arXiv subjects

Masaya Uchida

Publications and source records attributed to Masaya Uchida.

3 recordsLinked to original sources

arXiv2013

Measuring the orbital angular momentum of electron vortex beams using a forked grating

The present study experimentally examines how an electron vortex beam with orbital angular momentum (OAM) undergoes diffraction through a forked grating. The nth-order diffracted electron vortex beam after passing through a forked grating with a Burgers vector of 1 shows an OAM transfer of nh. Hence, the diffraction patterns become mirror asymmetric owing to the size difference between the electron beams. Such a forked grating, when used in combination with a pinhole located at the diffraction plane, could act as an analyzer to measure the OAM of input electrons.

quant-ph↗

arXiv2010

Epitaxially stabilized iridium spinel oxide without cations in the tetrahedral site

Single-crystalline thin film of an iridium dioxide polymorph Ir2O4 has been fabricated by the pulsed laser deposition of LixIr2O4 precursor and the subsequent Li-deintercalation using soft chemistry. Ir2O4 crystallizes in a spinel (AB2O4) without A cations in the tetrahedral site, which is isostructural to lambda-MnO2. Ir ions form a pyrochlore sublattice, which is known to give rise to a strong geometrical frustration. This Ir spinel was found to be a narrow gap insulator, in remarkable contrast to the metallic ground state of rutile-type IrO2. We argue that an interplay of strong spin-orbit coupling and a Coulomb repulsion gives rise to an insulating ground state as in a layered perovskite Sr2IrO4.

cond-mat.str-el↗

arXiv2008

Band Jahn-Teller Instability and Formation of Valence Bond Solid in a Mixed-Valent Spinel Oxide LiRh2O4

We have synthesized a new spinel oxide LiRh2O4 with a mixed-valent configuration of Rh3+ and Rh4+. At room temperature it is a paramagnetic metal, but on cooling, a metal-insulator transition occurs and a valence bond solid state is formed below 170 K. We argue that the formation of valence bond solid is promoted by a band Jahn-Teller transition at 230 K and the resultant confinement of t2g holes within the xy band. The band Jahn-Teller instability is also responsible for the observed enhanced thermoelectric power in the orbital disordered phase above 230 K.

cond-mat.str-el↗