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Masatoshi Imada

Publications and source records attributed to Masatoshi Imada.

At least 181 records · Page 10Linked to original sources

Effect of the Orbital Level Difference in Doped Spin-1 Chains

Doping of a two-orbital chain with mobile S=1/2 Fermions and strong Hund's rule couplings stabilizing the S=1 spins strongly depends on the presence of a level difference among these orbitals. By DMRG methods we find a finite spin gap upon doping and dominant pairing correlations without level-difference, whereas the presence of a level difference leads to dominant charge density wave (CDW) correlations with gapless spin-excitations. The string correlation function also shows qualitative differences between the two models.

cond-mat↗

Spin-1 chain doped with mobile S=1/2 fermions

We investigate doping of a two-orbital chain with mobile $S=1/2$ fermions as a valid model for $\rm Y_{2-x}Ca_xBaNiO_5$. The S=1 spins are stabilized by strong, ferromagnetic (fm) Hund's rule couplings. We calculate correlation functions and thermodynamic quantities by DMRG methods and find a new hierarchy of energy scales in the spin sector upon doping. Gapless spin-excitations are generated at a lower energy scale by interactions among itinerant polarons created by each hole and coexist with the larger scale of the gapful spin-liquid background of the S=1 chain accompanied by a finite string-order parameter.

cond-mat↗

Enhancement of Pairing Correlation and Spin Gap through Suppression of Single-Particle Dispersion in One-Dimensional Models

We investigate the effects of suppression of single-particle dispersion near the Fermi level on the spin gap and the singlet-pairing correlation by using the exact diagonalization method for finite-size systems. We consider strongly correlated one-dimensional models, which have flat band dispersions near wave number k=π/2, if the interactions are switched off. Our results for strongly correlated models show that the spin gap region expands as the single-particle dispersion becomes flatter. The region where the singlet-pairing correlation is the most dominant also expands in models with flatter band dispersions. Based on our numerical results, we propose a pairing mechanism induced by the flat-band dispersion.

cond-mat.str-el↗

Superconductivity from Flat Dispersion Designed in Doped Mott Insulators

Routes to enhance superconducting instability are explored for doped Mott insulators. With the help of insights for criticalities of metal-insulator transitions, geometrical design of lattice structure is proposed to control the instability. A guideline is to explicitly make flat band dispersions near the Fermi level without suppressing two-particle channels. In a one-dimensional model, numerical studies show that our prescription with finite-ranged hoppings realizes large enhancement of spin-gap and pairing dominant regions. We also propose several multi-band systems, where the pairing is driven by intersite Coulomb repulsion.

cond-mat.str-el↗

Quantum Effects in Resistance-Shunted Josephson Junctions

Thermodynamics and transport properties of resistance-shunted Josephson junctions are studied theoretically in the tight-binding limit E_C/E_J<<1, where E_C and E_J are a charging energy and a Josephson coupling energy respectively. Based on a phenomenological harmonic-oscillator model, weak coupling region K=R_Q/R<<1 is analytically studied, where R and R_Q=h/(2e)^2 are a shunted resistance and the quantum resistance. In addition to the effective bandwidth, we find that this multi-level system genuinely has a novel crossover at lower energy below which the density of states becomes strongly degenerate. These two energy scales control the linear DC responses, optical responses, and nonlinear I-V characteristics. The lower energy crossover indicates the existence of a new class of strongly-correlated phenomena beyond the framework of the Kondo problem.

cond-mat.supr-con↗

Single-Particle Pseudogap in Two-Dimensional Electron Systems

We investigate pseudogap phenomena in the 2D electron system. Based on the mode-mode coupling theory of antiferromagnetic (AFM) and $d_{x^2-y^2}$-wave superconducting ($d$SC) fluctuations, single-particle dynamics is analyzed. For the parameter values of underdoped cuprates, pseudogap structure grows in the single-particle spectral weight $A(k,ω)$ around the wave vector $(π,0)$ and $(0,π)$ below the pseudo-spin-gap temperature $\TPG$ signaled by the reduction of dynamical spin correlations in qualitative agreement with the experimental data. The calculated results for the overdoped cuprates also reproduce the absence of the pseudogap in the experiments. We also discuss limitations of our weak-coupling approach.

cond-mat.str-el↗

Control of Superconducting Correlations in High-Tc Cuprates

A strategy to enhance d-wave superconducting correlations is proposed based on our numerical study for correlated electron models for high-Tc cuprates. We observe that the pairing is enhanced when the single-electron level around (pi,0) is close to the Fermi level E_F, while the d-wave pairing interaction itself contains elements to disfavor the pairing due to shift of the (pi,0)-level. Angle-resolved photoemission results in the cuprates are consistently explained in the presence of the d-wave pairing interaction. Our proposal is the tuning of the (pi,0)-level under the many-body effects to E_F by optimal design of band structure.

cond-mat.supr-con↗

Effects of Orbital Degeneracy and Electron Correlation on Charge Dynamics in Perovskite Manganese Oxides

Taking the orbital degeneracy of $e_g$ conduction bands and the Coulomb interaction into account in a double-exchange model, we investigate charge dynamics of perovskite Mn oxides by the Lancz$\ddot{\rm o}$s diagonalization method. In the metallic phase near the Mott insulator, it is found that the optical conductivity for a spin-polarized two-dimensional system exhibits a weight transfer to a broad and incoherent structure within the lower-Hubbard band together with a suppressed Drude weight. It reproduces qualitative feature of the experimental results. As an orbital effect, we find that an anomalous charge correlation at quarter filling suppresses the coherent charge dynamics and signals precursor to the charge ordering.

cond-mat.str-el↗

Ordering and Fluctuation of Orbital and Lattice Distortion in Perovskite Manganese Oxides

Roles of orbital and lattice degrees of freedom in strongly correlated systems are investigated to understand electronic properties of perovskite Mn oxides such as La_{1-x}Sr_{x}MnO_{3}. An extended double-exchange model containing Coulomb interaction, doubly degenerate orbitals and Jahn-Teller coupling is derived under full polarization of spins with two-dimensional anisotropy. Quantum fluctuation effects of Coulomb interaction and orbital degrees of freedom are investigated by using the quantum Monte Carlo method. In undoped states, it is crucial to consider both the Coulomb interaction and the Jahn-Teller coupling in reproducing characteristic hierarchy of energy scales among charge, orbital-lattice and spin degrees of freedom in experiments. Our numerical results quantitatively reproduce the charge gap amplitude as well as the stabilization energy and the amplitude of the cooperative Jahn-Teller distortion in undoped compounds. Upon doping of carriers, in the absence of the Jahn-Teller distortion, critical enhancement of both charge compressibility and orbital correlation length is found with decreasing doping concentration. These are discussed as origins of strong incoherence in charge dynamics. With the Jahn-Teller coupling in the doped region, collapse of the Jahn-Teller distortion and instability to phase separation are obtained and favorably compared with experiments. These provide a possible way to understand the complicated properties of lightly doped manganites.

cond-mat.str-el↗

d_{x^2-y^2}-Wave Pairing Fluctuations and Pseudo Spin Gap in Two-Dimensional Electron Systems

Pseudogap phenomena of high-T_c cuprates are examined. In terms of AFM (antiferromagnetic) and dSC (d_{x^2-y^2}-wave superconducting) auxiliary fields introduced to integrate out the fermions, the effective action for 2D electron systems with AFM and dSC fluctuations is considered. By the self-consistent renormalization (SCR), the NMR relaxation rate T_1^{-1}, the spin correlation length ξ_σand the pairing correlation length ξ_d are calculated. From this calculation, a mechanism of the pseudogap formation emerges as the region of dominant d-wave short-range order (SRO) over AFM-SRO. When damping for the AFM fluctuation strongly depends on the dSC correlation length through the formation of precursor singlets around (π,0) and (0,π) points in the momentum space, the pseudogap appears in a region of the normal state characterized by decreasing 1/T_1T and increasing AFM correlation length with decrease in temperature. This reproduces a characteristic feature of the pseudogap phenomena in many underdoped cuprates. When the damping becomes insensitive to the dSC correlation length, the pseudogap region shrinks as in the overdoped cuprates.

cond-mat.str-el↗

Optical Conductivity of the Two-Dimensional Hubbard Model

Charge dynamics of the two-dimensional Hubbard model is investigated. Lancz$\ddot{\rm o}$s-diagonalization results for the optical conductivity and the Drude weight of this model are presented. Near the Mott transition, large incoherence below the upper-Hubbard band is obtained together with a remarkably suppressed Drude weight in two dimensions while the clearly coherent character is shown in one dimension. The two-dimensional results are consistent with previous results from quantum Monte Carlo calculations indicating that the Mott transition in this two-dimensional model belongs to the universality class characterized by the dynamical exponent of $z=4$.

cond-mat↗

Metal-Insulator Transition in Mn Perovskite Compounds

We discuss Mott insulating and metallic phases of a model with $e_g$ orbital degeneracy to understand physics of Mn perovskite compounds. Quantum Monte Carlo and Lanczos diagonalization results are discussed in this model. To reproduce experimental results on charge gap and Jahn-Teller distortions, we show that a synergy between the strong correlation effects and the Jahn-Teller coupling is important. The incoherent charge dynamics and strong charge fluctuations are characteristic of the metallic phase accompanied with critical enhancement of short-ranged orbital correlation near the insulator.

cond-mat.str-el↗

Effects of Electron Correlation, Orbital Degeneracy and Jahn-Teller Coupling in Perovskite Manganites

Roles of Coulomb interaction, orbital degeneracy and Jahn-Teller coupling in double-exchange models are examined for Mn perovskite oxides. We study the undoped Mott insulator as well as metal-insulator transitions by hole doping, and especially strong incoherence of ferromagnetic metal. We derive models where all the spins are fully polarized in two-dimensional planes as in the experimental indications, and investigate their ground-state properties by quantum Monte Carlo method. At half filling where the number of $e_{g}$ electron is one per site on average, the Coulomb interaction opens a Mott gap and induces a staggered orbital ordering. The opening of the Mott gap is, however, substantially slower than the mean-field results if the Jahn-Teller coupling is absent. The synergy between the strong correlation and the Jahn-Teller coupling largely enhances the Mott gap amplitude and reproduces realistic amplitudes and stabilization energy of the Jahn-Teller distortion. Upon doping, the orbital ordering stabilized by the Coulomb interaction is destroyed immediately. Toward the metal-insulator transition, the short-ranged orbital correlation is critically enhanced in metals, which should be related to strong incoherence of charge dynamics observed in experiments. Our model, moreover, exhibits a uniform ordering of $d_{x^{2}-y^{2}}$ orbital in a wide region of doping in agreement with experimental indications.

cond-mat.str-el↗

Metal-Insulator and Superconductor-Insulator Transitions in Correlated Electron Systems

Quantum transitions between the Mott insulator and metals by controlling filling in two-dimensional square lattice are characterized by a large dynamical exponent $z=4$ where the origin of unusual metallic properties near the Mott insulator are ascribed to the proximity of the transition. The scaling near the transition indicates the formation of flat dispersion area due to singular momentum dependence of the single-particle renormalization. The flat dispersion controls critical properties of the Mott transition. An instability of the flat dispersion to the d-wave superconducting order is discussed. We also discuss a case of the Mott transition for a model of Mn perovskite compounds with orbital degeneracy where orbital correlation length shows critical divergence toward the metal-insulator transition.

cond-mat.str-el↗

Numerical Study for the Ground State of Multi-Orbital Hubbard Models

Ground state properties of multi-orbital Hubbard models are investigated by the auxiliary field quantum Monte Carlo method. A Monte Carlo technique generalized to the multi-orbital systems is introduced and examined in detail. The algorithm contains non-trivial cases where the negative sign problem does not exist. We investigate one-dimensional systems with doubly degenerate orbitals by this new technique. Properties of the Mott insulating state are quantitatively clarified as the strongly correlated insulator, where the charge gap amplitude is much larger than the spin gap. The insulator-metal transitions driven by the chemical potential shows a universality class with the correlation length exponent $ν=1/2$, which is consistent with the scaling arguments. Increasing level split between two orbitals drives crossover from the Mott insulator with high spin state to the band insulator with low spin state, where the spin gap amplitude increases and becomes closer to the charge gap. Experimental relevance of our results especially to Haldane materials is discussed.

cond-mat.str-el↗

Thermodynamics and Optical Conductivity of a Dissipative Carrier in a Tight Binding Model

Thermodynamics and transport properties of a dissipative particle in a tight-binding model are studied through specific heat and optical conductivity. A weak coupling theory is constituted to study the crossover behavior between the low-temperature region and the high-temperature region analytically. We found that coherent part around zero frequency in the optical conductivity disappears for 0<s<2, where s is an exponent of a spectral function of the environment. Detailed calculation is performed for ohmic damping (s=1). In this case, the specific heat shows an unusual $T$-linear behavior at low temperatures, which indicates that the environment strongly influences the particle motion, and changes the low-energy states of the dissipative particle. The optical conductivity σ(ω) takes a non-Drude form even at zero temperature, and the high-frequency side behaves as ω^(2K-2), where K is a dimensionless damping strength. The high frequency side of the optical conductivity is independent of temperatures, while the low frequency side depends on the temperature, and behaves as T^(2K-2) at high temperatures. We also comment on the application of this model to the description of incoherent motion in correlated electron systems.

cond-mat.stat-mech↗

Dynamic Exponent of t-J and t-J-W Model

Drude weight of optical conductivity is calculated at zero temperature by exact diagonalization for the two-dimensional t-J model with the two-particle term, $W$. For the ordinary t-J model with $W$=0, the scaling of the Drude weight $D \propto δ^2$ for small doping concentration $δ$ is obtained, which indicates anomalous dynamic exponent $z$=4 of the Mott transition. When $W$ is switched on, the dynamic exponent recovers its conventional value $z$=2. This corresponds to an incoherent-to-coherent transition associated with the switching of the two-particle transfer.

cond-mat.str-el↗

Orbital Order Effect of Two-Dimensional Spin Gap System for CaV4O9

Effects of possible orbital order in magnetic properties of two-dimensional spin gap system for CaV$_4$O$_9$ are investigated theoretically. After analyzing experimental data, we show that single orbital models assumed in the literature are insufficient to reproduce the data. To understand the origin of the discrepancy, we assume that in $d^1$ state of V, $d_{xz}$ and $d_{yz}$ orbitals have substantial contributions in the lowest-energy atomic level which leads to a double-degeneracy. We study possible configurations of the orbital order. By exact diagonalization and perturbation expansion, we calculate the susceptibility, wavenumber dependence of low-lying excitations and equal-time spin-spin correlations which is related to integrated intensity of the neutron inelastic scattering. These quantities sensitively depend on the configuration of the orbital order. The calculated results for some configurations of the orbital order reproduce many experimental results much better than the previous single-orbital models. However some discrepancy still remains to completely reproduce all of the reported experimental results. To understand the origin of these discrepancies, we point out the possible importance of the partially occupied $d_{xy}$ orbital in addition to orbital order of partially filled $d_{xz}$ and $d_{yz}$ orbitals.

cond-mat.str-el↗