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Matteo Savaresi

Publications and source records attributed to Matteo Savaresi.

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Strain-induced dynamic control over the population of quantum emitters in two-dimensional materials

The discovery of quantum emitters (QEs) in two-dimensional materials (2D) has triggered a surge of research to assess their suitability for quantum photonics. While their microscopic origin is still the subject of intense studies, position-controlled QEs are routinely fabricated using static strain gradients, which are used to drive excitons towards localized regions of the crystal where quantum light emission takes place. However, the use of strain in a dynamic fashion to control the brightness of single-photon sources in 2D materials has not been explored so far. In this work, we address this challenge by introducing a novel hybrid semiconductorpiezoelectric device in which WSe2 monolayers are integrated onto piezoelectric pillars that provide both static and dynamic strains. The static strains are first used to induce the formation of QEs, whose emission shows photon anti-bunching. Their energy and brightness are then controlled via the application of voltages to the piezoelectric pillars. Numerical simulations combined with drift-diffusion equations show that these effects are due to a strain-induced modification of the confining-potential landscape, which in turn leads to a net redistribution of excitons among the different QEs. Our work provides a method to dynamically control the brightness of single photon sources based on 2D materials.

cond-mat.mtrl-sci

Strain-tunable Single Photon Sources in WSe2 Monolayers

The appearance of single photon sources in atomically thin semiconductors holds great promises for the development of a flexible and ultra-compact quantum technology, in which elastic strain engineering can be used to tailor their emission properties. Here, we show a compact and hybrid 2D-semiconductor-piezoelectric device that allows for controlling the energy of single photons emitted by quantum emitters localized in wrinkled WSe2 monolayers. We demonstrate that strain fields exerted by the piezoelectric device can be used to tune the energy of localized excitons in WSe2 up to 18 meV in a reversible manner, while leaving the single photon purity unaffected over a wide range. Interestingly, we find that the magnitude and in particular the sign of the energy shift as a function of stress is emitter dependent. With the help of finite element simulations we suggest a simple model that explains our experimental observations and, furthermore, discloses that the type of strain (tensile or compressive) experienced by the quantum emitters strongly depends on their localization across the wrinkles. Our findings are of strong relevance for the practical implementation of single photon devices based on two-dimensional materials as well as for understanding the effects of strain on their emission properties.

cond-mat.mes-hall