arXiv subjects

Masanobu Iwanaga

Publications and source records attributed to Masanobu Iwanaga.

12 recordsLinked to original sources

arXiv2026

Finite-Size Effect Induced Spatial-Spectral Mode Splitting in Membrane Metasurfaces

This work reports the spatial-spectral engineering and finite-size quantization of optical modes within a triangular-lattice silicon nitride membrane metasurface. Truncating the lattice into a finite square cavity breaks translational symmetry and lifts modal degeneracy, splitting optical modes into discrete cavity-envelope sub-modes. High-resolution photoluminescence (PL) scanning reveals distinct spatial field distributions. The corner-localized sub-mode features the highest Q-factor due to multipolar far-field destructive interference, whereas the core-localized sub-mode exhibits strong radiative coupling. PL mapping reveals a symmetric, four-fold clover-like wavelength arrangement. These results demonstrate that boundary-induced deterministic symmetry can override underlying lattice characteristics, offering a robust strategy for precise spatial-spectral tailoring of light-matter interactions at the nanoscale.

physics.optics↗

arXiv2026

Single-nanoparticle detection using quasi-bound states in the continuum supported by silicon metasurfaces

The detection of single particles or molecules represents a critical milestone in the development of biosensing technologies. Recently developed optical sensors based on quasi-bound states in the continuum (qBICs) have primarily focused on detecting global refractive index changes, aiming to simultaneously enhance both refractive index sensitivity and quality ($Q$) factors. However, sensors capable of resolving local refractive index perturbations, such as the binding of a nanometer-sized molecule on a surface, remain elusive and have not yet been demonstrated in BIC geometries due to the limited $Q$ factors and relatively large mode volumes. Here, we demonstrate low-contrast BIC metasurfaces that can perform sensing with a virus-sized single-nanoparticle resolution. The qBIC resonance operating at the critical coupling condition exhibits an experimental $Q$ factor of 4.5 x 10$^4$ in heavy water. The strong interaction between the localized electric field and polystyrene nanoparticles with a diameter of 100 nm enable the experimental observation of step-like resonance wavelength shifts, serving as signatures of individual particle binding events. Furthermore, binding-induced modifications to the qBIC resonance alter the optical confinement and asymmetry factor, inducing changes not only in the resonance wavelength but also in the linewidth and amplitude with single-particle sensitivity. Combined with position-insensitive response and free-space accessible features, low-contrast BIC metasurfaces provide a user-friendly platform for next-generation single-molecule sensing integrated with microfluidic systems.

physics.optics↗

arXiv2024

Low-Contrast BIC Metasurfaces with Quality Factors Exceeding 100,000

Dielectric metasurfaces operating at quasi-bound states in the continuum (qBICs) can achieve exceptionally high radiative quality ($\textit{Q}$) factors by introducing small asymmetries into their unit cells. However, fabrication imperfections often impose major limitations on the experimentally observed $\textit{Q}$ factors. In this study, we experimentally demonstrate BIC metasurfaces with a record-high $\textit{Q}$ factor of 101,486 under normal excitation of light in the telecom wavelength range achieved by employing low-contrast silicon pairs. Our findings show that such ultrahigh-$\textit{Q}$ factors can be attained by leveraging both the high radiative $\textit{Q}$ factors of higher-order qBIC modes and reduced scattering losses in shallow-etched designs. Additionally, we demonstrate stable sub-picometer-level wavelength fluctuations in water, with a limit of detection of $10^{-5}$ for environmental refractive index changes. The proposed approach can be extended to BIC metasurfaces with many other configurations and operating wavelengths for ultrahigh-$\textit{Q}$ applications in both fundamental physics and advanced devices.

physics.optics↗

arXiv2023

Vibrational coupling to quasi-bound states in the continuum under tailored coupling conditions

Photonic resonance modes can be spectrally coupled to the vibrational modes of molecules in the mid-infrared regime through interactions between localized electric fields and nearby molecules. According to recent studies, radiative loss engineering of coupled systems is a promising approach for tailoring coupling conditions and enhancing the molecular signals. However, this strategy has only been realized using the localized surface plasmon resonances of metal nanostructures, which suffer from increased ohmic loss in the mid-infrared region and face serious limitations in achieving high quality (Q) factors. In this study, we adopt silicon-based metasurfaces formed on silicon-on-insulator wafers to achieve high Q factors and tune the coupling conditions between the quasi-bound states in the continuum (qBICs) and molecular vibrations. The coupling between the resonance mode and polymethyl methacrylate molecules is tailored from weak to strong coupling regimes by simply changing the structural asymmetry parameter and utilizing the intrinsically high Q factors of the qBIC modes. In addition, we identify the optimal asymmetry parameter that maximizes the enhanced molecular signal, opening a route toward realizing highly sensitive surface-enhanced infrared spectroscopy using complementary metal-oxide semiconductor compatible all-dielectric materials.

physics.optics↗

arXiv2007

Diamagnetic nature of stratified thin metals in visible range

It is numerically demonstrated that effectively strong diamagnetic resonance emerges at visible frequencies in stratified metal-dielectric metamaterials. The effective optical constants are extracted by two-complex reflectivity method. It is clarified that the effective diamagnetic response originates from local diamagnetism at stratified thin metals. The effective diamagnetism is crucially sensitive to the sturucture of unitcell. The effective diamagnetic response is always associated with effective plasma frequency and is therefore regarded as a magnetic component of the collective excitation.

physics.optics↗

arXiv2007

Reciprocal transmittances and reflectances: An elementary proof

We present an elementary proof concerning reciprocal transmittances and reflectances. The proof is direct, simple, and valid for the diverse objects that can be absorptive and induce diffraction and scattering, as long as the objects respond linearly and locally to electromagnetic waves. The proof enables students who understand the basics of classical electromagnetics to grasp the physical basis of reciprocal optical responses. In addition, we show an example to demonstrate reciprocal response numerically and experimentally.

physics.optics↗

arXiv2007

Effective optical constants in stratified metal-dielectric metameterial

We present effective optical constants of stratified metal-dielectric metameterial. The effective constants are determined by two complex reflectivity method (TCRM). TCRM reveals full components of effective permittivity and permeability tensors and indicates the remarkable anisotropy of metallic and dielectric components below effective plasma frequency. On the other hand, above the plasma frequency, one of the effective refractive indexes takes a positive value less than unity and is associated with small loss. The photonic states are confirmed by the distribution of electromagnetic fields.

physics.optics↗

arXiv2005

Full optical responses of one-dimensional metallic photonic crystal slabs

We reveal all the linear optical responses, reflection, transmission, and, diffraction, of typical one-dimensional metallic photonic crystal slabs (MPhCS) with the periodicity of a half micrometer. Maxwell equations for the structure of deep grooves are solved numerically with good precision by using the formalism of scattering matrix, without assuming perfect conductivity. We verify characteristic optical properties such as nearly perfect transmission and reflection. Moreover, we present large reflective diffraction and show that, in the energy range where diffraction channels are open, the photonic states in the MPhCS originate from surface plasmon polaritons.

cond-mat.mtrl-sci↗

arXiv2005

Photoacoustic wave propagating from normal into superconductive phases in Pb single crystals

Photoacoustic (PA) wave has been examined in a superconductor of the first kind, Pb single crystal. The PA wave is induced by optical excitation of electronic state and propagates from normal into superconductive phases below T$_{\rm C}$. It is clearly shown by wavelet analysis that the measured PA wave includes two different components. The high-frequency component is MHz-ultrasonic and the relative low-frequency one is induced by thermal wave. The latter is observed in a similar manner irrespective of T$_{\rm C}$. On the other hand, the MHz-frequency component is obviously enhanced below T$_{\rm C}$. The behavior is reproduced by the change of attenuation of longitudinal ultrasonic wave and is consistent with BCS theory.

cond-mat.mtrl-sci↗

arXiv2005

Photoacoustic detection of phase transitions at low temperatures in CsPbCl$_3$ crystals

Phase transitions in CsPbCl$_3$ crystals have been explored by photoacoustic (PA) method in a wide temperature range of 150--300 K. The PA signals, induced by ns-pulsed laser excitation of electronic states and detected with a piezoelectric transducer, are thermoelastic ultrasonic waves lasting for hundreds of microseconds. The wavelet analysis of the PA wave has clarified that the thermoelastic wave includes several MHz components. The PA signals have been made use of in order to examine phase transitions at low temperatures in the crystal. Changes of PA signals indicate that two phase transitions take place at low temperatures around 200 K. The types of phase transitions are discussed taking into recent experimatal results.

cond-mat.mtrl-sci↗

arXiv2002

Exciton-relaxation dynamics in lead halides

We survey recent comprehensive studies of exciton relaxation in the crystals of lead halides. The luminescence and electron-spin-resonance studies have revealed that excitons in lead bromide spontaneously dissociate and both electrons and holes get self-trapped individually. Similar relaxation has been also clarified in lead chloride. The electron-hole separation is ascribed to repulsive correlation via acoustic phonons. Besides, on the basis of the temperature profiles of self-trapped states, we discuss the origin of luminescence components which are mainly induced under one-photon excitation into the exciton band in lead fluoride, lead chloride, and lead bromide.

cond-mat.mtrl-sci↗

arXiv2002

Self-trapped electrons and holes in PbBr$_2$ crystals

We have directly observed self-trapped electrons and holes in PbBr$_{2}$ crystals with electron-spin-resonance (ESR) technique. The self-trapped states are induced below 8 K by two-photon interband excitation with pulsed 120-fs-width laser light at 3.10 eV. Spin-Hamiltonian analyses of the ESR signals have revealed that the self-trapping electron centers are the dimer molecules of Pb$_2$$^{3+}$ along the crystallographic a axis and the self-trapping hole centers are those of Br$_2$$^-$ with two possible configurations in the unit cell of the crystal. Thermal stability of the self-trapped electrons and holes suggests that both of them are related to the blue-green luminescence band at 2.55 eV coming from recombination of spatially separated electron-hole pairs.

cond-mat.mtrl-sci↗