arXiv subjects

Matteo Clerici

Publications and source records attributed to Matteo Clerici.

At least 19 recordsLinked to original sources

arXiv2026

Single-pump hybrid nonlinearities in transparent conductors

Low-index transparent conducting oxides have attracted significant attention because ultrafast optical excitation in these materials can induce exceptionally large temporal index gradients. Due to this remarkable nonlinear optical behaviour, this material platform enables sub-picosecond, all-optical control of photon energy and momentum, with growing relevance for integrated photonics, quantum optics, and optical computation. Owing to their hybrid electronic structure, transparent conductors exhibit both intraband and interband nonlinearities, previously accessed using dual-colour excitation with near-infrared and ultraviolet pumps. Here, we show that both excitation regimes can be activated using a single, intense near-infrared pump. Above a threshold intensity, the pump drives hot-electron intraband dynamics while simultaneously generating higher harmonics that trigger interband excitation. The interplay of these two effects sharpens the temporal features of the recorded transmissivity which in turn substantially broadens the effective material bandwidth. Finally, by comparing linear and circular pumping conditions, we further demonstrate that the observed interband nonlinearities originate from harmonic generation rather than from direct multiphoton absorption. Our results provide key insights into the strong-field optical response in these time-varying photonic materials, opening new frontiers for the ultra-fast manipulation of photons in both classic and quantum regimes.

physics.optics↗

arXiv2025

Quantum-enhanced second harmonic generation beyond the photon pairs regime

Two-photon processes are crucial in applications like microscopy and microfabrication, but their low cross-section requires intense illumination and limits, e.g., the penetration depth in nonlinear microscopy. Entangled states have been proposed to enhance the efficiency of two-photon interactions and have shown effectiveness at low intensities. This quantum enhancement is generally believed to be lost at high intensities, for more than one photon per mode, raising doubts about its usefulness. We explored experimentally and theoretically two-photon processes driven by entangled photons at intensities beyond this threshold and compared the results with the classical case. We found that a quantum advantage can still be observed at nearly one order of magnitude higher intensities than previously assumed. Our findings show a potential path for exploiting quantum-enhanced two-photon processes in practical applications.

quant-ph↗

arXiv2024

Polarization Purity and Dispersion Characteristics of Nested Antiresonant Nodeless Hollow-Core Optical Fiber at Near- and Short-wave-IR Wavelengths for Quantum Communications

Advancements in quantum communication and sensing require improved optical transmission that ensures excellent state purity and reduced losses. While free-space optical communication is often preferred, its use becomes challenging over long distances due to beam divergence, atmospheric absorption, scattering, and turbulence, among other factors. In the case of polarization encoding, traditional silica-core optical fibers, though commonly used, struggle with maintaining state purity due to stress-induced birefringence. Hollow core fibers, and in particular nested antiresonant nodeless fibers (NANF), have recently been shown to possess unparalleled polarization purity with minimal birefringence in the telecom wavelength range using continuous-wave (CW) laser light. Here, we investigate a 1-km NANF designed for wavelengths up to the 2-$\mu$m waveband. Our results show a polarization extinction ratio between ~-30 dB and ~-70 dB across the 1520 to 1620 nm range in CW operation, peaking at ~-60 dB at the 2-$\mu$m design wavelength. Our study also includes the pulsed regime, providing insights beyond previous CW studies, e.g., on the propagation of broadband quantum states of light in NANF at 2 $\mu$m, and corresponding extinction-ratio-limited quantum bit error rates (QBER) for prepare-measure and entanglement-based quantum key distribution (QKD) protocols. Our findings highlight the potential of these fibers in emerging applications such as QKD, pointing towards a new standard in optical quantum technologies.

physics.optics↗

arXiv2023

High-power sub-picosecond filamentation at 1.03 μm with high repetition rates between 10 and 100 kHz

Filamentation has extensively been explored and is well understood at repetition rates <1 kHz due to the typical availability of multi-mJ laser systems at a moderate average power. The advent of high-power Yb-lasers opened new possibilities for filamentation research. However, so far, high average power Yb systems have mostly been explored to increase the driving pulse energy to several hundreds of mJ and not at significantly higher repetition rates. In this paper, we study, for the first time, long filaments at unprecedented high repetition rates of 10, 40, and 100 kHz using a 500-W Yb-doped thin-disk amplifier driver operating with sub-700 fs pulses. We compare the filament length, density hole, and fluorescence at a constant peak power but different repetition rates and find a strong dependence on filament length and density depletion with repetition rate. Our analysis reveals the emergence of a significant stationary density depletion at repetition rates of 40 and 100 kHz. The corresponding reduction in the breakdown threshold by increasing the laser repetition rate observed in our study signifies a promising avenue for enhancing the efficiency and reliability of electric discharge triggering in various scenarios. Using capacitive plasma probe measurements, we address the limitations of fluorescence imaging-based measurements and demonstrate a systematic underestimation of filament length. This work contributes to a deeper understanding of the interplay between laser repetition rates, filamentation, and heat-driven density depletion effects from high-repetition-rate high-power laser systems and will contribute to guiding future research, making use of filaments at high repetition rates.

physics.optics↗

arXiv2022

Electro-Optical Sampling of Single-Cycle THz Fields with Single-Photon Detectors

Electro-optical sampling of Terahertz fields with ultrashort pulsed probes is a well-established approach for directly measuring the electric field of THz radiation. This technique usually relies on balanced detection to record the optical phase shift brought by THz-induced birefringence. The sensitivity of electro-optical sampling is, therefore, limited by the shot noise of the probe pulse, and improvements could be achieved using quantum metrology approaches using, e.g., NOON states for Heisenberg-limited phase estimation. We report on our experiments on THz electro-optical sampling using single-photon detectors and a weak squeezed vacuum field as the optical probe. Our approach achieves field sensitivity limited by the probe state statistical properties using phase-locked single-photon detectors and paves the way for further studies targeting quantum-enhanced THz sensing.

quant-ph↗

arXiv2022

An all-dielectric metasurface polarimeter

The polarization state of light is a key parameter in many imaging systems. For example, it can image mechanical stress and other physical properties that are not seen with conventional imaging, and can also play a central role in quantum sensing. However, polarization is more difficult to image and polarimetry typically involves several independent measurements with moving parts in the measurement device. Metasurfaces with interleaved designs have demonstrated sensitivity to either linear or circular/elliptical polarization states. Here we present an all-dielectric meta-polarimeter for direct measurement of any arbitrary polarization states from a single unit-cell design. By engineering a completely asymmetric design, we obtained a metasurface that can excite eigenmodes of the nanoresonators, thus displaying a unique diffraction pattern for not only any linear polarization state but all elliptical polarization states (and handedness) as well. The unique diffraction patterns are quantified into Stokes parameters with a resolution of 5$^{\circ}$ and with a polarization state fidelity of up to $99\pm1$%. This holds promise for applications in polarization imaging and quantum state tomography.

physics.optics↗

arXiv2021

Near-maximal two-photon entanglement for quantum communications at 2.1 $μ$m

Owing to a reduced solar background and low propagation losses in the atmosphere, the 2- to 2.5-$μ$m waveband is a promising candidate for daylight quantum communication. This spectral region also offers low losses and low dispersion in hollow-core fibers and in silicon waveguides. We demonstrate for the first time near-maximally entangled photon pairs at 2.1 $μ$m that could support device independent quantum key distribution (DIQKD) assuming sufficiently high channel efficiencies. The state corresponds to a positive secure-key rate (0.254 bits/pair, with a quantum bit error rate of 3.8%) based on measurements in a laboratory setting with minimal channel loss and transmission distance. This is promising for the future implementation of DIQKD at 2.1 $μ$m.

quant-ph↗

arXiv2020

Fast and slow nonlinearities in ENZ materials

Novel materials, with enhanced light-matter interaction capabilities, play an essential role in achieving the lofty goals of nonlinear optics. Recently, Epsilon-Near-Zero (ENZ) media have emerged as a promising candidate to enable the enhancement of several nonlinear processes including refractive index modulation and harmonic generation. Here, we analyze the optical nonlinearity of ENZ media to clarify the commonalities with other nonlinear media and its unique properties. We focus on transparent conducting oxides (TCOs) as the family of ENZ media with near zero permittivity in the near-infrared (telecom) band. We investigate the instantaneous and delayed nonlinearities. By identifying their common origin from the band nonparabolicity, we show that their relative strength is entirely determined by a ratio of the energy and momentum relaxation (or dephasing) times. Using this framework, we compare ENZ materials against the many promising nonlinear media that have been investigated in literature and show that while ENZ materials do not radically outpace the strength of traditional materials in either the fast or slow nonlinearity, they pack key advantages such as an ideal response time, intrinsic slow light enhancement, and broadband nature in a compact platform making them a valuable tool for ultrafast photonics applications for decades to come.

physics.optics↗

arXiv2020

Two-photon Quantum Interference and Entanglement at 2 μm

Quantum-enhanced optical systems operating within the 2- to 2.5-$μ$m spectral region have the potential to revolutionize emerging applications in communications, sensing, and metrology. However, to date, sources of entangled photons have been realized mainly in the near-infrared 700- to 1550-nm spectral window. Here, using custom-designed lithium niobate crystals for spontaneous parametric down-conversion and tailored superconducting nanowire single-photon detectors, we demonstrate two-photon interference and polarization-entangled photon pairs at 2090 nm. These results open the 2- to 2.5-$μ$m mid-infrared window for the development of optical quantum technologies such as quantum key distribution in next-generation mid-infrared fiber communication systems and future Earth-to-satellite communications.

quant-ph↗

arXiv2020

Adiabatic frequency shifting in epsilon near zero materials: The role of group velocity

We investigate adiabatic frequency conversion using epsilon near zero (ENZ) materials and show that while the maximum frequency conversion for a given change of permittivity does not exhibit increase in the vicinity of ε=0 condition. However, that change can be achieved in a shorter length, and if the pump is also in the ENZ vicinity, at a lower pump intensity. This slow propagation effect makes the conversion efficiency in the ENZ material comparable to that in microresonators and other structured slow light schemes, but unlike the latter no nanofabrication is required for ENZ materials which constitutes their major advantage over alternative frequency conversion approaches.

physics.optics↗

arXiv2019

Broad frequency shift of parametric processes in Epsilon-Near-Zero time-varying media

The ultrafast changes of material properties induced by short laser pulses can lead to frequency shift of reflected and transmitted radiation. Recent reports highlight how such a frequency shift is enhanced in the spectral regions where the material features a near-zero real part of the permittivity. Here we investigate the frequency shift for fields generated by four-wave mixing with a nonlinear polarisation oscillating at twice the pump frequency. In our experiment we observe a frequency shift of more than 60 nm (compared to the pulse width of ~40 nm) for the phase conjugated radiation generated by a 500 nm Aluminium-doped Zinc Oxide (AZO) film pumped close to the epsilon-near-zero wavelength. Our results indicate applications of time-varying media for nonlinear optics and frequency conversion.

physics.optics↗

arXiv2019

Polarisation and Transparency of Relativistically Rotating Two-Level Atoms

Electromagnetism and light-matter interaction in rotating systems is a rich area of ongoing research. We study the interaction of light with a gas of non-interacting two-level atoms confined to a rotating disk. We numerically solve the optical Bloch equations to investigate the how relativistic rotation affects the atoms' polarisation and inversion. The results are used to predict the steady-state stimulated emission seen by an observer at rest with the optical source in the laboratory frame. Competing physical effects due to time dilation and motion-induced detuning strongly modify solutions to the Bloch equations when the gas's velocity becomes relativistic. We account for the non-inertial motion by including acceleration-dependent excitation and emission rates, arising from a generalised Unruh effect. The effective thermal vacuum resulting from large accelerations de-polarises the gas while driving it towards population inversion, negating coherent driving due to the external light source. The results illustrate the intuitive, special-relativistic approach of assigning instantaneously comoving frames to understand non-inertial motion's influence when only local fields are physically significant.

physics.optics↗

arXiv2017

Towards On-Chip Integrated Optical Quantum Frequency Combs

Recent development in quantum photonics allowed to start the process of bringing photonic-quantum-based systems out of the lab into real world applications. As an example, devices for the exchange of a cryptographic key secured by the law of quantum mechanics are currently commercially available. In order to further boost this process, the next step is to migrate the results achieved by means of bulky and expensive setups to miniaturized and affordable devices. Integrated quantum photonics is exactly addressing this issue. In this paper we briefly review the most recent advancements in the generation of quantum states of light (at the core of quantum cryptography and computing) on chip. In particular, we focus on optical microcavities, as they can offer a solution to the issue of low efficiency (low number of photons generated) typical of the materials mostly used in integrated platforms. In addition, we show that specifically designed microcavities can also offer further advantages, such as compatibility with existing telecom standard (thus allowing to exploit the existing fiber network) and quantum memories (necessary in turns to extend the communication distance), as well as longitudinal multimode character. This last property (i.e. the increased dimensionality necessary for describing the quantum state of a photon) is achieved thanks to the generating multiple photon pairs on a frequency comb corresponding to the microcavity resonances. Further achievements include the possibility to fully exploit the polarization degree of freedom also for integrated devices. These results pave the way to the generation of integrated quantum frequency combs, that in turn may find application as quantum computing platform.

physics.optics↗

arXiv2017

Optical time reversal from time-dependent Epsilon-Near-Zero media

Materials with a spatially uniform but temporally varying optical response have applications ranging from magnetic field-free optical isolators to fundamental studies of quantum field theories. However, these effects typically become relevant only for time-variations oscillating at optical frequencies, thus presenting a significant hurdle that severely limits the realisation of such conditions. Here we present a thin-film material with a permittivity that pulsates (uniformly in space) at optical frequencies and realises a time-reversing medium of the form originally proposed by Pendry [Science 322, 71 (2008)]. We use an optically pumped, 500 nm thick film of epsilon-near-zero (ENZ) material based on Al-doped zinc oxide (AZO). An incident probe beam is both negatively refracted and time-reversed through a reflected phase-conjugated beam. As a result of the high nonlinearity and the refractive index that is close to zero, the ENZ film leads to time reversed beams (simultaneous negative refraction and phase conjugation) with near-unit efficiency and greater-than-unit internal conversion efficiency. The ENZ platform therefore presents the time-reversal features required e.g. for efficient subwavelength imaging, all-optical isolators and fundamental quantum field theory studies.

physics.optics↗

arXiv2016

Linearizing nonlinear optics

In the framework of linear optics, light fields do not interact with each other in a medium. Yet, when their field amplitude becomes comparable to the electron binding energies of matter, the nonlinear motion of these electrons emits new dipole radiation whose amplitude, frequency and phase differ from the incoming fields. Such high fields are typically achieved with ultra-short, femtosecond (1fs = 10-15 sec.) laser pulses containing very broad frequency spectra. Here, the matter not only couples incoming and outgoing fields but also causes different spectral components to interact and mix through a convolution process. In this contribution, we describe how frequency domain nonlinear optics overcomes the shortcomings arising from this convolution in conventional time domain nonlinear optics1. We generate light fields with previously inaccessible properties because the uncontrolled coupling of amplitudes and phases is turned off. For example, arbitrary phase functions are transferred linearly to the second harmonic frequency while maintaining the exact shape of the input power spectrum squared. This nonlinear control over output amplitudes and phases opens up new avenues for applications based on manipulation of coherent light fields. One could investigate c.f. the effect of tailored nonlinear perturbations on the evolution of discrete eigenmodes in Anderson localization2. Our approach might also open a new chapter for controlling electronic and vibrational couplings in 2D-spectroscopy3 by the geometrical optical arrangement.

physics.optics↗

arXiv2015

Observation of image pair creation and annihilation from superluminal scattering sources

The invariance of the speed of light implies a series of consequences related to our perception of simultaneity and of time itself. Whilst these consequences are experimentally well studied for subluminal speeds, the kinematics of superluminal motion lack direct evidence. Using high temporal resolution imaging techniques, we demonstrate that if a source approaches an observer at superluminal speeds, the temporal ordering of events is inverted and its image appears to propagate backwards. If the source changes its speed, crossing the interface between sub- and super-luminal propagation, we observe image pair annihilation and creation. These results show that it is not possible to unambiguously determine the kinematics of an event from imaging and time-resolved measurements alone.

physics.optics↗

arXiv2015

Two-dimensional materials and the coherent control of nonlinear optical interactions

Deeply sub-wavelength two-dimensional films may exhibit extraordinarily strong nonlinear effects. Here we show that 2D films exhibit the remarkable property of a phase-controllable nonlinearity, i.e., the amplitude of the nonlinear polarisation wave in the medium can be controlled via the pump beam phase and determines whether a probe beam will "feel" or not the nonlinearity. This is in stark contrast to bulk nonlinearites where propagation in the medium averages out any such phase dependence. We perform a series of experiments in graphene that highlight some of the consequences of the optical nonlinearity phase-dependence, {such as} the coherent control of nonlinearly diffracted beams, single-pump-beam {induced} phase-conjugation and the demonstration of a nonlinear mirror characterised by negative reflection. The observed phase sensitivity is not specific to graphene but rather is solely a result of the dimensionality and is therefore expected in all 2D materials.

physics.optics↗

arXiv2015

Experimental characterisation of nonlocal photon superfluids

Quantum gases of atoms and exciton-polaritons are nowadays a well established theoretical and experimental tool for fundamental studies of quantum many-body physics and suggest promising applications to quantum computing. Given their technological complexity, it is of paramount interest to devise other systems where such quantum many-body physics can be investigated at a lesser technological expense. Here we examine a relatively well-known system of laser light propagating through thermo-optical defocusing media: based on a hydrodynamical description of light as a quantum fluid of interacting photons, we investigate such systems as a valid, room temperature alternative to atomic or exciton-polariton condensates for studies of many-body physics. First, we show that by using a technique traditionally used in oceanography, it is possible to perform a direct measurement of the single-particle part of the dispersion relation of the elementary excitations on top of the photon fluid and to detect its global flow. Then, using a pump-and-probe set-up, we investigate the collective nature of low-wavevector sound modes of the fluid and observe signatures of superfluid behaviour.

physics.optics↗