arXiv subjects

Masayuki Toyoda

Publications and source records attributed to Masayuki Toyoda.

3 recordsLinked to original sources

arXiv2026

High-field magneto-optical imaging of superconducting critical states beyond 10 T using a paramagnetic garnet sensor

Spatially resolved characterization of the critical current density Jc in superconductors under high magnetic fields is crucial for both fundamental understanding and practical applications. However, conventional techniques primarily provide bulk-averaged values, making it difficult to resolve local variations of Jc, especially in high magnetic fields. In this work, we develop a magneto-optical imaging (MOI) technique that enables visualization of superconducting critical states in steady magnetic fields up to 13 T. This is achieved by employing a paramagnetic Nd-garnet indicator combined with a polarizing microscope system. Using this method, we directly image the magnetic flux distribution in a bulk single crystal of an iron-based superconductor Ba(Fe1-xCox)2As2 (x = 0.075) at 12 K and 20 K across the entire sample area (approximately 1 mm). From the measured magnetic field distributions, we quantitatively reconstruct the spatial distribution of the critical current density. The extracted field dependence of Jc is in good agreement with that obtained from conventional magnetization measurements. Furthermore, we demonstrate vector mapping of current flow within the sample by converting the magnetic field distribution into local current-density distributions. Our results establish high-field MOI as a powerful approach for spatially resolved evaluation of superconducting critical states and provide a new pathway for investigating inhomogeneous current transport in superconductors under high magnetic fields.

cond-mat.supr-con↗

arXiv2018

Magnetic Structural Unit with Convex Geometry: a Building Block Hosting an Exchange-striction-driven Magnetoelectric Coupling

We perform a combined experimental and theoretical study of a magnetic-field ($B$) induced evolution of magnetic and ferroelectric properties in an antiferromagnetic material Pb(TiO)Cu$_4$(PO$_4$)$_4$, whose structure is characterized by a staggered array of Cu$_4$O$_{12}$ magnetic units with convex geometry known as square cupola. Our experiments show a $B$-induced phase transition from a previously reported low-$B$ linear magnetoelectric phase to a new high-$B$ magnetoelectric phase, which accompanies a 90$^\circ$ flop of electric polarization and gigantic magnetodielectric effect. Moreover, we observe a $B$-induced sign reversal of ferroelectric polarization in the high-$B$ phase. Our model and first-principles calculations reveal that the observed complex magnetoelectric behavior is well explained in terms of a $B$-dependent electric polarization generated in each Cu$_4$O$_{12}$ unit by the so-called exchange striction mechanism. The present study demonstrates that the materials design based on the magnetic structural unit with convex geometry deserves to be explored for developing strong magnetoelectric couplings.

cond-mat.mtrl-sci↗

arXiv2008

Exchange Interaction and $T_c$ in Alkaline-earth-metal-oxide-based DMS without Magnetic Impurities: First Principle Pseudo-SIC and Monte Carlo Calculation

The prospects of half-metallic ferromagnetism being induced by the incorporation of C atoms into alkaline-earth-metal-oxides are investigated by the first principle calculation. The origin of the ferromagnetism is discussed through the calculation of the electronic structure and exchange coupling constant by using the pseudo-potential-like self-interaction-corrected local spin density method. The Curie temperature ($T_c$) is also predicted by employing the Monte Carlo simulation. It is shown that by taking the electron self-interaction into account, the half-metallic ferromagnetism induced by C in the host materials is more stabilized in comparison with the standard LDA case, and the C's $2p$ electron states in the bandgap become more localized resulting in the predominance of the short-ranged exchange interaction. While the ferromagnetism in MgO$_{1-x}$C$_x$ is stabilized due to the exchange interaction of the $1st$-nearest neighbor pairs and might be suppressed by the anti-ferromagnetic super-exchange interaction at higher $x$, the ferromagnetism in CaO$_{1-x}$C$_x$, SrO$_{1-x}$C$_x$, and BaO$_{1-x}$C$_x$ is stabilized by both the $1st$- and $2nd$-nearest neighbor pairs, and $T_c$ monotonously increases with the C concentration.

cond-mat.mtrl-sci↗