arXiv subjects

Masahiro Sato

Publications and source records attributed to Masahiro Sato.

At least 37 records · Page 2Linked to original sources

arXiv2024

Electric-field control of magnetic anisotropies: applications to Kitaev spin liquids and topological spin textures

Magnetic anisotropies often originate from the spin-orbit coupling and determine magnetic ordering patterns. We develop a microscopic theory for DC electric-field controls of magnetic anisotropies in magnetic Mott insulators and discuss its applications to Kitaev materials and topological spin textures. Throughout this paper, we take a microscopic approach based on Hubbard-like lattice models, tight-binding models with on-site interactions. We derive a low-energy spin Hamiltonian from a fourth-order perturbation expansion of the Hubbard-like model. We show in the presence of a strong intra-atomic spin-orbit coupling that DC electric fields add non-Kitaev interactions such as a Dzyaloshinskii-Moriya interaction and an off-diagonal $Γ'$ interaction to the Kitaev-Heisenberg model and can induce a topological quantum phase transition between Majorana Chern insulating phases. We also investigate the inter-atomic Rashba spin-orbit coupling and its effects on topological spin textures. DC electric fields turn out to create and annihilate magnetic skyrmions, hedgehogs, and chiral solitons. We propose several methods of creating topological spin textures with external electromagnetic fields. Our theory clarifies that the strong but feasible electric field can control Kitaev spin liquids and topological spin textures.

cond-mat.str-el↗

arXiv2024

Microscopic theory of spin Seebeck effect in antiferromagnets

We develop a microscopic theory for the spin Seebeck effect (SSE) in Néel and canted phases of antiferromagnetic insulators. We calculate the DC spin current tunneling from the antiferromagnet to an attached metal, incorporating the spin-wave theory and the non-equilibrium Green's function approach. Our result shows a sign change of the spin current at the spin-flop phase transition between Néel and canted phases, which is in agreement with a recent experiment for the SSE of $\rm Cr_2O_3$ in a semi-quantitative level. The sign change can be interpreted from the argument based on the density of states of up- and down-spin magnons, which is related to the polarized-neutron scattering spectra. The theory also demonstrates that the spin current in the Néel phase is governed by the magnon correlation, while that in the canted phase consists of two parts: Contributions from not only the magnon dynamics but also the static transverse magnetization. This result leads to a prediction that at sufficiently low temperatures, the spin current non-monotonically changes as a function of magnetic field in the canted phase. Towards a more unified understanding of the SSE in antiferromagnets, we further discuss some missing links of theories of SSE: Interface properties, effects of the transverse spin moment in the canted phase, the spin-orbit coupling in the metal, etc. Finally, we compare the SSE of antiferromagnets with those of different magnetic phases such as ferromagnets, ferrimagnets, an one-dimensional spin liquid, a spin-nematic liquid, and a spin-Peierls (dimerized) phase.

cond-mat.str-el↗

arXiv2023

Peltier effect of phonon driven by ac electromagnetic waves

Steady current in metals induces a thermal gradient, a phenomenon known as the Peltier effect. The Peltier effect is one of the fundamental phenomena in the thermoelectric properties of materials and is also used in applications such as refrigerators. In this work, we show that an analogous phenomenon occurs by phonons in a material subject to linearly-polarized light. Under light illumination, an energy current of phonons occurs through a nonlinear optical effect similar to the bulk photovoltaic effect. We formulate the nonlinear Peltier coefficient of the photogalvanic energy current carried by phonons using nonlinear response theory. From the general formula, we show that the photogalvanic energy current occurs only in a non-centrosymmetric system with two or more optical phonon bands. We demonstrate the generation of the photogalvanic energy current using a one-dimensional ion chain with three ions in a unit cell, which predicts the generation of an experimentally observable energy current using available THz-infrared light sources.

cond-mat.mes-hall↗

arXiv2023

Imprinting spiral Higgs waves onto superconductors with vortex beams

A vortex beam, akin to a quantized vortex in superfluids, possesses inherent orbital angular momentum (OAM), resulting in the propagation of a spiral-shaped wavefront. Here we demonstrate that a pulsed vortex beam with OAM in the terahertz frequency band can induce a spiral Higgs wave, which is a spiral-shaped oscillation mode of the superconducting order parameter. By utilizing the gauge-invariant theory for the superconducting order, we demonstrate that the phase mode is driven to screen the longitudinal magnetic field of the vortex beam, which facilitates the imprinting of the spiral-shaped wavefront and the transfer of OAM to the condensate. Furthermore, we find that increasing the OAM of light amplifies the intensity of the third harmonic generation. These findings highlight the potential of terahertz vortex beams as a spectroscopic probe of collective modes.

cond-mat.supr-con↗

arXiv2023

Generation of third-harmonic spin oscillation from strong spin precession induced by terahertz magnetic near fields

The ability to drive a spin system to state far from the equilibrium is indispensable for investigating spin structures of antiferromagnets and their functional nonlinearities for spintronics. While optical methods have been considered for spin excitation, terahertz (THz) pulses appear to be a more convenient means of direct spin excitation without requiring coupling between spins and orbitals or phonons. However, room-temperature responses are usually limited to small deviations from the equilibrium state because of the relatively weak THz magnetic fields in common approaches. Here, we studied the magnetization dynamics in a HoFeO3 crystal at room temperature. A custom-made spiral-shaped microstructure was used to locally generate a strong multicycle THz magnetic near field perpendicular to the crystal surface; the maximum magnetic field amplitude of about 2 T was achieved. The observed time-resolved change in the Faraday ellipticity clearly showed second- and third-order harmonics of the magnetization oscillation and an asymmetric oscillation behaviour. Not only the ferromagnetic vector M but also the antiferromagnetic vector L plays an important role in the nonlinear dynamics of spin systems far from equilibrium.

physics.optics↗

arXiv2021

Large photogalvanic spin current by magnetic resonance in bilayer Cr trihalides

Magnetic materials show rich optical responses related to the magnetic order. These phenomena reflect the nature of their excitations, providing a powerful probe for the magnetic states and a way to control them. In recent years, such studies were extended to the optical control of spin current using nonlinear optical response similar to the photogalvanic effect. However, neither a candidate material nor a general formula for calculating the photogalvanic spin current is known so far. In this work, we develop a general theory for the photogalvanic spin current through a magnetic resonance process. Using the nonlinear response formalism, we find the nonlinear conductivity consists of two contributions that involve one and two magnon bands; the latter is a contribution unknown to date. We argue that the two-band process produces a large photogalvanic spin current in the antiferromagnetic phase of bilayer CrI$_3$ and CrBr$_3$, whose resonance frequency can be tuned between GHz-THz range by an external magnetic field. Our findings open a route to the studies on the photogalvanic effect of spin angular momentum in realistic setups.

cond-mat.mes-hall↗

arXiv2021

Nonequilibrium steady states in the Floquet-Lindblad systems: van Vleck's high-frequency expansion approach

Nonequilibrium steady states (NESSs) in periodically driven dissipative quantum systems are vital in Floquet engineering. We develop a general theory for high-frequency drives with Lindblad-type dissipation to characterize and analyze NESSs based on the high-frequency (HF) expansion with linear algebraic numerics and without numerically solving the time evolution. This theory shows that NESSs can deviate from the Floquet-Gibbs state depending on the dissipation type. We show the validity and usefulness of the HF-expansion approach in concrete models for a diamond nitrogen-vacancy (NV) center, a kicked open XY spin chain with topological phase transition under boundary dissipation, and the Heisenberg spin chain in a circularly-polarized magnetic field under bulk dissipation. In particular, for the isotropic Heisenberg chain, we propose the dissipation-assisted terahertz (THz) inverse Faraday effect in quantum magnets. Our theoretical framework applies to various time-periodic Lindblad equations that are currently under active research.

cond-mat.mes-hall↗

arXiv2021

Quantized edge magnetizations and their symmetry protection in one-dimensional quantum spin systems

The bulk electric polarization works as a nonlocal order parameter that characterizes topological quantum matters. Motivated by a recent paper [H. Watanabe \textit{et al.}, Phys. Rev. B {\bf 103}, 134430 (2021)], we discuss magnetic analogs of the bulk polarization in one-dimensional quantum spin systems, that is, quantized magnetizations on the edges of one-dimensional quantum spin systems.The edge magnetization shares the topological origin with the fractional edge state of the topological odd-spin Haldane phases. Despite this topological origin, the edge magnetization can also appear in topologically trivial quantum phases. We develop straightforward field theoretical arguments that explain the characteristic properties of the edge magnetization. The field theory shows that a U(1) spin-rotation symmetry and a site-centered or bond-centered inversion symmetry protect the quantization of the edge magnetization. We proceed to discussions that quantum phases on nonzero magnetization plateaus can also have the quantized edge magnetization that deviates from the magnetization density in bulk. We demonstrate that the quantized edge magnetization distinguishes two quantum phases on a magnetization plateau separated by a quantum critical point. The edge magnetization exhibits an abrupt stepwise change from zero to $1/2$ at the quantum critical point because the quantum phase transition occurs in the presence of the symmetries protecting the quantization of the edge magnetization. We also show that the quantized edge magnetization can result from the spontaneous ferrimagnetic order.

cond-mat.str-el↗

arXiv2021

Triplon current generation in solids

A triplon refers to a fictitious particle that carries angular momentum $S = 1$ corresponding to the elementary excitation in a broad class of quantum dimerized spin systems. Such systems without magnetic order have long been studied as a testing ground for quantum properties of spins. Although triplons have been found to play a central role in thermal and magnetic properties in dimerized magnets with singlet correlation, a spin angular momentum flow carried by triplons, a triplon current, has not been detected yet. Here we report spin Seebeck effects induced by a triplon current: triplon spin Seebeck effect, using a spin-Peierls system CuGeO$_3$. The result shows that the heating-driven triplon transport induces spin current whose sign is positive, opposite to the spin-wave cases in magnets. The triplon spin Seebeck effect persists far below the spin-Peierls transition temperature, being consistent with a theoretical calculation for triplon spin Seebeck effects.

cond-mat.mtrl-sci↗

arXiv2021

Linear and Nonlinear Optical Responses in Kitaev Spin Liquids

We theoretically study THz-light-driven high-harmonic generation (HHG) in the spin-liquid states of the Kitaev honeycomb model with a magnetostriction coupling between spin and electric polarization. To compute the HHG spectra, we numerically solve the Lindblad equation, taking account of the dissipation effect. We find that isotropic Kitaev models possess a dynamical symmetry, which is broken by a static electric field, analogous to HHG in electron systems. We show that the HHG spectra exhibit characteristic continua of Majorana fermion excitations, and their broad peaks can be controlled by applying static electric or magnetic fields. In particular, the magnetic-field dependence of the HHG spectra drastically differs from those of usual ordered magnets. These results indicate that an intense THz laser provides a powerful tool to observe dynamic features of quantum spin liquids.

cond-mat.str-el↗

arXiv2021

Approximation Theory Based Methods for RKHS Bandits

The RKHS bandit problem (also called kernelized multi-armed bandit problem) is an online optimization problem of non-linear functions with noisy feedback. Although the problem has been extensively studied, there are unsatisfactory results for some problems compared to the well-studied linear bandit case. Specifically, there is no general algorithm for the adversarial RKHS bandit problem. In addition, high computational complexity of existing algorithms hinders practical application. We address these issues by considering a novel amalgamation of approximation theory and the misspecified linear bandit problem. Using an approximation method, we propose efficient algorithms for the stochastic RKHS bandit problem and the first general algorithm for the adversarial RKHS bandit problem. Furthermore, we empirically show that one of our proposed methods has comparable cumulative regret to IGP-UCB and its running time is much shorter.

cs.LG↗

arXiv2021

Control of superexchange interactions with DC electric fields

We discuss DC electric-field controls of superexchange interactions. We first present generic results about antiferromagnetic and ferromagnetic superexchange interactions valid in a broad class of Mott insulators, where we also estimate typical field strength to observe DC electric-field effects: $\sim 1~\mathrm{MV/cm}$ for inorganic Mott insulators such as transition-metal oxides and $\sim 0.1~\mathrm{MV/cm}$ for organic ones. Next, we apply these results to geometrically frustrated quantum spin systems. Our theory widely applies to (quasi-)two-dimensional and thin-film systems and one-dimensional quantum spin systems on various lattices such as square, honeycomb, triangular, and kagome ones. In this paper, we give our attention to those on the square lattice and on the chain. For the square lattice, we show that DC electric fields can control a ratio of the nearest-neighbor and next-nearest-neighbor exchange interactions. In some realistic cases, DC electric fields make the two next-nearest-neighbor interactions nonequivalent and eventually turns the square-lattice quantum spin system into a deformed triangular-lattice one. For the chain, DC electric fields can induce singlet-dimer and Haldane-dimer orders. We show that the DC electric-field-induced spin gap $\propto |\boldsymbol E|^{2/3}$ in the Heisenberg antiferromagnetic chain will reach $\sim 10~\%$ of the dominant superexchange interaction in the case of a spin-chain compound $\mathrm{KCuMoO_4(OH)}$ when the DC electric field of $\sim 1~\mathrm{MV/cm}$ is applied.

cond-mat.str-el↗

arXiv2021

Online Evaluation Methods for the Causal Effect of Recommendations

Evaluating the causal effect of recommendations is an important objective because the causal effect on user interactions can directly leads to an increase in sales and user engagement. To select an optimal recommendation model, it is common to conduct A/B testing to compare model performance. However, A/B testing of causal effects requires a large number of users, making such experiments costly and risky. We therefore propose the first interleaving methods that can efficiently compare recommendation models in terms of causal effects. In contrast to conventional interleaving methods, we measure the outcomes of both items on an interleaved list and items not on the interleaved list, since the causal effect is the difference between outcomes with and without recommendations. To ensure that the evaluations are unbiased, we either select items with equal probability or weight the outcomes using inverse propensity scores. We then verify the unbiasedness and efficiency of online evaluation methods through simulated online experiments. The results indicate that our proposed methods are unbiased and that they have superior efficiency to A/B testing.

cs.LG↗

arXiv2021

Submodular Bandit Problem Under Multiple Constraints

The linear submodular bandit problem was proposed to simultaneously address diversified retrieval and online learning in a recommender system. If there is no uncertainty, this problem is equivalent to a submodular maximization problem under a cardinality constraint. However, in some situations, recommendation lists should satisfy additional constraints such as budget constraints, other than a cardinality constraint. Thus, motivated by diversified retrieval considering budget constraints, we introduce a submodular bandit problem under the intersection of $l$ knapsacks and a $k$-system constraint. Here $k$-system constraints form a very general class of constraints including cardinality constraints and the intersection of $k$ matroid constraints. To solve this problem, we propose a non-greedy algorithm that adaptively focuses on a standard or modified upper-confidence bound. We provide a high-probability upper bound of an approximation regret, where the approximation ratio matches that of a fast offline algorithm. Moreover, we perform experiments under various combinations of constraints using a synthetic and two real-world datasets and demonstrate that our proposed methods outperform the existing baselines.

cs.LG↗

arXiv2021

Causality-Aware Neighborhood Methods for Recommender Systems

The business objectives of recommenders, such as increasing sales, are aligned with the causal effect of recommendations. Previous recommenders targeting for the causal effect employ the inverse propensity scoring (IPS) in causal inference. However, IPS is prone to suffer from high variance. The matching estimator is another representative method in causal inference field. It does not use propensity and hence free from the above variance problem. In this work, we unify traditional neighborhood recommendation methods with the matching estimator, and develop robust ranking methods for the causal effect of recommendations. Our experiments demonstrate that the proposed methods outperform various baselines in ranking metrics for the causal effect. The results suggest that the proposed methods can achieve more sales and user engagement than previous recommenders.

cs.IR↗

arXiv2020

An Intuitionistic Set-theoretical Model of Fully Dependent CCω

Werner's set-theoretical model is one of the simplest models of CIC. It combines a functional view of predicative universes with a collapsed view of the impredicative sort Prop. However this model of Prop is so coarse that the principle of excluded middle holds. Following our previous work, we interpret Prop into a topological space (a special case of Heyting algebra) to make the model more intuitionistic without sacrificing simplicity. We improve on that work by providing a full interpretation of dependent product types, using Alexandroff spaces. We also extend our approach to inductive types by adding support for lists.

cs.LO↗

arXiv2020

Spin-current version of solar cells in non-centrosymmetric magnetic insulators

Photovoltaic effect, e.g., solar cells, converts light into DC electric current. This phenomenon takes place in various setups such as in noncentrosymmetric crystals and semiconductor pn junctions. Recently, we proposed a theory for producing DC spin current in magnets using electromagnetic waves, i.e., the spin-current counterpart of the solar cells. Our calculation shows that the nonlinear conductivity for the spin current is nonzero in a variety of noncentrosymmetric magnets, implying that the phenomenon is ubiquitous in inversion-asymmetric materials with magnetic excitations. Intuitively, this phenomenon is a bulk photovoltaic effect of magnetic excitations, where electrons and holes, visible light, and inversion-asymmetric semiconductors are replaced with magnons or spinons, THz or GHz waves, and asymmetric magnetic insulators, respectively. We also show that the photon-driven spin current is shift current type, and as a result, the current is stable against impurity scattering. This bulk photovoltaic spin current is in sharp contrast to that of well-known spin pumping that takes place at the interface between a magnet and a metal.

cond-mat.str-el↗

arXiv2020

Unbiased Learning for the Causal Effect of Recommendation

Increasing users' positive interactions, such as purchases or clicks, is an important objective of recommender systems. Recommenders typically aim to select items that users will interact with. If the recommended items are purchased, an increase in sales is expected. However, the items could have been purchased even without recommendation. Thus, we want to recommend items that results in purchases caused by recommendation. This can be formulated as a ranking problem in terms of the causal effect. Despite its importance, this problem has not been well explored in the related research. It is challenging because the ground truth of causal effect is unobservable, and estimating the causal effect is prone to the bias arising from currently deployed recommenders. This paper proposes an unbiased learning framework for the causal effect of recommendation. Based on the inverse propensity scoring technique, the proposed framework first constructs unbiased estimators for ranking metrics. Then, it conducts empirical risk minimization on the estimators with propensity capping, which reduces variance under finite training samples. Based on the framework, we develop an unbiased learning method for the causal effect extension of a ranking metric. We theoretically analyze the unbiasedness of the proposed method and empirically demonstrate that the proposed method outperforms other biased learning methods in various settings.

cs.LG↗