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Mats Larsson

Publications and source records attributed to Mats Larsson.

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Data-Driven Predictive Control for Wide-Area Power Oscillation Damping

We study damping of inter-area oscillations in transmission grids using voltage-source-converter-based high-voltage direct-current (VSC-HVDC) links. Conventional power oscillation damping controllers rely on system models that are difficult to obtain in practice. Data-driven Predictive Control (DPC) addresses this limitation by replacing explicit models with data. We apply AutoRegressive with eXogenous inputs (ARX)-based predictive control and its Transient Predictive Control (TPC) variant, and compare them with Data-enabled Predictive Control (DeePC) and two standard model-based controllers. The methods are evaluated in simulation on a system exhibiting both inter-area and local oscillation modes. ARX-based predictive control and DeePC both achieve effective damping, while the ARX-based methods require less online computation. Using warm-started, pre-factorized operator-splitting solvers, ARX/TPC control actions are computed in less than 1ms. These results demonstrate that DPC is a viable approach for power-system oscillation damping for the given test case.

eess.SY

Wavelength-Dependent Photodissociation of Iodomethylbutane

Ultrashort XUV pulses of the Free-Electron-LASer in Hamburg (FLASH) were used to investigate laser-induced fragmentation patterns of the prototypical chiral molecule 1-iodo-2-methyl-butane (C$_5$H$_{11}$I) in a pump-probe scheme. Ion velocity-map images and mass spectra of optical-laser-induced fragmentation were obtained for subsequent FEL exposure with photon energies of 63 eV and 75 eV. These energies specifically address the iodine 4d edge of neutral and singly charged iodine, respectively. The presented ion spectra for two optical pump-laser wavelengths, i.e., 800 nm and 267 nm, reveal substantially different cationic fragment yields in dependence on the wavelength and intensity. For the case of 800-nm-initiated fragmentation, the molecule dissociates notably slower than for the 267-nm pump. The results underscore the importance of considering optical-laser wavelength and intensity in the dissociation dynamics of this prototypical chiral molecule that is a promising candidate for future studies of its asymmetric nature.

physics.chem-ph

Attosecond soft X-ray pulses generated by chirp-dispersed manipulation in an XFEL reveal nonlinear core-electron dynamics in neon

Free-electron lasers have demonstrated their capability of generating intense attosecond X-ray pulses, which are the key to studying electron dynamics at their natural time scale and in specifically targeted electronic states, but come at the expanse of complicated generation schemes and stochastic pulse shapes. Here, we demonstrate a novel and simple operation concept based on the manipulation of the electron-bunch chirp-dispersion and working with the full 4.5 MHz repetition rate at the European XFEL in Germany. With a high-fidelity single-shot temporal characterisation, we detect X-ray pulses with durations of down to 200 attoseconds and peak powers reaching into the terawatt regime at ~1 keV photon energy. As a direct application, we present simultaneous measurements of nonlinear X-ray-matter interaction via time-resolved electron spectroscopy. Using the derived temporal pulse information and restricting the durations to a regime where individual X-ray pulses are shorter than the single-core-hole life time in neon atoms, we reveal an otherwise hidden peak-intensity dependence in the nonlinear dynamics of double-core-hole formation. Our results open the field of attosecond science to the investigation of electronic processes not only in the ground state but also in systems driven far off their equilibrium. They shed light on highly transient intermediate steps in complex electronic dynamics and thus promise to help build the conceptual bridge between fundamental physical processes and chemical photo-reactions.

physics.optics

Opportunities for Gas-Phase Science at Short-Wavelength Free-Electron Lasers with Undulator-Based Polarization Control

Free-electron lasers (FELs) are the world's most brilliant light sources with rapidly evolving technological capabilities in terms of ultrabright and ultrashort pulses over a large range of accessible photon energies. Their revolutionary and innovative developments have opened new fields of science regarding nonlinear light-matter interaction, the investigation of ultrafast processes from specific observer sites, and approaches to imaging matter with atomic resolution. A core aspect of FEL science is the study of isolated and prototypical systems in the gas phase with the possibility of addressing well-defined electronic transitions or particular atomic sites in molecules. Notably for polarization-controlled short-wavelength FELs, the gas phase offers new avenues for investigations of nonlinear and ultrafast phenomena in spin orientated systems, for decoding the function of the chiral building blocks of life as well as steering reactions and particle emission dynamics in otherwise inaccessible ways. This roadmap comprises descriptions of technological capabilities of facilities worldwide, innovative diagnostics and instrumentation, as well as recent scientific highlights, novel methodology and mathematical modeling. The experimental and theoretical landscape of using polarization controllable FELs for dichroic light-matter interaction in the gas phase will be discussed and comprehensively outlined to stimulate and strengthen global collaborative efforts of all disciplines.

physics.atom-ph

Boundary Objects and their Use in Agile Systems Engineering

Agile methods are increasingly introduced in automotive companies in the attempt to become more efficient and flexible in the system development. The adoption of agile practices influences communication between stakeholders, but also makes companies rethink the management of artifacts and documentation like requirements, safety compliance documents, and architecture models. Practitioners aim to reduce irrelevant documentation, but face a lack of guidance to determine what artifacts are needed and how they should be managed. This paper presents artifacts, challenges, guidelines, and practices for the continuous management of systems engineering artifacts in automotive based on a theoretical and empirical understanding of the topic. In collaboration with 53 practitioners from six automotive companies, we conducted a design-science study involving interviews, a questionnaire, focus groups, and practical data analysis of a systems engineering tool. The guidelines suggest the distinction between artifacts that are shared among different actors in a company (boundary objects) and those that are used within a team (locally relevant artifacts). We propose an analysis approach to identify boundary objects and three practices to manage systems engineering artifacts in industry.

cs.SE

Dimethylsilanone generation from pyrolysis of polysiloxanes filled with nanosized silica and ceria/silica

Polydimethylsiloxane (PDMS) is a widely used organosilicon polymer often employed in formulations with fine oxide particles for various high temperature applications. Although PDMS is considered to be thermally stable and chemically inert, it is not always clear how the oxide filler influences its thermoresistance, decomposition chemistry and what reactive products are formed in the underlying thermal reactions. In this work we use temperature programmed desorption mass spectrometry (TPD MS) to study the pyrolysis of PDMS and its composites with nanosized silica and ceria/silica. Our results suggest that the elusive organosilicon compound - dimethylsilanone is generated from PDMS over a broad temperature range (in some cases starting at 70$°$C). The presence of nano-oxides catalyzed this process. Ions characteristic of the fragmentation of dimethylsilanone under electron ionization were assigned with the aid of DFT structure calculations. Possible reaction mechanisms for generating dimethylsilanone were discussed in the context of the calculated kinetic parameters. Observed accompanying products of PDMS pyrolysis, such as tetramethylcyclodisiloxane and hexamethylcyclotrisiloxane, indicate that multiple channels are involved in the dimethylsilanone release.

physics.chem-ph

Landau's Nobel Prize in Physics

Work of Lev Landau had a profound impact on the physics in 20th century. Landau had created the paradigms that had framed the conversations on the outstanding problems in physics for decades. He has laid the foundations for our understanding of quantum matter such as superfluidity, superconductivity and the theory of Fermi Liquid. Here we present sampled Nobel Archive data on the winning nomination that led to the Nobel Prize in Physics in 1962.

physics.hist-ph