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Matteo Ciardi

Publications and source records attributed to Matteo Ciardi.

15 recordsLinked to original sources

Static-Field Shielding of Bosonic Molecules: Evaporation to Degeneracy and Self-Bound Droplets

The strong, tunable dipolar interactions of ultracold molecules make them a powerful platform for quantum many-body physics, but reaching degeneracy by evaporative cooling requires suppressing inelastic collisions. Microwave collisional shielding has enabled the preparation of degenerate Fermi gases and Bose-Einstein condensates of polar molecules, whereas static electric field shielding has been limited to fermionic species, which are less prone to inelastic loss. We demonstrate static-field F\"{o}rster shielding of bosonic $^{23}$Na$^{87}$Rb molecules, suppressing two-body loss by up to four orders of magnitude. Within a bound-state-free electric-field window, three-body loss is also strongly suppressed, enabling efficient evaporation. Evaporating with an efficiency of 2.09(9), we increase the phase-space density of the gas by two orders of magnitude, reaching degeneracy with 7200(1000) molecules. We observe self-bound droplets at the end of evaporation over a wide range of field strengths, emerging from either degenerate or non-degenerate parent gases. We perform Path Integral Monte Carlo simulations, which suggest that the observed droplets are filamentary in nature, and find good agreement with the experimentally observed droplet formation temperatures. Our results establish F\"{o}rster shielding as a single-field route to prepare degenerate gases and self-bound droplets of bosonic polar molecules.

cond-mat.quant-gas

Equilibrium and non-equilibrium phases of microwave-dressed polar molecules beyond rotational symmetries

Recent experiments on molecular droplets have opened a new frontier of self-organization in strongly dipolar quantum matter. Microwave-dressing of polar molecules permits to tune both the strength and the angular structure of long-range interactions, potentially promoting a rich spectrum of quantum phases, from superfluid droplets with varying geometry and insulating or supersolid droplet arrays to strongly correlated crystals of individual molecules. Using path-integral Monte Carlo simulations of large molecular ensembles, we demonstrate that experimentally observed droplet arrays emerge as a metastable non-equilibrium state from the quenching of a gas-droplet phase transition under entirely broken rotational symmetry of the microwave-induced interaction potential. We moreover find that a crystalline phase of molecules, predicted for antidipolar interactions, is absent under conditions of recent experiments. This is traced back to the lack of angular symmetry in currently employed microwave-dressing, which qualitatively reshapes the many-body energy landscape and cannot be captured by effective scalar interaction parameters. Our results provide the first direct comparison of ab initio simulations and experiments and establish interaction anisotropy as a key aspect of molecular quantum gases.

cond-mat.quant-gas

Extended Bose-Hubbard Model on Small Grids: Exact Diagonalization and Monte Carlo Studies

The superfluid-insulator transition in systems of lattice bosons is usually analyzed in the framework of the Bose-Hubbard model, and has been extensively studied by theory and simulations. Less attention has been paid to the remnants of the transition in truncated lattices, with or without periodic boundary conditions. Here we consider the hard-core limit of the extended Bose-Hubbard model on small square and triangular grids -- i.e., sections of the square and triangular lattices containing up to 13 sites. By mapping out the zero-temperature phase diagram through exact diagonalization, we find ground-state characteristics that are markedly different from those emerging in the thermodynamic limit, together with similarities. The dichotomy between superfluid-like and insulating-like behavior is then investigated in two-dimensional systems of a few interacting bosons in the continuum, subject to confining and optical-lattice potentials mimicking the $3\times 3$ square grid. Using path-integral Monte Carlo simulations, we compute kinetic and potential energies, as well as superfluidity and exchange-cycle statistics, finding hints of Bose-Hubbard behavior even in systems of just five particles.

cond-mat.quant-gas

Bilayer crystals in a polar-molecules system

We investigate the finite-temperature phase diagram of polar molecules confined in a quasi-two-dimensional geometry by a harmonic potential along the polarization axis. We employ Quantum Monte Carlo simulations to explore the strongly correlated regime accessible with current experimental setups. By tuning temperature and confinement strength, we identify a rich set of phases, including normal fluid, superfluid, supersolid, cluster crystal, and bilayer crystal states. Our results reveal the emergence of crystallization upon increasing temperature, highlighting the nontrivial role of thermal fluctuations in dipolar systems. In particular, we show that a bilayer crystal with one molecule per lattice site can be stabilized by varying the confinement strength at fixed interaction. Moreover, we show evidence of layering of superfluid states with phase coherence between the two layers. These findings provide insight into the interplay between interactions, confinement, and temperature in low-dimensional dipolar systems, and suggest new directions for engineering quantum phases with ultracold polar molecules.

cond-mat.quant-gas

Layering and superfluidity of soft-core bosons in shallow spherical traps

Fundamental theories and models of many-body physics can be probed in experiments on ultracold atoms held in place by electromagnetic fields. In particular, of considerable interest are systems under curved confinement, since they can yield exotic states of matter which would be impossible to obtain in flat space. In this study we focus on relatively small samples, where curvature effects are stronger, and analyze by Monte Carlo simulations the peculiar structure arising in an assembly of soft-core bosons subject to a weak trapping potential with spherical symmetry. Upon suitable tuning of the parameters, a hundred particles or so group together in clusters arranged in a shell with icosahedral symmetry. As the number of particles increases, a second shell gradually develops, concentric to (and partly overlapping with) the original one, where clusters are in perfect registry with the first shell, thus forming a dodecahedral pattern. Cluster arrangements with the symmetry of other polyhedra are seen for different sets of parameters. At low temperature the superfluid density is non-uniform in the radial direction; heating the system progressively, superfluidity eventually vanishes while still clusters are present, a behavior resembling the transition from supersolid to normal solid on a plane. Two shells of clusters are also observed in systems of classical or distinguishable quantum particles, but in those cases the shells are more fragile to thermal fluctuations. All these behaviors can in principle be tested in systems of Rydberg-dressed atoms loaded into a bubble trap.

cond-mat.quant-gas

Strongly dipolar molecular Bose-Einstein condensates: From few- to many-body physics

Recent advances in molecular cooling have enabled the realization of strongly dipolar Bose--Einstein condensates (BECs) of molecules, and BECs of many different molecular species may become experimentally accessible in the near future. Here, we explore the unique properties of such BECs and the new insights they may offer into dipolar quantum fluids and many-body physics. We explore which parameter regimes can realistically be achieved using currently available experimental techniques, discuss how to implement these techniques, and outline which molecular species are particularly well suited to explore exotic new states of matter. We further determine how state-of-the-art beyond mean-field theories, originally developed for weakly dipolar magnetic gases, can be pushed to their limits and beyond, and what other long-standing questions in the field of dipolar physics may realistically come within reach using molecular systems.

cond-mat.quant-gas

Self-bound monolayer crystals of ultracold polar molecules

We investigate the physics of ultracold dipolar molecules using path-integral quantum Monte Carlo simulations, and construct the complete phase diagram extending from weak to strong interactions and from small to mesoscopic particle numbers. Our calculations predict the formation of self-bound quantum droplets at interaction strengths lower than previously anticipated. For stronger interactions, the droplet continuously loses superfluidity as correlations develop, and is eventually found to undergo a transition to a crystalline monolayer that remains self-bound without external confinement. The spontaneous formation of such two-dimensional phases from a three-dimensional quantum gas is traced back to the peculiar anisotropic form of the dipole-dipole interaction generated by microwave-dressing of rotational molecular states. For sufficiently large particle numbers, crystallization takes place for comparably low interaction strengths that do not promote two-body bound states and should thus be observable in ongoing experiments without limitations from three-body recombination.

cond-mat.quant-gas

Transitional supersolidity in ion doped helium droplets

$^4$He nanodroplets doped with an alkali ion feature a snowball of crystallized layers surrounded by superfluid helium. For large droplets, we predict that a transitional supersolid layer can form, bridging between the solid core and the liquid bulk, where the $^4$He density displays modulations of icosahedral group symmetry. To identify the different phases, we combine density functional theory with the semiclassical Gaussian time-dependent Hartree method for localized many-body systems. This hybrid approach can handle large particle numbers and provides insight into the physical origin of the supersolid layer. For small droplets, we verify that the predictions of our approach are in excellent agreement with Path-Integral Monte Carlo calculations.

cond-mat.quant-gas

Effects of gravity on supersolid order in bubble-trapped bosons

Unveiling the principles behind self-organization in quantum systems is of paramount importance, both intrinsically and practically, in view of foreseeable technological applications. Recently, increasing attention is being paid to atomic systems in curved geometries, which are a promising platform for the discovery of new emergent phenomena. A notable example is that of a gas of ultracold atoms loaded into a thin spherical shell, according to a protocol introduced by Zobay and Garraway more than twenty years ago. However, gravity prevents a dilute assembly of atoms from uniformly spreading throughout the shell, which explains why experiments on the condensation and superfluidity of bubble-trapped gases are usually conducted in space under microgravity conditions. In this paper, we focus instead on strongly-interacting quantum particles in a bubble trap, choosing the cluster supersolid of soft-core bosons as testbed. To study the impact of gravity on supersolid order, we consider a gedanken experiment in which the strength of gravity relative to the core repulsion is gradually enhanced. Using path integral Monte Carlo simulations, we trace the parallel evolution of system structure and superfluidity at low temperature, finding that the latter is sizeable only when gravity is a small perturbation or, at the other extreme, so strong that particles are all gathered in one cluster at the bottom of the trap. Finally, we assess the relevance of gravity for the equilibrium behavior of ultracold Rydberg-dressed atoms in a bubble trap, concluding that in some cases clues of the supersolid phase in the absence of gravity could be found even in a laboratory on Earth.

cond-mat.quant-gas

Path Integral Monte Carlo Study of a Doubly-Dipolar Bose Gas

By combining first-principles path integral Monte Carlo methods and mean-field techniques, we explore the properties of cylindrically trapped doubly-dipolar Bose gases. We first verify the emergence of a pancake quantum droplet at low temperatures, validating previously mean-field calculations. In a regime of small doubly-dipolar interactions, first-principles calculations agree with the generalized Gross-Pitaevskii equation. Such an accordance disappears in a large interaction limit. Here the path integral Monte Carlo estimates the strong doubly-dipolar regime with accuracy. On the contrary, the Gross-Pitaevskii equation does not seize quantum fluctuations in full. We also provide a complete description of the system's quantum behavior in a wide range of parameters. When the system forms a droplet, the superfluid fraction exhibits an anisotropic behavior if compared to the usual Bose gas regime. Interestingly, we observe that the transition temperature from thermal gas to droplet results higher than that of the thermal gas to a Bose-Einstein condensate, indicating the robustness of the droplet against thermal fluctuations. Further, we investigate the anisotropic behavior of the superfluid fraction during the structural transition from a pancake to a cigar-shaped droplet by varying the ratio between electric and magnetic dipole interaction strengths. Our findings furnish evidence that the stability of doubly-dipolar Bose-Einstein condensates can be detected in experiments by means of dysprosium atoms.

cond-mat.quant-gas

Self-induced Bose glass phase in quantum cluster quasicrystals

We study the emergence of Bose glass phases in self sustained bosonic quasicrystals induced by a pair interaction between particles of Lifshitz-Petrich type. By using a mean field variational method designed in momentum space as well as Gross-Pitaevskii simulations we determine the phase diagram of the model. The study of the local and global superfluid fraction allows the identification of supersolid, super quasicrystal, Bose glass and insulating phases. The Bose glass phase emerges as a quasicrystal phase in which the global superfluidity is essentially zero, while the local superfluidity remains finite in certain ring structures of the quasicrystalline pattern. Furthermore, we perform continuous space Path Integral Monte Carlo simulations for a case in which the interaction between particles stabilizes a quasicrystal phase. Our results show that as the strength of the interaction between particles is increased the system undergoes a sequence of states consistent with the super quasicrystal, Bose glass, and quasicrystal insulator thermodynamic phases.

cond-mat.quant-gas

Supersolid phases of bosonic particles in a bubble trap

Confinement can have a considerable effect on the behavior of particle systems, and is therefore an effective way to discover new phenomena. A notable example is a system of identical bosons at low temperature under an external field mimicking an isotropic bubble trap, which constrains the particles to a portion of space close to a spherical surface. Using Path Integral Monte Carlo simulations, we examine the spatial structure and superfluid fraction in two emblematic cases. First, we look at soft-core bosons, finding the existence of supersolid cluster arrangements with polyhedral symmetry; we show how different numbers of clusters are stabilized depending on the trap radius and the particle mass, and we characterize the temperature behavior of the cluster phases. A detailed comparison with the behavior of classical soft-core particles is provided too. Then, we examine the case, of more immediate experimental interest, of a dipolar condensate on the sphere, demonstrating how a quasi-one-dimensional supersolid of clusters is formed on a great circle for realistic values of density and interaction parameters. Crucially, this supersolid phase is only slightly disturbed by gravity. We argue that the predicted phases can be revealed in magnetic traps with spherical-shell geometry, possibly even in a lab on Earth. Our results pave the way for future simulation studies of correlated quantum systems in curved geometries.

cond-mat.quant-gas

Quasicrystalline Bose glass in the absence of disorder and quasidisorder

We study the low-temperature phases of interacting bosons on a two-dimensional quasicrystalline lattice. By means of numerically exact Path Integral Monte Carlo simulations, we show that for sufficiently weak interactions the system is a homogeneous Bose-Einstein condensate, which develops density modulations for increasing filling factor. The simultaneous occurrence of sizeable condensate fraction and density modulation can be interpreted as the analogous, in a quasicrystalline lattice, of supersolid phases occurring in conventional periodic lattices. For sufficiently large interaction strength and particle density, global condensation is lost and quantum exchanges are restricted to specific spatial regions. The emerging quantum phase is therefore a Bose Glass, which here is stabilized in the absence of any source of disorder or quasidisorder, purely as a result of the interplay between quantum effects, particle interactions and quasicrystalline substrate. This finding clearly indicates that (quasi)disorder is not essential to observe Bose Glass physics. Our results are of interest for ongoing experiments on (quasi)disorder-free quasicrystalline lattices.

cond-mat.dis-nn

Zonal estimators for quasiperiodic bosonic many-body phases

In this work, we explore the relevant methodology for the investigation of interacting systems with contact interactions, and we introduce a class of zonal estimators for path-integral Monte Carlo methods, designed to provide physical information about limited regions of inhomogeneous systems.We demonstrate the usefulness of zonal estimators by their application to a system of trapped bosons in a quasiperiodic potential in two dimensions, focusing on finite temperature properties across a wide range of values of the potential. Finally, we comment on the generalization of such estimators to local fluctuations of the particle numbers and to magnetic ordering in multi-component systems, spin systems, and systems with nonlocal interactions.

cond-mat.quant-gas

Finite-temperature phases of trapped bosons in a two-dimensional quasiperiodic potential

We study a system of 2D trapped bosons in a quasiperiodic potential via ab initio Path Integral Monte Carlo simulations, focusing on its finite temperature properties, which have not yet been explored. Alongside the superfluid, normal fluid and insulating phases, we demonstrate the existence of a Bose glass phase, which is found to be robust to thermal fluctuations, up to about half of the critical temperature of the non-interacting system. Local quantities in the trap are characterized by employing zonal estimators, allowing us to trace a phase diagram; we do so for a set of parameters within reach of current experiments with quasi-2D optical confinement.

cond-mat.quant-gas