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Matias Kagias

Publications and source records attributed to Matias Kagias.

6 recordsLinked to original sources

Breaking order: Talbot effect with spinodal architectures

The Talbot effect describes the emergence of periodic patterns in perturbed propagating wave fields. The effect is well studied for perturbations from structurally coherent optics such as diffraction gratings. The emergence of freeform and metaoptical designs raises the question of whether comparable behavior can also be observed from complex, non-periodic structures. Here we demonstrate that stochastic structures inspired by recent metamaterial designs, display a strong Talbot-like behavior. Re-emergence of projected wavefronts through stochastic spinodal architectures at distinct propagation distances are proven theoretically and experimentally in the visible and hard X-ray regimes. A direct application of this phenomenon is X-ray dark-field imaging for characterizing artificial and natural meso-structured materials. Our work shows that spinodal X-ray optics effectively bridge the gap between the two opposing approaches in dark-field X-ray imaging that advocate for either spatially fully coherent (i.e gratings) or incoherent (i.e diffusers) optics. This opens opportunities for exploring a new dimension in the implementation of X-ray imaging methods. Given the impact and universality of the classical Talbot effect, we expect our work to enable new opportunities for characterizing and manipulating matter.

physics.optics

Photon density of states engineering with generative inverse design for scalable 3D photonic metamaterials

The photon density of states (pDOS) governs fundamental light matter interactions and is a critical parameter for designing next generation light driven technologies such as photocatalysis and solar energy harvesting. Achieving a target pDOS in 3D nanoarchitected structures remains challenging due to the nonlinear and non unique relationship between geometry and spectral response. Here, we present an end to end inverse design framework for tailoring the pDOS of 3D photonic metamaterials fabricated via the scalable nanofabrication approach of metasurface-based holographic lithography. A data driven forward surrogate model is constructed to predict frequency resolved pDOS spectra from metasurface diffraction parameters and lithographic thresholds. Inverse design is performed using a conditional generative adversarial network (cGAN) that generates candidate metasurface diffraction parameters for target pDOS features. 3D structures featuring high local pDOS were obtained across a broad normalized frequency range and consistently outperformed those in the original dataset. Structural analysis revealed that these high pDOS architectures fall into two predominant structural categories with similar rotational symmetry characteristics. Our work establishes the first inverse design strategy for 3D photonic metamaterials fabricated via holographic lithography.

physics.optics

High aspect ratio silicon structures by Displacement Talbot lithography and Bosch etching

Despite the fact that the resolution of conventional contact/proximity lithography can reach feature sizes down to ~0.5-0.6 micrometers, the accurate control of the linewidth and uniformity becomes already very challenging for gratings with periods in the range of 1-2 μm. This is particularly relevant for the exposure of large areas and wafers thinner than 300μm. If the wafer or mask surface is not fully flat due to any kind of defects, such as bowing/warpage or remaining topography of the surface in case of overlay exposures, noticeable linewidth variations or complete failure of lithography step will occur. We utilized the newly developed Displacement Talbot lithography to pattern gratings with equal lines and spaces and periods in the range of 1.0 to 2.4 μm. The exposures in this lithography process do not require contact between the mask and the wafer, which makes it essentially insensitive to surface planarity and enables exposures with very high linewidth uniformity on thin and even slightly deformed wafers. We demonstrated pattern transfer of such exposures into Si substrates by reactive ion etching using the Bosch process. An etching depth of 30 μm or more for the whole range of periods was achieved, which corresponds to very high aspect ratios up to 60:1. The application of the fabricated gratings in phase contrast x-ray imaging is presented.

physics.app-ph

Towards Sub-micrometer High Aspect Ratio X-ray Gratings by Atomic Layer Deposition of Iridium

X-ray grating interferometry is an excellent technique for X-ray phase contrast imaging and X-ray wavefront sensing with applications in materials science, biology and medical diagnosis. Among other requirements, the method depends on the availability of highly X-ray absorbing metallic gratings. Here, we report on the fabrication and characterization of high aspect ratio iridium gratings with a period of one micrometer and a depth of 30 micrometer combining deep reactive ion etching of silicon and atomic layer deposition of iridium. The implementation of such structures can greatly enhance the sensitivity of grating-based X-ray phase contrast imaging and thus, expand further its broad range of applications.

physics.app-ph

High aspect ratio metal microcasting by hot embossing for X-ray optics fabrication

Metal microstructured optical elements for grating-based X-ray phase-contrast interferometry were fabricated by using an innovative approach of microcasting: hot embossing technology with low melting temperature (280°C) metal alloy foils and silicon etched templates. A gold-tin alloy (80w%Au / 20w%Sn) was used to cast micro-gratings with pitch sizes in the range of 2 to 20 micrometers and depth of the structures up to 80 micrometers. The metal filling of the silicon template strongly depends on the wetting properties of the liquid metal on the groove surface. A thin metal wetting layer (20 nm of Ir or Au) was deposited before the casting in order to turn the template surface into hydrophilic with respect of the melted metal alloy. Temperature and pressure of the hot embossing process were optimized for a complete filling of the cavities in a low viscosity regime of the liquid metal, and for minimizing the shear force that might damage the silicon structures for small pitch grating. The new method has relevant advantages, such as being a low cost technique, fast and easily scalable to large area fabrication.

physics.app-ph

Anisotropic de Gennes narrowing in confined fluids

The collective diffusion of dense fluids in spatial confinement was studied by combining high-energy (21 keV) x-ray photon correlation spectroscopy and small-angle x-ray scattering from colloid-filled microfluidic channels. We found the structural relaxation in confinement to be slower compared to bulk. The collective dynamics is wave vector dependent, akin to de Gennes narrowing typically observed in bulk fluids. However, in stark contrast to bulk, the structure factor and de Gennes narrowing in confinement are anisotropic. These experimental observations are essential in order to develop a microscopic theoretical description of collective diffusion of dense fluids in confined geometries.

cond-mat.soft