arXiv subjects

Matthew Markham

Publications and source records attributed to Matthew Markham.

At least 37 records · Page 2Linked to original sources

arXiv2017

All-optical control of the silicon-vacancy spin in diamond at millikelvin temperatures

The silicon-vacancy center in diamond offers attractive opportunities in quantum photonics due to its favorable optical properties and optically addressable electronic spin. Here, we combine both to achieve all-optical coherent control of its spin states. We utilize this method to explore spin dephasing effects in an impurity-rich sample beyond the limit of phonon-induced decoherence: Employing Ramsey and Hahn-echo techniques at 12mK base temperature we identify resonant coupling to a substitutional nitrogen spin bath as the limiting decoherence source for the electron spin.

quant-ph↗

arXiv2017

Sub-millihertz magnetic spectroscopy with a nanoscale quantum sensor

Precise timekeeping is critical to metrology, forming the basis by which standards of time, length and fundamental constants are determined. Stable clocks are particularly valuable in spectroscopy as they define the ultimate frequency precision that can be reached. In quantum metrology, where the phase of a qubit is used to detect external fields, the clock stability is defined by the qubit coherence time, which determines the spectral linewidth and frequency precision. Here we demonstrate a quantum sensing protocol where the spectral precision goes beyond the sensor coherence time and is limited by the stability of a classical clock. Using this technique, we observe a precision in frequency estimation scaling in time $T$, as $T^{-3/2}$ for classical oscillating fields. The narrow linewidth magnetometer based on single spins in diamond is used to sense nanoscale magnetic fields with an intrinsic frequency resolution of 607 $μ$Hz, 8 orders of magnitude narrower than the qubit coherence time.

quant-ph↗

arXiv2017

Entanglement Distillation between Solid-State Quantum Network Nodes

The potential impact of future quantum networks hinges on high-quality quantum entanglement shared between network nodes. Unavoidable real-world imperfections necessitate means to improve remote entanglement by local quantum operations. Here we realize entanglement distillation on a quantum network primitive of distant electron-nuclear two-qubit nodes. We demonstrate the heralded generation of two copies of a remote entangled state through single-photon-mediated entangling of the electrons and robust storage in the nuclear spins. After applying local two-qubit gates, single-shot measurements herald the distillation of an entangled state with increased fidelity that is available for further use. In addition, this distillation protocol significantly speeds up entanglement generation compared to previous two-photon-mediated schemes. The key combination of generating, storing and processing entangled states demonstrated here opens the door to exploring and utilizing multi-particle entanglement on an extended quantum network.

quant-ph↗

arXiv2017

Coherent control of the silicon-vacancy spin in diamond

Spin impurities in diamond have emerged as a promising building block in a wide range of solid-state-based quantum technologies. The negatively charged silicon-vacancy centre combines the advantages of its high-quality photonic properties with a ground-state electronic spin, which can be read out optically. However, for this spin to be operational as a quantum bit, full quantum control is essential. Here, we report the measurement of optically detected magnetic resonance and the demonstration of coherent control of a single silicon-vacancy centre spin with a microwave field. Using Ramsey interferometry, we directly measure a spin coherence time, T2*, of 115 +/- 9 ns at 3.6 K. The temperature dependence of coherence times indicates that dephasing and decay of the spin arise from single phonon-mediated excitation between orbital branches of the ground state. Our results enable the silicon-vacancy centre spin to become a controllable resource to establish spin-photon quantum interfaces.

quant-ph↗

arXiv2016

Diamond optomechanical crystals

Cavity-optomechanical systems realized in single-crystal diamond are poised to benefit from its extraordinary material properties, including low mechanical dissipation and a wide optical transparency window. Diamond is also rich in optically active defects, such as the nitrogen-vacancy (NV) and silicon-vacancy (SiV) centers, which behave as atom-like systems in the solid state. Predictions and observations of coherent coupling of the NV electronic spin to phonons via lattice strain has motivated the development of diamond nanomechanical devices aimed at realization of hybrid quantum systems, in which phonons provide an interface with diamond spins. In this work, we demonstrate diamond optomechanical crystals (OMCs), a device platform to enable such applications, wherein the co-localization of ~ 200 THz photons and few to 10 GHz phonons in a quasi-periodic diamond nanostructure leads to coupling of an optical cavity field to a mechanical mode via radiation pressure. In contrast to other material systems, diamond OMCs operating in the resolved-sideband regime possess large intracavity photon capacity (> 10$^5$) and sufficient optomechanical coupling rates to reach a cooperativity of ~ 20 at room temperature, allowing for the observation of optomechanically induced transparency and the realization of large amplitude optomechanical self-oscillations.

cond-mat.mes-hall↗

arXiv2016

Spin dynamics of diamond nitrogen-vacancy centres at the ground state level anti-crossing and all-optical low frequency magnetic field sensing

We investigate the photo-induced spin dynamics of single nitrogen-vacancy (NV) centres in diamond near the electronic ground state level anti-crossing (GSLAC), which occurs at an axial magnetic field around 1024 G. Using optically detected magnetic resonance spectroscopy, we first find that the electron spin transition frequency can be tuned down to 100 kHz for the \NV{14} centre, while for the \NV{15} centre the transition strength vanishes for frequencies below about 2 MHz owing to the GSLAC level structure. Using optical pulses to prepare and readout the spin state, we observe coherent spin oscillations at 1024 G for the \NV{14}, which originate from spin mixing induced by residual transverse magnetic fields. This effect is responsible for limiting the smallest observable transition frequency, which can span two orders of magnitude from 100 kHz to tens of MHz depending on the local magnetic noise. A similar feature is observed for the \NV{15} centre at 1024 G. As an application of these findings, we demonstrate all-optical detection and spectroscopy of externally-generated fluctuating magnetic fields at frequencies from 8 MHz down to 500 kHz, using a \NV{14} centre. Since the Larmor frequency of most nuclear spin species lies within this frequency range near the GSLAC, these results pave the way towards all-optical, nanoscale nuclear magnetic resonance spectroscopy, using longitudinal spin cross-relaxation.

cond-mat.mes-hall↗

arXiv2016

Repeated quantum error correction on a continuously encoded qubit by real-time feedback

Reliable quantum information processing in the face of errors is a major fundamental and technological challenge. Quantum error correction protects quantum states by encoding a logical quantum bit (qubit) in multiple physical qubits. To be compatible with universal fault-tolerant computations, it is essential that the states remain encoded at all times and that errors are actively corrected. Here we demonstrate such active error correction on a continuously protected qubit using a diamond quantum processor. We encode a logical qubit in three long-lived nuclear spins, repeatedly detect phase errors by non-destructive measurements using an ancilla electron spin, and apply corrections on the encoded state by real-time feedback. The actively error-corrected qubit is robust against errors and multiple rounds of error correction prevent errors from accumulating. Moreover, by correcting correlated phase errors naturally induced by the environment, we demonstrate that encoded quantum superposition states are preserved beyond the dephasing time of the best physical qubit used in the encoding. These results establish a powerful platform for the fundamental investigation of error correction under different types of noise and mark an important step towards fault-tolerant quantum information processing.

quant-ph↗

arXiv2016

Quantum Zeno subspaces by repeated multi-spin projections

Repeated observations inhibit the coherent evolution of quantum states through the quantum Zeno effect. In multi-qubit systems this effect provides new opportunities to control complex quantum states. Here, we experimentally demonstrate that repeatedly projecting joint observables of multiple spins creates coherent quantum Zeno subspaces and simultaneously suppresses dephasing caused by the environment. We encode up to two logical qubits in these subspaces and show that the enhancement of the dephasing time with increasing number of projections follows a scaling law that is independent of the number of spins involved. These results provide new insights into the interplay between frequent multi-spin measurements and non-Markovian noise and pave the way for tailoring the dynamics of multi-qubit systems through repeated projections.

quant-ph↗

arXiv2016

Robust quantum-network memory using decoherence-protected subspaces of nuclear spins

The realization of a network of quantum registers is an outstanding challenge in quantum science and technology. We experimentally investigate a network node that consists of a single nitrogen-vacancy (NV) center electronic spin hyperfine-coupled to nearby nuclear spins. We demonstrate individual control and readout of five nuclear spin qubits within one node. We then characterize the storage of quantum superpositions in individual nuclear spins under repeated application of a probabilistic optical inter-node entangling protocol. We find that the storage fidelity is limited by dephasing during the electronic spin reset after failed attempts. By encoding quantum states into a decoherence-protected subspace of two nuclear spins we show that quantum coherence can be maintained for over 1000 repetitions of the remote entangling protocol. These results and insights pave the way towards remote entanglement purification and the realisation of a quantum repeater using NV center quantum network nodes.

quant-ph↗

arXiv2016

Ultrafast, all-optical coherent control of single silicon vacancy colour centres in diamond

Recently, the negatively charged silicon vacancy centre (SiV) in diamond has emerged as a novel promising system for quantum information processing (QIP) due to its superior spectral properties and advantageous electronic structure: The SiV offers an optically accessible Λ-type level structure with a large orbital level splitting even without the need of an external magnetic field and previous studies determined the ground state coherence time of the centre to be on the order of 35-45ns. While these studies already indicate the feasibility of an ultrafast all-optical coherent control of the SiV, no experimental realization has been presented so far. Here, we report on optical Rabi oscillations and Ramsey interference between the ground and the excited state of the SiV using 12 ps long, resonant rotation pulses. Moreover, utilizing a Λ-scheme, we demonstrate Raman-based coherent Rabi rotations and Ramsey interference within the ground state manifold using a single, 1ps long off-resonant pulse. These measurements prove the accessibility of the complete set of single-qubit operations relying solely on optical fields and pave the way for high-speed QIP applications using SiV centres.

quant-ph↗

arXiv2016

Quantum metrology enhanced by repetitive quantum error correction

The accumulation of quantum phase in response to a signal is the central mechanism of quantum sensing, as such, loss of phase information presents a fundamental limitation. For this reason approaches to extend quantum coherence in the presence of noise are actively being explored. Here we experimentally protect a room-temperature hybrid spin register against environmental decoherence by performing repeated quantum error correction whilst maintaining sensitivity to signal fields. We use a long-lived nuclear spin to correct multiple phase errors on a sensitive electron spin in diamond and realize magnetic field sensing beyond the timescales set by natural decoherence. The universal extension of sensing time, robust to noise at any frequency, demonstrates the definitive advantage entangled multi-qubit systems provide for quantum sensing and offers an important complement to quantum control techniques. In particular, our work opens the door for detecting minute signals in the presence of high frequency noise, where standard protocols reach their limits.

quant-ph↗

arXiv2016

Measuring nanoscale magnetic write head fields using a hybrid quantum register

The generation and control of nanoscale magnetic fields are of fundamental interest in material science and a wide range of applications. Nanoscale magnetic resonance imaging quantum spintronics for example require single spin control with high precision and nanoscale spatial resolution using fast switchable magnetic fields with large gradients. Yet, characterizing those fields on nanometer length scales at high band width with arbitrary orientation has not been possible so far. Here we demonstrate single electron and nuclear spin coherent control using the magnetic field of a hard disc drive write head. We use single electron spins for measuring fields with high spatial resolution and single nuclear spins for large band width measurements. We are able to derive field profiles from coherent spin Rabi oscillations close to GHz in fields with gradients of up to 10 mT/nm and measure all components of a static and dynamic magnetic field independent of its orientation. Our method paves the way for precision measurement of the magnetic fields of nanoscale write heads important for future miniaturization of the devices.

cond-mat.mes-hall↗

arXiv2015

Effect of Low-Damage Inductively Coupled Plasma on Shallow NV Centers in Diamond

Near-surface nitrogen-vacancy ({NV}) centers in diamond have been successfully employed as atomic-sized magnetic field sensors for external spins over the last years. A key challenge is still to develop a method to bring NV centers at nanometer proximity to the diamond surface while preserving their optical and spin properties. To that aim we present a method of controlled diamond etching with nanometric precision using an oxygen inductively coupled plasma (ICP) process. Importantly, no traces of plasma-induced damages to the etched surface could be detected by X-ray photoelectron spectroscopy (XPS) and confocal photoluminescence microscopy techniques. In addition, by profiling the depth of NV centers created by 5.0 keV of nitrogen implantation energy, no plasma-induced quenching in their fluorescence could be observed. Moreover, the developed etching process allowed even the channeling tail in their depth distribution to be resolved. Furthermore, treating a 12C isotopically purified diamond revealed a threefold increase in T2 times for NV centers with <4 nm of depth (measured by NMR signal from protons at the diamond surface) in comparison to the initial oxygen-terminated surface.

cond-mat.mtrl-sci↗

arXiv2015

Nanoimplantation and Purcell enhancement of single NV centers in photonic crystal cavities in diamond

We present the controlled creation of single nitrogen-vacancy (NV) centers via ion implantation at the center of a photonic crystal cavity which is fabricated in an ultrapure, single crystal diamond membrane. High-resolution placement of NV centers is achieved using collimation of a 5keV-nitrogen ion beam through a pierced tip of an atomic force microscope (AFM). We demonstrate coupling of the implanted NV centers' broad band fluorescence to a cavity mode and observe Purcell enhancement of the spontaneous emission. The results are in good agreement with a master equation model for the cavity coupling.

quant-ph↗

arXiv2014

All optical control of a single electron spin in diamond

Precise coherent control of the individual electronic spins associated with atom-like impurities in the solid state is essential for applications in quantum information processing and quantum metrology. We demonstrate all-optical initialization, fast coherent manipulation, and readout of the electronic spin of the negatively charged nitrogen-vacancy (NV$^-$) center in diamond at T$\sim$7K. We then present the observation of a novel double-dark resonance in the spectroscopy of an individual NV center. These techniques open the door for new applications ranging from robust manipulation of spin states using geometric quantum gates to quantum sensing and information processing.

quant-ph↗

arXiv2014

All-optical formation of coherent dark states of silicon-vacancy spins in diamond

Spin impurities in diamond can be versatile tools for a wide range of solid-state-based quantum technologies, but finding spin impurities which offer sufficient quality in both photonic and spin properties remains a challenge for this pursuit. The silicon-vacancy center has recently attracted a lot of interest due to its spin-accessible optical transitions and the quality of its optical spectrum. Complementing these properties, spin coherence is essential for the suitability of this center as a spin-photon quantum interface. Here, we report all-optical generation of coherent superpositions of spin states in the ground state of a negatively charged silicon-vacancy center using coherent population trapping. Our measurements reveal a characteristic spin coherence time, T2*, exceeding 250 nanoseconds at 4 K. We further investigate the role of phonon-mediated coupling between orbital states as a source of irreversible decoherence. Our results indicate the feasibility of all-optical coherent control of silicon-vacancy spins using ultrafast laser pulses.

quant-ph↗

arXiv2014

Unconditional quantum teleportation between distant solid-state qubits

Realizing robust quantum information transfer between long-lived qubit registers is a key challenge for quantum information science and technology. Here we demonstrate unconditional teleportation of arbitrary quantum states between diamond spin qubits separated by 3 meters. We prepare the teleporter through photon-mediated heralded entanglement between two distant electron spins and subsequently encode the source qubit in a single nuclear spin. By realizing a fully deterministic Bell-state measurement combined with real-time feed-forward we achieve teleportation in each attempt while obtaining an average state fidelity exceeding the classical limit. These results establish diamond spin qubits as a prime candidate for the realization of quantum networks for quantum communication and network-based quantum computing.

quant-ph↗

arXiv2012

Quantum interference of single photons from remote nitrogen-vacancy centers in diamond

We demonstrate quantum interference between indistinguishable photons emitted by two nitrogen-vacancy (NV) centers in distinct diamond samples separated by two meters. Macroscopic solid immersion lenses are used to enhance photon collection efficiency. Quantum interference is verified by measuring a value of the second-order cross-correlation function $g^{(2)}(0) = 0.35 \pm 0.04<0.5$. In addition, optical transition frequencies of two separated NV centers are tuned into resonance with each other by applying external electric fields. Extension of the present approach to generate entanglement of remote solid-state qubits is discussed.

quant-ph↗