arXiv subjects

Mathias Kläui

Publications and source records attributed to Mathias Kläui.

At least 55 records · Page 3Linked to original sources

arXiv2025

Ultrafast electron heating as the dominant driving force of photoinduced terahertz spin currents

Ultrafast spintronics strongly relies on the generation, transport, manipulation and detection of terahertz spin currents (TSCs). In F|HM stacks consisting of a ferromagnetic layer F and a heavy-metal layer HM, ultrafast spin currents are typically triggered by femtosecond optical laser pulses. A key open question is whether the initial step, optical excitation and injection of spin currents, can be controlled by tuning the photon energy of the femtosecond pulse. While many theoretical works suggest a marked impact of photon-energy and of highly excited non-thermal electrons, profound experimental evidence is lacking. Here, we use terahertz-emission spectroscopy to study TSCs triggered with two different photon energies of 1.5 eV and 3 eV. We study a wide range of magnetic systems covering metallic ferromagnets, ferrimagnetic insulators, half-metals, as well as systems including tunneling barriers, and rare-earth metallic alloys. We find that variation of the exciting photon energy does not change the dynamics and only slightly the amplitude of the induced TSC in all sample systems. Our results reveal that the ultrafast pump-induced heating of electrons is a highly efficient process for generating TSCs, whereas highly excited primary photoelectrons are of minor importance.

cond-mat.mes-hall↗

arXiv2025

Non-reciprocity in magnon mediated charge-spin-orbital current interconversion

In magnetic systems, angular momentum is carried by spin and orbital degrees of freedom. Nonlocal devices, comprising heavy-metal nanowires on magnetic insulators like yttrium iron garnet (YIG), enable angular momentum transport via magnons. These magnons are polarized by spin accumulation at the interface through the spin Hall effect (SHE) and detected via the inverse SHE (iSHE). The processes are generally reciprocal, as demonstrated by comparable efficiencies when reversing injector and detector roles. However, introducing Ru, which enables the orbital Hall effect (OHE), disrupts this reciprocity. In our system, magnons polarized through combined SHE and OHE and detected via iSHE are 35% more efficient than the reverse process. We attribute this nonreciprocity to nonzero spin vorticity, resulting from varying electron drift velocities across the Pt/Ru interface. This study highlights the potential of orbital transport mechanisms in influencing angular momentum transport and efficiency in nonlocal spintronic devices.

cond-mat.mtrl-sci↗

arXiv2025

Identifying Switching of Antiferromagnets by Spin-Orbit Torques

Antiferromagnets are promising candidates for ultrafast spintronic applications, leveraging current-induced spin-orbit torques. However, experimentally distinguishing between different switching mechanisms of the staggered magnetization (Néel vector) driven by current pulses remains a challenge. In an exemplary study of the collinear antiferromagnetic compound Mn$_2$Au, we demonstrate that slower thermomagnetoelastic effects predominantly govern switching over a wide parameter range. In the regime of short current pulses in the nanosecond range, however, we observe fully Néel spin-orbit torque driven switching. We show that this ultrafast mechanism enables the complete directional alignment of the Néel vector by current pulses in device structures.

physics.app-ph↗

arXiv2025

Triplet superconductivity by the orbital Rashba effect at surfaces of elemental superconductors

It is often assumed that in a superconductor without spin-triplet pairing, the formation of unconventional spin-triplet densities requires the spin-orbit interaction in combination with either broken inversion symmetry or broken time-reversal symmetry. Here, we show from first principles the existence of supercurrent-driven spin triplet densities on the surface of a variety of simple superconducting materials without spin-orbit coupling. We are able to attribute this phenomenon to the superconducting non-relativistic orbital Rashba Edelstein effect. Furthermore, we find that the spin-orbit induced spin moment is one order of magnitude smaller than the orbital moment, and has a vanishing effect on the total magnitude of the induced triplet density. Our findings imply the existence of a route to generate spin-currents without the use of heavy metals. Additionally, as an orbital moment can couple directly to a magnetic field, it shows that orbital physics is the dominant term that drives the superconducting diode effect.

cond-mat.supr-con↗

arXiv2025

Manipulating magnetization by orbital current from a light metal Ti

The orbital Hall effect, which does not rely on the spin-orbit coupling, has recently emerged as a promising mechanism for electrically manipulating magnetization in thin-film ferromagnets. Despite its potential, direct experimental observation of magnetization switching driven by orbital currents has been challenging, primarily because there is no direct exchange coupling between orbital angular momentum and local spin based magnetic moments. In this study, we present a compensated design to directly probe the contribution of orbital currents in the most promising light metal titanium (Ti), where symmetric layer structures allow zeroing out of the net spin current. By varying the thickness of the Ti layer in Ti(t)/Pt/Co/Pt/Co/Pt multilayers, we demonstrate the ability to control the magnetization switching polarity. We deduce the orbital charge conversion efficiency of the Ti layer to be approximately 0.17. These findings not only confirm the presence of the orbital Hall effect in Ti but also suggest that orbital currents may be promising candidates for developing energy-efficient magnetic devices with enhanced performance and scalability.

cond-mat.mtrl-sci↗

arXiv2025

Identification of orbital pumping from spin pumping and rectification effects

The recently predicted mechanism of orbital pumping enables the generation of pure orbital current from a precessing ferromagnet (FM) without the need for electrical current injection. This orbital current can be efficiently injected into an adjacent nonmagnetic material (NM) without being hampered by electrical conductivity mismatch. However, experimentally identifying this novel effect presents significant challenges due to the substantial background contributions from spin pumping and spin rectification effects (SREs). In this work, we disentangle the effects of orbital pumping from spin pumping in bilayer structures composed of Nb/Ni and Nb/$\mathrm{Fe_{60}Co_{20}B_{20}}$ by observing a sign reversal of the measured voltage. This reversal arises from the competing signs of the spin and orbital Hall effects in the Nb. We establish methods to differentiate the pumping signal from SREs by analyzing the distinct angular dependence of the measured voltage and its spatial dependence relative to the radio frequency excitation source.

cond-mat.mtrl-sci↗

arXiv2025

Realizing Quantitative Quasiparticle Modeling of Skyrmion Dynamics in Arbitrary Potentials

We demonstrate fully quantitative Thiele model simulations of magnetic skyrmion dynamics on previously unattainable experimentally relevant large length and time scales by ascertaining the key missing parameters needed to calibrate the experimental and simulation time scales and current-induced forces. Our work allows us to determine complete spatial pinning energy landscapes that enable quantification of experimental studies of diffusion in arbitrary potentials within the Lifson-Jackson framework. Our method enables us to ascertain the time scales, and by isolating the effect of ultra-low current density (order $10^6 A/m^2$) generated torques we directly infer the total force acting on the skyrmion for a quantitative modelling.

cond-mat.stat-mech↗

arXiv2025

Orbital torques and orbital pumping in two-dimensional rare-earth dichalcogenides

The design of spin-orbit torque properties in two-dimensional (2D) materials presents one of the challenges of modern spintronics. In this context, 2D layers involving rare-earth ions $-$ which give rise to robust magnetism, exhibit pronounced orbital polarization of the states, and carry strong spin-orbit interaction $-$ hold particular promise. Here, we investigate ferromagnetic Janus H-phase monolayers of 4$f$-Eu rare-earth dichalcogenides EuSP, EuSSe, and EuSCl using first-principles calculations. We demonstrate that all compounds exhibit significant spin-orbit torques which originate predominantly in the colossal current-induced orbital response on the Eu $f$-electrons. Moreover, we demonstrate that the corresponding orbital torques can be used to drive strong in-plane currents of orbital angular momentum with non-trivial direction of orbital polarization. Our findings promote $f$-orbital-based 2D materials as a promising platform for in-plane orbital pumping and spin-orbit torque applications, and motivate further research on educated design of orbital properties for orbitronics with 2D materials.

cond-mat.mes-hall↗

arXiv2025

Simulating Bloch points using micromagnetic and Heisenberg models

Magnetic Bloch points (BPs) are highly confined magnetization configurations, that often occur in transient spin dynamics processes. However, opposing chiralities of adjacent layers for instance in a FeGe bilayer stack can stabilize such magnetic BPs at the layer interface. These BPs configurations are metastable and consist of two coupled vortices (one in each layer) with same circularity and opposite polarity. Each vortex is stabilized by opposite sign Dzyaloshinskii-Moriya interactions. This stabilization mechanism potentially opens the door towards BP-based spintronic applications. An open question, from a methodological point of view, is whether the Heisenberg (HB) model approach (atomistic model) as to be used to study such systems or if the -- computationally more efficient -- micromagnetic (MM) models can be used and still obtain robust results. We are modelling and comparing the energetics and dynamics of a stable BP obtained using both HB and MM approaches. We find that an MM description of a stable BP leads qualitatively to the same results as the HB description, and that an appropriate mesh discretization plays a more important role than the chosen model. Further, we study the dynamics by shifting the BP with an applied in-plane field and investigating the relaxation after switching the filed off abruptly. The precessional motion of coupled vortices in a BP state can be drastically reduced compared to a classical vortex, which may be also an interesting feature for fast and efficient devices. A recent study has shown that a bilayer stack hosting BPs can be used to retain information [1].

cond-mat.mtrl-sci↗

arXiv2025

Imaging Topological Defect Dynamics Mediating 2D Skyrmion Lattice Melting

Topological defects are the key feature mediating 2D phase transitions. However, both resolution and tunability have been lacking to access the dynamics of the transitions. With dynamic Kerr microscopy, we directly capture the melting of a confined 2D magnetic skyrmion lattice with high resolution in real-time and -space. Skyrmions in magnetic thin films are two-dimensional, topologically non-trivial quasi-particles that provide rich dynamics as well as unique tunability as an essential ingredient for controlling phase behavior: We tune the skyrmion size and effective temperature on the fly to drive the two-step melting through an intermediate hexatic regime between the solid lattice and the isotropic liquid. We quantify the characteristic occurrence of topological defects mediating the transitions and reveal the so-far inaccessible dynamics of the lattice dislocations. The full real-time and -space imaging reveals the diffusion coefficient of the dislocations, which we find to be orders of magnitudes higher than that of the skyrmions.

cond-mat.stat-mech↗

arXiv2024

Laser-induced helicity and texture-dependent switching of nanoscale stochastic domains in a ferromagnetic film

Controlling magnetic textures at ever smaller length and time scales is of key fundamental and technological interest. Achieving nanoscale control often relies on finding an external stimulus that is able to act on that small length scales, which is highly challenging. A promising alternative is to achieve nanoscale control using the inhomogeneity of the magnetic texture itself. Using a multilayered ferromagnetic Pt/Co/Pt thin-film structure as a model system, we employ a magnetic force microscope to investigate the change in magnetic nanotextures induced by circularly polarized picosecond laser pulses. Starting from a saturated magnetic state, we find stochastic nucleation of complex nanotextured domain networks. In particular, the growth of these domains depends not only on their macroscopic magnetization but also on the complexity of the domain texture. This helicity and texture-dependent effect contrasts with the typical homogeneous growth of magnetic domains initiated by an effective magnetic field of a circularly polarized laser pulse. We corroborate our findings with a stochastic model for the nucleation of magnetic domains, in which the nucleation and annihilation probability not only depends on the helicity of light but also on the relative magnetization orientation of neighboring domains. Our results establish a new approach to investigate ultrafast nanoscale magnetism and photo-excitation across first-order phase transitions.

cond-mat.mtrl-sci↗

arXiv2024

Spin Seebeck in the weak exchange coupled van der Waals antiferromagnet

Spin Seebeck effect (SSE) refers to the creation of spin currents due to a temperature gradient in the magnetic materials or across magnet-normal metal interfaces, which can be electrically detected through the inverse spin Hall effect (ISHE) when in contact with heavy metals. It offers fundamental insights into the magnetic properties of materials, including the magnetic phase transition, static magnetic order, and magnon excitations. However, the SSE in van der Waals antiferromagnet is still elusive, especially across the spin-flip transition. Here, we demonstrate the SSE in the weak exchange coupled van der Waals antiferromagnet CrPS$_4$. The SSE increases as the magnetic field increases before the spin-flip transition due to the enhancement of the thermal spin current as a function of the applied field. A peak of SSE is observed at the spin-flip field, which is related to the magnon mode edges across the spin-flip field. Our results extend SSE research to van der Waals antiferromagnets and demonstrate an enhancement of SSE at the spin-flip transition.

physics.app-ph↗

arXiv2024

All-optical magnetometric characterization of the antiferromagnetic exchange-spring system Mn$_2$Au|Py by terahertz spin-torques

Antiferromagnetic materials have great potential for spintronic applications at terahertz (THz) frequencies. However, in contrast to ferromagnets, experimental studies of antiferromagnets are often challenging due to a lack of straightforward external control of the Néel vector $\mathbf{L}$. Here, we study an AFM|FM stack consisting of an antiferromagnetic metal layer (AFM) of the novel material Mn2Au and a ferromagnetic metal layer (FM) of NiFe. In this exchange-spring system, $\mathbf{L}$ of AFM Mn2Au can be controlled by the application of an external magnetic field B_ext. To characterize the AFM|FM stack as a function of the quasi-static $\mathbf{B}_{\mathrm{ext}}$, we perform THz-pump magneto-optic probe experiments. We identify signal components that can consistently be explained by the in-plane antiferromagnetic magnon mode excited by field-like Néel spin-orbit torques (NSOTs). Remarkably, we find that the $\mathbf{B}_{\mathrm{ext}}$- and THz-pump-induced changes in the optical response of the sample are dominated exclusively by the spin degrees of freedom of AFM. We fully calibrate the magnetic circular and magnetic linear optical birefringence of AFM and extract the efficiency of the NSOTs. Finally, by selective excitation of domains with different orientation of $\mathbf{L}$, we are able to determine the relative volume fraction of 0°, 90°, 180° and 270° domains distribution during the quasi-static reversal of $\mathbf{L}$ by $\mathbf{B}_{\mathrm{ext}}$. Our insights are an important prerequisite for future studies of ultrafast coherent switching of spins by THz NSOTs and show that THz-pump magneto-optic-probe experiments are a powerful tool to characterize magnetic properties of antiferromagnets.

cond-mat.mes-hall↗

arXiv2024

Inductive detection of inverse spin-orbit torques in magnetic heterostructures

The manipulation of magnetization via Magnetic torques is one of the most important phenomena in spintronics. In thin films, conventionally, a charge current flowing in a heavy metal is used to generate transverse spin currents and to exert torques on the magnetization of an adjacent ferromagnetic thin film layer. Here, in contrast to the typically employed heavy metals, we study spin-to-charge conversion in ferromagnetic heterostructures with large spin-orbit interaction that function as the torque-generating layers. In particular, we chose perpendicular magnetic anisotropy (PMA) multilayers [Co/Ni] and [Co/Pt] as the torque-generating layers and drive magnetization dynamics in metallic ferromagnetic thin film $\mathrm{Co_{20}Fe_{60}B_{20}}$ (CoFeB) layers with in-plane magnetic anisotropy (IMA). We investigate the spin dynamics driven by spin-orbit torque (SOT) and the concomitant charge current generation by the inverse SOT process using an inductive technique based on a vector network analyzer. In our experimental findings, we find that the SOTs generated by our multilayers are of a magnitude comparable to those produced by Pt, consistent with first-principles calculations. Furthermore, we noted a significant correlation between the SOT and the thickness of the CoFeB layer.

cond-mat.mtrl-sci↗

arXiv2024

Experimental realization of metastable target skyrmion states in continuous films

Target skyrmions (TSks) are topological spin textures where the out-of-plane component of the magnetization twists an integer number of $m$-$π$ rotations. Based on a magnetic multilayer stack in the form of $n\times$[CoFeB/MgO/Ta], engineered to host topological spin textures via dipole and DMI energies, we have successfully stabilized 1$π$, 2$π$ and 3$π$ target skyrmions by tuning material properties and thermal excitations close to room temperature. The nucleated textures, imaged via Kerr and Magnetic Force Microscopies, are stable at zero magnetic field and robust within a range of temperatures (tens of Kelvin) close to room temperature (RT = 292 K) and over long time scales (months). Under applied field (mT), the TSks collapse into the central skyrmion core, which resists against higher magnetic fields ($\approx$ 2 $\times$ TSk annihilation field), as the core is topologically protected. Micromagnetic simulations support our experimental findings, showing no TSk nucleation at 0 K, but a $\approx$ 30 $\%$ probability at 300 K for the experimental sample parameters. Our work provides a simple method to tailor spin textures in continuous films, enabling free movement in 2D space, creating a platform transferable to technological applications where the dynamics of the topological textures can be exploited beyond geometrical confinements.

cond-mat.mtrl-sci↗

arXiv2024

The role of magnetic dipolar interactions in skyrmion lattices

Magnetic skyrmions are promising candidates for information and storage technologies. In the last years, magnetic multilayer systems have been tuned to enable room-temperature skyrmions, stable even in the absence of external magnetic field. There are several models describing the properties of an isolated skyrmion in a homogeneous background for single repetition multilayer stack, however, the description on how the equilibrium skyrmion size in lattices scales with increasing the number of repetitions of the stack remains unaddressed. This question is essential for fundamental and practical perspectives, as the behaviour of an ensemble of skyrmions differs from the isolated case. Based on a multilayer stack hosting a skyrmion lattice, we have carried out a series of imaging experiments scaling up the dipolar interaction by repeating $n$ times the multilayer unit, from $n =1$ up to $n=30$. We have developed an analytical description for the skyrmion radius in the whole multilayer regime, $i.e.$, from thin to thick film limits. Furthermore, we provide insight on how nucleation by an externally applied field can give rise to a lattice with more skyrmions (thus, overfilled) than the predicted by the calculations.

cond-mat.mtrl-sci↗

arXiv2024

Stabilizing perpendicular magnetic anisotropy with strong exchange bias in PtMn/Co by magneto-ionics

Electric field control of magnetic properties offers a broad and promising toolbox for enabling ultra-low power electronics. A key challenge with high technological relevance is to master the interplay between the magnetic anisotropy of a ferromagnet and the exchange coupling to an adjacent antiferromagnet. Here, we demonstrate that magneto-ionic gating can be used to achieve a very stable out-of-plane (OOP) oriented magnetization with strong exchange bias in samples with as-deposited preferred in-plane (IP) magnetization. We show that the perpendicular interfacial anisotropy can be increased by more than a factor 2 in the stack Ta/Pt/PtMn/Co/HfO2 by applying -2.5 V gate voltage over 3 nm HfO2, causing a reorientation of the magnetization from IP to OOP with a strong OOP exchange bias of more than 50 mT. Comparing two thicknesses of PtMn, we identify a notable trade-off: while thicker PtMn yields a significantly larger exchange bias, it also results in a slower response to ionic liquid gating within the accessible gate voltage window. These results pave the way for post-deposition electrical tailoring of magnetic anisotropy and exchange bias in samples requiring significant exchange bias.

cond-mat.mtrl-sci↗

arXiv2024

Harnessing Orbital Hall Effect in Spin-Orbit Torque MRAM

Spin-Orbit Torque (SOT) Magnetic Random-Access Memory (MRAM) devices offer improved power efficiency, nonvolatility, and performance compared to static RAM, making them ideal, for instance, for cache memory applications. Efficient magnetization switching, long data retention, and high-density integration in SOT MRAM require ferromagnets (FM) with perpendicular magnetic anisotropy (PMA) combined with large torques enhanced by Orbital Hall Effect (OHE). We have engineered PMA [Co/Ni]$_3$ FM on selected OHE layers (Ru, Nb, Cr) and investigated the potential of theoretically predicted larger orbital Hall conductivity (OHC) to quantify the torque and switching current in OHE/[Co/Ni]$_3$ stacks. Our results demonstrate a $\sim$30\% enhancement in damping-like torque efficiency with a positive sign for the Ru OHE layer compared to a pure Pt, accompanied by a $\sim$20\% reduction in switching current for Ru compared to pure Pt across more than 250 devices, leading to more than a 60\% reduction in switching power. These findings validate the application of Ru in devices relevant to industrial contexts, supporting theoretical predictions regarding its superior OHC. This investigation highlights the potential of enhanced orbital torques to improve the performance of orbital-assisted SOT-MRAM, paving the way for next-generation memory technology.

physics.app-ph↗