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Matthias Althammer

Publications and source records attributed to Matthias Althammer.

At least 55 records · Page 3Linked to original sources

Spin transport in a magnetic insulator with zero effective damping

Applications based on spin currents strongly profit from the control and reduction of their effective damping and their transport properties. We here experimentally observe magnon mediated transport of spin (angular) momentum through a 13.4 nm thin yttrium iron garnet film with full control of the magnetic damping via spin-orbit torque. Above a critical spin-orbit torque, the fully compensated damping manifests itself as an increase of magnon conductivity by almost two orders of magnitude. We compare our results to theoretical expectations based on recently predicted current induced magnon condensates and discuss other possible origins of the observed critical behaviour.

cond-mat.mtrl-sci↗

High Spin-Wave Propagation Length Consistent with Low Damping in a Metallic Ferromagnet

We report ultra-low intrinsic magnetic damping in Co$_{\text{25}}$Fe$_{\text{75}}$ heterostructures, reaching the low $10^{-4}$ regime at room temperature. By using a broadband ferromagnetic resonance technique, we extracted the dynamic magnetic properties of several Co$_{\text{25}}$Fe$_{\text{75}}$-based heterostructures with varying ferromagnetic layer thickness. By estimating the eddy current contribution to damping, measuring radiative damping and spin pumping effects, we found the intrinsic damping of a 26\,nm thick sample to be $$α_{\mathrm{0}} \lesssim 3.18\times10^{-4}$. Furthermore, using Brillouin light scattering microscopy we measured spin-wave propagation lengths of up to $(21\pm1)\,\mathrm{μm}$ in a 26 nm thick Co$_{\text{25}}$Fe$_{\text{75}}$ heterostructure at room temperature, which is in excellent agreement with the measured damping.

cond-mat.mtrl-sci↗

Anomalous spin Hall angle of a metallic ferromagnet determined by a multiterminal spin injection/detection device

We report on the determination of the anomalous spin Hall angle in the ferromagnetic metal alloy cobalt-iron (Co$_{25}$Fe$_{75}$, CoFe). This is accomplished by measuring the spin injection/detection efficiency in a multiterminal device with nanowires of platinum (Pt) and CoFe deposited onto the magnetic insulator yttrium iron garnet (Y$_3$Fe$_5$O$_{12}$, YIG). Applying a spin-resistor model to our multiterminal spin transport data, we determine the magnon conductivity in YIG, the spin conductance at the YIG/CoFe interface and finally the anomalous spin Hall angle of CoFe as a function of its spin diffusion length in a single device. Our experiments clearly reveal a negative anomalous spin Hall angle of the ferromagnetic metal CoFe, but a vanishing ordinary spin Hall angle. This is in contrast to the results reported for the ferromagnetic metals Co and permalloy.

cond-mat.mes-hall↗

Spin-wave propagation in metallic CoFe films determined by microfocused frequency-resolved magneto-optic Kerr effect

We investigated the magnetization dynamics of a patterned Co$_{25}$Fe$_{75}$-based heterostructure with a novel optical measurement technique that we call microfocused frequency-resolved magneto optic Kerr effect ($μ$FR-MOKE). We measured the magnetic field dependence of the dynamical spin-wave susceptibility and recorded a spatial map of the spin-waves excited by a microwave antenna. We compare these results to those obtained on the same sample with the established microfocused Brillouin light scattering technique. With both techniques, we find a spin-wave propagation length of 5.6$μ$m at 10GHz. Furthermore, we measured the dispersion of the wavevector and the spin-wave propagation length as a function of the external magnetic field. These results are in good agreement with existing literature and with the employed Kalinkos-Slavin model.

cond-mat.mes-hall↗

Current direction anisotropy of the spin Hall magnetoresistance in nickel ferrite thin films with bulk-like magnetic properties

We utilize spin Hall magnetoresistance (SMR) measurements to experimentally investigate the pure spin current transport and magnetic properties of nickel ferrite (NiFe2O4,NFO)/normal metal (NM) thin film heterostructures. We use (001)-oriented NFO thin films grown on lattice-matched magnesium gallate substrates by pulsed laser deposition, which significantly improves the magnetic and structural properties of the ferrimagnetic insulator. The NM in our experiments is either Pt or Ta. A comparison of the obtained SMR magnitude for charge currents applied in the [100]- and [110]-direction of NFO yields a change of 50% for Pt at room temperature. We also investigated the temperature dependence of this current direction anisotropy and find that it is qualitatively different for the conductivity and the SMR magnitude. From our results we conclude that the observed current direction anisotropy may originate from an anisotropy of the spin mixing conductance or of the spin Hall effect in these Pt and Ta layers, and/or additional spin-galvanic contributions from the NFO/NM interface.

cond-mat.mes-hall↗

Pure spin currents in magnetically ordered insulator/normal metal heterostructures

Pure spin currents, i.e. the transport of angular momentum without an accompanying charge current, represent a new, promising avenue in modern spintronics from both a fundamental and an application point of view. Such pure spin currents can not only flow in electrical conductors via mobile charge carriers, but also in magnetically ordered electrical insulators as a flow of spin excitation quanta. Over the course of the last years remarkable results have been obtained in heterostructures consisting of magnetically ordered insulators interfaced with a normal metal, where a pure spin current flows across the interface. This topical review article deals with the fundamental principles, experimental findings and recent developments in the field of pure spin currents in magnetically ordered insulators. We here put our focus onto four different manifestations of pure spin currents in such heterostructures: The spin pumping effect, the longitudinal spin Seebeck effect, the spin Hall magnetoresistance and the all-electrical detection of magnon transport in non-local device concepts. In this article, we utilize a common theoretical framework to explain all four effects and explain important material systems (especially rare-earth iron garnets) used in the experiments. For each effect we introduce basic measurement techniques and detection schemes and discuss their application in the experiment. We account for the remarkable progress achieved in each field by reporting the recent progress in each field and by discussing research highlights obtained in our group. Finally, we conclude the review article with an outlook on future challenges and obstacles in the field of pure spin currents in magnetically ordered insulator / normal metal heterostructures.

cond-mat.mes-hall↗

Spin Hall magnetoresistance in antiferromagnet/heavy-metal heterostructures

We investigate the spin Hall magnetoresistance in thin film bilayer heterostructures of the heavy metal Pt and the antiferromagnetic insulator NiO. While rotating an external magnetic field in the easy plane of NiO, we record the longitudinal and the transverse resistivity of the Pt layer and observe an amplitude modulation consistent with the spin Hall magnetoresistance. In comparison to Pt on collinear ferrimagnets, the modulation is phase shifted by 90° and its amplitude strongly increases with the magnitude of the magnetic field. We explain the observed magnetic field-dependence of the spin Hall magnetoresistance in a comprehensive model taking into account magnetic field induced modifications of the domain structure in antiferromagnets. With this generic model we are further able to estimate the strength of the magnetoelastic coupling in antiferromagnets. Our detailed study shows that the spin Hall magnetoresistance is a versatile tool to investigate the magnetic spin structure as well as magnetoelastic effects, even in antiferromagnetic multidomain materials.

cond-mat.mes-hall↗

Magnetically Ordered Insulators for Advanced Spintronics

Magnetically ordered, electrically insulating materials pave the way towards novel spintronic devices. In these materials the flow of magnetic excitations such as magnons results in pure spin currents. These spin currents can be driven by gradients of the spin chemical potential and/or temperature such that they can play the same role in novel spintronic devices as charge currents in traditional electronic circuits. Connecting spin current based and charge current based devices requires spin to charge interconversion. This has been achieved by the spin Hall effect with an efficiency of several 10%. The recent progress in materials development and understanding of pure spin current physics opens up a plethora of novel device concepts and opportunities for fundamental studies.

physics.app-ph↗

Spin waves in coupled YIG/Co heterostructures

We investigate yttrium iron garnet (YIG)/cobalt (Co) heterostructures using broadband ferromagnetic resonance (FMR). We observe an efficient excitation of perpendicular standing spin waves (PSSWs) in the YIG layer when the resonance frequencies of the YIG PSSWs and the Co FMR line coincide. Avoided crossings of YIG PSSWs and the Co FMR line are found and modeled using mutual spin pumping and exchange torques. The excitation of PSSWs is suppressed by a thin aluminum oxide (AlOx) interlayer but persists with a copper (Cu) interlayer, in agreement with the proposed model.

cond-mat.mes-hall↗

Observation of the spin Nernst effect

The observation of the spin Hall effect triggered intense research on pure spin current transport. With the spin Hall effect, the spin Seebeck effect, and the spin Peltier effect already observed, our picture of pure spin current transport is almost complete. The only missing piece is the spin Nernst (-Ettingshausen) effect, that so far has only been discussed on theoretical grounds. Here, we report the observation of the spin Nernst effect. By applying a longitudinal temperature gradient, we generate a pure transverse spin current in a Pt thin film. For readout, we exploit the magnetization-orientation-dependent spin transfer to an adjacent Yttrium Iron Garnet layer, converting the spin Nernst current in Pt into a controlled change of the longitudinal thermopower voltage. Our experiments show that the spin Nernst and the spin Hall effect in Pt are of comparable magnitude, but differ in sign, as corroborated by first-principles calculations.

cond-mat.mes-hall↗

Magnon mode selective spin transport in compensated ferrimagnets

We investigate the generation of magnonic thermal spin currents and their mode selective spin transport across interfaces in insulating, compensated ferrimagnet/normal metal bilayer systems. The spin Seebeck effect signal exhibits a non-monotonic temperature dependence with two sign changes of the detected voltage signals. Using different ferrimagnetic garnets, we demonstrate the universality of the observed complex temperature dependence of the spin Seebeck effect. To understand its origin, we systematically vary the interface between the ferrimagnetic garnet and the metallic layer, and by using different metal layers we establish that interface effects play a dominating role. They do not only modify the magnitude of the spin Seebeck effect signal but in particular also alter its temperature dependence. By varying the temperature, we can select the dominating magnon mode and we analyze our results to reveal the mode selective interface transmission probabilities for different magnon modes and interfaces. The comparison of selected systems reveals semi-quantitative details of the interfacial coupling depending on the materials involved, supported by the obtained field dependence of the signal.

cond-mat.mtrl-sci↗

Impact of the interface quality of Pt/YIG(111) hybrids on their spin Hall magnetoresistance

We study the influence of the interface quality of Pt/Y$_3$Fe$_5$O$_{12}$(111) hybrids on their spin Hall magnetoresistance. This is achieved by exposing Y$_3$Fe$_5$O$_{12}$(111) single crystal substrates to different well-defined surface treatments prior to the Pt deposition. The quality of the Y$_3$Fe$_5$O$_{12}$(YIG) surface, the Pt/YIG interface and the Pt layer is monitored \textit{in-situ} by reflection high-energy electron diffraction and Auger electron spectroscopy as well as \textit{ex-situ} by atomic force microscopy and x-ray diffraction. To identify the impact of the different surface treatments on the spin Hall magnetoresistance, angle-dependent magnetoresistance measurements are carried out at room temperature. The largest spin Hall magnetoresistance is found in Pt/YIG fabricated by a two-step surface treatment consisting of a "piranha" etch process followed by an annealing step at $500^\circ$C in pure oxygen atmosphere. Our data suggest that the small SMR in Pt/YIG without any surface treatments of the YIG substrate prior to Pt deposition is caused by a considerable carbon agglomeration at the Y$_3$Fe$_5$O$_{12}$ surface.

cond-mat.mes-hall↗

Pure spin current transport in gallium doped zinc oxide

We study the flow of a pure spin current through zinc oxide by measuring the spin Hall magnetoresistance (SMR) in thin film trilayer samples consisting of bismuth-substituted yttrium iron garnet (Bi:YIG), gallium-doped zinc oxide (Ga:ZnO), and platinum. We investigate the dependence of the SMR magnitude on the thickness of the Ga:ZnO interlayer and compare to a Bi:YIG/Pt bilayer. We find that the SMR magnitude is reduced by almost one order of magnitude upon inserting a Ga:ZnO interlayer, and continuously decreases with increasing interlayer thickness. Nevertheless, the SMR stays finite even for a $12\;\mathrm{nm}$ thick Ga:ZnO interlayer. These results show that a pure spin current indeed can propagate through a several nm-thick degenerately doped zinc oxide layer. We also observe differences in both the temperature and the field dependence of the SMR when comparing tri- and bilayers. Finally, we compare our data to predictions of a model based on spin diffusion. This shows that interface resistances play a crucial role for the SMR magnitude in these trilayer structures.

cond-mat.mes-hall↗

Investigation of the tunnel magnetoresistance in junctions with a strontium stannate barrier

We experimentally investigate the structural, magnetic and electrical transport properties of La$_{0.67}$Sr$_{0.33}$MnO$_{3}$ based magnetic tunnel junctions with a SrSnO$_3$ barrier. Our results show that despite the large number of defects in the strontium stannate barrier, due to the large lattice mismatch, the observed tunnel magnetoresistance is comparable to tunnel junctions with a better lattice matched STiO$_3$ barrier, reaching values of up to 350% at T=5 K. Further analysis of the current-voltage characteristics of the junction and the bias voltage dependence of the observed tunnel magnetoresistance show a decrease of the TMR with increasing bias voltage. In addition, the observed TMR vanishes for T>200 K. Our results suggest that by employing a better lattice matched ferromagnetic electrode and thus reducing the structural defects in the strontium stannate barrier even larger TMR ratios might be possible in the future.

cond-mat.mes-hall↗

Spin Hall Magnetoresistance in a Canted Ferrimagnet

We study the spin Hall magnetoresistance effect in ferrimagnet/normal metal bilayers, comparing the response in collinear and canted magnetic phases. In the collinear magnetic phase, in which the sublattice magnetic moments are all aligned along the same axis, we observe the conventional spin Hall magnetoresistance. In contrast, in the canted phase, the magnetoresistance changes sign. Using atomistic spin model calculations of the magnetic configuration, we show that the electric transport for the different magnetic phases can be rationalized considering the individual sublattice moment orientations. This enables a magneto-transport based investigation of non-collinear magnetic textures.

cond-mat.mes-hall↗

Theory of spin Hall magnetoresistance (SMR) and related phenomena

We review the recently discovered spin Hall magnetoresistance (SMR) and related effects from a theoretical point of view. The SMR is observed in bilayers of a magnetic insulator and a metal, in which spin currents aregenerated in the normal metal due to the spin Hall effect. The associated angular momentum transfer to the ferromagnetic layer and thereby the electrical resistance is modulated by the angle between the applied current and the magnetization direction. The SMR provides a convenient tool to non-invasively measure the magnetization direction and spin-transfer torque to an insulator. We introduce the minimal theoretical instruments to calculate the SMR, i.e. spin diffusion theory and quantum mechanical boundary conditions. This leads to a small set of parameters that can be fitted to experiments. We discuss the limitations of the theory as well as alternative mechanisms such as the ferromagnetic proximity effect and Rashba spin-orbit torques, and point out new developments related to the SMR.

cond-mat.mtrl-sci↗

Non-local magnetoresistance in YIG/Pt nanostructures

We study the local and non-local magnetoresistance of thin Pt strips deposited onto yttrium iron garnet. The local magnetoresistive response, inferred from the voltage drop measured along one given Pt strip upon current-biasing it, shows the characteristic magnetization orientation dependence of the spin Hall magnetoresistance. We simultaneously also record the non-local voltage appearing along a second, electrically isolated, Pt strip, separated from the current carrying one by a gap of a few 100 nm. The corresponding non-local magnetoresistance exhibits the symmetry expected for a magnon spin accumulation-driven process, confirming the results recently put forward by Cornelissen et al. [1]. Our magnetotransport data, taken at a series of different temperatures as a function of magnetic field orientation, rotating the externally applied field in three mutually orthogonal planes, show that the mechanisms behind the spin Hall and the non-local magnetoresistance are qualitatively different. In particular, the non-local magnetoresistance vanishes at liquid Helium temperatures, while the spin Hall magnetoresistance prevails.

cond-mat.mtrl-sci↗

Longitudinal spin Seebeck effect contribution in transverse spin Seebeck effect experiments in Pt/YIG and Pt/NFO

We investigate the inverse spin Hall voltage of a 10nm thin Pt strip deposited on the magnetic insulators Y3Fe5O12 (YIG) and NiFe2O4 (NFO) with a temperature gradient in the film plane. We observe characteristics typical of the spin Seebeck effect, although we do not observe a change of sign of the voltage at the Pt strip when it is moved from hot to cold side, which is believed to be the most striking feature of the transverse spin Seebeck effect. Therefore, we relate the observed voltages to the longitudinal spin Seebeck effect generated by a parasitic out-of-plane temperature gradient, which can be simulated by contact tips of different material and heat conductivities and by tip heating. This work gives new insights into the interpretation of transverse spin Seebeck effect experiments, which are still under discussion.

cond-mat.mtrl-sci↗