Searcharxiv⌕ Search

arXiv subjects

Matías P. Grassi

Publications and source records attributed to Matías P. Grassi.

10 recordsLinked to original sources
arXiv2026

Mapping Reversal Pathways and Interaction Fields in Artificial Spin Ice

In artificial spin ice (ASI), magnetic interactions between nanomagnets determine both the stable states and the switching pathways under an applied field. Here, first-order reversal curve (FORC) measurements are used to map how these interactions govern magnetization reversal in square arrays as the element shape and spacing are varied. The FORC diagrams show that some geometries reverse more uniformly, whereas others exhibit broader, more asymmetric responses, indicating stronger interaction effects and more complex reversal pathways. Combined FORC analysis and micromagnetic simulations also capture subtle changes in internal magnetization textures during switching, linking local behavior within individual elements to collective behavior across the array. These results establish FORC as a practical tool for mapping and engineering interaction landscapes, with direct relevance to reconfigurable magnetic reservoirs and neuromorphic functionality.

cond-mat.mtrl-sci↗
arXiv2026

Probing deuterium-induced magnetic phase transitions in TbCo alloys with in-situ polarized neutron reflectometry

Hydrogen-based magneto-ionics is a promising approach for rapid magnetoelectric control of spintronic devices. Most investigations so far into the magneto-ionic manipulation of rare-earth transition-metal alloys have used electrochemical methods for evaluating the magnetoelectric properties, but this technique makes it difficult to discriminate between the effects of competing ionic species. In this work, we use atmospheric loading to evaluate the effect of an isotope of hydrogen, deuterium, on the magnetic properties of TbCo films using in-situ polarized neutron reflectometry. With this approach, we are able to simultaneously measure the magnetization, thickness expansion and deuterium concentration of TbCo films. We quantitatively observe the deuterium concentrations at which the paramagnetic phase transition occurs for a Tb-rich film, and the weakening of out-of-plane magnetic anisotropy for a Co-rich film. For the Tb-rich film the expansion of the film thickness is the primary mechanism identified for the paramagnetic phase transition, while for the Co-rich film no thickness expansion is observed. We also find that an oxidized interface is insensitive to deuterium loading, but remains exchange coupled to the rest of the film and can be indirectly manipulated by loading of deuterium in the alloy. We expect these results to be directly translatable to that of hydrogen.

cond-mat.mtrl-sci↗
arXiv2025

Long-Range Magnetic Order in Structurally Embedded Mesospin Metamaterials

Engineered assemblies of interacting magnetic elements-magnetic metamaterials-provide a powerful route to tailor collective magnetic order and dynamics. By structuring matter at the mesoscale, they bridge atomic magnetism and macroscopic functionality, enabling emergent behaviour inaccessible in conventional materials. However, realizing large-area metamaterials that combine high morphological uniformity with intrinsic long-range order has remained challenging, largely due to the structural disorder inherent to lithographic fabrication. Here we demonstrate a scalable route to structurally and magnetically coherent metamaterials by embedding iron-ions to form mesospins within a non-magnetic thin film palladium host matrix. Using controlled implantation, we realize morphologically uniform arrays that spontaneously develop extended antiferromagnetic order in the as-fabricated state - without the need of external annealing or field cycling. Resonant X-ray scattering and microscopy reveal sharp magnetic Bragg peaks modulated by the mesospin form factor, evidencing long-range antiferromagnetic order coupled to structural coherence. This embedded architecture establishes a platform for exploring coherent spin-photon interactions and functional X-ray scattering in magnetic metamaterials free from lithographic topography and disorder.

cond-mat.mes-hall↗
arXiv2025

Magnetic texture control in ion-implanted metamaterials

We study experimentally the impact of the additive fabrication method on the magnetic properties of Fe$^+$-implanted Pd square artificial spin ice lattices. Our findings show that the lattices exhibit a higher ordering temperature than their continuous film counterparts. This behavior is attributed to the additive fabrication process, which induces an inhomogeneous Fe concentration within the lattice building blocks. Moreover, the implantation process creates a magnetic depth profile, enabling temperature-dependent tunability of the magnetic thickness. These additional internal degrees of freedom broaden the design possibilities for magnetic metamaterials, allowing precise fine-tuning of their static and dynamic properties to achieve complex and customizable behaviors.

cond-mat.mes-hall↗
arXiv2024

Control of Ferrimagnetic Compensation and Perpendicular Anisotropy in Tb$_x$Co$_{(100-x)}$ with H$^{+}$ ion implantation

The tuning of magnetic properties through electrochemical loading of hydrogen has recently attracted significant interest as a way to manipulate magnetic devices with electric fields. In this paper we investigate quantitatively the magneto-ionic effect of hydrogen uptake on the magnetic properties of rare-earth transition metal alloy Tb$_x$Co$_{(100-x)}$ in the composition range of $x=10-39$ at.\% using ion implantation. Using this technique we are able to link changes in magnetic behaviour to exact concentrations of hydrogen, isolated from the movement of any other ions that would be a factor in electrochemical studies. The composition of the alloy has been varied alongside the hydrogen dose to characterize the effect of progressive hydrogen loading on the full range of $x$ displaying out-of-plane magnetic anisotropy. We find large changes in two important properties: the compensation composition and the Co-rich in-plane to out-of-plane magnetic anisotropy transition composition, both of which move by 6 at.\% towards higher Tb concentrations after hydrogen implantation. This shift in composition does not increase with a larger dose. From the changes in magnetization we attribute the change in compensation composition to a significant reduction of the moment on the Tb sublattice.

cond-mat.mtrl-sci↗
arXiv2024

Magnetic Order and Long-Range Interactions in Mesoscopic Ising Chains

We investigate the design of magnetic ordering in one-dimensional mesoscopic magnetic Ising chains by modulating long-range interactions. These interactions are affected by geometrical modifications to the chain, which adjust the energy hierarchy and the resulting magnetic ground states. Consequently, the magnetic ordering can be tuned between antiferromagnetic and dimer antiferromagnetic phases. These phases are experimentally observed in chains fabricated using both conventional electron-beam lithography and ion implantation techniques, demonstrating the feasibility of controlling magnetic properties at the mesoscale. The ability of attaining these magnetic structures by thermal annealing, underlines the potential of using such systems instead of simulated annealers in tackling combinatorial optimization tasks.

cond-mat.mes-hall↗
arXiv2024

Magnetic metamaterials by ion-implantation

We present a method for the additive fabrication of planar magnetic nanoarrays with minimal surface roughness. Synthesis is accomplished by combining electron-beam lithography, used to generate nanometric patterned masks, with ion implantation in thin films. By implanting $^{56}$Fe$^{+}$ ions, we are able to introduce magnetic functionality in a controlled manner into continuous Pd thin films, achieving 3D spatial resolution down to a few tens of nanometers. Our results demonstrate the application of this technique in fabricating square artificial spin ice lattices, which exhibit well-defined magnetization textures and interactions among the patterned magnetic elements.

cond-mat.mtrl-sci↗
arXiv2024

Modelling nanomagnet vertex dynamics through Coulomb charges

We investigate the magnetization dynamics in nanomagnet vertices often found in artificial spin ices. Our analysis involves creating a simplified model that depicts edge magnetization using magnetic charges. We utilize the model to explore the energy landscape, its associated curvatures, and the fundamental modes. Our study uncovers specific magnonic regimes and transitions between magnetization states, marked by zero-modes, which can be understood within the framework of Landau theory. To verify our model, we compare it with micromagnetic simulations, demonstrating a noteworthy agreement.

cond-mat.mes-hall↗
arXiv2023

Polymerization in magnetic metamaterials

We numerically study a mesoscopic system consisting of magnetic nanorings in the presence of thermal magnetization fluctuations. We find the formation of dipolar-field-mediated ``bonds" promoting the formation of annuli clusters, where the amount of bonds between two rings varies between zero and two. This system resembles the formation of polymers from artificial atoms, which in our case are the annuli and where the valency of the atom is set by the ring multipolarity. We investigate the thermodynamic properties of the resulting structures, and find a transition associated with the formation of the bonds. In addition, we find that the system has a tendency to form topological structures, with a distinct critical temperature in relation to the one for bond formation.

cond-mat.mes-hall↗