. We observed that a diamagnetic response near 70 K, indicative of the superconducting transition, persisted up to 23 GPa in KBr, whereas it disappeared above 11 GPa and 70 K in cBN. These results demonstrate the high sensitivity of Bi-2223 to the pressure environment and highlight the critical role of hydrostatic pressure in cuprate superconductors.

cond-mat.supr-con↗

arXiv2026

Optically detected magnetic resonance of nitrogen-vacancy centers in microdiamonds inside nanopolycrystalline diamond anvil cell

We demonstrated optically detected magnetic resonance (ODMR) of nitrogen-vacancy (NV) centers in microdiamonds inside a diamond anvil cell pressurized with nanopolycrystalline diamond (NPD) anvils. NPD exhibits high optical transparency, superior hardness, and low thermal conductivity, making it suitable for optical and spectroscopic measurements under high-pressure and high-temperature conditions. We observed the ODMR signal from an ensemble of NV centers under conditions where NV centers in microdiamonds served as markers for pressures exceeding 30 GPa, with a culet diameter of 600 $μ$m. We also performed ODMR measurements on multiple microdiamonds sealed inside a sample chamber and found that the resonance frequency varied with the pressure distribution. The combination of NPD and microdiamonds containing NV centers is auspicious for pressure and magnetic sensing under concurrent high-pressure and high-temperature conditions.

cond-mat.mtrl-sci↗

arXiv2025

Coherent control of solid-state defect spins via patterned boron-doped diamond circuit

Monolithic integration, which refers to the incorporation of all device functionalities within a single material, shows significant potential for creating scalable solid-state quantum devices. This study demonstrated the coherent control of nitrogen-vacancy (NV) spins using an electronic circuit monolithically integrated within diamond: a patterned, conductive boron-doped diamond (BDD) microwave waveguide. First, we validated the high-frequency performance of the circuit by characterizing its impedance up to the microwave range, confirming its capability for efficient microwave transmission. Then, using this monolithically integrated BDD--NV hybrid system, we performed optically detected magnetic resonance and observed noticeable Rabi oscillations driven by the metallic BDD circuit. Importantly, we verified that the BDD antenna has a minimal detrimental impact on the NV spins; microwave-induced heating is negligible under both pulsed and continuous driving, and the spin relaxation time ($T_1$) remains unperturbed. This approach paves the way for a new class of compact, robust, and versatile quantum platforms suitable for sensing and information processing in various environments.

physics.app-ph↗

arXiv2025

Enhancement of superconductivity on thin film of Sn under high pressure

We investigated the pressure effects of a superconductivity on thin films of Sn. Elemental superconductor Sn with a body-centered tetragonal structure, $β$-Sn, exhibits superconductivity below the superconducting transition temperature ($T_{\rm c}=3.72$ K) at ambient pressure. $T_{\rm c}$ of Sn increases with lowering dimension such as in thin film and nanowire growth, or by high-pressure application. For thin films, $T_{\rm c}$ exhibits a slight increase up to approximately 4 K compared to the bulk value, attributable to the crystalline size and lattice disorder. By applying pressure on a bulk Sn, $T_{\rm c}$ initially decreases from 3.72 K as the pressure increases. Further increasing pressure up to 10 GPa, $T_{\rm c}$ increases to 5.3 K with the structural transformation. However, the combination of these effects on thin films of Sn, namely, thin-film growth and pressure effects, remains underexplored. In this study, we combined film-growth and pressure-application techniques to further increase $T_{\rm c}$ using a diamond anvil cell with boron-doped diamond electrodes. The drop of the electrical resistance suggesting the onset of $T_{\rm c}$ on the thin film reached above 6 K in $γ$-Sn phase. Further, the upper critical magnetic field was drastically enhanced. Atomic force microscopy suggests that the refinement of the grain size of the thin film under the non-hydrostatic pressure conditions contributes to stabilizing the higher $T_{\rm c}$ of $γ$-Sn.

cond-mat.supr-con↗

arXiv2024

Pressure-induced anomalous enhancement in superconducting critical temperature of transition-metal chalcogenide Ta$_2$PdS$_6$ and Ta$_2$PdSe$_6$

The emergence of a second dome in the superconducting phase through pressure-driven manipulation of crystal structures in materials has attracted considerable attention. Transition metal chalcogenides (TMCs) represent a highly promising platform, as the second dome has been observed in several binary compounds. Recently, ternary TMCs such as Ta$_2$PdS$_6$ and Ta$_2$PdSe$_6$ have exhibited pressure-induced superconducting domes. In this study, we perform electrical transport measurements of Ta$_2$PdS$_6$ and Ta$_2$PdSe$_6$ under extremely high pressures exceeding 100 GPa, namely uninvestigated regions in previous reports, to reveal the emergence of the second dome. The superconducting critical temperatures (T$_c$) in both Ta$_2$PdS$_6$ and Ta$_2$PdSe$_6$ initially decrease with increasing pressure. Subsequently, the Tcs tend to enhance drastically above 100 GPa. Notably, the maximum T$_c$ in Ta$_2$PdS$_6$ is 11.2 K at 130.0 GPa, which is a relatively high record among the TMCs. The emergence of the second dome in Ta$_2$PdS$_6$ and Ta$_2$PdSe$_6$ opens further motivation for the investigation under extreme conditions beyond the first dome to find hidden ordered phases.

cond-mat.supr-con↗