arXiv subjects

Masamitsu Hayashi

Publications and source records attributed to Masamitsu Hayashi.

At least 19 recordsLinked to original sources

arXiv2026

Phase control of magnon-phonon coupling via magnetic field

We study the phase of the coupling between magnons and surface acoustic wave (SAW) phonons in magnetic thin films. The coupling constant changes from a real to a complex number as the external magnetic field is reduced. Below a transition field, the imaginary coupling constant allows SAW phonons to couple to overdamped magnons whose resonance frequency is close to zero and far from the SAW resonance. The strength of the imaginary coupling constant and the magnitude of the transition field both scale with magnetic damping. We find the coupling produces a broad, pronounced minimum in the SAW transmittance spectrum near zero magnetic field in a Ni/Ru/Ni synthetic antiferromagnet with large magnetic damping. These results demonstrate that the phase of the complex magnon-phonon coupling constant can be tuned via magnetic field in strongly damped magnets, offering a platform to explore novel regimes of magnon-phonon interactions.

cond-mat.mes-hall↗

arXiv2026

Tellurium Metasurface Beam Splitter with Pulse Laser-Controlled Anisotropy

Laser-programmable optical anisotropy offers a new route to developing reconfigurable metasurfaces without conventional nanofabrication processes. Here, we demonstrate a lithography-free approach based on spatial control of the crystallographic $c$ axis orientation in tellurium (Te) using pulse laser irradiation. As a proof of concept, we demonstrate a Te metasurface beam splitter by laser-written optical-axis patterning and experimentally confirm that its optical response is in good agreement with theoretical predictions and numerical simulations. By directly programming the local optical anisotropy, this method enables a simple fabrication process while offering the possibility of rewriting and dynamically reconfiguring device functionality. These features make this approach a promising platform for non-resonant active metasurfaces and other reconfigurable flat-optics applications.

cond-mat.mes-hall↗

arXiv2026

Photo-thermal origin of pulse laser induced orientation of crystallographic c axis in Tellurium thin films

Recent studies have shown that the orientation of crystallographic c axis of Tellurium thin films can be controlled using picosecond long laser pulses. This method provides spatially programmable control of the crystal orientation and is therefore highly attractive for practical applications in functional optical and electronic devices. Previously, it was suggested that laser-induced selective melting and recrystallization can cause the laser-induced reorientation. However, this interpretation remains inconclusive due to limited data. To clarify the mechanism, here we systematically study Te samples under different irradiation conditions. We find that the threshold fluence for inducing optical reorientation depends on the number of laser pulses. The results agrees well with a minimal kinetic model based on the Arrhenius law. Using the model developed, we investigate the condition required to control the optic axis in other two-dimensional materials, such as black phosphorus, WTe2, and SnSe. These findings provide a guide for developing functional electro-optical devices based on anisotropic materials.

cond-mat.mes-hall↗

arXiv2026

Polar and quadratic magneto-optical Kerr effects in nonmagnetic/ferromagnet bilayers for spin-orbit torque measurements

Recent studies have revealed that spin Hall magnetoresistance (SMR) contributes to both the anomalous and planar Hall resistances in nonmagnetic metal (NM)/ferromagnetic metal (FM) bilayers. This effect becomes pronounced when the NM layer exhibits a large spin Hall angle, as in W/CoFeB bilayers. In such systems, the ratio of planar to anomalous Hall resistances, normally small in single CoFeB layers, can approach unity. This unusually large ratio complicates the determination of spin-torque efficiency using harmonic Hall voltage measurements. To overcome this limitation, magneto-optical Kerr effect (MOKE) measurements have been proposed as an alternative approach. Here, we investigate the polar and quadratic MOKE components, which correspond to, respectively, the anomalous and planar Hall resistances in the low-frequency limit to clarify whether the MOKE measurements are suitable for characterizing the spin-torque efficiency. We find that the ratio of quadratic to polar MOKE signals in NM/FM bilayers is significantly smaller than the corresponding Hall resistance ratio, indicating that SMR contributes negligibly to the MOKE response in the visible range. Consequently, the spin-torque efficiency extracted from MOKE measurements agree well with those expected from the spin Hall angle of the NM layer. These results clarify the reason why MOKE measurements provide reliable determination of the spin-torque efficiency.

cond-mat.mes-hall↗

arXiv2026

Current induced magneto-optical Kerr effect as a probe of Dirac carriers in Bi$_{1-x}$Sb$_x$ alloy

We study the current-induced magneto-optical Kerr effect (MOKE) in Bi$_{1-x}$Sb$_x$ semi-metalic alloys. The MOKE signal is found to be the largest in pure Bi ($x=0$), exceeding that of transition metals by nearly four orders of magnitude, and decreases monotonically with increasing Sb concentration. We find the MOKE signal scales with the resistivity ($\rho$) as $\rho^{1.7 \pm 0.6}$ and with the mobility ($\mu_\mathrm{c}$) as $\mu_\mathrm{c}^{2.0 \pm 0.2}$. Model calculations show that such exponent can be accounted for if the Dirac electrons are responsible for the generation of spin current. This is in contrast to the $\rho^{2}$ and $\mu_\mathrm{c}^{-2}$ scaling of the MOKE signal induced by the free electrons in parabolic band. The scaling of the MOKE amplitude with the resistivity also partly accounts for the order of magnitude differences of the signal observed between metals, semimetals, and semiconductors. These results demonstrate that current induced MOKE serves as an effective means to characterize the nature of spin current in materials with diverse electronic structures.

cond-mat.mes-hall↗

arXiv2026

Comments on the formula to extract current-induced torques from the harmonic Hall voltage measurements

We examine the formulas commonly used to estimate current-induced spin-orbit torques from harmonic Hall voltage measurements. In particular, we focus on the factor of two discrepancy among expressions employed to fit harmonic Hall signals measured under an in-plane rotating magnetic field. By explicitly deriving the relevant relations, we clarify the origin of this discrepancy and present the correct form of the fitting formula. We further discuss the determination of the sign of the field-like torque from harmonic Hall voltage measurements, which depends on the assumed form of the current-induced torques.

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arXiv2025

Light-programmable reorientation of the crystallographic c-axis of Tellurium thin films

Tellurium (Te), a two-dimensional material with pronounced structural anisotropy, exhibits exceptional electrical and optical properties that are highly sensitive to its crystallographic orientation. However, conventional synthesis techniques offer limited control over the in-plane alignment of Te's crystallographic c-axis, hindering large-scale integration. Here, we report a novel, non-contact method to dynamically manipulate the c-axis orientation of Te thin films using linearly polarized picosecond laser pulses. We show that the c-axis can be omnidirectionally reoriented perpendicular to the laser polarization, even in initially polycrystalline films. This reorientation is fully reversible, allowing for rewritable and spatially selective control of the c-axis orientation post-deposition. Our light-driven approach enables programmable anisotropy in Te, opening new avenues for reconfigurable optoelectronic and photonic devices, such as active metasurfaces and CMOS-compatible architectures.

cond-mat.mes-hall↗

arXiv2025

Significant electron-magnon scattering in layered ferromagnet Cr$_2$Te$_3$

A layered ferromagnet Cr$_2$Te$_3$ is attracting growing interest because of its unique electronic and magnetic properties. Studies have shown that it exhibits sizable anomalous Hall effect (AHE) that changes sign with temperature. The origin of the AHE and the sign change, however, remains elusive. Here we show experimentally that electron-magnon scattering significantly contributes to the AHE in Cr$_2$Te$_3$ through magnon induced skew scattering, and that the sign change is caused by the competition with the Berry-curvature or impurity-induced side-jump contribution. The electron-magnon skew scattering is expected to arise from the exchange interaction between the itinerant Te $p$-electrons and the localized Cr $d$-electrons modified by the strong spin-orbit coupling on Te. These results suggest that the magnon-induced skew scattering can dominate the AHE in layered ferromagnets with heavy elements.

cond-mat.mes-hall↗

arXiv2025

Model calculations of the strains associated with surface acoustic waves

Magnon-phonon coupling has garnered increasing interest in condensed matter physics due to its fertile physics and potential applications in devices with novel functionalities. Surface acoustic waves (SAWs) are commonly employed as a source of coherent acoustic phonons. The strain associated with SAWs couples to magnetization of magnetic materials via magnetoelastic coupling and/or spin-rotation coupling. A typical SAW device is formed on a piezoelectric substrate with anisotropic crystal structure. Since the form of strain depends on the material parameters and structure of the SAW device, it is of vital importance to understand its character. In this paper, we present a comprehensive methodology to numerically calculate the SAW velocity, SAW excitation efficiency, lattice displacement and all strain components associated with SAW. LiNbO$_3$ is used as a prototypical material system. All quantities depend on the SAW propagation direction with respect to the crystalline axis and on the electrical boundary conditions. In contrast to non-piezoelectric isotropic media, we find that all shear strain components can be induced in LiNbO$_3$, with their amplitude and relative phase (with respect to the longitudinal strain) dependent on the propagation direction and the boundary conditions at the LiNbO$_3$ surface. These results offer a robust foundation for analyzing strain-driven magnon-phonon coupling mechanisms and contribute to designing strain-engineered functional magnonic and phononic devices.

cond-mat.mtrl-sci↗

arXiv2024

Spin current generation by acousto-electric evanescent wave

We experimentally demonstrate that a spin current can be induced by the acousto-electric evanescent wave, an electric field associated with surface acoustic waves (SAWs) that decay along the surface normal. A previous study showed that a magnetic-field-dependent dc voltage (acoustic voltage) emerges in heavy metal (HM)/ferromagnet (FM) bilayers under excitation of SAWs. The effect, referred to as the acoustic spin Hall effect, was understood by assuming a SAW-induced ac spin current rectified by the oscillation of the FM layer magnetization and the inverse spin Hall effect. However, the mechanism of the spin current generation remained unidentified. Here we measure the acoustic voltage as a function of the SAW propagation direction relative to the crystalline orientation of a LiNbO$_3$ substrate. We find that the magnetic field angle dependence of the acoustic voltage exhibits a phase shift depending on the SAW propagation direction. The result is consistently explained in terms of the acousto-electric evanescent wave generating the spin current in HM layer via the spin Hall effect, thus clarifies the origin of the acoustic spin Hall effect.

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arXiv2024

Electromagnetic evanescent field associated with surface acoustic wave: Response of metallic thin films

Surface acoustic waves (SAWs), coherent vibrational modes localized at solid surfaces, have been employed to manipulate and detect electronic and magnetic states in condensed-matter systems via strain. SAWs are commonly excited in a piezoelectric material, often the substrate. In such systems, SAWs not only generate strain but also electric field at the surface. Conventional analysis of the electric field accompanying the SAW invokes the electrostatic approximation, which may fall short in fully capturing its essential characteristics by neglecting the effect of the magnetic field. Here we study the electric and magnetic fields associated with SAWs without introducing the electrostatic approximation. The plane wave solution takes the form of an evanescent field that decays along the surface normal with a phase velocity equal to the speed of sound. If a metallic film is placed on the piezoelectric substrate, a time- and space-varying electric field permeates into the film with a decay length along the film normal defined by the skin depth and the SAW wavelength. For films with high conductivity, the phase of the electric field varies along the film normal. The emergence of the evanescent field is a direct consequence of dropping the electrostatic approximation, providing a simple but critical physical interpretation of the SAW-induced electromagnetic field.

cond-mat.mes-hall↗

arXiv2024

Acoustoelectric non-local spin wave power detector for studying magnon-phonon coupling

We have developed a simple detection scheme to study spin waves excited by surface acoustic wave (SAW) in ferromagnetic thin films. Metallic antennas made of Ta and a ferromagnetic element are placed along the SAW propagation path. The SAW excites spin waves in the ferromagnetic element and induces acoustoelectric current in the antennas, which are detected as a DC voltage. The DC voltage takes an extremum at the spin wave resonance condition, which demonstrates that the antenna acts as a non-local spin wave detector. The antennas placed before and after the ferromagnetic element along the SAW propagation path can probe spin wave excitation from reflected and transmitted SAWs, respectively. Interestingly, we find characteristics of spin wave excitations that are different for the reflected and transmitted SAWs: the former excites spin waves with larger frequency with broader linewidth compared to the latter. The results show that the antennas act as a non-local spin wave power detector and can be used to map out the spin wave spectra in a unique way, providing insights into the magnon-phonon coupling in magnetic nanostructures fabricated on phononic SAW devices.

cond-mat.mes-hall↗

arXiv2023

Magnon-phonon coupling of synthetic antiferromagnets in a surface acoustic wave cavity resonator

We use a surface acoustic wave (SAW) cavity resonator to study the coupling of acoustic magnons in a synthetic antiferromagnet (SAF) and the phonons carried by SAWs. The SAF is composed of a CoFeB/Ru/CoFeB trilayer and the scattering matrix of the SAW resonator is studied to assess the coupling. We find that the spectral linewidth of the SAW resonator is modulated when the frequency of the excited magnons approaches the SAW resonance frequency. Moreover, the linewidth modulation varies with the magnitude and orientation of the external magnetic field. Such change in the spectral linewidth can be well reproduced using macrospin-like model calculations. From the model analyses, we estimate the magnon-phonon coupling strength to be $\sim$15.6 MHz at a SAW resonance frequency of 1.8 GHz: the corresponding magnomechanical cooperativity is $\sim$0.66. As the spectral shape hardly changes in a CoFeB single layer reference sample under the same experimental condition, these results show that SAF provides an ideal platform to study magnon-phonon coupling in a SAW cavity resonator.

cond-mat.mes-hall↗

arXiv2023

On-chip all-electrical determination of the magnetoelastic coupling constant of magnetic heterostructures

We have developed an approach to determine the magnetoelastic coupling constant of magnetic layers in thin film heterostructures. The film is formed on a piezoelectric substrate between two interdigital transducers (IDT), a platform often used to construct a surface acoustic wave device. With the substrate piezoelectricity, strain is induced into the film by applying a dc voltage to the IDTs. The strain causes changes in the magnetization direction of the magnetic layer, which is probed by measuring changes, if any, in the transverse resistance of the heterostructure. We find the extracted magnetoelastic coupling constant of the magnetic layer (CoFeB) depends on the film stacking. Such change can be accounted for provided that the elastic properties of the layers that constitute the heterostructures are taken into account. The on-chip all-electrical approach described here provides a versatile means to quantitatively assess the magnetoelastic coupling constant of thin film heterostructures.

cond-mat.mes-hall↗

arXiv2023

Helicity resolved Raman spectroscopy of mono- and a few-layers thick PtSe$_2$

We studied helicity resolved Raman scattering in PtSe$_2$ flakes with different thicknesses. The peak amplitude of helicity-switched Raman scattering is significantly larger than that of helicity-conserved scattering for the in-plane $E_{g}$ mode, consistent with the Raman tensor analyses and conservation law of angular momentum. The peak amplitude of the helicity-switched $E_{g}$ mode is larger for the thinner flakes. In addition, we find Raman peaks near the energy levels of infrared (IR)-active $E_u$ and $A_{2u}$ modes, only for monolayer and a few-layers thick flakes. Interestingly, these peaks manifest themselves only for helicity-switched Raman scattering; they are nearly absent for helicity-conserved scattering.

cond-mat.mes-hall↗

arXiv2023

Cavity magnomechanical coupling with coupled magnon modes in a synthetic antiferromagnet

On-chip cavity magnomechanics is an emerging field exploring acoustic and magnonic functionalities of various ferromagnetic materials and structures using strongly confined phonons. It is expected that such cavity magnomechanics can be extended to multilayer ferromagnets, especially synthetic antiferromagnets (SAFs) that exhibit zero net magnetization through interlayer exchange coupling. However, the conventional theoretical framework for a single ferromagnet cannot be used directly because of the antiferromagnetic magnetization dynamics associated with the interlayer exchange coupling. In this paper, we theoretically investigate phonon-magnon coupling with a three-layer SAF. Our formulation of the phonon-magnon coupling constants reveals that the acoustic (optical) magnon mode dominantly couples to the cavity phonon when the magnetization angles in the two ferromagnetic layers are antiparallel (orthogonal). Moreover, numerical calculations including the effects of dipole-dipole interactions and in-plane uniaxial magnetic anisotropy allow us to predict phonon frequency shifts and linewidth broadening that can be detected in experiments. These theoretical insights would greatly help us to make a strategy for bringing the system into the strong coupling regime and to devise novel control protocols in analogy to cavity quantum electrodynamics and cavity optomechanics.

cond-mat.mes-hall↗

arXiv2023

Anisotropy of the spin Hall effect in a Dirac ferromagnet

We study the intrinsic spin Hall effect of a Dirac Hamiltonian system with ferromagnetic exchange coupling, a minimal model combining relativistic spin-orbit interaction and ferromagnetism. The energy bands of the Dirac Hamiltonian are split after introducing a Stoner-type ferromagnetic ordering which breaks the spherical symmetry of pristine Dirac model. The totally antisymmetric spin Hall conductivity (SHC) tensor becomes axially anisotropic along the direction of external electric field. Interestingly, the anisotropy does not vanish in the asymptotic limit of zero magnetization. We show that the ferromagnetic ordering breaks the spin degeneracy of the eigenfunctions and modifies the selection rules of the interband transitions for the intrinsic spin Hall effect. The difference in the selection rule between the pristine and the ferromagnetic Dirac phases causes the anisotropy of the SHC, resulting in a discontinuity of the SHC as the magnetization, directed orthogonal to the electric field, is reduced to zero in the ferromagnetic Dirac phase and enters the pristine Dirac phase.

cond-mat.mes-hall↗

arXiv2023

Anomalous Hall effect of light-driven three-dimensional Dirac electrons in bismuth

Recent advancement in laser technology has opened the path toward the manipulation of functionalities in quantum materials by intense coherent light. Here, we study three-dimensional (3D) Dirac electrons driven by circularly polarized light (CPL), when the photon energy lies within the Dirac bands. As an experimental realization of this setup, we irradiate a thin film sample of elemental bismuth, which is a well-known semimetal hosting 3D Dirac electrons, with mid-infrared CPL. We successfully observe the emergence of the anomalous Hall effect (AHE) via terahertz Faraday rotation that is both pump-helicity-dependent and instantaneous. We compare our experimental findings with the results of Floquet theory, which is a powerful framework for analyzing the electronic band structure driven by coherent light. The contribution from the band structures near the one-photon resonant positions to the AHE shows a field-strength dependence consistent with our experimental results. The effective Hamiltonian on which we base our model calculations also implies that a pair of "double Weyl points" emerge due to the CPL-induced hybridization between the occupied and unoccupied 3D Dirac bands. Our findings shed light on ultrafast control of material properties in nonlinear topological optics.

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