arXiv subjects

Mathias Weiler

Publications and source records attributed to Mathias Weiler.

At least 37 records · Page 2Linked to original sources

arXiv2023

Investigation of Spin-Wave Dynamics in Gyroid Nanostructures

A new concept in magnonics studies the dynamics of spin waves (SWs) in three-dimensional nanosystems. It is a natural evolution from conventionally used planar systems to explore magnetization configurations and dynamics in 3D nanostructures with lengths near intrinsic magnetic scales. In this work, we perform broadband ferromagnetic resonance (BBFMR) measurements and micromagnetic simulations of nanoscale magnetic gyroids - a periodic chiral structure consisting entirely of chiral triple junctions. Our results show unique properties of the network, such as the localization of the SW modes, evoking their topological properties, and the substantial sensitivity to the direction of the static magnetic field. The presented results open a wide range of applications in the emerging field of 3D magnonic crystals and spintronics.

cond-mat.mes-hall↗

arXiv2023

Symmetry and nonlinearity of spin wave resonance excited by focused surface acoustic waves

The use of a complex ferromagnetic system to manipulate GHz surface acoustic waves is a rich current topic under investigation, but the high-power nonlinear regime is under-explored. We introduce focused surface acoustic waves, which provide a way to access this regime with modest equipment. Symmetry of the magneto-acoustic interaction can be tuned by interdigitated transducer design which can introduce additional strain components. Here, we compare the impact of focused acoustic waves versus standard unidirectional acoustic waves in significantly enhancing the magnon-phonon coupling behavior. Analytical simulation results based on modified Landau-Lifshitz-Gilbert theory show good agreement with experimental findings. We also report nonlinear input power dependence of the transmission through the device. This experimental observation is supported by the micromagnetic simulation using mumax3 to model the nonlinear dependence. These results pave the way for extending the understanding and design of acoustic wave devices for exploration of acoustically driven spin wave resonance physics.

cond-mat.mtrl-sci↗

arXiv2023

Temperature dependent study of the spin dynamics of coupled Y$_3$Fe$_5$O$_{12}$/Gd$_3$Fe$_5$O$_{12}$/Pt trilayers

In this study, we investigate the dynamic response of a Y$_3$Fe$_5$O$_{12}$ (YIG)/ Gd$_3$Fe$_5$O$_{12}$ (GdIG)/ Pt trilayer system by measurements of the ferromagnetic resonance (FMR) and the pumped spin current detected by the inverse spin Hall effect. This trilayer system offers the unique opportunity to investigate the spin dynamics of the ferrimagnetic GdIG, close to its compensation temperature. We show that our trilayer acts as a highly tunable spin current source. Our experimental results are supported by micro-magnetic simulations. As the detected spin current in the top Pt layer is distinctly dominated by the GdIG layer, this gives the unique opportunity to investigate the excitation and dynamic properties of GdIG while comparing it to the broadband FMR absorption spectrum of the heterostructure.

cond-mat.mtrl-sci↗

arXiv2023

Coupling of ferromagnetic and antiferromagnetic spin dynamics in Mn$_{2}$Au/NiFe thin-film bilayers

We investigate magnetization dynamics of Mn$_{2}$Au/Py (Ni$_{80}$Fe$_{20}$) thin film bilayers using broadband ferromagnetic resonance (FMR) and Brillouin light scattering spectroscopy. Our bilayers exhibit two resonant modes with zero-field frequencies up to almost 40 GHz, far above the single-layer Py FMR. Our model calculations attribute these modes to the coupling of the Py FMR and the two antiferromagnetic resonance (AFMR) modes of Mn2Au. The coupling-strength is in the order of 1.6 T$\cdot$nm at room temperature for nm-thick Py. Our model reveals the dependence of the hybrid modes on the AFMR frequencies and interfacial coupling as well as the evanescent character of the spin waves that extend across the Mn$_{2}$Au/Py interface

cond-mat.mtrl-sci↗

arXiv2022

Hybrid magnetization dynamics in $\text{Cu}_\text{2}\text{OSeO}_\text{3}$/$\mathrm{NiFe}$ heterostructures

We investigate the coupled magnetization dynamics in heterostructures of a single crystal of the chiral magnet $\mathrm{Cu_2OSeO_3}$ (CSO) and a polycrystalline ferromagnet $\mathrm{NiFe}$ (Py) thin film using broadband ferromagnetic resonance (FMR) at cryogenic temperatures. We observe the excitation of a hybrid mode (HM) below the helimagnetic transition temperature of CSO. This HM is attributed to the spin dynamics at the CSO/Py interface. We study the HM by measuring its resonance frequencies for in plane rotations of the external magnetic field. We find that the HM exhibits dominantly four-fold anisotropy, in contrast to the FMR of CSO and Py.

cond-mat.mes-hall↗

arXiv2022

Parametric Excitation and Instabilities of Spin Waves driven by Surface Acoustic Waves

The parametric excitation of spin waves by coherent surface acoustic waves is demonstrated experimentally in metallic magnetic thin film structures. The involved magnon modes are analyzed with micro-focused Brillouin light scattering spectroscopy and complementary micromagnetic simulations combined with analytical modelling are used to determine the origin of the spin-wave instabilities. Depending on the experimental conditions, we observe spin-wave instabilities originating from different phonon-magnon and magnon-magnon scattering processes. Our results demonstrate that an efficient excitation of high amplitude, strongly nonlinear magnons in metallic ferromagnets is possible by surface acoustic waves, which opens novel ways to create micro-scaled nonlinear magnonic systems for logic and data processing that can profit from the high excitation efficiency of phonons using piezoelectricity.

cond-mat.other↗

arXiv2022

Reduced effective magnetization and damping by slowly-relaxing impurities in strained $γ$-$\mathrm{Fe_2O_3}$ thin films

We study the static and dynamic magnetic properties of epitaxially strained $γ$-$\mathrm{Fe_2O_3}$ (maghemite) thin films grown via pulsed-laser deposition on MgO substrates by SQUID magnetometry and cryogenic broadband ferromagnetic resonance experiments. SQUID magnetometry measurements reveal hysteretic magnetization curves for magnetic fields applied both in- and out of the sample plane. From the magnetization dynamics of our thin films, we find a small negative effective magnetization in agreement with a strain induced perpendicular magnetic anisotropy. Moreover, we observe a non-linear evolution of the ferromagnetic resonance-linewidth as function of the microwave frequency and explain this finding with a model based on slowly relaxing impurities, the so-called slow relaxor model. By investigating the magnetization dynamics in our maghemite thin films as a function of frequency and temperature, we can isolate the temperature dependent contribution of the slowly relaxing impurities to the resonance linewidth and, in particular, observe a sign change in the effective magnetization. This finding provides evidence for a transition of the magnetic anisotropy from a perpendicular easy axis to an easy in-plane anisotropy for reduced temperatures.

cond-mat.mes-hall↗

arXiv2022

Spin-wave frequency combs

We experimentally demonstrate the generation of spin-wave frequency combs based on the nonlinear interaction of propagating spin waves in a microstructured waveguide. By means of time and space-resolved Brillouin light scattering spectroscopy, we show that the simultaneous excitation of spin waves with different frequencies leads to a cascade of four-magnon scattering events which ultimately results in well-defined frequency combs. Their spectral weight can be tuned by the choice of amplitude and frequency of the input signals. Furthermore, we introduce a model for stimulated four-magnon scattering which describes the formation of spin-wave frequency combs in the frequency and time domain.

cond-mat.mes-hall↗

arXiv2021

Tunable Cooperativity in Coupled Spin--Cavity Systems

We experimentally study the tunability of the cooperativity in coupled spin--cavity systems by changing the magnetic state of the spin system via an external control parameter. As model system, we use the skyrmion host material Cu$_2$OSeO$_3$ coupled to a microwave cavity resonator. In the different magnetic phases we measure a dispersive coupling between the resonator and the magnon modes and model our results by using the input--output formalism. Our results show a strong tunability of the normalized coupling rate by magnetic field, allowing us to change the magnon--photon cooperativity from 1 to 60 at the phase boundaries of the skyrmion lattice state.

cond-mat.mes-hall↗

arXiv2021

Robust formation of nanoscale magnetic skyrmions in easy-plane thin film multilayers with low damping

We experimentally demonstrate the formation of room-temperature skyrmions with radii of about 25\,nm in easy-plane anisotropy multilayers with interfacial Dzyaloshinskii-Moriya interaction (DMI). We detect the formation of individual magnetic skyrmions by magnetic force microscopy and find that the skyrmions are stable in out-of-plane fields up to about 200 mT. We determine the interlayer exchange coupling as well as the strength of the interfacial DMI. Additionally, we investigate the dynamic microwave spin excitations by broadband magnetic resonance spectroscopy. From the uniform Kittel mode we determine the magnetic anisotropy and low damping $α_{\mathrm{G}} < 0.04$. We also find clear magnetic resonance signatures in the non-uniform (skyrmion) state. Our findings demonstrate that skyrmions in easy-plane multilayers are promising for spin-dynamical applications.

cond-mat.mtrl-sci↗

arXiv2021

Growth optimization of TaN for superconducting spintronics

We have optimized the growth of superconducting TaN thin films on \ch{SiO2} substrates via dc magnetron sputtering and extract a maximum superconducting transition temperature of $T_{\mathrm{c}}=5$ K as well as a maximum critical field $μ_0H_{\mathrm{c2}}=(13.8\pm0.1)$ T. To investigate the impact of spin-orbit interaction in superconductor/ferromagnet heterostructures, we then analyze the magnetization dynamics of both normal state and superconducting TaN/\ch{Ni80Fe20}(Permalloy, Py)-bilayers as a function of temperature using broadband ferromagnetic resonance (bbFMR) spectroscopy. The phase sensitive detection of the microwave transmission signal is used to quantitatively extract the inverse current-induced torques of the bilayers. The results are compared to our previous study on NbN/Py-bilayers. In the normal state of TaN, we detect a positive damping-like current-induced torque $σ_{\mathrm{d}}$ from the inverse spin Hall effect (iSHE) and a small field-like torque $σ_{\mathrm{f}}$ attributed to the inverse Rashba-Edelstein effect (iREE) at the TaN/Py-interface. In the superconducting state of TaN, we detect a negative $σ_{\mathrm{d}}$ attributed to the quasiparticle mediated inverse spin Hall effect (QMiSHE) and the unexpected manifestation of a large positive field-like $σ_{\mathrm{f}}$ of unknown origin matching our previous results for NbN/Py-bilayers.

cond-mat.mes-hall↗

arXiv2020

Nonreciprocal Dzyaloshinskii-Moriya magnetoacoustic waves

We study the interaction of surface acoustic waves with spin waves in ultra-thin CoFeB/Pt bilayers. Due to the interfacial Dzyaloshinskii-Moriya interaction (DMI), the spin wave dispersion is non-degenerate for oppositely propagating spin waves in CoFeB/Pt. In combination with the additional nonreciprocity of the magnetoacoustic coupling itself, highly nonreciprocal acoustic wave transmission through the magnetic film is observed. We systematically characterize the magnetoacoustic wave propagation in a thickness series of CoFeB($d$)/Pt samples as a function of magnetic field magnitude and direction, and at frequencies up to 7 GHz. We quantitatively model our results to extract the strength of the DMI and magnetoacoustic driving fields.

cond-mat.mes-hall↗

arXiv2020

High-throughput techniques for measuring the spin Hall effect

The spin Hall effect in heavy-metal thin films is routinely employed to convert charge currents into transverse spin currents and can be used to exert torque on adjacent ferromagnets. Conversely, the inverse spin Hall effect is frequently used to detect spin currents by charge currents in spintronic devices up to the terahertz frequency range. Numerous techniques to measure the spin Hall effect or its inverse were introduced, most of which require extensive sample preparation by multi-step lithography. To enable rapid screening of materials in terms of charge-to-spin conversion, suitable high-throughput methods for measuring the spin Hall angle are required. Here, we compare two lithography-free techniques, terahertz emission spectroscopy and broadband ferromagnetic resonance, to standard harmonic Hall measurements and theoretical predictions using the binary-alloy series Au$_x$Pt$_{1-x}$ as benchmark system. Despite being highly complementary, we find that all three techniques yield a spin Hall angle with approximately the same $x$~dependence, which is also consistent with first-principles calculations. Quantitative discrepancies are discussed in terms of magnetization orientation and interfacial spin-memory loss.

cond-mat.mes-hall↗

arXiv2020

Temperature-dependent spin-transport and current-induced torques in superconductor/ferromagnet heterostructures

We investigate the injection of quasiparticle spin currents into a superconductor via spin pumping from an adjacent FM layer.$\;$To this end, we use NbN/\ch{Ni80Fe20}(Py)-heterostructures with a Pt spin sink layer and excite ferromagnetic resonance in the Py-layer by placing the samples onto a coplanar waveguide (CPW). A phase sensitive detection of the microwave transmission signal is used to quantitatively extract the inductive coupling strength between sample and CPW, interpreted in terms of inverse current-induced torques, in our heterostructures as a function of temperature. Below the superconducting transition temperature $T_{\mathrm{c}}$, we observe a suppression of the damping-like torque generated in the Pt layer by the inverse spin Hall effect (iSHE), which can be understood by the changes in spin current transport in the superconducting NbN-layer. Moreover, below $T_{\mathrm{c}}$ we find a large field-like current-induced torque.

cond-mat.mes-hall↗

arXiv2020

Nonlinear losses in magnon transport due to four-magnon scattering

We report on the impact of nonlinear four-magnon scattering on magnon transport in microstructured Co25Fe75 waveguides with low magnetic damping. We determine the magnon propagation length with microfocused Brillouin light scattering over a broad range of excitation powers and detect a decrease of the attenuation length at high powers. This is consistent with the onset of nonlinear four-magnon scattering. Hence, it is critical to stay in the linear regime, when deriving damping parameters from the magnon propagation length. Otherwise, the intrinsic nonlinearity of magnetization dynamics may lead to a misinterpretation of magnon propagation lengths and, thus, to incorrect values of the magnetic damping of the system.

cond-mat.mtrl-sci↗

arXiv2020

Effect of interfacial oxidation layer in spin pumping experiments on Ni$_{80}$Fe$_{20}$/SrIrO$_3$ heterostructures

SrIrO$_3$ with its large spin-orbit coupling and low charge conductivity has emerged as a potential candidate for efficient spin-orbit torque magnetization control in spintronic devices. We here report on the influence of an interfacial oxide layer on spin pumping experiments in Ni$_{80}$Fe$_{20}$ (NiFe)/SrIrO$_3$ bilayer heterostructures. To investigate this scenario we have carried out broadband ferromagnetic resonance (BBFMR) measurements, which indicate the presence of an interfacial antiferromagnetic oxide layer. We performed in-plane BBFMR experiments at cryogenic temperatures, which allowed us to simultaneously study dynamic spin pumping properties (Gilbert damping) and static magnetic properties (such as the effective magnetization and magnetic anisotropy). The results for NiFe/SrIrO$_3$ bilayer thin films were analyzed and compared to those from a NiFe/NbN/SrIrO$_3$ trilayer reference sample, where a spin-transparent, ultra-thin NbN layer was inserted to prevent oxidation of NiFe. At low temperatures, we observe substantial differences in the magnetization dynamics parameters of these samples, which can be explained by an antiferromagnetic interfacial layer in the NiFe/SrIrO$_3$ bilayers.

cond-mat.mes-hall↗

arXiv2019

Spin transport in a magnetic insulator with zero effective damping

Applications based on spin currents strongly profit from the control and reduction of their effective damping and their transport properties. We here experimentally observe magnon mediated transport of spin (angular) momentum through a 13.4 nm thin yttrium iron garnet film with full control of the magnetic damping via spin-orbit torque. Above a critical spin-orbit torque, the fully compensated damping manifests itself as an increase of magnon conductivity by almost two orders of magnitude. We compare our results to theoretical expectations based on recently predicted current induced magnon condensates and discuss other possible origins of the observed critical behaviour.

cond-mat.mtrl-sci↗

arXiv2019

Exchange-enhanced Ultrastrong Magnon-Magnon Coupling in a Compensated Ferrimagnet

The ultrastrong coupling of (quasi-)particles has gained considerable attention due to its application potential and richness of the underlying physics. Coupling phenomena arising due to electromagnetic interactions are well explored. In magnetically ordered systems, the quantum-mechanical exchange-interaction should furthermore enable a fundamentally different coupling mechanism. Here, we report the observation of ultrastrong intralayer exchange-enhanced magnon-magnon coupling in a compensated ferrimagnet. We experimentally study the spin dynamics in a gadolinium iron garnet single crystal using broadband ferromagnetic resonance. Close to the ferrimagnetic compensation temperature, we observe ultrastrong coupling of clockwise and anticlockwise magnon modes. The magnon-magnon coupling strength reaches more than 30% of the mode frequency and can be tuned by varying the direction of the external magnetic field. We theoretically explain the observed phenomenon in terms of an exchange-enhanced mode-coupling mediated by a weak cubic anisotropy.

cond-mat.mtrl-sci↗