arXiv subjects

Matthias Bickermann

Publications and source records attributed to Matthias Bickermann.

4 recordsLinked to original sources

arXiv2026

Generation of continuous-wave laser light at 148.4 nm using cavity-enhanced second harmonic generation in $BaMgF_4$

We experimentally investigate the potential of $BaMgF_4$ crystals to create a continuous-wave (CW) solid state laser at the vacuum ultraviolet (VUV) wavelength of 148.4 nm via cavity-enhanced second harmonic generation. This investigation is motivated by the development of a nuclear optical clock based on a transition between the ground and isomeric state in the $^{229}Th$ nucleus. For this purpose, a $BaMgF_4$ crystal was grown, optically polished and periodically poled. The crystal was inserted into a power-enhancement cavity, resonant at the fundamental wavelength of 296.8 nm and the generated laser light at 148.4 nm was characterized. Within this proof-of-concept investigation, a VUV output power of typically ($16\pm1$) pW is obtained. This marks the first time that this type of crystal is used to generate VUV laser light. The experimental findings are compared to theoretical expectations and provide a clear path for future improvements.

physics.optics↗

arXiv2024

Evaluation and thermodynamic optimization of phase diagram of lithium niobate tantalate solid solutions

The phase diagram of the lithium niobate and lithium tantalate solid solutions was investigated using experimental data from differential thermal analysis (DTA) and crystal growth. We used XRF analysis to determine the elemental composition of crystals. Based on the Neumann-Kopp rule, essential data of end members lithium niobate (LN) and lithium tantalate (LT) was created. The heats of fusion of end members given by DTA measurements of LN (103 kJ/mol at 1531 K) and LT (289 kJ/mol at 1913 K) were given as input parameters to generate the data. This data served as the basis for calculating a phase diagram for LN and LT solid solutions. Finally, based on the experimental data and thermodynamic solution model, the phase diagram was optimized in the Calphad Factsage module. We also generated thermodynamic parameters for Gibb's excess energy of the solid solution. A plot of segregation coefficient as a function of Ta concentration was derived from the phase diagram.

cond-mat.mtrl-sci↗

arXiv2021

Photochromism and influence of point defect charge states on optical absorption in aluminum nitride (AlN)

In this work, we study the absorption properties of AlN in the range of 1.5 - 5.5 eV, as well as the meta-stable change in absorption induced by ultraviolet (UV) irradiation (photochromism), and the restoration of the initial state under the action of irradiation of 2 - 4 eV or elevated temperatures. UV irradiation results in a decrease of the absorption coefficient from 110 cm$^{-1}$ to 55 cm$^{-1}$ at 4.7 eV while in the visible range the absorption coefficient increases from values below 5 cm$^{-1}$ to ~35 cm$^{-1}$. Measurements with two linear polarizations, parallel and perpendicular to the optical axis, provide determination of several different absorption bands at 2.6, 2.8, 3.4, 4.0, 4.5, and 4.8 eV. The bands at 2.6 eV and 3.4 eV identify the defect levels near to the valence band, while the band peaking at 2.8 eV is related to the conduction band. The photochromism allows controlling the absorption of light in two related spectral ranges because the decrease of UV absorption and increase of the visible absorption are related to switching the charge state of the same defects.

cond-mat.mtrl-sci↗

arXiv2020

Phase diagram studies for the growth of (Mg,Zr):SrGa$_{12}$O$_{19}$ crystals

By differential thermal analysis a concentration field suitable for the growth of Zr, Mg codoped strontium hexagallate crystals was observed that corresponds well with experimental results from Mateika and Laurien, J. Crystal Growth 52 (1981) 566-572. It was shown that the melting point of doped crystal is ca. 60 K higher than that of undoped crystals. This higher melting points indicates hexagallate phase stabilization by Zr, Mg codoping, and increases the growth window, compared to undoped SrO-Ga$_2$O$_3$ melts.

cond-mat.mtrl-sci↗